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A. Stolz

Publications and source records attributed to A. Stolz.

At least 19 recordsLinked to original sources

Abrasion-fission reactions at intermediate energies

The availability of high-intensity, heavy-ion beams coupled to sensitive, large solid-angleacceptance spectrometers has enabled a detailed examination of the fission fragments produced in induced-fission reactions. The abrasion-fission process involves the formation of projectile-like prefragments in violent nuclear collisions at relative energies in excess of 100 MeV/u. At intermediate energies below this threshold, experiments suggest a change in the prefragment kinematic qualities. Information regarding the influence of this transitional phase upon the evolution of nuclei approaching the point of scission is scarce. In this article, data are presented for over 200 nuclei from nickel to palladium produced in abrasion-fission reactions of a 80 MeV/u 238U beam. Cross sections were obtained following yield measurements performed for the principal charge states of the identified fission fragments and a detailed analysis of the ion transmission. A full kinematic analysis of the fission fragments has been performed using the LISE++ software package, where the trajectory of an ion passing through a spectrometer can be reconstructed based upon measurements at the focal plane. The results obtained at the S800 spectrograph are compared with predictions obtained with a three-fission progenitor (3EER) model. Systematic studies of fission-fragment properties continue to provide a valuable experimental benchmark for theoretical efforts directed toward describing this complex decay channel, that is important in the context of planning experiments to explore the neutron-rich region of the nuclear chart at rare-isotope beam facilities.

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Design of the High Rigidity Spectrometer at FRIB

A High Rigidity Spectrometer (HRS) has been designed for experiments at the Facility for Rare-Isotope Beams (FRIB) at Michigan State University (MSU). The HRS will allow experiments to be performed with the most exotic neutron-rich isotopes at high beam energies ($\gtrsim$100MeV/u). The HRS consists of an analysis beamline called the High-Transmission Beamline (HTBL) and the spectrometer proper called the Spectrometer Section. The maximum magnetic rigidity of the HRS is 8Tm, which corresponds to the rigidities at which rare-isotope beams are optimally produced at FRIB. The resolving power, angular acceptance, and momentum acceptance are set to match the anticipated scientific program. An ion-optical design developed for the HRS is described in detail, along with the specifications of the associated magnet and detector systems.

physics.ins-det

Multi-layer Thick Gas Electron Multiplier (M-THGEM): a new MPDG structure for high-gain operation at low-pressure

The operating principle and performances of the Multi-layer Thick Gaseous Electron Multiplier (M-THGEM) is presented. The M-THGEM is a novel hole-type gaseous electron multiplier produced by multi-layer printed circuit board technology; it consists of a densely perforated assembly of multiple insulating substrate sheets (e.g., FR-4), sandwiched between thin metallic-electrode layers. The electron avalanche processes occur along the successive multiplication stages within the M-THGEM holes, under the action of strong dipole fields resulting from the application of suitable potential differences between the electrodes. The present work focuses on investigation of two different geometries: a two-layer M-THGEM (either as single or double-cascade detector) and a single three-layer M-THGEM element, tested in various low-pressure He-based gas mixtures. The intrinsically robust confinement of the avalanche volume within the M-THGEM holes provides an efficient suppression of the photon-induced secondary effects, resulting in a high-gain operation over a broad pressure range, even in pure noble gas. The operational principle, main properties (maximum achievable gain, long-term stability, energy resolution, etc.) under different irradiation conditions, as well as capabilities and potential applications are discussed.

physics.ins-det

Proton spectroscopy of 48Ni, 46Fe, and 44Cr

Results of decay spectroscopy on nuclei in vicinity of the doubly magic 48Ni are presented. The measurements were performed with a Time Projection Chamber with optical readout which records tracks of ions and protons in the gaseous volume. Six decays of 48Ni including four events of two-proton ground-state radioactivity were recorded. An advanced reconstruction procedure yielded the 2p decay energy for 48Ni of Q2p = 1.29(4) MeV. In addition, the energy spectra of \b{eta}-delayed protons emitted in the decays of 44Cr and 46Fe, as well as half-lives and branching ratios were determined. The results were found to be consistent with the previous measurements made with Si detectors. A new proton line in the decay of 44Cr corresponding to the decay energy of 760 keV is reported. The first evidence for the \b{eta}2p decay of 46 Fe, based on one clear event, is shown.

