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A. Verdini

Publications and source records attributed to A. Verdini.

At least 19 recordsLinked to original sources

Self-Aligned Metallic-Semiconducting Phosphorus Nanoarrays Driven by Facet Engineering

Two-dimensional (2D) materials often require specific substrate terminations for epitaxial stabilization, yet the search for suitable templates has largely focused on low-index metal surfaces, which may not provide the optimal conditions for the growth of new phases. Here, we show that crystal-facet engineering on curved Cu surfaces enables the stabilization, within a single preparation step, of two distinct 2D phosphorus phases with different electronic properties. Hexagonal blue phosphorene forms on Cu(111) terraces, whereas a previously unreported skewed-square phosphorus phase is stabilized on Cu(513) facets. By combining complementary microscopy and spectroscopy techniques with theoretical calculations, we determine the structural and electronic properties of this new phase, which displays semiconducting character, in contrast to the metallic behavior of blue phosphorene. The coexistence of these two competing phases gives rise to a metal-to-semiconducting transition of the 2D phosphorus layer over the substrate. Locally, the competition between the two phases gives rise to self-aligned nanoarrays of alternating metallic and semiconducting phosphorus terraces. These results establish crystal-facet engineering as a practical route for discovering and stabilizing emergent 2D material phases on high-index substrates, while also enabling the engineering of nanostructures with tailored electronic properties through a simple and scalable growth process.

cond-mat.mtrl-sci

Radial and angular evolution of magnetic cloud signatures in the turbulent solar wind: virtual spacecraft analysis

Interplanetary coronal mass ejections (ICMEs) carry magnetic clouds (MCs), large-scale structures with average radial widths about a fifth of an astronomical unit at Earth's orbit. ICMEs display substructures in white light images and reveal rich dynamics across many spatial scales when directly measured by spacecraft. A spacecraft encounter with an ICME can result in smoothly rotating MC intervals or less organised magnetic obstacle (MO) ones. We investigate how the interplay of expansion, turbulence, and internal cloud dynamics affects magnetic cloud properties, which are reflected in the plasma signatures measured by spacecraft. We perform high-resolution 2.5D MHD simulations of a magnetic flux rope cross-section, which is embedded in the turbulent, expanding solar wind with the expanding box model. We probe the local plasma properties, and thus the flux rope signatures and angular coherence, with virtual spacecraft. Our simulations reproduce clear and stable MC signatures when the flux rope core is intercepted by virtual spacecraft. Disordered MO signatures appear at the edges of the flux rope, and are attributed to both expansion and turbulent transport. We vary some key physical parameters of the flux rope and the environment to understand their effect on the observed coherence and signatures. The pace of the expanding flow controls the angular extent of MC signatures, whereas the intensity of interplanetary turbulence controls how asymmetric and distorted the flux rope appears at 1 AU. The geometry of spacecraft encounters determines whether MC or MO signatures are observed. The presence of a magnetic structure which can result in MO signatures is strongly controlled by the flux rope's initial/early magnetic configuration: MO signatures can only be observed when the axial flux rope field is spatially not well confined by the rope's own magnetic tension, and disappear otherwise.

astro-ph.SR

The essential role of multi-point measurements in investigations of turbulence, three-dimensional structure, and dynamics: the solar wind beyond single scale and the Taylor Hypothesis

Space plasmas are three-dimensional dynamic entities. Except under very special circumstances, their structure in space and their behavior in time are not related in any simple way. Therefore, single spacecraft in situ measurements cannot unambiguously unravel the full space-time structure of the heliospheric plasmas of interest in the inner heliosphere, in the Geospace environment, or the outer heliosphere. This shortcoming leaves numerous central questions incompletely answered. Deficiencies remain in at least two important subjects, Space Weather and fundamental plasma turbulence theory, due to a lack of a more complete understanding of the space-time structure of dynamic plasmas. Only with multispacecraft measurements over suitable spans of spatial separation and temporal duration can these ambiguities be resolved. We note that these characterizations apply to turbulence across a wide range of scales, and also equally well to shocks, flux ropes, magnetic clouds, current sheets, stream interactions, etc. In the following, we will describe the basic requirements for resolving space-time structure in general, using turbulence' as both an example and a principal target or study. Several types of missions are suggested to resolve space-time structure throughout the Heliosphere.

physics.space-ph

Scale dependence and cross-scale transfer of kinetic energy in compressible hydrodynamic turbulence at moderate Reynolds numbers

