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A. V. Zayats

Publications and source records attributed to A. V. Zayats.

17 recordsLinked to original sources

Frozen Surface Modes on a Moving Interface

Spatio-temporal modulation enables synthetic motion at effective velocities approaching the speed of light, providing new regimes for light-matter interaction. Traditional Cherenkov-type effects arise when the velocity of an emitter matches or exceeds the phase velocity of electromagnetic modes supported by a medium. Here, we study dispersive systems in which phase and group velocities differ markedly. Specifically, we explore the case of group-velocity matching for surface waves, where the emitter moves at the same velocity as the flow of energy. This gives rise to frozen surface modes which are stationary in the emitter frame, accompanied by resonant energy accumulation. The result is a dramatic increase of the local density of optical states, the power extracted from the emitter, and the optomechanical forces and torques it experiences. Since surface modes naturally exhibit slow group velocities, this is accessible at lower relative speeds than phase-velocity effects. This phenomenon provides a route to enhanced light-matter interaction via real or synthetic motion.

physics.optics↗

Roadmap on structured waves

Structured waves are ubiquitous for all areas of wave physics, both classical and quantum, where the wavefields are inhomogeneous and cannot be approximated by a single plane wave. Even the interference of two plane waves, or a single inhomogeneous (evanescent) wave, provides a number of nontrivial phenomena and additional functionalities as compared to a single plane wave. Complex wavefields with inhomogeneities in the amplitude, phase, and polarization, including topological structures and singularities, underpin modern nanooptics and photonics, yet they are equally important, e.g., for quantum matter waves, acoustics, water waves, etc. Structured waves are crucial in optical and electron microscopy, wave propagation and scattering, imaging, communications, quantum optics, topological and non-Hermitian wave systems, quantum condensed-matter systems, optomechanics, plasmonics and metamaterials, optical and acoustic manipulation, and so forth. This Roadmap is written collectively by prominent researchers and aims to survey the role of structured waves in various areas of wave physics. Providing background, current research, and anticipating future developments, it will be of interest to a wide cross-disciplinary audience.

physics.optics↗

Transverse spinning of unpolarized light

It is well known that spin angular momentum of light, and therefore that of photons, is directly related to their circular polarization. Naturally, for totally unpolarized light, polarization is undefined and the spin vanishes. However, for nonparaxial light, the recently discovered transverse spin component, orthogonal to the main propagation direction, is largely independent of the polarization state of the wave. Here we demonstrate, both theoretically and experimentally, that this transverse spin survives even in nonparaxial fields (e.g., tightly focused or evanescent) generated from a totally unpolarized light source. This counterintuitive phenomenon is closely related to the fundamental difference between the degrees of polarization for 2D paraxial and 3D nonparaxial fields. Our results open an avenue for studies of spin-related phenomena and optical manipulation using unpolarized light.

physics.optics↗

Circular Dichroism Enhancement in Plasmonic Nanorod Metamaterials

Optical activity is a fundamental phenomenon originating from the chiral nature of crystals and molecules. While intrinsic chiroptical responses of ordinary chiral materials to circularly polarized light are relatively weak, they can be enhanced by specially tailored nanostructures. Here, nanorod metamaterials, comprising a dense array of vertically aligned gold nanorods, is shown to provide significant enhancement of the circular dichroism response of an embedded material. A nanorod composite, acting as an artificial uniaxial crystal, is filled with chiral mercury sulfide nanocrystals embedded in a transparent polymer. The nanorod based metamaterial, being inherently achiral, enables optical activity enhancement or suppression. Unique properties of inherently achiral structures to tailor optical activities pave a way for flexible characterization of optical activity of molecules and nanocrystal-based compounds.

