arXiv subjects

A. Zilges

Publications and source records attributed to A. Zilges.

At least 19 recordsLinked to original sources

arXiv2025

Deviations from the Porter-Thomas Distribution due to Nonstatistical $\gamma$ Decay below the $^{150}$Nd Neutron Separation Threshold

We introduce a new method for the study of fluctuations of partial transition widths based on nuclear resonance fluorescence experiments with quasimonochromatic linearly polarized photon beams below particle separation thresholds. It is based on the average branching of decays of $J=1$ states of an even-even nucleus to the $2^+_1$ state in comparison to the ground state. Between 5 and 7 MeV, a constant average branching ratio for $\gamma$ decays from $1^-$ states of 0.490(16) is observed for the nuclide $^{150}$Nd. Assuming $\chi^2$-distributed partial transition widths, this average branching ratio is related to a degree of freedom of $\nu = 1.93(12)$, rejecting the validity of the Porter-Thomas distribution, requiring $\nu=1$. The observed deviation can be explained by nonstatistical effects in the $\gamma$-decay behavior with contributions in the range of 9.4(10)% up to 94(10)%.

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arXiv2023

Direct demonstration of the two-phonon structure of the $J^{\pi} = 1_{4742~\mathrm{keV}}^{-}$ state of $^{88}$Sr

We have studied the decay pattern of the $J^{\pi} = 1_{4742~\mathrm{keV}}^{-}$ state of $^{88}$Sr to probe its quadrupole-octupole coupled two-phonon structure. In particular, a unique fingerprint to prove the two-phonon nature is the $E2$ decay strength of the $1_{4742~\mathrm{keV}}^{-} \to 3_{1}^{-}$ transition into the one-octupole-phonon state. $\gamma$-ray spectroscopy was performed after the $\beta$-decay of $^{88}$Rb to obtain the necessary sensitivity for this weak-intensity decay branch. Sufficient amounts of $^{88}$Rb (T$_{1/2}$ = 17.8 min) were produced by neutron activation of natural Rb in the TR IGA Mark II reactor. The results show that the $B(E2)$ value of the $1_{4742~\mathrm{keV}}^{-} \to 3_{1}^{-}$ transition is equal to the $B(E2)$ of the $2_{1}^{+} \to 0_{1}^{+}$ transition, directly demonstrating the quadrupole-octupole coupled two-phonon nature of the $1^-$ state. A comparison of the results with energy-density functional plus quasiparticle-phonon model calculations shows rema rkable agreement, corroborating this assignment.

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arXiv2023

Experimental study of excited states of ${}^{62}$Ni via one-neutron $(d,p)$ transfer up to the neutron-separation threshold and characteristics of the pygmy dipole resonance states

The degree of collectivity of the Pygmy Dipole Resonance (PDR) is an open question. Recently, Ries {\it et al.} have suggested the onset of the PDR beyond $N=28$ based on the observation of a significant $E1$ strength increase in the Cr isotopes and proposed that the PDR has its origin in a few-nucleon effect. Earlier, Inakura {\it et al.} had predicted by performing systematic calculations using the random-phase approximation (RPA) with the Skyrme functional SkM* that the $E1$ strength of the PDR strongly depends on the position of the Fermi level and that it displays a clear correlation with the occupation of orbits with orbital angular momenta less than $3\hbar$ $(l \leq 2)$. To further investigate the microscopic structures causing the possible formation of a PDR beyond the $N=28$ neutron shell closure, we performed a $^{61}$Ni$(d,p){}^{62}$Ni experiment at the John D. Fox Superconducting Linear Accelerator Laboratory of Florida State University. To determine the angular momentum transfer populating possible $J^{\pi} = 1^-$ states and other excited states of ${}^{62}$Ni, angular distributions and associated single-neutron transfer cross sections were measured with the Super-Enge Split-Pole Spectrograph. A number of $J^{\pi} = 1^-$ states were observed below the neutron-separation threshold after being populated through $l=2$ angular momentum transfers. A comparison to available $(\gamma,\gamma')$ data for ${}^{58,60}$Ni provides evidence that the $B(E1)$ strength shifts further down in energy. The $(d,p)$ data clearly prove that $l=0$ strength, i.e., the neutron $(2p_{3/2})^{-1}(3s_{1/2})^{+1}$ one-particle-one-hole configuration plays only a minor role for $1^-$ states below the neutron-separation threshold in ${}^{62}$Ni.

