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A. Shevchenko

Publications and source records attributed to A. Shevchenko.

10 recordsLinked to original sources

High temperature transitions in Ruddlesden-Popper nickelates La$_{n+1}$Ni$_{n}$O$_{3n+1}$

The discovery of superconductivity at $15\,\mathrm{K}$ in the infinite-layer nickelate $(\mathrm{Nd},\mathrm{Sr})\mathrm{NiO}_2$, followed by superconductivity at $80\,\mathrm{K}$ in the Ruddlesden--Popper phase $\mathrm{La}_3\mathrm{Ni}_2\mathrm{O}_7$, has ushered in a new era of nickelate research. Despite this progress, large discrepancies between reports exist. Here, we investigate the complete series of bulk-stable $\mathrm{La}_{n+1}\mathrm{Ni}_n\mathrm{O}_{3n+1}$ compounds using a comprehensive set of experimental techniques, including PXRD, single-crystal XRD, electron microscopy, heat capacity, differential scanning calorimetry, magnetic susceptibility, and transport measurements, over a broad temperature range from $2$ to $1000\,\mathrm{K}$. By studying high-quality single crystals, we identify a previously underappreciated high-temperature phase transition in Ruddlesden--Popper nickelates $\mathrm{La}_{n+1}\mathrm{Ni}_n\mathrm{O}_{3n+1}$ distinct from the one going to a tetragonal phase.

cond-mat.supr-con

Inverse-designed 3D laser nanoprinted phase masks to extend the depth of field of imaging systems

In optical imaging, achieving high resolution often comes at the expense of a shallow depth of field. This means that when using a standard microscope, any minor movement of the object along the optical axis can cause the image to become blurry. To address this issue, we exploit inverse design techniques to optimise a phase mask which, when inserted into a standard microscope, extends the depth of field by a factor of approximately four without compromising the microscope's resolution. Differentiable Fourier optics simulations allow us to rapidly iterate towards an optimised design in a hybrid fashion, starting with gradient-free Bayesian optimisation and proceeding to a local gradient-based optimisation. To fabricate the device, a commercial two-photon 3D laser nanoprinter is used, in combination with a two-step pre-compensation routine, providing high fabrication speed and much better than subwavelength accuracy. We find excellent agreement between our numerical predictions and the measurements upon integrating the phase mask into a microscope and optically characterising selected samples. The phase mask enables us to conduct simultaneous multiplane imaging of objects separated by distances that cannot be achieved with the original microscope.

physics.optics

Learning velocity model for complex media with deep convolutional neural networks

The paper considers the problem of velocity model acquisition for a complex media based on boundary measurements. The acoustic model is used to describe the media. We used an open-source dataset of velocity distributions to compare the presented results with the previous works directly. Forward modeling is performed using the grid-characteristic numerical method. The inverse problem is solved using deep convolutional neural networks. Modifications for a baseline UNet architecture are proposed to improve both structural similarity index measure quantitative correspondence of the velocity profiles with the ground truth. We evaluate our enhancements and demonstrate the statistical significance of the results.

cs.LG

Interferometric description of optical metamaterials

We introduce a simple theoretical model that describes the interaction of light with optical metamaterials in terms of interfering optical plane waves. In this model, a metamaterial is considered to consist of planar arrays of densely packed nanoparticles. In the analysis, each such array reduces to an infinitely thin homogeneous sheet. The transmission and reflection coefficients of this sheet are found to be equal to those of an isolated nanoparticle array and, therefore, they are easy to evaluate numerically for arbitrary shapes and arrangements of the particles. The presented theory enables fast calculation of electromagnetic fields interacting with a metamaterial slab of an arbitrary size, which, for example, can be used to retrieve the effective refractive index and wave impedance in the material. It is also shown to accurately describe optically anisotropic metamaterials that in addition exhibit strong spatial dispersion, such as bifacial metamaterials.

physics.optics

Calculating the electromagnetic characteristics of bifacial optical nanomaterials

