arXiv subjects

A. T. Bollinger

Publications and source records attributed to A. T. Bollinger.

14 recordsLinked to original sources

arXiv2022

Single-photon detection using high-temperature superconductors

The detection of individual quanta of light is important for quantum computation, fluorescence lifetime imaging, single-molecule detection, remote sensing, correlation spectroscopy, and more. Thanks to their broadband operation, high detection efficiency, exceptional signal-to-noise ratio, and fast recovery times, superconducting nanowire single-photon detectors (SNSPDs) have become a critical component in these applications. The operation of SNSPDs based on conventional superconductors, which have a low critical temperature ($T_c$), requires costly and bulky cryocoolers. This motivated exploration of other superconducting materials with higher $T_c$ that would enable single-photon detection at elevated temperatures, yet this task has proven exceedingly difficult. Here we show that with proper processing, high-$T_c$ cuprate superconductors can meet this challenge. We fabricated superconducting nanowires (SNWs) out of thin flakes of Bi$_2$Sr$_2$CaCu$_2$O$_{8+δ}$ and La$_{1.55}$Sr$_{0.45}$CuO$_4$/La$_2$CuO$_4$ (LSCO-LCO) bilayer films and demonstrated their single-photon response up to $25$ and $8$ K, respectively. The single-photon operation is revealed through the linear scaling of the photon count rate (PCR) on the radiation power. Both of our cuprate-based SNSPDs exhibited single-photon sensitivity at the technologically-important $1.5$ $μ$m telecommunications wavelength. Our work expands the family of superconducting materials for SNSPD technology, opens the prospects of raising the temperature ceiling, and raises important questions about the underlying mechanisms of single-photon detection by unconventional superconductors.

cond-mat.supr-con↗

arXiv2022

Colossal transverse magnetoresistance due to nematic superconducting phase fluctuations in a copper oxide

Electronic anisotropy (or `nematicity') has been detected in all main families of cuprate superconductors by a range of experimental techniques -- electronic Raman scattering, THz dichroism, thermal conductivity, torque magnetometry, second-harmonic generation -- and was directly visualized by scanning tunneling microscope (STM) spectroscopy. Using angle-resolved transverse resistance (ARTR) measurements, a very sensitive and background-free technique that can detect 0.5$\%$ anisotropy in transport, we have observed it also in La$_{2-x}$Sr$_{x}$CuO$_{4}$ (LSCO) for $0.02 \leq x \leq 0.25$. Arguably the key enigma in LSCO is the rotation of the nematic director with temperature; this has not been seen before in any material. Here, we address this puzzle by measuring the angle-resolved transverse magnetoresistance (ARTMR) in LSCO. We report a discovery of colossal transverse magnetoresistance (CTMR) -- an order-of-magnitude drop in the transverse resistivity in the magnetic field of $6\,$T, while none is seen in the longitudinal resistivity. We show that the apparent rotation of the nematic director is caused by superconducting phase fluctuations, which are much more anisotropic than the normal-electron fluid, and their respective directors are not parallel. This qualitative conclusion is robust and follows straight from the raw experimental data. We quantify this by modelling the measured (magneto-)conductivity by a sum of two conducting channels that correspond to distinct anisotropic Drude and Cooper-pair effective mass tensors. Strikingly, the anisotropy of Cooper-pair stiffness is significantly larger than that of the normal electrons, and it grows dramatically on the underdoped side, where the fluctuations become effectively quasi-one dimensional.

cond-mat.supr-con↗

arXiv2020

Surface Josephson plasma waves in a high-temperature superconductor

Electron density oscillations with acoustic dispersions and sustained at boundaries between different media provide information about surface and interface properties of hetero-structures. In ultra-thin metallic films these plasmonic excitations are heavily damped. Superconductivity is predicted to reduce dissipation allowing detection of these resonances. Emerging low-loss interface Cooper-pair waves have been studied before, however, the observation of surface-confined Josephson plasmons has remained elusive. Here, we report on generation and coupling to these excitations in an ultrathin single-crystal film of high-temperature superconductor La1.85Sr0.15CuO4. The film becomes brighter than Au below the critical temperature when probed with sub-gap THz photons. We show that the enhanced signal in the superconducting state, which can be visualized with a spatial resolution better than λ/3,000, originates from near-field coupling of light to surface Josephson plasmons. Our results open a path towards non-invasive investigation of enhanced superconductivity in artificial multilayers, buried interface states in topological hetero-structures, and non-linear phenomena in Josephson devices.

