arXiv subjects

A. V. Plyukhin

Publications and source records attributed to A. V. Plyukhin.

15 recordsLinked to original sources

arXiv2019

Fractional Langevin equation from damped bath dynamics

We consider the stochastic dynamics of a system linearly coupled to a hierarchical thermal bath with two well-separated inherent timescales: one slow, and one fast. The slow part of the bath is modeled as a set of harmonic oscillators and taken into account explicitly, while the effects of the fast part of the bath are simulated by dissipative and stochastic Langevin forces, uncorrelated in space and time, acting on oscillators of the slow part of the bath. We demonstrate for this model the robust emergence of a fractional Langevin equation with a power-law decaying memory kernel. The conditions of such an emergence and the specific value of the fractional exponent depend only on the asymptotic low-frequency spectral properties of the slow part of the bath.

cond-mat.stat-mech↗

arXiv2018

Intrinsic ratchets: A Hamiltonian approach

An asymmetric Brownian particle subjected to an external time-dependent force may acquire a net drift velocity, and thus operate as a motor or ratchet, even if the external force is represented by an unbiased time-periodic function or by a zero-centered noise. For an adequate description of such ratchets, a conventional Langevin equation linear in the particle's velocity is insufficient, and one needs to take into account the first nonlinear correction to the dissipation force which emerges beyond the weak coupling limit. We derived microscopically the relevant nonlinear Langevin equation by extending the standard projection operation technique beyond the weak coupling limit. The particle is modeled as a rigid cluster of atoms and its asymmetry may be geometrical, compositional (when a cluster is composed of atoms of different types), or due to a combination of both factors. The drift velocity is quadratic in the external force's amplitude and increases with decreasing the force's frequency (for a periodic force) and inverse correlation time (for a fluctuating force). The maximum value of the drift velocity is independent on the particle's mass and achieved in the adiabatic limit, i.e. for an infinitely slow change of the external field.

cond-mat.stat-mech↗

arXiv2015

Autonomous Brownian motor driven by nonadiabatic variation of internal parameters

We discuss an autonomous motor based on a Brownian particle driven from thermal equilibrium by periodic in time variation of the internal potential through which the particle interacts with molecules of the surrounding thermal bath. We demonstrate for such a motor the absence of a linear response regime: The average driving force and drift velocity are shown to be quadratic in both the frequency and amplitude of the variation. The adiabatic approximation (of an infinitely slow variation) and the leading correction to it (linear in the variation's frequency) both lead to zero drift and are insufficient to describe the motor's operation.

cond-mat.stat-mech↗

arXiv2013

Quasirelativistic Langevin equation

We address the problem of a microscopic derivation of the Langevin equation for a weakly relativistic Brownian particle. A non-covariant Hamiltonian model is adopted, in which the free motion of particles is described relativistically, while their interaction is treated classically, i.e. by means of action-to-a-distance interaction potentials. Relativistic corrections to the classical Langevin equation emerge as nonlinear dissipation terms and originate from the nonlinear dependence of the relativistic velocity on momentum. On the other hand, similar nonlinear dissipation forces also appear as classical (non-relativistic) corrections to the weak-coupling approximation. It is shown that these classical corrections, which are usually ignored in phenomenological models, may be of the same order of magnitude, if not larger than relativistic ones. The interplay of relativistic corrections and classical beyond-the-weak-coupling contributions determines the sign of the leading nonlinear dissipation term in the Langevin equation, and thus is qualitatively important.

cond-mat.stat-mech↗

arXiv2013

Brownian diode: Molecular motor based on a semi-permeable Brownian particle with internal potential drop

A model of an autonomous isothermal Brownian motor with an internal propulsion mechanism is considered. The motor is a Brownian particle which is semi-transparent for molecules of surrounding ideal gas. Molecular passage through the particle is controlled by a potential similar to that in the transition rate theory, i.e. characterized by two stationary states with a finite energy difference separated by a potential barrier. The internal potential drop maintains the diode-like asymmetry of molecular fluxes through the particle, which results in the particle's stationary drift.

cond-mat.stat-mech↗

arXiv2012

Stochastic dynamics beyond the weak coupling limit: thermalization

We discuss the structure and asymptotic long-time properties of coupled equations for the moments of a Brownian particle's momentum derived microscopically beyond the lowest approximation in the weak coupling parameter. Generalized fluctuation-dissipation relations are derived and shown to ensure convergence to thermal equilibrium at any order of perturbation theory.

cond-mat.stat-mech↗

arXiv2011

Nonergodic solutions of the generalized Langevin equation

It is known that in the regime of superlinear diffusion, characterized by zero integral friction (vanishing integral of the memory function), the generalized Langevin equation may have non-ergodic solutions which do not relax to equilibrium values. It is shown that the equation may have non-ergodic (non-stationary) solutions even if the integral of the memory function is finite and diffusion is normal.

