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A. Zdeb

Publications and source records attributed to A. Zdeb.

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Microscopic description of cluster radioactivity fission valleys along isotopic and isotonic chains

Cluster radioactivity has been successfully described as a super-asymmetric fission mode within the microscopic self-consistent Gogny Hartree-Fock-Bogoliubov approximation [Phys. Rev. C 84, 044608 (2011)]. For nuclei preserving the neutron-to-proton $N/Z$ ratio of the doubly magic $^{208}$Pb, a cluster radioactivity fission valley has been identified. Such a valley can also be found both in actinides and super-heavy nuclei. In this paper, chains of isotopes and isotones are examined to determine the limits of existence of the cluster radioactivity fission mode. It is shown that the super-asymmetric valley can be found in a wide range of the nuclear chart. Nevertheless, the valley flattens more and more when diverging from the isospin asymmetry of $^{208}$Pb. For neutron-deficient nuclei with $N/Z <$ 1.41, it is found that the valley diminishes before reaching the scission point, and cluster radioactivity can not be observed.

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Microscopic pairing in fission dynamics

Nuclear fission can be modelled as a quantum tunneling process driven by the interplay between the nuclear binding energy and the collective inertia. Within the Wentzel-Kramers-Brillouin formalism, spontaneous fission half-lives can be obtained by minimizing the action integral in the multidimensional space of collective degrees of freedom. Hence, including the relevant collective variables is crucial for properly describing spontaneous fission probabilities. Pairing correlations play an essential role in this evaluation since the collective inertia decreases as the inverse of the square of the pairing gap, and, therefore, they should be considered as a relevant degree of freedom on the same footing as deformation parameters. In this work, we show that the spontaneous fission half-lives in fermium isotopes can be reproduced in a microscopic theory by considering the least-action fission path in a two-dimensional space with constraints on the quadrupole moment and pairing correlations. We consider two microscopic quantities as degrees of freedom associated with pairing: the pairing gap parameter $\Delta$, and the particle number fluctuations $\langle \Delta N^2 \rangle$. Least-action paths, computed using the Dijkstra algorithm, are compared with minimum-energy paths, highlighting the importance of pairing correlations as a dynamical degree of freedom.

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HFB3: an axial HFB solver with Gogny forces using a 2-center HO basis (C++/Python)

The HFB3 program solves the axial nuclear Hartree-Fock-Bogoliubov (HFB) equations using bases formed by either one or two sets of deformed Harmonic Oscillator (HO) solutions with D1-type and D2-type Gogny effective nucleon-nucleon interactions. Using two sets of HO solutions shifted along the z-axis (2-center basis) allows to accurately describe highly elongated nuclear systems while keeping a moderate basis size, making this type of basis very convenient for the description of the nuclear fission process. For the description of odd-even and odd-odd systems, the equal-filling-approximation is used. Several observables can be calculated by the program, including the mean values of the multipole moments, nuclear radii, inertia tensors following Adiabatic Time-Dependent Hartree-Fock-Bogoliubov (ATDHFB) or Generator Coordinate Method (GCM) prescriptions, local and non-local one-body densities, local and non-local pairing densities, some fission fragment properties, etc. The program can ensure that the mean values associated with some specific operators take pre-defined values (constraints). Such constraints can be set on the usual multipole moments (for protons, neutrons or total mass). This program can be used as a monoprocess and monothreaded CLI executable, or through full-featured Python bindings (available through the Python Package Index PyPI).

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Pairing in fission: Mean-field and collective inertias study

Pairing plays a crucial role in the microscopic description of nuclear fission. Microscopic methods provide access to three quantities related to pairing, namely, the pairing gap ($\Delta$), the particle number fluctuations ($ \Delta \hat{N}^2 $), and the quenching factor (QF). The aim of this work is to analyse the impact of each of these quantities on the static description of the fission process.

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Fission Fragment Mass and Kinetic Energy Yields of Fermium Isotopes

A rapidly converging 4-dimensional Fourier shape parametrization is used to model the fission process of heavy nuclei. Potential energy landscapes are computed within the macroscopic-microscopic approach, on top of which the multi-dimensional Langevin equation is solved to describe the fission dynamics. Charge equilibration at scission and de-excitation by neutron evaporation of the primary fragments after scission is investigated. The model describes various observables, including fission-fragment mass, charge, and kinetic energy yields, as well as post-scission neutron multiplicities and, most importantly, their correlations, which are crucial to unravel the complexity of the fission process. The parameters of the dynamical model were tuned to reproduce experimental data obtained from thermal neutron-induced fission of $^{235}$U, which allows us to discuss the transition from asymmetric to symmetric fission along the Fm isotopic chain.