cond-mat.supr-con↗

arXiv2018

Scale-invariant magnetoresistance in a cuprate superconductor

The anomalous metallic state in high-temperature superconducting cuprates is masked by the onset of superconductivity near a quantum critical point. Use of high magnetic fields to suppress superconductivity has enabled a detailed study of the ground state in these systems. Yet, the direct effect of strong magnetic fields on the metallic behavior at low temperatures is poorly understood, especially near critical doping, $x=0.19$. Here we report a high-field magnetoresistance study of thin films of \LSCO cuprates in close vicinity to critical doping, $0.161\leq x\leq0.190$. We find that the metallic state exposed by suppressing superconductivity is characterized by a magnetoresistance that is linear in magnetic field up to the highest measured fields of $80$T. The slope of the linear-in-field resistivity is temperature-independent at very high fields. It mirrors the magnitude and doping evolution of the linear-in-temperature resistivity that has been ascribed to Planckian dissipation near a quantum critical point. This establishes true scale-invariant conductivity as the signature of the strange metal state in the high-temperature superconducting cuprates.

cond-mat.str-el↗

arXiv2017

Insulator to Metal Transition in WO$_3$ Induced by Electrolyte Gating

Tungsten oxide and its associated bronzes (compounds of tungsten oxide and an alkali metal) are well known for their interesting optical and electrical characteristics. We have modified the transport properties of thin WO$_3$ films by electrolyte gating using both ionic liquids and polymer electrolytes. We are able to tune the resistivity of the gated film by more than five orders of magnitude, and a clear insulator-to-metal transition is observed. To clarify the doping mechanism, we have performed a series of incisive operando experiments, ruling out both a purely electronic effect (charge accumulation near the interface) and oxygen-related mechanisms. We propose instead that hydrogen intercalation is responsible for doping WO$_3$ into a highly conductive ground state and provide evidence that it can be described as a dense polaronic gas.

cond-mat.supr-con↗

arXiv2012

Emergence of superconductivity from the dynamically heterogeneous insulating state in La_{2-x}Sr_{x}CuO_{4}

A central issue for copper oxides is the nature of the insulating ground state at low carrier densities and the emergence of high-temperature superconductivity from that state with doping. Even though this superconductor-insulator transition (SIT) is a zero-temperature transition, measurements are not usually carried out at low temperatures. Here we use magnetoresistance to probe both the insulating state at very low temperatures and the presence of superconducting fluctuations in La_{2-x}Sr_{x}CuO_{4}(LSCO) films, for doping levels that range from the insulator to the superconductor (x=0.03-0.08). We observe that the charge glass behavior, characteristic of the insulating state, is suppressed with doping, but it coexists with superconducting fluctuations that emerge already on the insulating side of the SIT. The unexpected quenching of the superconducting fluctuations by the competing charge order at low temperatures provides a new perspective on the mechanism for the SIT.

cond-mat.supr-con↗

arXiv2011

History dependent magnetoresistance in lightly doped La_{2-x}Sr_{x}CuO_{4} thin films

The in-plane magnetoresistance (MR) in atomically smooth La_{2-x}Sr_{x}CuO_{4} thin films grown by molecular-beam-epitaxy was measured in magnetic fields B up to 9 T over a wide range of temperatures T. The films, with x=0.03 and x=0.05, are insulating, and the positive MR emerges at T<4 K. The positive MR exhibits glassy features, including history dependence and memory, for all orientations of B. The results show that this behavior, which reflects the onset of glassiness in the dynamics of doped holes, is a robust feature of the insulating state.

cond-mat.str-el↗

arXiv2008

High-temperature interface superconductivity between metallic and insulating cuprates

High-temperature superconductivity confined to nanometer-size interfaces has been a long standing goal because of potential applications^{1,2} and the opportunity to study quantum phenomena in reduced dimensions^{3,4}. However, this is a challenging target: in conventional metals the high electron density restricts interface effects such as carrier depletion/accumulation to a region much narrower than the coherence length, the scale necessary for superconductivity to occur. In contrast, in copper oxides the carrier density is low while the critical temperature (T_c) is high and the coherence length very short; so, this provides a breakthrough opportunity but at a price: the interface must be atomically perfect. Here we report on superconductivity in bilayers consisting of an insulator (La_2CuO_4) and a metal (La_{1.55}Sr_{0.45}CuO_{4}), neither of which is superconducting in isolation. However, in bilayers T_c is either ~15 K or ~30 K, depending on the layering sequence. This highly robust phenomenon is confined within 2-3 nm from the interface. If such a bilayer is exposed to ozone, T_c exceeds 50 K and this enhanced superconductivity is also shown to originate from the interface layer about 1-2 unit cell thick. Enhancement of T_c in bilayer systems was observed previously^5 but the essential role of the interface was not recognized at the time. Our results demonstrate that engineering artificial heterostructures provides a novel, unconventional way to fabricate stable, quasi two-dimensional high T_c phases and to significantly enhance superconducting properties in known or new superconductors.

