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A. V. Poshakinskiy

Publications and source records attributed to A. V. Poshakinskiy.

At least 37 records · Page 2Linked to original sources

Excitation and coherent control of spin qudit modes with sub-MHz spectral resolution

Quantum bit or qubit is a two-level system, which builds the foundation for quantum computation, simulation, communication and sensing. Quantum states of higher dimension, i.e., qutrits (D = 3) and especially qudits (D = 4 or higher), offer significant advantages. Particularly, they can provide noise-resistant quantum cryptography, simplify quantum logic and improve quantum metrology. Flying and solid-state qudits have been implemented on the basis of photonic chips and superconducting circuits, respectively. However, there is still a lack of room-temperature qudits with long coherence time and high spectral resolution. The silicon vacancy centers in silicon carbide (SiC) with spin S = 3/2 are quite promising in this respect, but until now they were treated as a canonical qubit system. Here, we apply a two-frequency protocol to excite and image multiple qudit modes in a SiC spin ensemble under ambient conditions. Strikingly, their spectral width is about one order of magnitude narrower than the inhomogeneous broadening of the corresponding spin resonance. By applying Ramsey interferometry to these spin qudits, we achieve a spectral selectivity of 600 kHz and a spectral resolution of 30 kHz. As a practical consequence, we demonstrate absolute DC magnetometry insensitive to thermal noise and strain fluctuations.

quant-ph↗

Optomechanical Kerker effect

Tunable directional scattering is of paramount importance for operation of antennas, routing of light, and design of topologically protected optical states. For visible light scattered on a nanoparticle the directionality could be provided by the Kerker effect, exploiting the interference of electric and magnetic dipole emission patterns. However, magnetic optical resonances in small sub-100-nm particles are relativistically weak. Here, we predict inelastic scattering with the unexpectedly strong tunable directivity up to 5.25 driven by a trembling of small particle without any magnetic resonance. The proposed optomechanical Kerker effect originates from the vibration-induced multipole conversion. We also put forward an optomechanical spin Hall effect, the inelastic polarization-dependent directional scattering. Our results uncover an intrinsically multipolar nature of the interaction between light and mechanical motion. They apply to a variety of systems from cold atoms to two-dimensional materials to superconducting qubits and can be instructive to engineer chiral optomechanical coupling.

physics.optics↗

Multiwall nanotubes of molybdenum disulfide as optical resonators

We study the optical properties of MoS$_2$ nanotubes (NTs) with walls comprising dozens of monolayers. We reveal strong peaks in micro-photoluminescence ($μ$-PL) spectra when detecting the light polarized along the NT axis. We develop a model describing the optical properties of the nanotubes acting as optical resonators which support the quantization of whispering gallery modes inside the NT wall. The experimental observation of the resonances in $μ$-PL allows one to use them as a contactless method of the estimation of the wall width. Our findings open a way to use such NTs as polarization-sensitive components of nanophotonic devices.

cond-mat.mes-hall↗

Persistent Spin Helix Manipulation by Optical Doping of a CdTe Quantum Well

Time-resolved Kerr-rotation microscopy explores the influence of optical doping on the persistent spin helix in a [001]-grown CdTe quantum well at cryogenic temperatures. Electron spin diffusion dynamics reveal a momentum-dependent effective magnetic field providing SU(2) spin-rotation symmetry, consistent with kinetic theory. The Dresselhaus and Rashba spin-orbit coupling parameters are extracted independently from rotating the spin helix with external magnetic fields applied parallel and perpendicular to the effective magnetic field. Most importantly, a non-uniform spatiotemporal precession pattern is observed. The kinetic theory framework of spin diffusion allows for modeling of this finding by incorporating the photocarrier density into the Rashba ($α$) and the Dresselhaus ($β_3$) parameters. Corresponding calculations are further validated by an excitation-density dependent measurement. This work shows universality of the persistent spin helix by its observation in a II-VI compound and the ability to fine-tune it by optical doping.

cond-mat.mes-hall↗

Gate-Control of Anisotropic Spin Transport and Spin Helix Dynamics in a Modulation-Doped GaAs Quantum Well

Electron spin transport and dynamics are investigated in a single, high-mobility, modulation-doped, GaAs quantum well using ultrafast two-color Kerr-rotation micro-spectroscopy, supported by qualitative kinetic theory simulations of spin diffusion and transport. Evolution of the spins is governed by the Dresselhaus bulk and Rashba structural inversion asymmetries, which manifest as an effective magnetic field that can be extracted directly from the experimental coherent spin precession. A spin precession length L-SOI is defined as one complete precession in the effective magnetic field. It is observed that application of (a) an out-of-plane electric field changes the spin decay time and L-SOI through the Rashba component of the spin-orbit coupling, (b) an in-plane magnetic field allows for extraction of the Dresselhaus and Rashba parameters, and (c) an in-plane electric field markedly modifies both the L-SOI and diffusion coefficient. While simulations reproduce the main features of the experiments, the latter results exceed the corresponding simulations and extend previous studies of drift-current-dependent spin-orbit interactions.