We introduce a formalism that describes the interaction of light with bifacial optical nanomaterials. They are artificial noncentrosymmetric materials in which counter-propagating waves behave differently. We derive electromagnetic material parameters for uniaxial crystalline media in terms of the complex transmission and reflection coefficients of a single layer of the constituent nanoscatterers, which makes the numerical evaluation of these parameters very efficient. In addition, we present generalized Fresnel coefficients for such bifacial nanomaterials and investigate the fundamental role of higher-order electromagnetic multipoles on the bifaciality. We find that two counter-propagating waves in the material must experience the same refractive index, but they can have dramatically different wave impedances. The use of our model in practice is demonstrated with a particular example of a bifacial nanomaterial that exhibits a directional impedance matching to the surrounding medium.

physics.optics

Electromagnetic multipole theory for optical nanomaterials

Optical properties of natural or designed materials are determined by the electromagnetic multipole moments that light can excite in the constituent particles. In this work we present an approach to calculate the multipole excitations in arbitrary arrays of nanoscatterers in a dielectric host medium. We introduce a simple and illustrative multipole decomposition of the electric currents excited in the scatterers and link this decomposition to the classical multipole expansion of the scattered field. In particular, we find that completely different multipoles can produce identical scattered fields. The presented multipole theory can be used as a basis for the design and characterization of optical nanomaterials.

physics.optics

Electric dipole-free interaction of visible light with silver metadimers

In subwavelength-sized particles, light-induced multipole moments of orders higher than the electric dipole are usually negligibly small, which allows for the light-matter interaction to be accurately treated within the electric dipole approximation. In this work we show that in a specially designed meta-atom, a disc metadimer, the electric quadrupole and magnetic dipole can be the only excitable multipoles. This condition is achieved in a narrow but tunable spectral range of visible light both for individual metadimers and for a periodic array of such particles. The electromagnetic fields scattered by the metadimers fundamentally differ from those created by electric dipoles. A metamaterial composed of such metadimers will therefore exhibit unusual optical properties.

physics.optics

Level density of 2+ states in 40Ca from high energy-resolution (p,p') experiments

The level density of 2+ states in 40Ca has been extracted in the energy region of the isoscalar giant quadrupole resonance (ISGQR) from a fluctuation analysis of high energy-resolution p,p') data taken at incident energies of 200 MeV at the K600 magnetic spectrometer of iThemba LABS, South Africa. Quasi-free scattering cross sections were calculated to estimate their role as a background contribution to the spectra and found to be small. The shape of the background was determined from the discrete wavelet transform of the spectra using a biorthogonal wavelet function normalized at the lowest particle separation threshold. The experimental results are compared to widely used phenomenological and microscopic models.

nucl-ex

Fine structure of the isoscalar giant quadrupole resonance in 40Ca due to Landau damping?

The fragmentation of the Isoscalar Giant Quadrupole Resonance (ISGQR) in 40Ca has been investigated in high energy-resolution experiments using proton inelastic scattering at E_p = 200 MeV. Fine structure is observed in the region of the ISGQR and its characteristic energy scales are extracted from the experimental data by means of a wavelet analysis. The experimental scales are well described by Random Phase Approximation (RPA) and second-RPA calculations with an effective interaction derived from a realistic nucleon-nucleon interaction by the Unitary Correlation Operator Method (UCOM). In these results characteristic scales are already present at the mean-field level pointing to their origination in Landau damping, in contrast to the findings in heavier nuclei and also to SRPA calculations for 40Ca based on phenomenological effective interactions, where fine structure is explained by the coupling to two-particle two-hole (2p-2h) states.

nucl-ex

Trapping atoms on a transparent permanent-magnet atom chip

We describe experiments on trapping of atoms in microscopic magneto-optical traps on an optically transparent permanent-magnet atom chip. The chip is made of magnetically hard ferrite-garnet material deposited on a dielectric substrate. The confining magnetic fields are produced by miniature magnetized patterns recorded in the film by magneto-optical techniques. We trap Rb atoms on these structures by applying three crossed pairs of counter-propagating laser beams in the conventional magneto-optical trapping (MOT) geometry. We demonstrate the flexibility of the concept in creation and in-situ modification of the trapping geometries through several experiments.

quant-ph