arXiv subjects

A. Schilling

Publications and source records attributed to A. Schilling.

At least 19 recordsLinked to original sources

arXiv2025

Reconstruction of proton relative stopping power with a granular calorimeter detector model

Proton computed tomography (pCT) aims to facilitate precise dose planning for hadron therapy, a promising and effective method for cancer treatment. Hadron therapy utilizes protons and heavy ions to deliver well focused doses of radiation, leveraging the Bragg peak phenomenon to target tumors while sparing healthy tissues. The Bergen pCT Collaboration aims to develop a novel pCT scanner, and accompanying reconstruction algorithms to overcome current limitations. This paper focuses on advancing the track- and image reconstruction algorithms, thereby enhancing the precision of the dose planning and reducing side effects of hadron therapy. A neural network aided track reconstruction method is presented.

physics.comp-ph↗

arXiv2024

Low-Temperature Heat Transport under Phonon Confinement in Nanostructures

Heat transport in bulk materials is well described using the Debye theory of 3D vibrational modes (phonons) and the acoustic match model. However, in cryogenic nanodevices, phonon wavelengths exceed device dimensions, leading to confinement effects that standard models fail to address. With the growing application of low-temperature devices in communication, sensing, and quantum technologies, there is an urgent need for models that accurately describe heat transport under confinement. We introduce a computational approach to obtain phonon heat capacity and heat transport rates between solids in various confined geometries, that can be easily integrated into, e.g., the standard two-temperature model. Confinement significantly reduces heat capacity and may slow down heat transport. We have validated our model in experiments on strongly disordered NbTiN superconducting nanostructures, widely used in highly efficient single-photon detectors, and we argue that confinement is due to their polycrystalline granular structure. These findings point to potential advances in cryogenic device performance through tailored material and microstructure engineering.

cond-mat.mes-hall↗

arXiv2024

Performance of the electromagnetic and hadronic prototype segments of the ALICE Forward Calorimeter

We present the performance of a full-length prototype of the ALICE Forward Calorimeter (FoCal). The detector is composed of a silicon-tungsten electromagnetic sampling calorimeter with longitudinal and transverse segmentation (FoCal-E) of about 20$X_0$ and a hadronic copper-scintillating-fiber calorimeter (FoCal-H) of about 5$λ_{\rm int}$. The data were taken between 2021 and 2023 at the CERN PS and SPS beam lines with hadron (electron) beams up to energies of 350 (300) GeV. Regarding FoCal-E, we report a comprehensive analysis of its response to minimum ionizing particles across all pad layers. The longitudinal shower profile of electromagnetic showers is measured with a layer-wise segmentation of 1$X_0$. As a projection to the performance of the final detector in electromagnetic showers, we demonstrate linearity in the full energy range, and show that the energy resolution fulfills the requirements for the physics needs. Additionally, the performance to separate two-showers events was studied by quantifying the transverse shower width. Regarding FoCal-H, we report a detailed analysis of the response to hadron beams between 60 and 350 GeV. The results are compared to simulations obtained with a Geant4 model of the test beam setup, which in particular for FoCal-E are in good agreement with the data. The energy resolution of FoCal-E was found to be lower than 3% at energies larger than 100 GeV. The response of FoCal-H to hadron beams was found to be linear, albeit with a significant intercept that is about factor 2 larger than in simulations. Its resolution, which is non-Gaussian and generally larger than in simulations, was quantified using the FWHM, and decreases from about 16% at 100 GeV to about 11% at 350 GeV. The discrepancy to simulations, which is particularly evident at low hadron energies, needs to be further investigated.

physics.ins-det↗

arXiv2023

Fundamental limits of few-layer NbSe$_2$ microbolometers at terahertz frequencies

