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A. Spyrou

Publications and source records attributed to A. Spyrou.

At least 37 records · Page 2Linked to original sources

Enhanced low-energy $γ$-decay strength of $^{70}$Ni and its robustness within the shell model

Neutron-capture reactions on very neutron-rich nuclei are essential for heavy-element nucleosynthesis through the rapid neutron-capture process, now shown to take place in neutron-star merger events. For these exotic nuclei, radiative neutron capture is extremely sensitive to their $γ$-emission probability at very low $γ$ energies. In this work, we present measurements of the $γ$-decay strength of $^{70}$Ni over the wide range $1.3 \leq E_γ \leq 8 $ MeV. A significant enhancement is found in the $γ$-decay strength for transitions with $E_γ< 3$ MeV. At present, this is the most neutron-rich nucleus displaying this feature, proving that this phenomenon is not restricted to stable nuclei. We have performed $E1$-strength calculations within the quasiparticle time-blocking approximation, which describe our data above $E_γ\simeq 5$ MeV very well. Moreover, large-scale shell-model calculations indicate an $M1$ nature of the low-energy $γ$ strength. This turns out to be remarkably robust with respect to the choice of interaction, truncation and model space, and we predict its presence in the whole isotopic chain, in particular the neutron-rich $^{72,74,76}\mathrm{Ni}$.

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r-Process Nucleosynthesis: Connecting Rare-Isotope Beam Facilities with the Cosmos

This is an exciting time for the study of r-process nucleosynthesis. Recently, a neutron star merger GW170817 was observed in extraordinary detail with gravitational waves and electromagnetic radiation from radio to gamma rays. The very red color of the associated kilonova suggests that neutron star mergers are an important r-process site. Astrophysical simulations of neutron star mergers and core collapse supernovae are making rapid progress. Detection of both, electron neutrinos and antineutrinos from the next galactic supernova will constrain the composition of neutrino-driven winds and provide unique nucleosynthesis information. Finally FRIB and other rare-isotope beam facilities will soon have dramatic new capabilities to synthesize many neutron-rich nuclei that are involved in the r-process. The new capabilities can significantly improve our understanding of the r-process and likely resolve one of the main outstanding problems in classical nuclear astrophysics. However, to make best use of the new experimental capabilities and to fully interpret the results, a great deal of infrastructure is needed in many related areas of astrophysics, astronomy, and nuclear theory. We will place these experiments in context by discussing astrophysical simulations and observations of r-process sites, observations of stellar abundances, galactic chemical evolution, and nuclear theory for the structure and reactions of very neutron-rich nuclei. This review paper was initiated at a three-week International Collaborations in Nuclear Theory program in June 2016 where we explored promising r-process experiments and discussed their likely impact, and their astrophysical, astronomical, and nuclear theory context.

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Confirmation of the isomeric state in 26P

We report the independent experimental confirmation of an isomeric state in the proton drip-line nucleus $^{26}$P. The $γ$-ray energy and half-life determined are 164.4 $\pm$ 0.3 (sys) $\pm$ 0.2 (stat) keV and 104 $\pm$ 14 ns, respectively, which are in agreement with the previously reported values. These values are used to set a semi-empirical limit on the proton separation energy of $^{26}$P, with the conclusion that it can be bound or unbound.

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Low-lying level structure of $^{56}$Cu and its implications on the rp process

The low-lying energy levels of proton-rich $^{56}$Cu have been extracted using in-beam $γ$-ray spectroscopy with the state-of-the-art $γ$-ray tracking array GRETINA in conjunction with the S800 spectrograph at the National Superconducting Cyclotron Laboratory at Michigan State University. Excited states in $^{56}$Cu serve as resonances in the $^{55}$Ni(p,$γ$)$^{56}$Cu reaction, which is a part of the rp-process in type I x-ray bursts. To resolve existing ambiguities in the reaction Q-value, a more localized IMME mass fit is used resulting in $Q=639\pm82$~keV. We derive the first experimentally-constrained thermonuclear reaction rate for $^{55}$Ni(p,$γ$)$^{56}$Cu. We find that, with this new rate, the rp-process may bypass the $^{56}$Ni waiting point via the $^{55}$Ni(p,$γ$) reaction for typical x-ray burst conditions with a branching of up to $\sim$40$\%$. We also identify additional nuclear physics uncertainties that need to be addressed before drawing final conclusions about the rp-process reaction flow in the $^{56}$Ni region.