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arXiv2020

International Workshop on Next Generation Gamma-Ray Source

A workshop on The Next Generation Gamma-Ray Sources sponsored by the Office of Nuclear Physics at the Department of Energy, was held November 17--19, 2016 in Bethesda, Maryland. The goals of the workshop were to identify basic and applied research opportunities at the frontiers of nuclear physics that would be made possible by the beam capabilities of an advanced laser Compton beam facility. To anchor the scientific vision to realistically achievable beam specifications using proven technologies, the workshop brought together experts in the fields of electron accelerators, lasers, and optics to examine the technical options for achieving the beam specifications required by the most compelling parts of the proposed research programs. An international assembly of participants included current and prospective $γ$-ray beam users, accelerator and light-source physicists, and federal agency program managers. Sessions were organized to foster interactions between the beam users and facility developers, allowing for information sharing and mutual feedback between the two groups. The workshop findings and recommendations are summarized in this whitepaper.

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arXiv2020

Accessing the Single-Particle Structure of the Pygmy Dipole Resonance in $^{208}$Pb

New experimental data on the neutron single-particle character of the Pygmy Dipole Resonance (PDR) in $^{208}$Pb are presented. They were obtained from $(d,p)$ and resonant proton scattering experiments performed at the Q3D spectrograph of the Maier-Leibnitz Laboratory in Garching, Germany. The new data are compared to the large suite of complementary, experimental data available for $^{208}$Pb and establish $(d,p)$ as an additional, valuable, experimental probe to study the PDR and its collectivity. Besides the single-particle character of the states, different features of the strength distributions are discussed and compared to Large-Scale-Shell-Model (LSSM) and energy-density functional (EDF) plus Quasiparticle-Phonon Model (QPM) theoretical approaches to elucidate the microscopic structure of the PDR in $^{208}$Pb.

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arXiv2020

Probing the Z = 6 spin-orbit shell gap with (p,2p) quasi-free scattering reactions

The evolution of the traditional nuclear magic numbers away from the valley of stability is an active field of research. Experimental efforts focus on providing key spectroscopic information that will shed light into the structure of exotic nuclei and understanding the driving mechanism behind the shell evolution. In this work, we investigate the Z = 6 spin-orbit shell gap towards the neutron dripline. To do so, we employed $^{A}$N(p,2p)$^{A-1}$C quasi-free scattering reactions to measure the proton component of the 2$^+_1$ state of $^{16,18,20}$C. The experimental findings support the notion of a moderate reduction of the proton 1p$_{1/2}$-1p$_{3/2}$ spin-orbit splitting, at variance to recent claims for a prevalent Z = 6 magic number towards the neutron dripline.

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arXiv2020

Experimental techniques to study the $γ$ process for nuclear astrophysics at the Cologne accelerator laboratory

The nuclear astrophysics setup at the Institute for Nuclear Physics, University of Cologne, Germany is dedicated to measurements of total and partial cross sections of charged-particle induced reactions at astrophysically relevant energies. These observables are key ingredients for reaction network calculations of various stellar scenarios, and crucial for the understanding of the nucleosynthesis of elements. The experiments utilize the high-efficiency $γ$-ray spectrometer HORUS, and the 10 MV FN-Tandem accelerator. An updated target chamber as well as further experimental methods established in the last years will be presented which allow to measure cross sections down to the nb region. The reliability of the measured cross sections is proven by a $^{89}$Y(p,$γ$)$^{90}$Zr commissioning experiment. Additionally, an application for nuclear astrophysics will be presented. The results of a $^{93}$Nb(p,$γ$)$^{94}$Mo experiment will be discussed as well as their deviations compared to formerly reported results.

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arXiv2018

Fine structure of the pygmy quadrupole resonance in $^{112,114}$Sn isotopes

The electric quadrupole response in $^{112,114}$Sn isotopes is investigated by energy-density functional (EDF) and three-phonon quasiparticle-phonon model (QPM) theory with special emphasis on 2$^+$ excitations located above the first collective quadrupole state and below 5 MeV. Additional quadrupole strength clustering as a sequence of states similar to the recently observed pygmy quadrupole resonance in $^{124}$Sn is found. The spectral distributions and transition densities of these 2$^+$ states show special features being compatible with oscillations of a neutron skin against the isospin-symmetric nuclear core. Furthermore, two new ($p$, $p' γ$) Doppler-shift attenuation (DSA) coincidence experiments were performed at the SONIC@HORUS setup. Quadrupole states with excitation energies up to 4.2 MeV were populated in $^{112,114}$Sn. Lifetimes and branching ratios were measured allowing for the determination of the reduced quadrupole transition strengths to the ground state. A stringent comparison of the new data to EDF+QPM theory in $^{112}$Sn and $^{114}$Sn isotopes hints at the occurrence of a low-energy quadrupole mode of unique character which could be interpreted as pygmy quadrupole resonance.

