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A. Zawadowski

Publications and source records attributed to A. Zawadowski.

34 records · Page 2Linked to original sources

Theory of STM Spectroscopy of Kondo Ions on Metal Surfaces

The conduction electron density of states nearby a single magnetic impurity, as measured recently by scanning tunneling microscopy (STM), is calculated. It is shown that the Kondo effect induces a narrow Fano resonance as an intrinsic feature in the conduction electron density of states. The line shape varies with the distance between STM tip and impurity, in qualitative agreement with experiments, and is sensitive to details of the band structure. For a Co impurity the experimentally observed width and shift of the Kondo resonance are in accordance with those obtained from a combination of band structure and strongly correlated calculations.

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Theory of the Fano Resonance in the STM Tunneling Density of States due to a Single Kondo Impurity

The conduction electron density of states nearby single magnetic impurities, as measured recently by scanning tunneling microscopy (STM), is calculated, taking into account tunneling into conduction electron states only. The Kondo effect induces a narrow Fano resonance in the conduction electron density of states, while scattering off the d-level generates a weakly energy dependent Friedel oscillation. The line shape varies with the distance between STM tip and impurity, in qualitative agreement with experiments, but is very sensitive to details of the band structure. For a Co impurity the experimentally observed width and shift of the Kondo resonance are in accordance with those obtained from a combination of band structure and strongly correlated calculations.

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Theory of magnetoresistance in films of dilute magnetic alloys

Earlier a magnetic anisotropy for magnetic impurities nearby the surface of non-magnetic host was proposed in order to explain the size dependence of the Kondo effect in dilute magnetic alloys. Recently Giordano has measured the magnetoresistance of dilute Au(Fe) films for different thicknesses well above the Kondo temperature $T_K$. In this way he verified the existence of that anisotropy even for such a case where the Kondo effect is not dominating. For detailed comparison of that suggestion with experiments, the magnetic field dependence of the magnetoresistance is calculated in the lowest approximation, thus in the second order of the exchange coupling. The strength of the anisotropy is very close to earlier estimates deduced from the size dependence of the Kondo resistivity amplitude.

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Dephasing in Metals by Two-Level Systems in the 2-Channel-Kondo Regime

We point out a novel, non-universal contribution to the dephasing rate 1/τ_ϕ\equiv γ_ϕof conduction electrons in metallic systems: scattering off non-magnetic two-level systems (TLSs) having almost degenerate Kondo ground states. In the regime Δ_{ren} < T < T_K (Δ_{ren} = renormalized level splitting, T_K = Kondo temperature), such TLSs exhibit non-Fermi-liquid physics that can cause γ_ϕ, which generally decreases with decreasing T, to seemingly saturate in a limited temperature range before vanishing for T \to 0. This could explain the saturation of dephasing recently observed in gold wires [Mohanty et al. Phys. Rev. Lett. 78, 3366 (1997)].

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Spin-Orbit-Induced Kondo Size Effect in Thin Films with 5/2-spin Impurities

Recently, for spin $S=5/2$ impurities quite different size dependence of the Kondo contribution to the resistivity was found experimentally than for S=2. Therefore previous calculation about the effect of the spin-orbit-induced magnetic anisotropy on the Kondo amplitude of the resistivity is extended to the case of $S=5/2$ impurity spin which differs from the integer spin case as the ground state is degenerated. In this case the Kondo contribution remains finite when the sample size goes to zero and the thickness dependence in the Kondo resistivity is much weaker for Cu(Mn). The behavior of the Kondo coefficient as a function of the thickness depends on the Kondo temperature, that is somewhat stronger for larger $T_K$. Comparing our results with a recent experiment in thin Cu(Mn) films, we find a good agreement.

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Neutron Scattering and the B_{1g} Phonon in the Cuprates

The momentum dependent lineshape of the out-of-phase oxygen vibration as measured in recent neutron scattering measurements is investigated. Starting from a microscopic coupling of the phonon vibration to a local crystal field, the phonon lineshift and broadening is calculated as a function of transfered momentum in the superconducting state of YBa$_{2}$Cu$_{3}$O$_{7}$. It is shown that the anisotropy of the density of states, superconducting energy gap, and the electron-phonon coupling are all crucial in order to explain these experiments.

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Physical origin of the buckling in CuO$_2$: Electron-phonon coupling and Raman spectra

It is shown theoretically that the buckling of the CuO$_{2}$ planes in certain cuprate systems can be explained in terms of an electric field across the planes which originates from different valences of atoms above and below the plane. This field results also in a strong coupling of the Raman-active out-of-phase vibration of the oxygen atoms ($B_{1g}$ mode) to the electronic charge transfer between the two oxygens in the CuO$_{2}$ plane. Consequently, the electric field can be deduced from the Fano-type line shape of the $B_{1g}$ phonon. Using the electric field estimated from the electron-phonon coupling the amplitude of the buckling is calculated and found to be in good agreement with the structural data. Direct experimental support for the idea proposed is obtained in studies of YBa$_{2}$Cu$_{3}$O$_{6+x}$ and Bi$_{2}$Sr$_{2}$(Ca$_{1-x}$Y$_{x}$)Cu$_{2}$O$_{8}$ with different oxygen and yttrium doping, respectively, including antiferromagnetic samples. In the latter compound, symmetry breaking by replacing Ca partially by Y leads to an enhancement of the electron-phonon coupling by an order of magnitude.