We investigate properties of the scale dependence and cross-scale transfer of kinetic energy in compressible three-dimensional hydrodynamic turbulence, by means of two direct numerical simulations of decaying turbulence with initial Mach numbers M = 1/3 and M = 1, and with moderate Reynolds numbers, R_lambda ~ 100. The turbulent dynamics is analyzed using compressible and incompressible versions of the dynamic spectral transfer (ST) and the Karman-Howarth-Monin (KHM) equations. We find that the nonlinear coupling leads to a flux of the kinetic energy to small scales where it is dissipated; at the same time, the reversible pressure-dilatation mechanism causes oscillatory exchanges between the kinetic and internal energies with an average zero net energy transfer. While the incompressible KHM and ST equations are not generally valid in the simulations, their compressible counterparts are well satisfied and describe, in a quantitatively similar way, the decay of the kinetic energy on large scales, the cross-scale energy transfer/cascade, the pressure dilatation, and the dissipation. There exists a simple relationship between the KHM and ST results through the inverse proportionality between the wave vector k and the spatial separation length l as k l ~ 3^1/2. For a given time the dissipation and pressure-dilatation terms are strong on large scales in the KHM approach whereas the ST terms become dominant on small scales; this is owing to the complementary cumulative behavior of the two methods. The effect of pressure dilatation is weak when averaged over a period of its oscillations and may lead to a transfer of the kinetic energy from large to small scales without a net exchange between the kinetic and internal energies. Our results suggest that for large-enough systems there exists an inertial range for the kinetic energy cascade ...

physics.flu-dyn

Magnetic field turbulence in the solar wind at sub-ion scales: in situ observations and numerical simulations

We investigate the transition of the solar wind turbulent cascade from MHD to sub-ion range by means of a detail comparison between in situ observations and hybrid numerical simulations. In particular we focus on the properties of the magnetic field and its component anisotropy in Cluster measurements and hybrid 2D simulations. First, we address the angular distribution of wave-vectors in the kinetic range between ion and electron scales by studying the variance anisotropy of the magnetic field components. When taking into account the single-direction sampling performed by spacecraft in the solar wind, the main properties of the fluctuations observed in situ are also recovered in our numerical description. This result confirms that solar wind turbulence in the sub-ion range is characterized by a quasi-2D gyrotropic distribution of k-vectors around the mean field. We then consider the magnetic compressibility associated with the turbulent cascade and its evolution from large-MHD to sub-ion scales. The ratio of field-aligned to perpendicular fluctuations, typically low in the MHD inertial range, increases significantly when crossing ion scales and its value in the sub-ion range is a function of the total plasma beta only, as expected from theoretical predictions, with higher magnetic compressibility for higher beta. Moreover, we observe that this increase has a gradual trend from low to high beta values in the in situ data; this behaviour is well captured by the numerical simulations. The level of magnetic field compressibility that is observed in situ and in the simulations is in fairly good agreement with theoretical predictions, especially at high beta, suggesting that in the kinetic range explored the turbulence is supported by low-frequency and highly-oblique fluctuations in pressure balance, like kinetic Alfvén waves or other slowly evolving coherent structures.

physics.space-ph

Turbulence vs. fire hose instabilities: 3-D hybrid expanding box simulations

The relationship between a decaying plasma turbulence and proton fire hose instabilities in a slowly expanding plasma is investigated using three-dimensional (3-D) hybrid expanding box simulations. We impose an initial ambient magnetic field along the radial direction, and we start with an isotropic spectrum of large-scale, linearly-polarized, random-phase Alfvenic fluctuations with zero cross-helicity. A turbulent cascade rapidly develops and leads to a weak proton heating that is not sufficient to overcome the expansion-driven perpendicular cooling. The plasma system eventually drives the parallel and oblique fire hose instabilities that generate quasi-monochromatic wave packets that reduce the proton temperature anisotropy. The fire hose wave activity has a low amplitude with wave vectors quasi-parallel/oblique with respect to the ambient magnetic field outside of the region dominated by the turbulent cascade and is discernible in one-dimensional power spectra taken only in the direction quasi-parallel/oblique with respect to the ambient magnetic field; at quasi-perpendicular angles the wave activity is hidden by the turbulent background. These waves are partly reabsorbed by protons and partly couple to and participate in the turbulent cascade. Their presence reduces kurtosis, a measure of intermittency, and the Shannon entropy but increases the Jensen-Shannon complexity of magnetic fluctuations; these changes are weak and anisotropic with respect to the ambient magnetic field and it's not clear if they can be used to indirectly discern the presence of instability-driven waves.