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arXiv2018

Shape coexisistence and collective low-spin states in $^{112,114}$Sn studied with the $(p,p'γ)$ DSA coincidence technique

Proton-scattering experiments followed by the coincident spectroscopy of $γ$ rays have been performed at the Institute for Nuclear Physics of the University of Cologne to excite low-spin states in $^{112}$Sn and $^{114}$Sn, to determine their lifetimes and extract reduced transitions strengths $B(ΠL)$. The combined spectroscopy setup SONIC@HORUS has been used to detect the scattered protons and the emitted $γ$ rays of excited states in coincidence. The novel $(p,p'γ)$ DSA coincidence technique was employed to measure sub-ps nuclear level lifetimes. 74 level lifetimes $τ$ of states with $J = 0 - 6$ were determined. In addition, branching ratios were deduced which allowed the investigation of the intruder configuration in both nuclei. Here, $sd$ IBM-2 mixing calculations were added which support the coexistence of the two configurations. Furthermore, members of the expected QOC quintuplet are proposed in $^{114}$Sn for the first time. The $1^-$ candidate in $^{114}$Sn fits perfectly into the systematics observed for the other stable Sn isotopes. The $E2$ transition strengths observed for the low-spin members of the so-called intruder band support the existence of shape coexistence in $^{112,114}$Sn. The collectivity in this configuration is comparable to the one observed in the Pd nuclei, i.e. the 0p-4h nuclei. Strong mixing between the $0^+$ states of the normal and intruder configuration might be observed in $^{114}$Sn. The general existence of QOC states in $^{112,114}$Sn is supported by the observation of QOC candidates with $J \neq 1$.

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arXiv2018

High-resolution $(p,t)$ study of low-spin states in $^{240}$Pu: Octupole excitations, $α$ clustering, and other structure features

A high-resolution $(p,t)$ experiment at $E_{p}$= 24 MeV was performed to populate low-spin states in the actinide nucleus ${}^{240}$Pu. The Q3D magnetic spectrograph of the Maier-Leibnitz Laboratory (MLL) in Munich (Germany) was used to identify the ejected tritons via $dE/E$ particle identification with its focal-plane detection system. Angular distributions were measured at nine different Q3D angles to assign spin and parity to the excited states based on a comparison with coupled-channels DWBA calculations. In total, 209 states have been excited in $^{240}$Pu up to an excitation energy of 3 MeV. Many previously known states have also been observed and their spin-parity assignments were confirmed. However, many of the populated states have been seen for the first time. The low-spin one-octupole phonon excitations, i.e. $K^π = 0^-,1^-,2^-,3^-$, could be observed and a new candidate for the $K = 3$ projection is proposed. Furthermore, the double-octupole or $α$-cluster structure of the $0^+_2$ state in $^{240}$Pu has been studied in more detail. It is shown that the $0^+_2$ state in $^{230}$Th has a distinctly different structure. In addition, strongly excited $1^-$ states have been observed at 1.5\,MeV and 1.8\,MeV in $^{240}$Pu. The present study suggests that similar states might be observed in $^{230}$Th. At least two different and distinct structures for $J^π = 0^+$ states are present in the actinides. These are pairing states and states with enhanced octupole correlations. We have shown that it is crucial to consider negative-parity single-particle states being admixed to some $K^π = 0^+_2$ rotational bands to understand the $α$-decay hindrance factors and enhanced $E1$-decay rates. Based on our analysis, we have identified the double-octupole or $α$-cluster $K^π = 0^+$ candidates from $^{224}$Ra to $^{240}$Pu.