The rapid development of infrared spectroscopy, observational astronomy, and scanning near-field microscopy has been enabled by the emergence of sensitive mid- and far-infrared photodetectors. Owing to their exceptional signal-to-noise ratio and fast photoresponse, superconducting hot-electron bolometers (HEBs) have become a critical component in these applications. While superconducting HEBs are traditionally made from sputtered superconducting thin films like Nb or NbN, the potential of layered van der Waals (vdW) superconductors is untapped at THz frequencies. Here, we report the fabrication of superconducting HEBs out of few-layer NbSe$_2$ microwires. By improving the interface between NbSe$_2$ and metal leads connected to a broadband antenna, we overcome the impedance mismatch between this vdW superconductor and the radio frequency (RF) readout circuitry that allowed us to achieve large responsivity THz detection over the range from 0.13 to 2.5 THz with minimum noise equivalent power of 7~pW$\sqrt{Hz}$. Using the heterodyne sub-THz mixing technique, we reveal that NbSe$_2$ superconducting HEBs are relatively fast and feature a characteristic response time in the nanosecond range limited by the slow heat escape to the bath through a SiO$_2$ layer, on which they are assembled, in agreement with energy relaxation model. Our work expands the family of materials for superconducting HEBs technology, reveals NbSe$_2$ as a promising platform, and offers a reliable protocol for the in-lab production of custom bolometers using the vdW assembly technique.

cond-mat.supr-con↗

arXiv2023

Single-photon detection using large-scale high-temperature MgB$_2$ sensors at 20 K

Ultra-fast single-photon detectors with high current density and operating temperature can benefit space and ground applications, including quantum optical communication systems, lightweight cryogenics for space crafts, and medical use. Here we demonstrate magnesium diboride (MgB$_2$) thin-film superconducting microwires capable of single-photon detection at 1.55 $μ$m optical wavelength. We used helium ions to alter the properties of MgB$_2$, resulting in microwire-based detectors exhibiting single-photon sensitivity across a broad temperature range of up to 20 K, and detection efficiency saturation for 1 $μ$m wide microwires at 3.7 K. Linearity of detection rate vs incident power was preserved up to at least ~100 Mcps. Despite the large active area of up to 400$\times$400 $μ$m$^2$, the reset time was found to be as low as $\sim1$ ns. Our research provides new possibilities for breaking the operating temperature limit and maximum single-pixel count rate, expanding the detector area, and raises inquiries about the fundamental mechanisms of single-photon detection in high-critical-temperature superconductors.

cond-mat.supr-con↗

arXiv2023

Phonon heat capacity and disorder: new opportunities for performance enhancement of superconducting devices

We experimentally study for the first time the self-heating normal domain in magnetic field using nanowires made of granular NbTiN films with sub-10~nm thicknesses. Specifically, we found that at temperatures below 10 K, the heat capacity of phonons in such films is reduced with respect to predictions of the Debye model. Moreover, as the temperature decreases, the phonon heat capacity reduces quicker than the Debye prediction. These effects strengthen when the film thickness decreases. We attribute the observed reduction in the heat capacity to the size effect, which arises from the confinement of phonon modes within the grains; a phenomenon that has been predicted but not yet observed. These findings hold great importance in understanding the role of heat transport in superconducting electronic devices and have the potential for practical applications in mid-infrared photon sensing with superconducting nanowire detectors.

cond-mat.supr-con↗

arXiv2021

Magnetoconductance and photoresponse properties of disordered NbTiN films

We report on the study of phonon properties and electron-phonon coupling in thin NbTiN films, which are intensively exploited in superconducting devices. Studied NbTiN films with thicknesses less than 10~nm are disordered with respect to electron transport, the Ioffe-Regel parameter of $k_F l_e = 2.5-3.0$ ($k_F$ is the Fermi wave vector and $l_e$ is the electron mean free path), and inelastic electron-phonon interaction, the product $q_T l_e \ll 1$ ($q_T$ is the wave vector of a thermal phonon). By means of magnetoconductance and photoresponse techniques, we derived the inelastic electron-phonon scattering rate $1/τ_{e-ph}$ and determined sound velocities and phonon heat capacities. In the temperature range from 12 to 20~K, the scattering rate varies with temperature as $1/τ_{e-ph}\propto T^{3.45\pm0.05}$; its value extrapolated to 10~K amounts to approximately 16~ps. Making a comparative analysis of our films and other films used in superconducting devices, such as polycrystalline granular NbN and amorphous WSi, we found a systematic reduction of the sound velocity in all these films by about 50\% as compared to the corresponding bulk crystalline materials. A corresponding increase in the phonon heat capacities in all these films is, however, less than the Debye model predicts. We attribute these findings to reduced film dimensionality and film morphology.