cond-mat.mes-hall↗

Resonant photonic crystals based on van der Waals heterostructures

We propose to use 2D monolayers possessing optical gaps and high exciton oscillator strength as an element of one-dimensional resonant photonic crystals. We demonstrate that such systems are promising for the creation of effective and compact delay units. In the transition-metal-dichalcogenide-based structures where the frequencies of Bragg and exciton resonances are close, a propagating short pulse can be slowed down by few picoseconds while the pulse intensity decreases only 2 - 5 times. This is realized at the frequency of the "slow" mode situated within the stopband. The pulse retardation and attenuation can be controlled by detuning the Bragg frequency from the exciton resonance frequency.

cond-mat.mtrl-sci↗

Spin and optical properties of silicon vacancies in silicon carbide (a review)

We discuss the fine structure and spin dynamics of spin-3/2 centers associated with silicon vacancies in silicon carbide. The centers have optically addressable spin states which makes them highly promising for quantum technologies. The fine structure of the spin centers turns out to be highly sensitive to mechanical pressure, external magnetic and electric fields, temperature variation, etc., which can be utilized for efficient room-temperature sensing, particularly by purely optical means or through the optically detected magnetic resonance. We discuss the experimental achievements in magnetometry and thermometry based on the spin state mixing at level anticrossings in an external magnetic field and the underlying microscopic mechanisms. We also discuss spin fluctuations in an ensemble of vacancies caused by interaction with environment.

cond-mat.mes-hall↗

Coherent Electron Zitterbewegung

Zitterbewegung is a striking consequence of relativistic quantum mechanics which predicts that free Dirac electrons exhibit a rapid trembling motion even in the absence of external forces. The trembling motion of an electron results from the interference between the positive and the negative-energy solutions of the Dirac equation, separated by one MeV, leading to oscillations at extremely high frequencies which are out of reach experimentally. Recently, it was shown theoretically that electrons in III-V semiconductors are governed by similar equations in the presence of spin-orbit coupling. The small energy splittings up to meV result in Zitterbewegung at much smaller frequencies which should be experimentally accessible as an AC current. Here, we demonstrate the Zitterbewegung of electrons in a solid. We show that coherent electron Zitterbewegung can be triggered by initializing an ensemble of electrons in the same spin states in strained n-InGaAs and is probed as an AC current at GHz frequencies. Its amplitude is shown to increase linearly with both the spin-orbit coupling strength and the Larmor frequency of the external magnetic field. The latter dependence is the hallmark of the dynamical generation mechanism of the oscillatory motion of the Zitterbewegung. Our results demonstrate that relativistic quantum mechanics can be studied in a rather simple solid state system at moderate temperatures. Furthermore, the large amplitude of the AC current at high precession frequencies enables ultra-fast spin sensitive electric read-out in solids.

cond-mat.mes-hall↗

Phonoritonic crystals with synthetic magnetic field for acoustic diode

We develop a rigorous theoretical framework to describe light-sound interaction in the laser-pumped periodic multiple-quantum-well structure accounting for the hybrid phonon-polariton excitations, termed as phonoritons. We show that phonoritons exhibit the pumping-induced synthetic magnetic field in the artificial "coordinate-energy" space, that makes transmission of left- and right- going waves different. The transmission nonreciprocity allows to use such phonoritonic crystals with realistic parameters as optically controlled nanoscale acoustic diodes.

cond-mat.mes-hall↗

Multiple quantum wells for PT-symmetric phononic crystals

We demonstrate that the parity-time symmetry for sound is realized in the laser-pumped multiple-quantum-well structure. Breaking of the parity-time symmetry for the phonons with wave vectors corresponding to the Bragg condition makes the structure a highly-selective acoustic wave amplifier. Single-mode distributed feedback phonon lasing is predicted for structures with realistic parameters.

cond-mat.mes-hall↗

All-optical dc nanotesla magnetometry using silicon vacancy fine structure in isotopically purified silicon carbide

We uncover the fine structure of a silicon vacancy in isotopically purified silicon carbide (4H-$^{28}$SiC) and find extra terms in the spin Hamiltonian, originated from the trigonal pyramidal symmetry of this spin-3/2 color center. These terms give rise to additional spin transitions, which are otherwise forbidden, and lead to a level anticrossing in an external magnetic field. We observe a sharp variation of the photoluminescence intensity in the vicinity of this level anticrossing, which can be used for a purely all-optical sensing of the magnetic field. We achieve dc magnetic field sensitivity of 87 nT Hz$^{-1/2}$ within a volume of $3 \times 10^{-7}$ mm$^{3}$ at room temperature and demonstrate that this contactless method is robust at high temperatures up to at least 500 K. As our approach does not require application of radiofrequency fields, it is scalable to much larger volumes. For an optimized light-trapping waveguide of 3 mm$^{3}$ the projection noise limit is below 100 fT Hz$^{-1/2}$.