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arXiv2017

Combining γ-ray and particle spectroscopy with SONIC@HORUS

The particle spectrometer SONIC for particle-$γ$ coincidence measurements was commissioned at the Institute for Nuclear Physics in Cologne, Germany. SONIC consists of up to 12 silicon $\mathitΔE$-$E$ telescopes with a total solid angle coverage of 9%, and will complement HORUS, a $γ$-ray spectrometer with 14 HPGe detectors. The combined setup SONIC@HORUS is used to investigate the $γ$-decay behaviour of low-spin states up to the neutron separation threshold excited by light-ion inelastic scattering and transfer reactions using beams provided by a 10 MV FN Tandem accelerator. The particle-$γ$ coincidence method will be presented using data from a $^{92}$Mo(p,p'$γ$) experiment. In a $^{119}$Sn(d,X) experiment, excellent particle identification has been achieved because of the good energy resolution of the silicon detectors of approximately 20 keV. Due to the non-negligible momentum transfer in the reaction, a Doppler correction of the detected $γ$-ray energy has to be performed, using the additional information from measuring the ejectile energy and direction. The high sensitivity of the setup is demonstrated by the results from a $^{94}$Mo(p,p'$γ$) experiment, where small $γ$-decay branching ratios have been deduced.

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arXiv2016

The decay of quadrupole-octupole $1^-$ states in $^{40}$Ca and $^{140}$Ce

Background: Two-phonon excitations originating from the coupling of two collective one-phonon states are of great interest in nuclear structure physics. One possibility to generate low-lying $E1$ excitations is the coupling of quadrupole and octupole phonons. Purpose: In this work, the $γ$-decay behavior of candidates for the $(2_1^+\otimes 3_1^-)_{1^-}$ state in the doubly-magic nucleus $^{40}$Ca and in the heavier and semi-magic nucleus $^{140}$Ce is investigated. Methods: $(\vecγ,γ')$ experiments have been carried out at the High Intensity $γ$-ray Source (HI$γ$S) facility in combination with the high-efficiency $γ$-ray spectroscopy setup $γ^3$ consisting of HPGe and LaBr$_3$ detectors. The setup enables the acquisition of $γ$-$γ$ coincidence data and, hence, the detection of direct decay paths. Results: In addition to the known ground-state decays, for $^{40}$Ca the decay into the $3^-_1$ state was observed, while for $^{140}$Ce the direct decays into the $2^+_1$ and the $0^+_2$ state were detected. The experimentally deduced transition strengths and excitation energies are compared to theoretical calculations in the framework of EDF theory plus QPM approach and systematically analyzed for $N=82$ isotones. In addition, negative parities for two $J=1$ states in $^{44}$Ca were deduced simultaneously. Conclusions: The experimental findings together with the theoretical calculations support the two-phonon character of the $1^-_1$ excitation in the light-to-medium-mass nucleus $^{40}$Ca as well as in the stable even-even $N=82$ nuclei.

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arXiv2016

Magnetic dipole excitations of $^{50}$Cr

The low-lying $M1$-strength of the open-shell nucleus $^{50}$Cr has been studied with the method of nuclear resonance fluorescence up to 9.7 MeV, using bremsstrahlung at the superconducting Darmstadt linear electron accelerator S-DALINAC and Compton backscattered photons at the High Intensity $γ$-ray Source (HI$γ$S) facility between 6 and 9.7 MeV of the initial photon energy. Fifteen $1^{+}$ states have been observed between 3.6 and 9.7 MeV. Following our analysis, the lowest $1^{+}$ state at 3.6 MeV can be considered as an isovector orbital mode with some spin admixture. The obtained results generally match the estimations and trends typical for the scissors-like mode. Detailed calculations within the Skyrme Quasiparticle Random-Phase-Approximation method and the Large-Scale Shell Model justify our conclusions. The calculated distributions of the orbital current for the lowest $1^{+}$-state suggest the schematic view of Lipparini and Stringari (isovector rotation-like oscillations inside the rigid surface) rather than the scissors-like picture of Lo Iudice and Palumbo. The spin M1 resonance is shown to be mainly generated by spin-flip transitions between the orbitals of the $fp$-shell.

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arXiv2015

Lifetime measurement of excited low-spin states via the $(p,p^{\prime}γ$) reaction

In this article a method for lifetime measurements in the sub-picosecond regime via the Doppler-shift attenuation method (DSAM) following the inelastic proton scattering reaction is presented. In a pioneering experiment we extracted the lifetimes of 30 excited low-spin states of $^{96}$Ru, taking advantage of the coincident detection of scattered protons and de-exciting $γ$-rays as well as the large number of particle and $γ$-ray detectors provided by the SONIC@HORUS setup at the University of Cologne. The large amount of new experimental data shows that this technique is suited for the measurement of lifetimes of excited low-spin states, especially for isotopes with a low isotopic abundance, where $(n,n^{\prime}γ$) or - in case of investigating dipole excitations - ($γ,γ^{\prime}$) experiments are not feasible due to the lack of sufficient isotopically enriched target material.