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Nonlinear Optical Rectennas

We introduce strongly-coupled optical gap antennas to interface optical radiation with current-carrying electrons at the nanoscale. The transducer relies on the nonlinear optical and electrical properties of an optical antenna operating in the tunneling regime. We discuss the underlying physical mechanisms controlling the conversion and demonstrate that a two-wire optical antenna can provide advanced optoelectronic functionalities beyond tailoring the electromagnetic response of a single emitter. Interfacing an electronic command layer with a nanoscale optical device may thus be facilitated by the optical rectennas discussed here.

physics.optics

Production cross sections from 82Se fragmentation as indications of shell effects in neutron-rich isotopes close to the drip-line

Production cross sections for neutron-rich nuclei from the fragmentation of a 82Se beam at 139 MeV/u were measured. The longitudinal momentum distributions of 126 neutron-rich isotopes of elements 11 <= Z <= 32 were scanned using an experimental approach of varying the target thickness. Production cross sections with beryllium and tungsten targets were determined for a large number of nuclei including several isotopes first observed in this work. These are the most neutron-rich nuclides of the elements 22 <= Z <= 25 (64Ti, 67V, 69Cr, 72Mn). One event was registered consistent with 70Cr, and another one with 75Fe. The production cross sections are correlated with Qg systematics to reveal trends in the data. The results presented here confirm our previous result from a similar measurement using a 76Ge beam, and can be explained with a shell model that predicts a subshell closure at N = 34 around Z = 20. This is demonstrated by systematic trends and calculations with the Abrasion-Ablation model that are sensitive to separation energies.

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Production cross sections of neutron rich isotopes from a 82Se beam

Production cross sections for neutron-rich nuclei from the fragmentation of a 82Se beam at 139 MeV/u were measured. The longitudinal momentum distributions of 122 neutron-rich isotopes of elements $11 \le Z \le 32$ were determined by varying the target thickness. Production cross sections with beryllium and tungsten targets were determined for a large number of nuclei including several isotopes first observed in this work. These are the most neutron-rich nuclides of the elements $22 \le Z \le 25$ (64Ti, 67V, 69Cr, 72Mn). One event was registered consistent with 70Cr, and another one with 75Fe. A one-body Qg systematics is used to describe the production cross sections based on thermal evaporation from excited prefragments. The current results confirm those of our previous experiment with a 76Ge beam: enhanced production cross sections for neutron-rich fragments near Z=20.

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Beta-delayed proton emission in the 100Sn region

Beta-delayed proton emission from nuclides in the neighborhood of 100Sn was studied at the National Superconducting Cyclotron Laboratory. The nuclei were produced by fragmentation of a 120 MeV/nucleon 112Sn primary beam on a Be target. Beam purification was provided by the A1900 Fragment Separator and the Radio Frequency Fragment Separator. The fragments of interest were identified and their decay was studied with the NSCL Beta Counting System (BCS) in conjunction with the Segmented Germanium Array (SeGA). The nuclei 96Cd, 98Ing, 98Inm and 99In were identified as beta-delayed proton emitters, with branching ratios bp = 5.5(40)%, 5.5+3 -2%, 19(2)% and 0.9(4)%, respectively. The bp for 89Ru, 91,92Rh, 93Pd and 95Ag were deduced for the first time with bp = 3+1.9 -1.7%, 1.3(5)%, 1.9(1)%, 7.5(5)% and 2.5(3)%, respectively. The bp = 22(1)% for 101Sn was deduced with higher precision than previously reported. The impact of the newly measured bp values on the composition of the type-I X-ray burst ashes was studied.