physics.space-ph

[Plasma 2020 Decadal] The essential role of multi-point measurements in turbulence investigations: the solar wind beyond single scale and beyond the Taylor Hypothesis

This paper briefly reviews a number of fundamental measurements that need to be made in order to characterize turbulence in space plasmas such as the solar wind. It has long been known that many of these quantities require simultaneous multipoint measurements to attain a proper characterization that would reveal the fundamental physics of plasma turbulence. The solar wind is an ideal plasma for such an investigation, and it now appears to be technologically feasible to carry out such an investigation, following the pioneering Cluster and MMS missions. Quantities that need to be measured using multipoint measurements include the two-point, two-time second correlation function of velocity, magnetic field and density, and higher order statistical objects such as third and fourth order structure functions. Some details of these requirements are given here, with a eye towards achieving closure on fundamental questions regarding the cascade rate, spectral anisotropy, characteristic coherent structures, intermittency, and dissipation mechanisms that describe plasma turbuelence, as well as its variability with plasma parameters in the solar wind. The motivation for this discussion is the current planning for a proposed Helioswarm mission that would be designed to make these measurements,leading to breakthrough understanding of the physics of space and astrophysical turbulence.

physics.space-ph

Three-dimensional simulations of solar wind turbulence with the hybrid code CAMELIA

We investigate the spectral properties of plasma turbulence from fluid to sub-ion scales by means of high-resolution three-dimensional (3D) numerical simulations performed with the hybrid particle-in-cell (HPIC) code CAMELIA. We produce extended turbulent spectra with well-defined power laws for the magnetic, ion bulk velocity, density, and electric fluctuations. The present results are in good agreement with previous two-dimensional (2D) HPIC simulations, especially in the kinetic range of scales, and reproduce several features observed in solar wind spectra. By providing scaling tests on many different architectures and convergence studies, we prove CAMELIA to represent a very efficient, accurate and reliable tool for investigating the develpoment of the turbulent cascade in the solar wind, being able to cover simultaneously several decades in wavenumber, also in 3D.

astro-ph.SR

Sub-structure formation in starless cores

Motivated by recent observational searches of sub-structure in starless molecular cloud cores, we investigate the evolution of density perturbations on scales smaller than the Jeans length embedded in contracting isothermal clouds, adopting the same formalism developed for the expanding Universe and the solar wind. We find that initially small amplitude, Jeans-stable perturbations (propagating as sound waves in the absence of a magnetic field), are amplified adiabatically during the contraction, approximately conserving the wave action density, until they either become nonlinear and steepen into shocks at a time $t_{\rm nl}$, or become gravitationally unstable when the Jeans length decreases below the scale of the perturbations at a time $t_{\rm gr}$. We evaluate analytically the time $t_{\rm nl}$ at which the perturbations enter the non-linear stage using a Burgers' equation approach, and we verify numerically that this time marks the beginning of the phase of rapid dissipation of the kinetic energy of the perturbations. We then show that for typical values of the rms Mach number in molecular cloud cores, $t_{\rm nl}$ is smaller than $t_{\rm gr}$, and therefore density perturbations likely dissipate before becoming gravitational unstable. Solenoidal modes grow at a faster rate than compressible modes, and may eventually promote fragmentation through the formation of vortical structures.

astro-ph.SR

Magnetic reconnection as a driver for a sub-ion scale cascade in plasma turbulence

A new path for the generation of a sub-ion scale cascade in collisionless plasma turbulence, triggered by magnetic reconnection, is uncovered by means of high-resolution two-dimensional hybrid-kinetic simulations employing two complementary approaches, Lagrangian and Eulerian, and different driving mechanisms. The simulation results provide clear numerical evidences that the development of power-law energy spectra below the so-called ion break occurs as soon as the first magnetic reconnection events take place, regardless of the actual state of the turbulent cascade at MHD scales. In both simulations, the reconnection-mediated small-scale energy spectrum of parallel magnetic fluctuations exhibits a very stable spectral slope of ~-2.8, whether or not a large-scale turbulent cascade has already fully developed. Once a quasi-stationary turbulent state is achieved, the spectrum of the total magnetic fluctuations settles towards a spectral index of -5/3 in the MHD range and of ~-3 at sub-ion scales.