cond-mat.supr-con↗

arXiv2008

Determination of the Superconductor-Insulator Phase Diagram for One-Dimensional Wires

We establish the superconductor-insulator phase diagram for quasi-one dimensional wires by measuring a large set of MoGe nanowires. This diagram is consistent with the Chakravarty-Schmid-Bulgadaev phase boundary, namely with the critical resistance being equal to R_Q = h/4e^2. We find that transport properties of insulating nanowires exhibit a weak Coulomb blockade behavior.

cond-mat.supr-con↗

arXiv2006

Dichotomy in short superconducting nanowires: thermal phase slippage vs. Coulomb blockade

Quasi-one-dimensional superconductors or nanowires exhibit a transition into a nonsuperconducting regime, as their diameter shrinks. We present measurements on ultrashort nanowires (~40-190 nm long) in the vicinity of this quantum transition. Properties of all wires in the superconducting phase, even those close to the transition, can be explained in terms of thermally activated phase slips. The behavior of nanowires in the nonsuperconducting phase agrees with the theories of the Coulomb blockade of coherent transport through mesoscopic normal metal conductors. Thus it is concluded that the quantum transition occurs between two phases: a "true superconducting phase" and an "insulating phase". No intermediate, "metallic" phase was found.

cond-mat.supr-con↗

arXiv2006

Magnetic field enhancement of superconductivity in ultra-narrow wires

We study the effect of an applied magnetic field on sub-10nm wide MoGe and Nb superconducting wires. We find that magnetic fields can enhance the critical supercurrent at low temperatures, and does so more strongly for narrower wires. We conjecture that magnetic moments are present, but their pair-breaking effect, active at lower magnetic fields, is suppressed by higher fields. The corresponding microscopic theory, which we have developed, quantitatively explains all experimental observations, and suggests that magnetic moments have formed on the wire surfaces.

cond-mat.supr-con↗

arXiv2004

Influence of high magnetic fields on superconducting transition of one-dimensional Nb and MoGe nanowires

The effects of strong magnetic field on superconducting Nb and MoGe nanowires with diameter $\sim10$ nm have been studied. We have found that the Langer-Ambegaokar-McCumber-Halperin (LAMH) theory of thermally activated phase slips is applicable in a wide range of magnetic fields and describes well the temperature dependence of the wire resistance, over eleven orders of magnitude. The field dependence of the critical temperature, $T_{c}$, extracted from the LAMH fits is in good quantitative agreement with the theory of pair-breaking perturbations that takes into account both spin and orbital contributions. The extracted spin-orbit scattering time agrees with an estimate $τ_{so}\simeq τ(\hbar c/ Ze^{2})^{4}$, where $τ$ is the elastic scattering time and $Z$ is the atomic number.

cond-mat.supr-con↗

arXiv2004

Phase slips in superconducting films with constrictions

A system of two coplanar superconducting films seamlessly connected by a bridge is studied. We observe two distinct resistive transitions as the temperature is reduced. The first one, occurring in the films, shows some properties of the Berezinskii-Kosterlitz-Thouless (BKT) transition. The second apparent transition (which is in fact a crossover) is related to freezing out of thermally activated phase slips (TAPS) localized on the bridge. We also propose a powerful indirect experimental method allowing an extraction of the sample's zero-bias resistance from high-current-bias measurements. Using direct and indirect measurements, we determined the resistance $R(T)$ of the bridges within a range of {\em eleven orders of magnitude}. Over such broad range, the resistance follows a simple relation $R(T)=R_N \text{exp} [-(c/t)(1-t)^{3/2}]$, where $c=ΔF(0) / kT_c$ is the normalized free energy of a phase slip at zero temperature, $t=T/T_c$ is normalized temperature, and $R_N$ is the normal resistance of the bridge.

cond-mat.supr-con↗

arXiv2004

The effect of morphology on the superconductor-insulator transition in 1-D nanowires

We study the effect of morphology on the low temperature behavior of superconducting nanowires of length $\approx$100 nm. A well-defined superconductor-insulator transition (SIT) is observed only in homogenous wires, in which case the transition occurs when the normal resistance is close to $h/4e^2$. Inhomogeneous wires, on the other hand, exhibit a mixed behavior, such that signatures of the superconducting and insulating regimes can be observed in the same sample. The resistance versus temperature curves of inhomogeneous wires show multiple steps, each corresponding to a weak link constriction (WLC) present in the wire. Similarly, each WLC generates a differential resistance peak when the bias current reaches the critical current of the WLC. Due to the presence of WLCs an inhomogeneous wire splits into a sequence of weakly interacting segments where each segment can act as a superconductor or as an insulator. Thus the entire wire then shows a mixed behavior.

cond-mat.supr-con↗