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Spontaneous fission half-lives of actinides and super-heavy elements

Spontaneous fission half-lives of actinide and super-heavy nuclei are calculated, using the least-action integral, through the WKB tunneling probability of the barrier that appears in the deformation landscape obtained in the macroscopic-microscopic potential-energy surface. This deformation-energy landscape is obtained using a Fourier shape parametrization with 4 deformation parameters, taking into account the nuclear elongation, left-right asymmetry, neck formation and non-axiality degrees of freedom. The collective inertia tensor entering the WKB half-life expression is given through the so-called irrotational flow approach, successfully used in nuclear fission to reproduce observables that characterize the nuclear system in the vicinity of the scission configurations, such as fragment mass or charge distributions. For a comparisons, we have also used the so-called phenomenological mass parameter depending only on the center-of-mass difference of the forming fission fragments. Our approach is shown to be able to reproduce empirical fission half-lives of all here considered nuclei to within 3 orders of magnitude.

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Scission configuration in the self-consistent calculations with neck constraint

The calculations of the potential energy surface are essential in the theoretical description of the fission process. In the constrained self-consistent approach, the smooth evolution of nuclear shape is described from the ground state until a very elongated one with a narrow neck. In all microscopic calculations, the rupture of the neck at scission is associated with a substantial change of nuclear matter density distribution and rapid energy decrease. In this paper, we show that there is no discontinuity of the potential energy surface at scission when multi-constrained calculations are applied with the neck constraint. An early rupture of the neck at lower quadrupole and octupole moments is discussed as competitive with the conventional fission path. We discuss the neck properties in the scission configuration. We find that the neck radius in the asymmetric fission mode cannot decrease below 2 fm, and the nuclear matter density cannot decrease below the saturation density. In the compact fission mode, nuclear density may go down to half of the saturation density before the rupture of the neck.

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Description of the multidimensional potential energy surface in fission of $^{252}$Cf and $^{258}$No

The microscopic studies on nuclear fission require the evaluation of the potential energy surface as a function of the collective coordinates. A reasonable choice of constraints on multipole moments should be made to describe the topography of the surface completely within a reasonable amount of computing time. We present a detailed analysis of fission barriers in the self-consistent Hartree-Fock-Bogoliubov approach with the D1S parametrization of the Gogny nucleon-nucleon interaction. Two heavy isotopes representing different spontaneous fission modes - $^{252}$Cf (asymmetric) and $^{258}$No (bimodal) - have been chosen for the analysis. We have shown the existence of complicated structures on the energy surface that can not be fully described in two-dimensional calculations. We analyze apparent problems that can be encountered in this type of calculations: multiple solutions for given constraints and transitions between various potential energy surfaces. We present possible solutions on how to deal with these issues.

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Cluster Radioactivity in Super Heavy Nuclei

Cluster radioactivity is an exotic nuclear decay observed in actinides where a light nucleus is emitted while the remaining heavy mass residue is the doubly magic $^{208}$Pb or a nucleus in its neighborhood. We have investigated this type of decay in heavier nuclei up to Lv $(Z=116)$ within a microscopic theory. It has been found that super asymmetric fission with $^{208}$Pb as heavy fragment may be dominant decay channel in some super heavy nuclei. This reaction is closely related with cluster radioactivity.

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Fission dynamics of $^{252}$Cf

The time-dependent generator coordinate method with the gaussian overlap approximation (TDGCM+GOA) formalism is applied to describe the fission of $^{252}$Cf. We perform analysis of fission from the initial states laying in the energetic range from the ground state to the state located 4 MeV above the fission barrier. The fission fragment mass distributions, obtained for different parity, energy of levels and types of mixed states, are calculated and compared with experimental data. The impact of the total time of wave packet propagation on the final results is studied as well. The weak dependence of obtained mass yields on the initial conditions is shown.

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Fission fragment mass yield deduced from density distribution in the pre-scission configuration

Static self-consistent methods usually allow to determine the most probable fission fragments mass asymmetry. We have applied random neck rupture mechanism to the nuclei in the configuration at the end of fission paths. Fission fragment mass distributions have been deduced from the pre-scission nuclear density distribution obtained from the self-consistent calculations. Potential energy surfaces as well as nuclear shapes have been calculated in the fully microscopic theory, namely the constrained Hartree-Fock-Bogolubov model with the effective Gogny D1S density-dependent interaction. The method has been applied for analysis of fission of Fm-256,258, Cf-252 and Hg-180 and compared with the experimental data.

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On spontaneous fission and alpha-decay half-lives of atomic nuclei

It is shown, that the Gamow-like model with only one adjustable parameter - radius constant is able to reproduce well the alpha-decay half-lives for all even-even nuclei with the proton number larger than 50. The systematics for odd-A and odd-odd isotopes can be also well described when ones introduces an additional hindrance factor. Similar model based on the W. J. Swiatecki idea from 1955 is developed to reproduce the spontaneous fission half-lives of transactinide nuclei. The achieved accuracy of reproduction of the data is better than that obtained in more advanced theories.

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Spontaneous fission half-lives of nuclei in a phenomenological model

A simple phenomenological model, based on the Świ{\c a}tecki idea for evaluation of the spontaneous fission half-lives is proposed. The model contains only one adjustable parameter fixed to the data for even-even nuclei and two additional hindrance factors to the life-times, which give the effect of odd particles. A good agreement with the experimental data for all fissioning nuclei is achieved.

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