cond-mat.mtrl-sci↗

Spatiotemporal spin fluctuations caused by spin-orbit-coupled Brownian motion

We develop a theory of thermal fluctuations of spin density emerging in a two-dimensional electron gas. The spin fluctuations probed at spatially separated spots of the sample are correlated due to Brownian motion of electrons and spin-obit coupling. We calculate the spatiotemporal correlation functions of the spin density for both ballistic and diffusive transport of electrons and analyze them for different types of spin-orbit interaction including the isotropic Rashba model and persistent spin helix regime. The measurement of spatial spin fluctuations provides direct access to the parameters of spin-orbit coupling and spin transport in conditions close to the thermal equilibrium.

cond-mat.mes-hall↗

Phase spectroscopy of topological invariants in photonic crystals

We propose a method of measuring topological invariants of a photonic crystal through phase spectroscopy. We show how the Chern numbers can be deduced from the winding numbers of the reflection coefficient phase. An explicit proof of existence of edge states in system with nonzero reflection phase winding number is given. The method is illustrated for one- and two-dimensional photonic crystals of nontrivial topology.

cond-mat.mes-hall↗

Excitation of spin density and current by coherent light pulses in QWs

We study the orbital and spin dynamics of charge carriers induced by non-overlapping linearly polarized light pulses in semiconductor quantum wells (QWs). It is shown that such an optical excitation with coherent pulses leads to a spin orientation of photocarriers and an electric current. The effects are caused by the interference of optical transitions driven by individual pulses. The distribution of carriers in the spin and momentum spaces depends on the QW crystallographic orientation and can be efficiently controlled by the pulse polarizations, time delay and phase shift between the pulses, as well as an external magnetic field.

cond-mat.mes-hall↗

Resonant Brillouin scattering of excitonic polaritons in multiple-quantum-well structures

We present theoretical and experimental study of resonant Brillouin scattering of excitonic polaritons in one-dimensional multiple-quantum-well structure. We obtain general analytical results for the scattering light spectra, valid for arbitrary quantum well arrangement. Application of our theory to the specific case of short-period superlattice shows a perfect quantitative agreement with experimental results for the height, width and position of the Brillouin scattering peaks and allows us to determine the energy, radiative and nonradiative decay rates of quantum well excitons. We reveal the signatures of excitonic polariton formation in the scattering spectra and show, that the spectral width and height are strongly sensitive to the number of wells in the sample.

cond-mat.mes-hall↗

Magnetic Field Effect on Electron Spin Dynamics in (110) GaAs Quantum wells

We study the electron spin relaxation in both symmetric and asymmetric GaAs/AlGaAs quantum wells (QWs) grown on (110) substrates in an external magnetic field B applied along the QW normal. The spin polarization is induced by circularly polarized light and detected by time-resolved Kerr rotation technique. In the asymmetric structure, where a δ-doped layer on one side of the QW produces the Rashba contribution to the conduction-band spin-orbit splitting, the lifetime of electron spins aligned along the growth axis exhibits an anomalous dependence on B in the range 0<B<0.5 T; this results from the interplay between the Dresselhaus and Rashba effective fields which are perpendicular to each other. For larger magnetic fields, the spin lifetime increases, which is the consequence of the cyclotron motion of the electrons and is also observed in (001)-grown quantum wells. The experimental results are in agreement with the calculation of the spin lifetimes in (110)- grown asymmetric quantum wells described by the point group Cs where the growth direction is not the principal axis of the spin-relaxation-rate tensor.

cond-mat.mes-hall↗

Radiative topological states in resonant photonic crystals

We present a theory of topological edge states in one-dimensional resonant photonic crystals with a compound unit cell. Contrary to the traditional electronic topological states the states under consideration are radiative, i.e., they decay in time due to the light escape through the structure boundaries. We demonstrate that the states survive despite their radiative decay and can be detected both in time- and frequency-dependent light reflection.

cond-mat.mes-hall↗

Time-resolved second-order correlations of microcavity photons

The time dependence of the correlations between the photons, emitted from the microcavity with embedded quantum dot under incoherent pumping, is studied theoretically. Analytical expressions for the second-order correlation function g2(t) are presented in strong and weak coupling regimes. At moderate pumping the correlation function demonstrates Rabi oscillations, while at larger pumping it shows monoexponential decay. The decay time of the correlations nonmonotonously depends on the pumping value and has a maximum corresponding to the self-quenching transition.

cond-mat.mes-hall↗