cond-mat.supr-con↗

arXiv2020

Magnetism and anomalous transport in the Weyl semimetal PrAlGe: Possible route to axial gauge fields

In magnetic Weyl semimetals, where magnetism breaks time-reversal symmetry, large magnetically sensitive anomalous transport responses are anticipated that could be useful for topological spintronics. The identification of new magnetic Weyl semimetals is therefore in high demand, particularly since in these systems Weyl node configurations may be easily modified using magnetic fields. Here we explore experimentally the magnetic semimetal PrAlGe, and unveil a direct correspondence between easy-axis Pr ferromagnetism and anomalous Hall and Nernst effects. With sizes of both the anomalous Hall conductivity and Nernst effect in good quantitative agreement with first principles calculations, we identify PrAlGe as a system where magnetic fields can connect directly to Weyl nodes via the Pr magnetization. Furthermore, we find the predominantly easy-axis ferromagnetic ground state co-exists with a low density of nanoscale textured magnetic domain walls. We describe how such nanoscale magnetic textures could serve as a local platform for tunable axial gauge fields of Weyl fermions.

cond-mat.str-el↗

arXiv2016

Characteristics of superconducting tungsten silicide WxSi1-x for single photon detection

Superconducting properties of three series of amorphous WxSi1-x films with different thickness and stoichiometry were investigated by dc transport measurements in a magnetic field up to 9 T. These amorphous WxSi1-x films were deposited by magnetron co-sputtering of the elemental source targets onto silicon substrates at room temperature and patterned in form of bridges by optical lithography and reactive ion etching. Analysis of the data on magnetoconductivity allowed us to extract the critical temperature, superconducting coherence length, magnetic penetration depth, and diffusion coefficient of electrons in the normal state as a function of film thickness for each stoichiometry. Two basic time constants were derived from transport and time-resolving measurements. A dynamic process of the formation of a hot-spot was analyzed in the framework of a diffusion-based vortex-entry model. We used the two stage diffusion approach and defined a hotspot size by assuming that the quasi-particles and normal-state electrons have the equal diffusion constant. Our findings are consistent with the most recent results on a hot-spot relaxation time in the WxSi1-x superconducting nanowire single-photon detector. In the 5 nm thick W0.85Si0.15 film the hot-spot has a diameter of 105 nm at the peak of the number of non-equilibrium quasi-particles.

cond-mat.supr-con↗

arXiv2016

Superconducting single X-ray photon detector based on W0.8Si0.2

We fabricated a superconducting single X-ray photon detector based on W0.8Si0.2, and we characterized its basic detection performance for keV-photons at different temperatures. The detector has a critical temperature of 4.97 K, and it is able to be operated up to 4.8 K, just below the critical temperature. The detector starts to react to X-ray photons at relatively low bias currents, less than 1% of Ic at T = 1.8 K, and it shows a saturated count rate dependence on bias current at all temperatures, indicating that the optimum internal quantum efficiency can always be reached. Dark counts are negligible up to the highest investigated bias currents (99% of Ic) and operating temperature (4.8 K). The latching effect affects the detector performance at all temperatures due to the fast recovery of the bias current; however, further modifications of the device geometry are expected to reduce the tendency for latching.

physics.ins-det↗

arXiv2016

Field-induced transition of the magnetic ground state from A-type antiferromagnetic to ferromagnetic order in CsCo2Se2

We report on the magnetic properties of CsCo$_2$Se$_2$ with ThCr$_2$Si$_2$ structure, which we have characterized through a series of magnetization and neutron diffraction measurements. We find that CsCo$_2$Se2$_2$ undergoes a phase transition to an antiferromagnetically ordered state with a Néel temperature of $T_{\rm N} \approx$ 66 K. The nearest neighbour interactions are ferromagnetic as observed by the positive Curie-Weiss temperature of $Θ\approx$ 51.0 K. We find that the magnetic structure of CsCo$_2$Se$_2$ consists of ferromagnetic sheets, which are stacked antiferromagnetically along the tetragonal \textit{c}-axis, generally referred to as A-type antiferromagnetic order. The observed magnitude of the ordered magnetic moment at $T$ = 1.5 K is found to be only 0.20(1)$μ_{\rm Bohr}$/Co. Already in comparably small magnetic fields of $μ_0 H_{MM}$(5K) $\approx$ 0.3 T, we observe a metamagnetic transition that can be attributed to spin-rearrangements of CsCo$_2$Se$_2$, with the moments fully ferromagnetically saturated in a magnetic field of $μ_0 H_{\rm FM}$(5K) $\approx$ 6.4 T. We discuss the entire experimentally deduced magnetic phase diagram for CsCo$_2$Se$_2$ with respect to its unconventionally weak magnetic coupling. Our study characterizes CsCo$_2$Se$_2$, which is chemically and electronically posed closely to the $A_xFe_{2-y}Se_2$ superconductors, as a host of versatile magnetic interactions.