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Enhanced Electron-Phonon Coupling and its Irrelevance to High T$_{c}$ Superconductivity

It is argued that the origin of the buckling of the CuO$_{2}$ planes in certain cuprates as well as the strong electron-phonon coupling of the $B_{1g}$ phonon is due to the electric field across the planes induced by atoms with different valence above and below. The magnitude of the electric field is deduced from new Raman results on YBa$_{2}$Cu$_{3}$O$_{6+x}$ and Bi$_{2}$Sr$_{2}$(Ca$_{1-x}$Y$_{x}$)Cu$_{2}$O$_{8}$ with different O and Y doping, respectively. In the latter case it is shown that the symmetry breaking by replacing Ca partially by Y enhances the coupling by an order of magnitude, while the superconducting $T_c$ drops to about two third of its original value.

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Comment on ``Point-Contact Study of Fast and Slow Two-Level Fluctuators in Metallic Glasses'' by Keijsers, Shklyarevskii and van Kempen

We point out that a recent experiment by Keijsers, Shklyarevskii and van Kempen [Phys. Rev. Lett. 77, 3411 (1996)] on metallic glass point contacts containing two-level systems (TLS) effectively measures for the first time the conductance contributions of individual TLSs (previous experiments averaged over a distribution of TLSs). For this case the predictions of the Kozub-Kulik theory for the TLS-electron interaction differ from those of the Vladar-Zawadowski theory, the latter giving much better agreement with experiment.

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Exotic Kondo Effects in Metals: Magnetic Ions in a Crystalline Electric Field and Tunneling Centers

This review article provides an overview of the physics of the two-channel Kondo impurity model as manifested in two-level systems in metals and certain actinide/lanthanide ions in metals. Basic models are presented, followed by a discussion of the multiplicative renormalization group, numerical renormalization group, non-crossing approximation, conformal field theory, abelian bosonization, and Bethe-ansatz approaches to the models. An extensive discussion of experiment is presented for both classes of models, with critical attention paid to the relevance of the models to the data. Finally, a last section details other models which are related, approaches to the lattice via two impurity and infinite dimension models, and the connection of these models to exotic odd-frequency superconductivity. Also available at http://onsager.ucdavis.edu/~cox/REVIEW/drmpmain2.ps.gz

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Spin-Orbit-Induced Magnetic Anisotropy for Impurities in Metallic Samples I. Surface Anisotropy

Motivated by the recent measurements of Kondo resistivity in thin films and wires, where the Kondo amplitude is suppressed for thinner samples, the surface anisotropy for magnetic impurities is studied. That anisotropy is developed in those cases where in addition to the exchange interaction with the impurity there is strong spin-orbit interaction for conduction electrons around the impurity in the ballistic region. The asymmetry in the neighborhood of the magnetic impurity exhibits the anisotropy axis $n$ which, in the case of a plane surface, is perpendicular to the surface. The anisotropy energy is $ΔE=K_d (nS)^2$ for spin $S$, and the anisotropy constant $K_d$ is inversionally proportional to distance $d$ measured from the surface and $K_d>0$. Thus at low temperature the spin is frozen in a singlet or doublet of lowest energy. The influence of that anisotropy on the electrical resistivity is the subject of the following paper (part II).

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Spin-Orbit-Induced Magnetic Anisotropy for Impurities in Metallic Samples II. Finite Size Dependence in the Kondo Resistivity

The electrical resistivity including the Kondo resistivity increase at low temperature is calculated for thin films of dilute magnetic alloys. Assuming that in the non-magnetic host the spin-orbit interaction is strong like in Au and Cu, the magnetic impurities have a surface anisotropy calculated in part I. That anisotropy hinders the motion of the spin. Including that anisotropy the effective electron-impurity coupling is calculated by using the second order renormalization group equations. The amplitude of the Kondo resistivity contribution is reduced as the position of the impurity approaches the surface but the increase occurs approximately at the bulk Kondo temperature. Different proximity effects observed by Giordano are also explained qualitatively where the films of magnetic alloys are covered by pure second films with different mean free path. The theory explains the experimental results in those cases where a considerable amount of impurities is at the surface inside the ballistic region.