physics.space-ph

Mirror instability in the turbulent solar wind

The relationship between a decaying strong turbulence and the mirror instability in a slowly expanding plasma is investigated using two-dimensional hybrid expanding box simulations. We impose an initial ambient magnetic field perpendicular to the simulation box, and we start with a spectrum of large-scale, linearly-polarized, random-phase Alfvenic fluctuations which have energy equipartition between kinetic and magnetic fluctuations and vanishing correlation between the two fields. A turbulent cascade rapidly develops, magnetic field fluctuations exhibit a Kolmogorov-like power-law spectrum at large scales and a steeper spectrum at sub-ion scales. The imposed expansion (taking a strictly transverse ambient magnetic field) leads to generation of an important perpendicular proton temperature anisotropy that eventually drives the mirror instability. This instability generates large-amplitude, nonpropagating, compressible, pressure-balanced magnetic structures in a form of magnetic enhancements/humps that reduce the perpendicular temperature anisotropy.

physics.space-ph

Parametric decay of parallel and oblique Alfven waves in the expanding solar wind

The long-term evolution of large-amplitude Alfven waves propagating in the solar wind is investigated by performing two-dimensional MHD simulations within the expanding box model. The linear and nonlinear phases of the parametric decay instability are studied for both circularly polarized waves in parallel propagation and for arc-polarized waves in oblique propagation. The non-monochromatic case is also considered. In the oblique case, the direct excitation of daughter modes transverse to the local background field is found for the first time in an expanding environment, and this transverse cascade seems to be favored for monochromatic mother waves. The expansion effect reduces the instability growth rate, and it can even suppress its onset for the lowest frequency modes considered here, possibly explaining the persistence of these outgoing waves in the solar wind.

astro-ph.SR

Coupling the solar surface and the corona: coronal rotation, Alfvén wave-driven polar plumes

The dynamical response of the solar corona to surface and sub-surface perturbations depends on the chromospheric stratification, and specifically on how efficiently these layers reflect or transmit incoming Alfvén waves. While it would be desirable to include the chromospheric layers in the numerical simulations used to study such phenomena, that is most often not feasible. We defined and tested a simple approximation allowing the study of coronal phenomena while taking into account a parametrised chromospheric reflectivity. We addressed the problems of the transmission of the surface rotation to the corona and that of the generation of polar plumes by Alfvén waves (Pinto et al., 2010, 2011). We found that a high (yet partial) effective chromospheric reflectivity is required to properly describe the angular momentum balance in the corona and the way the surface differential rotation is transmitted upwards. Alfvén wave-driven polar plumes maintain their properties for a wide range of values for the reflectivity, but they become bursty (and eventually disrupt) when the limit of total reflection is attained.

astro-ph.SR

Reflection and dissipation of Alfvén waves in interstellar clouds

Context: Supersonic nonthermal motions in molecular clouds are often interpreted as long-lived magnetohydrodynamic (MHD) waves. The propagation and amplitude of these waves is affected by local physical characteristics, most importantly the gas density and the ionization fraction. Aims: We study the propagation, reflection and dissipation of Alfvén waves in molecular clouds deriving the behavior of observable quantities such as the amplitudes of velocity fluctuations and the rate of energy dissipation. Methods: We formulated the problem in terms of Elsässer variables for transverse MHD waves propagating in a one-dimensional inhomogeneous medium, including the dissipation due to collisions between ions and neutrals and to a nonlinear turbulent cascade treated in a phenomenological way. We considered both steady-state and time-dependent situations and solved the equations of the problem numerically with an iterative method and a Lax-Wendroff scheme, respectively. Results: Alfvén waves incident on overdense regions with density profiles typical of cloud cores embedded in a diffuse gas suffer enhanced reflection in the regions of the steepest density gradient, and strong dissipation in the core's interior. These effects are especially significant when the wavelength is intermediate between the critical wavelength for propagation and the typical scale of the density gradient. For larger wave amplitudes and/or steeper input spectra, the effects of the perpendicular turbulent cascade result in a stronger energy dissipation in the regions immediately surrounding the dense core. Conclusions: The results may help to interpret the sharp decrease of line width observed in the environments of low-mass cloud cores in several molecular transitions.