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arXiv2015

Origin of Low-Lying Enhanced E1 Strength in Rare-Earth Nuclei

The experimental $E1$ strength distribution below 4 MeV in rare-earth nuclei suggests a local breaking of isospin symmetry. In addition to the octupole states, additional $1^-$ states with enhanced E1 strength have been observed in rare-earth nuclei by means of ($γ,γ'$) experiments. By reproducing the experimental results, the spdf interacting boson model calculations provide further evidence for the formation of an $α$ cluster in medium-mass nuclei and might provide a new understanding of the origin of low-lying E1 strength.

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arXiv2015

The 106Cd(alpha,alpha)106Cd elastic scattering in a wide energy range for gamma-process studies

Alpha elastic scattering angular distributions of the 106Cd(alpha,alpha)106Cd reaction were measured at three energies around the Coulomb barrier to provide a sensitive test for the alpha + nucleus optical potential parameter sets. Furthermore, the new high precision angular distributions, together with the data available from the literature were used to study the energy dependence of the locally optimized α+nucleus optical potential in a wide energy region ranging from E_Lab = 27.0 MeV down to 16.1 MeV. The potentials under study are a basic prerequisite for the prediction of alpha-induced reaction cross sections and thus, for the calculation of stellar reaction rates used for the astrophysical gamma process. Therefore, statistical model predictions using as input the optical potentials discussed in the present work are compared to the available 106Cd + alpha cross section data.

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arXiv2015

Experimental constraints on the $γ$-ray strength function in $^{90}$Zr using partial cross sections of the $^{89}$Y(p,$γ$)$^{90}$Zr reaction

Partial cross sections of the $^{89}$Y(p,$γ$)$^{90}$Zr reaction have been measured to investigate the $γ$-ray strength function in the neutron-magic nucleus $^{90}$Zr. For five proton energies between $E_p=3.65$ MeV and $E_p=4.70$ MeV, partial cross sections for the population of seven discrete states in $^{90}$Zr have been determined by means of in-beam $γ$-ray spectroscopy. Since these $γ$-ray transitions are dominantly of $E1$ character, the present measurement allows an access to the low-lying dipole strength in $^{90}$Zr. A $γ$-ray strength function based on the experimental data could be extracted, which is used to describe the total and partial cross sections of this reaction by Hauser-Feshbach calculations successfully. Significant differences with respect to previously measured strength functions from photoabsorption data point towards deviations from the Brink-Axel hypothesis relating the photo-excitation and de-excitation strength functions.

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arXiv2015

Total and partial cross sections of the $^{112}$Sn($α,γ$)$^{116}$Te reaction measured via in-beam $γ$-ray spectroscopy

An extended database of experimental data is needed to address uncertainties of the nuclear-physics input parameters for Hauser-Feshbach calculations. Especially $α$+nucleus optical model potentials at low energies are not well known. The in-beam technique with an array of high-purity germanium (HPGe) detectors was successfully applied to the measurement of absolute cross sections of an ($α$,$γ$) reaction on a heavy nucleus at sub-Coulomb energies. The total and partial cross-section values were measured by means of in-beam $γ$-ray spectroscopy. Total and partial cross sections were measured at four different $α$-particle energies from $E_α= 10.5$ MeV to $E_α= 12$ MeV. The measured total cross-section values are in excellent agreement with previous results obtained with the activation technique, which proves the validity of the applied method. The experimental data was compared to Hauser-Feshbach calculations using the nuclear reaction code TALYS. A modified version of the semi-microscopic $α$+nucleus optical model potential OMP 3, as well as modified proton and $γ$ widths, are needed in order to obtain a good agreement between experimental data and theory. It is found, that a model using a local modification of the nuclear-physics input parameters simultaneously reproduces total cross sections of the $^{112}$Sn($α$,$γ$) and $^{112}$Sn($α$,p) reactions. The measurement of partial cross sections turns out to be very important in this case in order to apply the correct $γ$-ray strength function in the Hauser-Feshbach calculations. The model also reproduces cross-section values of $α$-induced reactions on $^{106}$Cd, as well as of ($α$,n) reactions on $^{115,116}$Sn, hinting at a more global character of the obtained nuclear-physics input.

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