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Completing the nuclear reaction puzzle of the nucleosynthesis of 92Mo

One of the greatest questions for modern physics to address is how elements heavier than iron are created in extreme, astrophysical environments. A particularly challenging part of that question is the creation of the so-called p-nuclei, which are believed to be mainly produced in some types of supernovae. The lack of needed nuclear data presents an obstacle in nailing down the precise site and astrophysical conditions. In this work, we present for the first time measurements on the nuclear level density and average strength function of $^{92}$Mo. State-of-the-art p-process calculations systematically underestimate the observed solar abundance of this isotope. Our data provide stringent constraints on the $^{91}$Nb$(p,γ)^{92}$Mo reaction rate, which is the last unmeasured reaction in the nucleosynthesis puzzle of $^{92}$Mo. Based on our results, we conclude that the $^{92}$Mo abundance anomaly is not due to the nuclear physics input to astrophysical model calculations.

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Beta-delayed gamma decay of 26P: Possible evidence of a proton halo

Background: Measurements of $β$ decay provide important nuclear structure information that can be used to probe isospin asymmetries and inform nuclear astrophysics studies. Purpose: To measure the $β$-delayed $γ$ decay of $^{26}$P and compare the results with previous experimental results and shell-model calculations. Method: A $^{26}$P fast beam produced using nuclear fragmentation was implanted into a planar germanium detector. Its $β$-delayed $γ$-ray emission was measured with an array of 16 high-purity germanium detectors. Positrons emitted in the decay were detected in coincidence to reduce the background. Results: The absolute intensities of $^{26}$P $β$-delayed $γ$-rays were determined. A total of six new $β$-decay branches and 15 new $γ$-ray lines have been observed for the first time in $^{26}$P $β$-decay. A complete $β$-decay scheme was built for the allowed transitions to bound excited states of $^{26}$Si. $ft$ values and Gamow-Teller strengths were also determined for these transitions and compared with shell model calculations and the mirror $β$-decay of $^{26}$Na, revealing significant mirror asymmetries. Conclusions: A very good agreement with theoretical predictions based on the USDB shell model is observed. The significant mirror asymmetry observed for the transition to the first excited state ($δ=51(10)\%$) may be evidence for a proton halo in $^{26}$P.

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Two-Neutron Sequential Decay of $^{24}$O

A two-neutron unbound excited state of $^{24}$O was populated through a (d,d') reaction at 83.4 MeV/nucleon. A state at $E = 715 \pm 110$ (stat) $\pm 45 $ (sys) keV with a width of $Γ< 2$ MeV was observed above the two-neutron separation energy placing it at 7.65 $\pm$ 0.2 MeV with respect to the ground state. Three-body correlations for the decay of $^{24}$O $\rightarrow$ $^{22}$O + $2n$ show clear evidence for a sequential decay through an intermediate state in $^{23}$O. Neither a di-neutron nor phase-space model for the three-body breakup were able to describe these correlations.

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Population of 13Be in a Nucleon Exchange Reaction

The neutron-unbound nucleus 13Be was populated with a nucleon-exchange reaction from a 71 MeV/u secondary 13B beam. The decay energy spectrum was reconstructed using invariant mass spectroscopy based on 12Be fragments in coincidence with neutrons. The data could be described with an s-wave resonance at E = 0.73(9) MeV with a width of Gamma = 1.98(34) MeV and a d-wave resonance at E = 2.56(13) MeV with a width of Gamma = 2.29(73) MeV. The observed spectral shape is consistent with previous one-proton removal reaction measurements from 14B.

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Observation of Doppler broadening in $β$-delayed proton-$γ$ decay

Background: The Doppler broadening of $γ$-ray peaks due to nuclear recoil from $β$-delayed nucleon emission can be used to measure the energies of the nucleons. This method has never been tested using $β$-delayed proton emission or applied to a recoil heavier than $A=10$. Purpose: To test and apply this Doppler broadening method using $γ$-ray peaks from the $^{26}$P($βpγ$)$^{25}$Al decay sequence. Methods: A fast beam of $^{26}$P was implanted into a planar Ge detector, which was used as a $^{26}$P $β$-decay trigger. The SeGA array of high-purity Ge detectors was used to detect $γ$ rays from the $^{26}$P($βpγ$)$^{25}$Al decay sequence. Results: Radiative Doppler broadening in $β$-delayed proton-$γ$ decay was observed for the first time. The Doppler broadening analysis method was verified using the 1613 keV $γ$-ray line for which the proton energies were previously known. The 1776 keV $γ$ ray de-exciting the 2720 keV $^{25}$Al level was observed in $^{26}$P($βpγ$)$^{25}$Al decay for the first time and used to determine that the center-of-mass energy of the proton emission feeding the 2720-keV level is 5.1 $\pm$ 1.0 (stat.) $\pm$ 0.6 (syst.) MeV, corresponding to a $^{26}$Si excitation energy of 13.3 $\pm$ 1.0 (stat.) $\pm$ 0.6 (syst.) MeV for the proton-emitting level. Conclusions: The Doppler broadening method has been demonstrated to provide practical measurements of the energies for $β$-delayed nucleon emissions populating excited states of nuclear recoils at least as heavy as $A=25$.