cond-mat.stat-mech↗

arXiv2010

Stochastic process leading to wave equations in dimensions higher than one

Stochastic processes are proposed whose master equations coincide with classical wave, telegraph, and Klein-Gordon equations. Similar to predecessors based on the Goldstein-Kac telegraph process, the model describes the motion of particles with constant speed and transitions between discreet allowed velocity directions. A new ingredient is that transitions into a given velocity state depend on spatial derivatives of other states populations, rather than on populations themselves. This feature requires the sacrifice of the single-particle character of the model, but allows to imitate the Huygens' principle and to recover wave equations in arbitrary dimensions.

cond-mat.stat-mech↗

arXiv2009

Thermophoresis as persistent random walk

In a simple model of a continuous random walk a particle moves in one dimension with the velocity fluctuating between V and -V. If V is associated with the thermal velocity of a Brownian particle and allowed to be position dependent, the model accounts readily for the particle's drift along the temperature gradient and recovers basic results of the conventional thermophoresis theory.

cond-mat.stat-mech↗

arXiv2008

Generalized Fokker-Planck equation, Brownian motion, and ergodicity

Microscopic theory of Brownian motion of a particle of mass $M$ in a bath of molecules of mass $m\ll M$ is considered beyond lowest order in the mass ratio $m/M$. The corresponding Langevin equation contains nonlinear corrections to the dissipative force, and the generalized Fokker-Planck equation involves derivatives of order higher than two. These equations are derived from first principles with coefficients expressed in terms of correlation functions of microscopic force on the particle. The coefficients are evaluated explicitly for a generalized Rayleigh model with a finite time of molecule-particle collisions. In the limit of a low-density bath, we recover the results obtained previously for a model with instantaneous binary collisions. In general case, the equations contain additional corrections, quadratic in bath density, originating from a finite collision time. These corrections survive to order $(m/M)^2$ and are found to make the stationary distribution non-Maxwellian. Some relevant numerical simulations are also presented.

cond-mat.stat-mech↗

arXiv2008

Quasi-one-dimensional disordered systems: fluctuations, transport and interplay

In a one dimensional lattice thermal fluctuations destroy the long-range order making particles of the lattice move on a scale much larger than the lattice spacing. We discuss the assumption that this motion may be responsible for the transport of localized electrons in a system of weakly coupled chains. The model with diffusing localization sites gives a temperature-independent mobility with a crossover to an activated dependence at high temperature. This prediction is consistent with and might account for experimental results on discotic liquid crystals and certain biopolymers.

cond-mat.soft↗

arXiv2007

Transient rectification of Brownian diffusion with asymmetric initial distribution

In an ensemble of non-interacting Brownian particles, a finite systematic average velocity may temporarily develop, even if it is zero initially. The effect originates from a small nonlinear correction to the dissipative force, causing the equation for the first moment of velocity to couple to moments of higher order. The effect may be relevant when a complex system dissociates in a viscous medium with conservation of momentum.

cond-mat.stat-mech↗

arXiv2006

Does a Brownian particle equilibrate?

The conventional equations of Brownian motion can be derived from the first principles to order $λ^2=m/M$, where $m$ and $M$ are the masses of a bath molecule and a Brownian particle respectively. We discuss the extension to order $λ^4$ using a perturbation analysis of the Kramers-Moyal expansion. For the momentum distribution such method yields an equation whose stationary solution is inconsistent with Boltzmann-Gibbs statistics. This property originates entirely from non-Markovian corrections which are negligible in lowest order but contribute to order $λ^4$.

cond-mat.stat-mech↗

arXiv2005

Hitchhiking transport in quasi-one-dimensional systems

In the conventional theory of hopping transport the positions of localized electronic states are assumed to be fixed, and thermal fluctuations of atoms enter the theory only through the notion of phonons. On the other hand, in 1D and 2D lattices, where fluctuations prevent formation of long-range order, the motion of atoms has the character of the large scale diffusion. In this case the picture of static localized sites may be inadequate. We argue that for a certain range of parameters, hopping of charge carriers among localization sites in a network of 1D chains is a much slower process than diffusion of the sites themselves. Then the carriers move through the network transported along the chains by mobile localization sites jumping occasionally between the chains. This mechanism may result in temperature independent mobility and frequency dependence similar to that for conventional hopping.

cond-mat.dis-nn↗

arXiv2005

On the higher order corrections to the Fokker-Planck equation

The Rayleigh model of nonlinear Brownian motion is revisited in which the heavy particle of mass M interacts with ideal gas molecules of mass m via instantaneous collisions. Using the van Kampen method of expansion of the master equation, non-linear corrections to the Fokker-Planck equation are obtained up to sixth order in the small parameter m/M, improving earlier results. The role and origin of non-Gaussian statistics of the random force in the corresponding Langevin equation are also discussed.

cond-mat.stat-mech↗