physics.optics↗

Structural second-order nonlinearity in metamaterials

Nonlinear processes are at the core of many optical technologies including lasers, information processing, sensing, and security, and require optimised materials suitable for nanoscale integration. Here we demonstrate the emergence of a strong bulk second-order nonlinear response in a composite plasmonic nanorod material comprised of centrosymmetric materials. The metamaterial provides equally strong generation of the p-polarized second harmonic light in response to both s- and p-polarized excitation. We develop an effective-medium description of the underlying physics, compare its predictions to the experimental results and analyze the limits of its applicability. We show that while the effective medium theory adequately describes the nonlinear polarization, the process of emission of second harmonic light cannot be described in the same framework. The work provides an understanding of the emergent nonlinear optical response in composites and opens a doorway to new nonlinear optical platform designs for integrated nonlinear photonics.

physics.optics↗

Spin-orbit interactions of light

Light carries spin and orbital angular momentum. These dynamical properties are determined by the polarization and spatial degrees of freedom of light. Modern nano-optics, photonics, and plasmonics, tend to explore subwavelength scales and additional degrees of freedom of structured, i.e., spatially-inhomogeneous, optical fields. In such fields, spin and orbital properties become strongly coupled with each other. We overview the fundamental origins and important applications of the main spin-orbit interaction phenomena in optics. These include: spin-Hall effects in inhomogeneous media and at optical interfaces, spin-dependent effects in nonparaxial (focused or scattered) fields, spin-controlled shaping of light using anisotropic structured interfaces (metasurfaces), as well as robust spin-directional coupling via evanescent near fields. We show that spin-orbit interactions are inherent in all basic optical processes, and they play a crucial role at subwavelength scales and structures in modern optics.

physics.optics↗

Influence of photoexcitation depth on luminescence spectra of bulk GaAs single crystals: application to defect structure characterization

The results of investigation of bulk GaAs photoluminescence are presented taken from near-surface layers of different thicknesses using for excitation the light with the wavelengths which are close but some greater than the excitonic absorption resonances (so-called "bulk" photoexcitation). Only the excitonic and band-edge luminescence is seen under the interband excitation, while under the "bulk" excitation, the spectra are much more informative. The interband excited spectra of all the samples investigated in the present work are practically identical, whereas the bulk excited PL spectra are different for different samples and excitation depths and provide the information on the deep-level point defect composition of the bulk materials.

cond-mat.mtrl-sci↗

Influence of Photoexcitation Depth on Luminescence Spectra of Bulk GaAs Single Crystals and Defect Structure Characterization

The results of investigation of bulk GaAs photoluminescence are presented taken from near-surface layers of different thicknesses using for excitation the light with the wavelengths which are close but some greater than the excitonic absorption resonances (so-called bulk photoexcitation). Only the excitonic and band-edge luminescence is seen under the interband excitation, while under the bulk excitation, the spectra are much more informative. The interband excited spectra of all the samples investigated in the present work are practically identical, whereas the bulk excited PL spectra are different for different samples and excitation depths and provide the information on the deep-level point defect composition of the bulk materials.

cond-mat.mtrl-sci↗

Amplification of surface plasmon polaritons in the presence of nonlinearity and spectral signatures of threshold crossover

We describe effects of nonlinearity on propagation of surface plasmon polaritons (SPPs) at an interface between a metal and an amplifying medium of the externally pumped two-level atoms. Using Maxwell equations we derive the nonlinear dispersion law and demonstrate that, the nonlinear saturation of the linear gain leads to formation of stationary SPP modes with the intensities independent from the propagation distance. Transition to the regime of stationary propagation is similar to the threshold crossover in lasers and leads to narrowing of the SPP spectrum.

physics.optics↗

Single-photon excitation of surface plasmon polaritons

We provide the quantum mechanical description of the excitation of surface plasmon polaritons on metal surfaces by single-photons. An attenuated-reflection setup is described for the quantum excitation process in which we find remarkably efficient photon-to-surface plasmon wavepacket-transfer. Using a fully quantized treatment of the fields, we introduce the Hamiltonian for their interaction and study the quantum statistics during transfer with and without losses in the metal.