astro-ph.GA

On the origin of the 1/f spectrum in the solar wind magnetic field

We present a mechanism for the formation of the low frequency 1/f magnetic spectrum based on numerical solutions of a shell reduced-MHD model of the turbulent dynamics inside the sub-Alfvénic solar wind. We assign reasonably realistic profiles to the wind speed and the density along the radial direction, and a radial magnetic field. Alfvén waves of short periodicity (600 s) are injected at the base of the chromosphere, penetrate into the corona and are partially reflected, thus triggering a turbulent cascade. The cascade is strong for the reflected wave while it is weak for the outward propagating waves. Reflection at the transition region recycles the strong turbulent spectrum into the outward weak spectrum, which is advected beyond the Alfvénic critical point without substantial evolution. There, the magnetic field has a perpendicular power-law spectrum with slope close to the Kolmogorov -5/3. The parallel spectrum is inherited from the frequency spectrum of large (perpendicular) eddies. The shape is a double power-law with slopes of -1 and -2 at low and high frequencies respectively, the position of the break depending on the injected spectrum. We suggest that the double power-law spectrum measured by Helios at 0.3 AU, where the average magnetic field is not aligned with the radial (contrary to our assumptions) results from the combination of such different spectral slopes. At low frequency the parallel spectrum dominates with its characteristic 1/f shape, while at higher frequencies its steep spectral slope (-2) is masked by the more energetic perpendicular spectrum (slope -5/3).

astro-ph.SR

Time delays in quasi-periodic pulsations observed during the X2.2 solar flare on 2011 February 15

We report observations of quasi-periodic pulsations (QPPs) during the X2.2 flare of 2011 February 15, observed simultaneously in several wavebands. We focus on fluctuations on time scale 1-30 s and find different time lags between different wavebands. During the impulsive phase, the Reuven Ramaty High Energy Solar Spectroscopic Imager (RHESSI) channels in the range 25-100 keV lead all the other channels. They are followed by the Nobeyama RadioPolarimeters at 9 and 17 GHz and the Extreme Ultra-Violet (EUV) channels of the Euv SpectroPhotometer (ESP) onboard the Solar Dynamic Observatory (SDO). The Zirconium and Aluminum filter channels of the Large Yield Radiometer (LYRA) onboard the Project for On-Board Autonomy (PROBA2) satellite and the SXR channel of ESP follow. The largest lags occur in observations from the Geostationary Operational Environmental Satellite (GOES), where the channel at 1-8 Å leads the 0.5-4 Å channel by several seconds. The time lags between the first and last channels is up to 9 s. We identified at least two distinct time intervals during the flare impulsive phase, during which the QPPs were associated with two different sources in the Nobeyama RadioHeliograph at 17 GHz. The radio as well as the hard X-ray channels showed different lags during these two intervals. To our knowledge, this is the first time that time lags are reported between EUV and SXR fluctuations on these time scales. We discuss possible emission mechanisms and interpretations, including flare electron trapping.

astro-ph.SR

Relating Energy Level Alignment and Amine-Linked Single Molecule Junction Conductance

Using photoemission spectroscopy, we determine the relationship between electronic energy level alignment at a metal-molecule interface and single-molecule junction transport data. We measure the position of the highest occupied molecular orbital (HOMO) relative to the Au metal Fermi level for three 1,4-benzenediamine derivatives on Au(111) and Au(110) with ultraviolet and resonant x-ray photoemission spectroscopy. We compare these results to scanning tunnelling microscope based break-junction measurements of single molecule conductance and to first-principles calculations. We find that the energy difference between the HOMO and Fermi level for the three molecules adsorbed on Au(111) correlate well with changes in conductance, and agree well with quasiparticle energies computed from first-principles calculations incorporating self-energy corrections. On the Au(110) which present Au atoms with lower-coordination, critical in break-junction conductance measurements, we see that the HOMO level shifts further from the Fermi level. These results provide the first direct comparison of spectroscopic energy level alignment measurements with single molecule junction transport data.

cond-mat.mes-hall

Coupling Photosphere and Corona: Linear and Turbulent Regimes

In a recent work Grappin et al. [1] have shown that low- frequency movements can be transmitted from one footpoint to the other along a magnetic loop, thus mimicking a friction effect of the corona on the photosphere, and invalidating the line-tying approximation. We consider here successively the effect of high frequencies and turbulent damping on the process. We use a very simple atmospheric model which allows to study analytically the laminar case, and to study the turbulent case both using simple phenomenological arguments and a more sophisticated turbulence model [2]. We find that, except when turbulent damping is such that all turbulence is damped during loop traversal, coupling still occurs between distant footpoints, and moreover the coronal field induced by photospheric movements saturates at finite values.

astro-ph.SR