cond-mat.str-el↗

arXiv2014

Low-temperature magnetic fluctuations in the Kondo insulator SmB6

We present the results of a systematic investigation of the magnetic properties of the three-dimensional Kondo topological insulator SmB6 using magnetization and muon-spin relaxation/rotation (muSR) measurements. The muSR measurements exhibit magnetic field fluctuations in SmB6 below 15 K due to electronic moments present in the system. However, no evidence for magnetic ordering is found down to 19 mK. The observed magnetism in SmB6 is homogeneous in nature throughout the full volume of the sample. Bulk magnetization measurements on the same sample show consistent behavior. The agreement between muSR, magnetization, and NMR results strongly indicate the appearance of intrinsic bulk magnetic in-gap states associated with fluctuating magnetic fields in SmB6 at low temperature.

cond-mat.str-el↗

arXiv2012

Intrinsic instability at the Bose-Einstein condensation of bosonic quasiparticles in magnetic insulators

Starting from a phenomenological standard energy functional to describe the condensation of a dilute gas of bosonic quasiparticles in magnetic insulators, we find that the inclusion of a perturbation term that explicitly violates the axial symmetry significantly modifies the details of the resulting Bose Einstein condensation. Systems with an originally axial symmetry must show an intrinsic tendency to spontaneously violate this symmetry as soon as the condensation sets in, and the phase transition at the respective critical field may even become of first order. We can explain a number of features in the experimental data of various insulating spin systems, such as a slightly nonlinear magnetization near the critical field as well as hysteresis effects and peculiarities in the energy-level scheme of TlCuCl3. We also offer a consistent explanation for certain anomalies in the magnetocaloric effect and in the magnetization of BaCuSi2O6 by assuming a spontaneous violation of axial symmetry at the magnetic phase transition on an energy scale of about 1 micro-eV. The resulting anisotropy gap in the magnetic excitation spectrum, that inevitably forms at the critical field of all such systems, lifts the linear Goldstone mode and is therefore seriously limiting the lifetime of magnetic condensates to a few nanoseconds at most.

cond-mat.str-el↗

arXiv2012

Superconductivity and magnetism in RbxFe2-ySe2: Impact of thermal treatment on mesoscopic phase separation

An extended study of the superconducting and normal-state properties of various as-grown and post-annealed RbxFe2-ySe2 single crystals is presented. Magnetization experiments evidence that annealing of RbxFe2-ySe2 at 413 K, well below the onset of phase separation Tp=489 K, neither changes the magnetic nor the superconducting properties of the crystals. In addition, annealing at 563 K, well above Tp, suppresses the superconducting transition temperature Tc and leads to an increase of the antiferromagnetic susceptibility accompanied by the creation of ferromagnetic impurity phases, which are developing with annealing time. However, annealing at T=488K=Tp increases Tc up to 33.3 K, sharpens the superconducting transition, increases the lower critical field, and strengthens the screening efficiency of the applied magnetic field. Resistivity measurements of the as-grown and optimally annealed samples reveal an increase of the upper critical field along both crystallographic directions as well as its anisotropy. Muon spin rotation and scanning transmission electron microscopy experiments suggest the coexistence of two phases below Tp: a magnetic majority phase of Rb2Fe4Se5 and a non-magnetic minority phase of Rb0.5Fe2Se2. Both microscopic techniques indicate that annealing the specimens just at Tp does not affect the volume fraction of the two phases, although the magnetic field distribution in the samples changes substantially. This suggests that the microstructure of the sample, caused by mesoscopic phase separation, is modified by annealing just at Tp, leading to an improvement of the superconducting properties of RbxFe2-ySe2 and an enhancement of Tc.