quant-ph↗

Digital resolution enhancement in surface plasmon microscopy

The use of photonic crystal and negative refractive index materials is known to improve resolution of optical microscopy and lithography devices down to 80 nm level. Here we demonstrate that utilization of well-known digital image recovery techniques allows us to further improve resolution of optical microscope down to 30 nm level. Our microscope is based on a flat dielectric mirror deposited onto an array of nanoholes in thin gold film. This two-dimensional photonic crystal mirror may have either positive or negative effective refractive index as perceived by surface plasmon polartions in the visible frequency range. The optical images formed by the mirror are enhanced using simple digital filters.

physics.optics↗

Diffraction grating revisited: a high-resolution plasmonic dispersive element

The spectral dispersion of light is critical in applications ranging from spectroscopy to sensing and optical communication technologies. We demonstrate that ultra-high spectral dispersion can be achieved with a finite-size surface plasmon polaritonic (SPP) crystal. The 3D to 2D reduction in light diffraction dimensions due to interaction of light with collective electron modes in a metal is shown to increase the dispersion by some two orders of magnitude, due to a two-stage process: (i) conversion of the incident light to SPP Bloch waves on a nanostructured surface and (ii) Bloch waves traversing the SPP crystal boundary. This has potential for high-resolution spectrograph applications in photonics, optical communications and lab-on-a-chip, all within a planar device which is compact and easy to fabricate.

cond-mat.str-el↗

High-contrast modulation of light with light by control of surface plasmon polariton wave coupling

We have demonstrated a new mechanism for modulating light with light by controlling the efficiency with which light is coupled into a plasmon polariton wave. An optical fluence of 15 mJ/cm^2 in the control channel is sufficient to achieve nearly a 10-fold intensity modulation of the signal beam reflected from a Glass/MgF_2/Ga structure. The mechanism depends on a nanoscale light-induced structural transformation in the gallium layer and has transient switching times of the order of a few tens of nanoseconds. It offers high modulation contrast for signals in the visible and near infrared spectral ranges.

cond-mat.mtrl-sci↗

Broken Time Reversal of Light Interaction with Planar Chiral Nanostructures

We report unambiguous experimental evidence of broken time reversal symmetry for the interaction of light with an artificial non-magnetic material. Polarized colour images of planar chiral gold-on-silicon nanostructures consisting of arrays of gammadions show intriguing and unusual symmetry: structures, which are geometrically mirror images, loose their mirror symmetry in polarized light. The symmetry of images can only be described in terms of anti-symmetry (black-and-white symmetry) appropriate to a time-odd process. The effect results from a transverse chiral non-local electromagnetic response of the structure and has some striking resemblance with the expected features of light scattering on anyon matter.

cond-mat.mtrl-sci↗

Optical control of photon tunneling through an array of nanometer scale cylindrical channels

We report first observation of photon tunneling gated by light at a different wavelength in an artificially created array of nanometer scale cylindrical channels in a thick gold film. Polarization properties of gated light provide strong proof of the enhanced nonlinear optical mixing in nanometric channels involved in the process. This suggests the possibility of building a new class of "gated" photon tunneling devices for massive parallel all-optical signal and image processing.

cond-mat.str-el↗

Light controlled photon tunneling

Recent measurements of photon tunneling through individual subwavelength pinholes in a gold film covered with a layer of polydiacetylene (Phys. Rev. Letters 88, 187402 (2002)) provided strong indication of "photon blockade" effect similar to Coulomb blockade phenomenon observed in single-electron tunneling experiments. Here we report first observation of photon tunneling been blocked (gated) by light at a different wavelength. This observation suggests possibility of building new class of photon tunneling gating devices for all-optical signal processing.

cond-mat.str-el↗

Single-photon tunneling

Strong evidence of a single-photon tunneling effect, a direct analog of single-electron tunneling, has been obtained in the measurements of light tunneling through individual subwavelength pinholes in a thick gold film covered with a layer of polydiacetylene. The transmission of some pinholes reached saturation because of the optical nonlinearity of polydiacetylene at a very low light intensity of a few thousands photons per second. This result is explained theoretically in terms of "photon blockade", similar to the Coulomb blockade phenomenon observed in single-electron tunneling experiments. The single-photon tunneling effect may find many applications in the emerging fields of quantum communication and information processing.

cond-mat.str-el↗