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Three-body correlations in the ground-state decay of 26O

Background: Theoretical calculations have shown that the energy and angular correlations in the three-body decay of the two-neutron unbound O26 can provide information on the ground-state wave function, which has been predicted to have a dineutron configuration and 2n halo structure. Purpose: To use the experimentally measured three-body correlations to gain insight into the properties of O26, including the decay mechanism and ground-state resonance energy. Method: O26 was produced in a one-proton knockout reaction from F27 and the O24+n+n decay products were measured using the MoNA-Sweeper setup. The three-body correlations from the O26 ground-state resonance decay were extracted. The experimental results were compared to Monte Carlo simulations in which the resonance energy and decay mechanism were varied. Results: The measured three-body correlations were well reproduced by the Monte Carlo simulations but were not sensitive to the decay mechanism due to the experimental resolutions. However, the three-body correlations were found to be sensitive to the resonance energy of O26. A 1σ upper limit of 53 keV was extracted for the ground-state resonance energy of O26. Conclusions: Future attempts to measure the three-body correlations from the ground-state decay of O26 will be very challenging due to the need for a precise measurement of the O24 momentum at the reaction point in the target.

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Search for unbound 15Be states in the 3n+12Be channel

15Be is expected to have low-lying 3/2+ and 5/2+ states. A first search did not observe the 3/2+ [A. Spyrou et al., Phys. Rev. C 84, 044309 (2011)], however, a resonance in 15Be was populated in a second attempt and determined to be unbound with respect to 14Be by 1.8(1) MeV with a tentative spin-parity assignment of 5/2+ [J. Snyder et al., Phys. Rev. C 88, 031303(R) (2013)]. Search for the predicted 15Be 3/2+ state in the three-neutron decay channel. A two-proton removal reaction from a 55 MeV/u 17C beam was used to populate neutron-unbound states in 15Be. The two-, three-, and four-body decay energies of the 12Be + neutron(s) detected in coincidence were reconstructed using invariant mass spectroscopy. Monte Carlo simulations were performed to extract the resonance and decay properties from the observed spectra. The low-energy regions of the decay energy spectra can be described with the first excited unbound state of 14Be (E_x=1.54 MeV, E_r=0.28 MeV). Including a state in 15Be that decays through the first excited 14Be state slightly improves the fit at higher energies though the cross section is small. A 15Be component is not needed to describe the data. If the 3/2+ state in 15Be is populated, the decay by three-neutron emission through 14Be is weak, less than or equal to 11% up to 4 MeV. In the best fit, 15Be is unbound with respect to 12Be by 1.4 MeV (unbound with respect to $14Be by 2.66 MeV) with a strength of 7%.

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Novel technique for constraining r-process (n,$γ$) reaction rates

A novel technique has been developed, which will open exciting new opportunities for studying the very neutron-rich nuclei involved in the r-process. As a proof-of-principle, the $γ$-spectra from the $β$-decay of $^{76}$Ga have been measured with the SuN detector at the National Superconducting Cyclotron Laboratory. The nuclear level density and $γ$-ray strength function are extracted and used as input to Hauser-Feshbach calculations. The present technique is shown to strongly constrain the $^{75}$Ge($n,γ$)$^{76}$Ge cross section and reaction rate.

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Measurement of the $^{58}$Ni($α$,$γ$)$^{62}$Zn reaction and its astrophysical impact

Cross section measurements of the $^{58}$Ni($α$,$γ$)$^{62}$Zn reaction were performed in the energy range $E_α=5.5-9.5$ MeV at the Nuclear Science Laboratory of the University of Notre Dame, using the NSCL Summing NaI(Tl) detector and the $γ$-summing technique. The measurements are compared to predictions in the statistical Hauser-Feshbach model of nuclear reactions using the SMARAGD code. It is found that the energy dependence of the cross section is reproduced well but the absolute value is overestimated by the prediction. This can be remedied by rescaling the $α$ width by a factor of 0.45. Stellar reactivities were calculated with the rescaled $α$ width and their impact on nucleosynthesis in type Ia supernovae has been studied. It is found that the resulting abundances change by up to 5\% when using the new reactivities.