cond-mat.supr-con↗

arXiv2012

Magnetic-field dependence of count rates in superconducting thin-film TaN single-photon detectors

We have studied the magnetic-field dependence of both dark-count rates and photon-count rates in a superconducting nanowire single-photon detector made of TaN in external magnetic fields $|μ_0H| < 10$ mT perpendicular to the plane of the underlying meander structure and at $T = 4$ K. The dark-count rates show a characteristic field-dependence, which is asymmetric with respect to magnetic field direction. The field- and the current dependence of the dark counts can be quantitatively well explained if one assumes that the critical current is reduced to $\approx50%$ at the $180^\circ$ meander turns when compared to a straight strip, and the observed asymmetry can be modeled assuming that the turnarounds are not all strictly equal. Surprisingly, the photon count rates do not show any significant field dependence, which seems to be at odds with existing detection models invoking vortex crossings.

cond-mat.supr-con↗

arXiv2012

Synthesis of a new alkali metal-organic solvent intercalated iron selenide superconductor with Tc{\approx}45K

We report on a new iron selenide superconductor with a TC onset of 45K and the nominal composition Lix(C5H5N)yFe2-zSe2, synthesized via intercalation of dissolved alkaline metal in anhydrous pyridine at room temperature. This superconductor exhibits a broad transition, reaching zero resistance at 10K. Magnetization measurements reveal a superconducting shielding fraction of approximately 30%. Analogous phases intercalated with Na, K and Rb were also synthesized and characterized. The superconducting transition temperature of Lix(C5H5N)yFe2-zSe2 is clearly enhanced in comparison to the known superconductors FeSe0.98 (Tc ~ 8K) and AxFe2-ySe2 (TC ~ 27-32K) and is in close agreement with critical temperatures recently reported for Lix(NH3)yFe2-zSe2. Post-annealing of intercalated material (Lix(C5H5N)yFe2-zSe2) at elevated temperatures drastically enlarges the c-parameter of the unit cell (~44%) and increases the amount of superconducting shielding fraction to nearly 100%. Our findings indicate a new synthesis road leading to possibly even higher critical temperatures in this class of materials by intercalation of organic compounds between Fe-Se layers.

cond-mat.supr-con↗

arXiv2011

Experimental tests for macroscopic phase coherence in magnetic-quasiparticle condensates of insulating spin systems

For most kinds of already known Bose-Einstein condensates experimental evidence for the existence of a macroscopic coherent quantum state has been provided, e.g., from the observation of interference phenomena, the formation vortices, the detection of Josephson effects, or even by the manifestation of superfluid behaviour. However, none of these hallmarks for a true, macroscopic phase-coherent state has ever been reported for any insulating spin system in a solid in which magnetic bosonic quasiparticles are thought to condense close to a quantum critical point. We describe an attempt to detect superfluid behaviour in TlCuCl3, and discuss in more detail a proposal for an experiment in which the a.c. Josephson effect can be probed by using a device composed of two weakly coupled magnetic insulators with different critical fields. We conclude that the detection of the a.c. Josephson effect is feasible for a proper choice of compounds with realistic material parameters.

cond-mat.supr-con↗

arXiv2011

Differential-thermal analysis around and below the critical temperature Tc of various low-Tc superconductors: A comparative study

We present specific-heat data on the type-II superconductors V3Si, LuNi2B2C and NbSe2 which were acquired with a low-temperature thermal analysis (DTA) technique. We compare our data with available literature data on these superconductors. In the first part we show that the DTA technique allows for fast measurements while providing a very high resolution on the temperature scale. Sharp features in the specific heat such as at the one at the transition to superconductivity are resolved virtually without instrumental broadening. In the second part we investigate the magnetic-field dependence of the specific heats of V3Si and LuNi2B2C at a fixed temperature T=7.5K to demonstrate that DTA techniques also allow for sufficiently precise measurements of absolute values of cp even in the absence of a sharp phase transition. The corresponding data for V3Si and LuNi2B2C are briefly discussed.

cond-mat.supr-con↗