A. Savici | Searcharxiv

arXiv2004

Site-Dilution in quasi one-dimensional antiferromagnet Sr2(Cu1-xPdx)O3: reduction of Neel Temperature and spatial distribution of ordered moment sizes

We investigate the Neel temperature of Sr2CuO3 as a function of the site dilution at the Cu (S=1/2) sites with Pd (S=0), utilizing the muon spin relaxation (muSR) technique. The Neel temperature, which is Tn=5.4K for the undoped system, becomes significantly reduced for less than one percent of doping Pd, giving a support for the previous proposal for the good one-dimensionality. The Pd concentration dependence of the Neel temperature is compared with a recent theoretical study (S. Eggert, I. Affleck and M.D.P. Horton, Phys. Rev. Lett. 89, 47202 (2002)) of weakly coupled one-dimensional antiferromagnetic chains of S=1/2 spins, and a quantitative agreement is found. The inhomogeneity of the ordered moment sizes is characterized by the muSR time spectra. We propose a model that the ordered moment size recovers away from the dopant S=0 sites with a recovery length of ξ= 150-200 sites. The origin of the finite recovery length ξfor the gapless S=1/2 antiferromagnetic chain is compared to the estimate based on the effective staggered magnetic field from the neighboring chains.

cond-mat.str-el↗

arXiv2003

Two dimensional nature of superconductivity in intercalated layered systems Li$_{x}$HfNCl and Li$_{x}$ZrNCl: muon spin relaxation and magnetization measurements

We report muon spin relaxation ($μ$SR) and magnetization measurements, together with synthesis and characterization, of the Li-intercalated layered superconductors Li$_{x}$HfNCl and Li$_{x}$ZrNCl with/without co-intercalation of THF (tetrahydrofuran) or PC (propylene carbonate). The 3-dimensional (3-d) superfluid density $n_{s}/m^{*}$ (superconducting carrier density / effective mass), as well as the two dimensional superfluid density $n_{s2d}/m^{*}_{ab}$ (2-dimensional (2-d) area density of superconducting carriers / ab-plane effective mass), have been derived from the $μ$SR results of the magnetic-field penetration depth $λ_{ab}$ observed with external magnetic field applied perpendicular to the 2-d honeycomb layer of HfN / ZrN. In a plot of $T_{c}$ versus $n_{s2d}/m^{*}_{ab}$, most of the results lie close to the linear relationship found for underdoped high-$T_{c}$ cuprate (HTSC) and layered organic BEDT superconductors. In Li$_{x}$ZrNCl without THF intercalation, the superfluid density and $T_{c}$ for $x$ = 0.17 and 0.4 do not show much difference, reminiscent of $μ$SR results for some overdoped HTSC systems. Together with the absence of dependence of $T_{c}$ on average interlayer distance among ZrN / HfN layers, these results suggest that the 2-d superfluid density $n_{s2d}/m^{*}_{ab}$ is a dominant determining factor for $T_{c}$ in the intercalated nitride-chloride systems. We also report $μ$SR and magnetization results on depinning of flux vortices, and the magnetization results for the upper critical field $H_{c2}$ and the penetration depth $λ$. Reasonable agreement was obtained between $μ$SR and magnetization estimates of $λ$. We discuss the two dimensional nature of superconductivity in the nitride-chloride systems based on these results.

cond-mat.supr-con↗