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Classical-Nova Contribution to the Milky Way's $^{26}$Al Abundance: Exit Channel of the Key $^{25}$Al($p,γ$)$^{26}$Si Resonance

Classical novae are expected to contribute to the 1809-keV Galactic $γ$-ray emission by producing its precursor $^{26}$Al, but the yield depends on the thermonuclear rate of the unmeasured $^{25}$Al($p,γ$)$^{26}$Si reaction. Using the $β$ decay of $^{26}$P to populate the key $J^π=3^+$ resonance in this reaction, we report the first evidence for the observation of its exit channel via a $1741.6 \pm 0.6 (\textrm{stat}) \pm 0.3 (\textrm{syst})$ keV primary $γ$ ray, where the uncertainties are statistical and systematic, respectively. By combining the measured $γ$-ray energy and intensity with other experimental data on $^{26}$Si, we find the center-of-mass energy and strength of the resonance to be $E_r = 414.9 \pm 0.6(\textrm{stat}) \pm 0.3 (\textrm{syst}) \pm 0.6(\textrm{lit.})$ keV and $ωγ= 23 \pm 6 (\textrm{stat})^{+11}_{-10}(\textrm{lit.})$ meV, respectively, where the last uncertainties are from adopted literature data. We use hydrodynamic nova simulations to model $^{26}$Al production showing that these measurements effectively eliminate the dominant experimental nuclear-physics uncertainty and we estimate that novae may contribute up to 30% of the Galactic $^{26}$Al.

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Measurement of the $^{90, 92}$Zr(p,$γ$)$^{91,93}$Nb reactions for the nucleosynthesis of elements around A=90

Cross section measurements of the reactions $^{90, 92}$Zr(p,$γ$)$^{91,93}$Nb were performed using the NSCL SuN detector at the University of Notre Dame. These reactions are part of the nuclear reaction flow for the synthesis of the light p nuclei. For the $^{90}$Zr(p,$γ$)$^{91}$Nb reaction the new measurement resolves the disagreement between previous results. For the $^{92}$Zr(p,$γ$)$^{93}$Nb reaction the present work reports the first measurement of this reaction cross section. Both reaction cross sections are compared to theoretical calculations and a very good agreement with the standard NON-SMOKER model is observed.

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Exploiting neutron-rich radioactive ion beams to constrain the symmetry energy

The Modular Neutron Array (MoNA) and 4 Tm Sweeper magnet were used to measure the free neutrons and heavy charged particles from the radioactive ion beam induced 32Mg + 9Be reaction. The fragmentation reaction was simulated with the Constrained Molecular Dynamics model(CoMD), which demonstrated that the of the heavy fragments and free neutron multiplicities were observables sensitive to the density dependence of the symmetry energy at sub-saturation densities. Through comparison of these simulations with the experimental data constraints on the density dependence of the symmetry energy were extracted. The advantage of radioactive ion beams as a probe of the symmetry energy is demonstrated through examination of CoMD calculations for stable and radioactive beam induced reactions.

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Novel techniques to search for neutron radioactivity

Two new methods to observe neutron radioactivity are presented. Both methods rely on the production and decay of the parent nucleus in flight. The relative velocity measured between the neutron and the fragment is sensitive to half-lives between ~1 and ~100 ps for the Decay in Target (DiT) method. The transverse position measurement of the neutron in the Decay in a Magnetic Field (DiMF) method is sensitive to half-lives between 10 ps and 1 ns.

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Systematic study of (p,γ) reactions on Ni isotopes

A systematic study of the radiative proton capture reaction for all stable nickel isotopes is presented. The results were obtained using 2.0 - 6.0 MeV protons from the 11 MV tandem Van de Graaff accelerator at the University of Notre Dame. The γ-rays were detected by the NSCL SuN detector utilising the γ-summing technique. The results are compared to a compilation of earlier measurements and discrepancies between the previous data are resolved. The experimental results are also compared to the theoretical predictions obtained using the NON-SMOKER and SMARAGD codes. Based on these comparisons an improved set of astrophysical reaction rates is proposed for the (p,γ) reactions on the stable nickel isotopes as well as for the 56Ni(p,γ)57Cu reaction.

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