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Beta-decay of nuclei around Se-90. Search for signatures of a N=56 sub-shell closure relevant the r-process

Nuclear structure plays a significant role on the rapid neutron capture process (r-process) since shapes evolve with the emergence of shells and sub-shells. There was some indication in neighboring nuclei that we might find examples of a new N=56 sub-shell, which may give rise to a doubly magic Se-90 nucleus. Beta-decay half lives of nuclei around Se-90 have been measured to determine if this nucleus has in fact a doubly-magic character. The fragmentation of Xe-136 beam at the National Superconducting Cyclotron Laboratory at Michigan State University was used to create a cocktail of nuclei in the A=90 region. We have measured the half lives of twenty-two nuclei near the r-process path in the A=90 region. The half lives of As-88 and Se-90 have been measured for the first time. The values were compared with theoretical predictions in the search for nuclear-deformation signatures of a N=56 sub-shell, and its possible role in the emergence of a potential doubly-magic Se-90. The impact of such hypothesis on the synthesis of heavy nuclei, particularly in the production of Sr, Y and Zr elements was investigated with a weak r-process network. The new half lives agree with results obtained from a standard global QRPA model used in r-process calculations, indicating that Se-90 has a quadrupole shape incompatible with a closed N=56 sub-shell in this region. The impact of the measured Se-90 half-life in comparison with a former theoretical predication associated with a spherical half-life on the weak-r-process is shown to be strong.

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Time-of-flight mass measurements for nuclear processes in neutron star crusts

The location of electron capture heat sources in the crust of accreting neutron stars depends on the masses of extremely neutron-rich nuclei. We present first results from a new implementation of the time-of-flight technique to measure nuclear masses of rare isotopes at the National Superconducting Cyclotron Laboratory. The masses of 16 neutron-rich nuclei in the scandium -- nickel range were determined simultaneously, improving the accuracy compared to previous data in 12 cases. The masses of $^{61}${V}, $^{63}${Cr}, $^{66}${Mn}, and $^{74}${Ni} were measured for the first time with mass excesses of $-30.510(890)$ MeV, $-35.280(650)$ MeV, $-36.900(790)$ MeV, and $-49.210(990)$ MeV, respectively. With the measurement of the $^{66}$Mn mass, the locations of the two dominant electron capture heat sources in the outer crust of accreting neutron stars that exhibit superbursts are now experimentally constrained. We find that the location of the $^{66}$Fe$\rightarrow^{66}$Mn electron capture transition occurs significantly closer to the surface than previously assumed because our new experimental Q-value is 2.1 MeV (2.6$σ$) smaller than predicted by the FRDM mass model.

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High-spin μs isomeric states in 96Ag

The isomeric and β decays of the N = Z +2 nucleus 96Ag were investigated at NSCL. A cascade of γ-ray transitions originating from the de-excitation of a μs isomer was observed for the first time and was found in coincidence with two previously-known transitions with energies of 470 and 667 keV. The isomeric half-life was determined as 1.45(7) μs, more precise than previously reported. The existence of a second, longer-lived μs isomer, associated with a 743-keV transition, is also proposed here. Shell model results within the (p_{3/2}p_{1/2}f_{5/2}g_{9/2}) model space, using the jj44b interaction, reproduced level energies and isomeric decay half-lives reasonably well.

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Beta-Delayed Proton Emission Branches in 43Cr

The beta+ decay of very neutron deficient 43Cr has been studied by means of an imaging time projection chamber which allowed recording tracks of charged particles. Events of beta-delayed emission of one-, two-, and three protons were clearly identified. The absolute branching ratios for these channels were determined to be 81(4)%, 7.1(4)%, and 0.08(3)%, respectively. The 43Cr is thus established as the second case in which the beta-3p decay occurs. Although the feeding to the proton-bound states in 43V is expected to be negligible, the large branching ratio of 12(4)% for decays without proton emission is found.

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Half-lives and branchings for β-delayed neutron emission for neutron-rich Co-Cu isotopes in the r-process

The β decays of very neutron-rich nuclides in the Co-Zn region were studied experimentally at the National Superconducting Cyclotron Laboratory using the NSCL β-counting station in conjunction with the neutron detector NERO. We measured the branchings for β-delayed neutron emission (Pn values) for 74Co (18 +/- 15%) and 75-77Ni (10 +/- 2.8%, 14 +/- 3.6%, and 30 +/- 24%, respectively) for the first time, and remeasured the Pn values of 77-79Cu, 79,81Zn, and 82Ga. For 77-79Cu and for 81Zn we obtain significantly larger Pn values compared to previous work. While the new half-lives for the Ni isotopes from this experiment had been reported before, we present here in addition the first half-life measurements of 75Co (30 +/- 11 ms) and 80Cu (170+110 -50 ms). Our results are compared with theoretical predictions, and their impact on various types of models for the astrophysical rapid neutron-capture process (r-process) is explored. We find that with our new data, the classical r-process model is better able to reproduce the A = 78-80 abundance pattern inferred from the solar abundances. The new data also influence r-process models based on the neutrino-driven high-entropy winds in core collapse supernovae.