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Instability of the marginal commutative model of tunneling centers interacting with metallic environment: Role of the electron-hole symmetry breaking

The role of the electron-hole symmetry breaking is investigated for a symmetrical commutative two-level system in a metal using the multiplicative renormalization group in a straightforward way. The role of the symmetries of the model and the path integral technique are also discussed in detail. It is shown that the electron-hole symmetry breaking may make the model non-commutative and generate the assisted tunneling process which is, however, too small itself to drive the system into the vicinity of the two-channel Kondo fixed point. While these results are in qualitative agreement with those of Moustakas and Fisher (Phys. Rev. B 51, 6908 (1995), ibid 53, 4300 (1996)) the scaling equations turn out to be essentially different. We show that the main reason for this difference is that the procedure for the elimination of the high energy degrees of freedom used by Moustakas and Fisher leaves only the free energy invariant, however, the couplings generated are not connected to the dynamical properties in a straightforward way and should be interpreted with care. These latter results might have important consequences in other cases where the path integral technique is used to produce the scaling equations and calculate physical quantities.

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Multiband Electronic Raman Scattering in Bilayer Superconductors

A theory of electronic Raman scattering in the presence of several energy bands crossing the Fermi surface is developed. The contributions to the light scattering cross section are calculated for each band and it is shown that the cross section can be written in terms of the sum of the single band contributions and a mixing term which only contributes to the fully symmetric channels $(A_{1g})$. Particular emphasis is placed on screening in bilayer superconductors. Since any charge fluctuation with long range character in real space is screened by the Coulomb interaction, the relevant fluctuations in a single layer case are induced between different parts of the Fermi surface. In a single band $d$-wave superconductor the scattering at energy transfer twice the maximum gap $Δ_{max}$ is dominated by those parts of the Fermi surface where $Δ^2({\bf k})$ is largest. As a consequence, the fully symmetric ($A_{1g}$) scattering is screened. In the case of a bilayer superconductor however, the charge transfer is possible between layers inside the unit cell. Therefore a formalism is considered which is valid for general band structure, superconducting energy gaps, and inter-layer hopping matrix elements. The spectra is calculated for La 2:1:4 and Y 1:2:3 as representative single and bilayer superconductors. The mixing term is found to be negligible and thus the response is well approximated by the sum of the contributions from the individual bands. The theory imposes strong constraints on both the magnitude and symmetry of the energy gap for the bilayer cuprates, and indicates that a nearly identical energy gap of $d_{x^{2}-y^{2}}$ symmetry provides a best fit to the data. However, the $A_{1g}$ part of the spectrum depends sensitively on many parameters.

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Charge transfer fluctuation, $d-$wave superconductivity, and the $B_{1g}$ Raman phonon in the Cuprates: A detailed analysis

The Raman spectrum of the $B_{1g}$ phonon in the superconducting cuprate materials is investigated theoretically in detail in both the normal and superconducting phases, and is contrasted with that of the $A_{1g}$ phonon. A mechanism involving the charge transfer fluctuation between the two oxygen ions in the CuO$_2$ plane coupled to the crystal field perpendicular to the plane is discussed and the resulting electron-phonon coupling is evaluated. Depending on the symmetry of the phonon the weight of different parts of the Fermi surface in the coupling is different. This provides the opportunity to obtain information on the superconducting gap function at certain parts of the Fermi surface. The lineshape of the phonon is then analyzed in detail both in the normal and superconducting states. The Fano lineshape is calculated in the normal state and the change of the linewidth with temperature below T$_{c}$ is investigated for a $d_{x^{2}-y^{2}}$ pairing symmetry. Excellent agreement is obtained for the $B_{1g}$ phonon lineshape in YBa$_{2}$Cu$_{3}$O$_{7}$. These experiments, however, can not distinguish between $d_{x^{2}-y^{2}}$ and a highly anisotropic $s$-wave pairing.

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Theory of Orbital Kondo Effect with Assisted Hopping in Strongly Correlated Electron Systems: Parquet Equations, Superconductivity and Mass Enhancement

Orbital Kondo effect is treated in a model, where additional to the conduction band there are localized orbitals close to the Fermi energy. If the hopping between the conduction band and the localized heavy orbitals depends on the occupation of the atomic orbitals in the conduction band then orbital Kondo correlation occurs. The noncommutative nature of the coupling required for the Kondo effect is formally due to the form factors associated with the assisted hopping which in the momentum representation depends on the momenta of the conduction electrons involved. The leading logarithmic vertex corrections are due to the local Coulomb interaction between the electrons on the heavy orbital and in the conduction band. The renormalized vertex functions are obtained as a solution of a closed set of differential equations and they show power behavior. The amplitude of large renormalization is determined by an infrared cutoff due to finite energy and dispersion of the heavy particles. The enhanced assisted hopping rate results in mass enhancement and attractive interaction in the conduction band. The superconductivity transition temperature calculated is largest for intermediate mass enhancement, $m^*/m \approx 2-3$. For larger mass enhancement the small one particle weight ($Z$) in the Green's function reduces the transition temperature which may be characteristic for other

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