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Production of very neutron-rich nuclei with a 76Ge beam

Production cross sections for neutron-rich nuclei from the fragmentation of a 76Ge beam at 132 MeV/u were measured. The longitudinal momentum distributions of 34 neutron-rich isotopes of elements 13 <= Z <= 27 were scanned using a novel experimental approach of varying the target thickness. Production cross sections with beryllium and tungsten targets were determined for a large number of nuclei including 15 isotopes first observed in this work. These are the most neutron-rich nuclides of the elements 17 <= Z <= 25 (50Cl, 53Ar, 55,56K, 57,58Ca, 59,60,61Sc, 62,63Ti, 65,66V, 68Cr,70Mn). A one-body Qg systematics is used to describe the production cross sections based on thermal evaporation from excited prefragments. Some of the fragments near 58Ca show anomalously large production cross sections.

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Evidence for a change in the nuclear mass surface with the discovery of the most neutron-rich nuclei with 17<Z <25

The results of measurements of the production of neutron-rich nuclei by the fragmentation of a 76-Ge beam are presented. The cross sections were measured for a large range of nuclei including fifteen new isotopes that are the most neutron-rich nuclides of the elements chlorine to manganese (50-Cl, 53-Ar, 55,56-K, 57,58-Ca, 59,60,61-Sc, 62,63-Ti, 65,66-V, 68-Cr, 70-Mn). The enhanced cross sections of several new nuclei relative to a simple thermal evaporation framework, previously shown to describe similar production cross sections, indicates that nuclei in the region around 62-Ti might be more stable than predicted by current mass models and could be an indication of a new island of inversion similar to that centered on 31-Na.

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Beta-decay half-lives and beta-delayed neutron emission probabilities of nuclei in the region below A=110, relevant for the r-process

Measurements of the beta-decay properties of r-process nuclei below A=110 have been completed at the National Superconducting Cyclotron Laboratory, at Michigan State University. Beta-decay half-lives for Y-105, Zr-106,107 and Mo-111, along with beta-delayed neutron emission probabilities of Y-104, Mo-109,110 and upper limits for Y-105, Zr-103,104,105,106,107 and Mo-108,111 have been measured for the first time. Studies on the basis of the quasi-random phase approximation are used to analyze the ground-state deformation of these nuclei.

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New isotope 44Si and systematics of the production cross sections of the most neutron-rich nuclei

The results of measurements of the production of neutron-rich nuclei by the fragmentation of a 48Ca beam at 142 MeV/u are presented. Evidence was found for the production of a new isotope that is the most neutron-rich silicon nuclide, 44Si, in a net neutron pick-up process. A simple systematic framework was found to describe the production cross sections based on thermal evaporation from excited prefragments that allows extrapolation to other weak reaction products.

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Projectile Fragmentation of $^{86}$Kr at 64 MeV/nucleon

We measured fragmentation cross sections produced using the primary beam of $^{86}$Kr at 64 MeV/nucleon on $^9$Be and $^{181}$Ta targets. The cross sections were obtained by integrating the momentum distributions of isotopes with 25<Z<36 measured using the RIPS fragment separator at RIKEN. The cross-section ratios obtained with the $^{181}$Ta and $^{9}$Be targets depend on the fragment masses, contrary to the simple geometrical models. We compared the extracted cross sections to EPAX; an empirical parameterization of fragmentation cross sections. Predictions from current EPAX parameterization severely overestimate the production cross sections of very neutron-rich isotopes. Attempts to obtain another set of EPAX parameters specific to the reaction studied here, to extrapolate the neutron-rich nuclei more accurately have not been very successful, suggesting that accurate predictions of production cross sections of nuclei far from the valley of stability require information of nuclear properties which are not present in EPAX.

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