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Aavishkar A. Patel

Publications and source records attributed to Aavishkar A. Patel.

At least 19 recordsLinked to original sources

Extended strange metal regime in a pure nematic quantum critical superconductor

High-temperature superconductivity often emerges from a strange metallic state, where the electrical resistivity exhibits a linear-in-temperature dependence over an anomalously extended temperature range. The prevailing belief is that magnetic critical fluctuations gives rise to strange metallicity, enhancing the superconducting transition temperature. Here, using high pulsed magnetic fields, we have uncovered the strange metallic ground state hidden below the superconducting dome of nonmagnetic FeSe$_{1-x}$Te$_{x}$, which harbors a quantum critical point (QCP) of pure electronic nematicity, characterized by spontaneous rotational symmetry breaking. Unlike the conventional quantum criticality, this strange metallic state does not appear in a fan-shaped region above the singular QCP but spans a wide compositional range, where pairing interactions are strengthened by nonmagnetic nematic critical fluctuations. This stands in sharp contrast to the much cleaner system FeSe$_{1-x}$S$_{x}$, which displays a quantum critical fan above nematic QCP, indicating that disorder-induced spatial randomness of the nematic fluctuations likely enlarges the QCP of FeSe$_{1-x}$Te$_{x}$ into an extended region of criticality, as suggested by relevant hybrid Quantum Monte Carlo simulations. These observations highlight superconductivity promoted by a unique interplay between pure nematic critical fluctuations, strange metallicity and disorder, providing new insight into the emergence of non-Fermi-liquid transport in various correlated materials.

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Influence of Harris disorder on quantum-critical superconductivity

In the Hertz theory, a quantum critical metal is described by the coupling of a Fermi surface to fluctuations of a Landau-damped bosonic field $ϕ$, which may represent either an order parameter or a Higgs field for a transition without symmetry breaking. Scattering from $ϕ$ produces non-Fermi-liquid behavior in the normal state, while the same fluctuations mediate enhanced Cooper pairing. By the Harris criterion, symmetry-preserving disorder couples most strongly to the coefficient of the $ϕ^2$ term, locally tuning the system toward or away from criticality. This random mass (``Harris disorder'') leads to a finite density of localized low-energy $ϕ$ modes even when the fermionic states remain extended and continue to provide Landau damping. We study the onset of pairing mediated by these localized overdamped bosonic modes. Starting from a real-space linearized Usadel equation for the two-particle propagator, we show that the localized bosonic wave functions generate both a spatially random pairing vertex and an effective random potential for Cooper pairs. Numerical solution, a self-consistent Born approximation, and Lifshitz-tail analysis reveal two regimes of the pairing instability. At high temperatures, pairing nucleates compact superconducting puddles on the most localized bosonic modes. At lower temperatures, an extended pairing eigenstate appears, but its transition scale and spatial structure remain strongly affected by mesoscopic correlation effects and enhanced probability of returns to favorable regions of the localized bosonic glue. The resulting distribution of local pairing scales has a power-law tail, in contrast to the stretched-exponential tails of disordered BCS superconductors. This mechanism provides a route to broad gap inhomogeneity and superconducting puddles in quantum-critical metals, and offers an interpretation of STM measurements of the cuprates.

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Fractionalized Fermi liquids and the cuprate phase diagram

We review a theoretical framework for the cuprate superconductors, rooted in a fractionalized Fermi liquid (FL*) description of the intermediate-temperature pseudogap phase at low doping. The FL* theory predicted hole pockets each of fractional area $p/8$ at hole doping $p$, in contrast to the area $p/4$ in spin density wave theory. Magnetotransport measurements, including observation of the Yamaji angle, show clear evidence of hole pocket quasiparticles which can tunnel coherently between square lattice layers, and are consistent with the FL* description. The FL* phase of a single-band model is described using a layer construction with a pair of ancilla qubits on each site: the Ancilla Layer Model (ALM). Fluctuations are described by the SU(2) gauge theory of a background spin liquid with critical Dirac spinons. A Monte Carlo study of the thermal SU(2) gauge theory transforms the hole pockets into Fermi arcs in photoemission. One route to confinement of FL* upon lowering temperature yields a $d$-wave superconductor via a Kosterlitz-Thouless transition of $h/(2e)$ vortices, with nodal Bogoliubov quasiparticles featuring anisotropic velocities and vortices surrounded by charge order halos. Increasing doping from the FL* phase in the ALM drives a transition to a conventional Fermi liquid (FL) at large doping, passing through an intermediate strange metal regime. We formulate a theory of the FL*-FL metal-metal transition without a symmetry-breaking order parameter, using a critical quantum `charge' liquid of mobile electrons in the presence of disorder, developed via an extension of the Sachdev-Ye-Kitaev model to two spatial dimensions. At low temperatures, and across optimal and over doping, we address the regimes of extended non-Fermi liquid behavior by Griffiths effects near quantum phase transitions in disordered metals.

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Superlinear Hall angle and carrier mobility from non-Boltzmann magnetotransport in the spatially disordered Yukawa-Sachdev-Ye-Kitaev model on a square lattice

Exact numerical results for the dc magnetoconductivity tensor of the two-dimensional spatially disordered Yukawa-Sachdev-Ye-Kitaev (2D-YSYK) model on a square lattice, at first order in applied perpendicular magnetic field, are obtained from the self-consistent disorder-averaged solution of the 2D-YSYK saddle-point equations. This system describes fermions endowed with a Fermi surface and coupled to a bosonic scalar field through spatially random Yukawa interactions. The resulting local and energy-dependent fermionic self-energies are employed in the Kubo formalism to calculate the longitudinal and Hall conductivities, the Hall coefficient, the carrier mobility, and the cotangent of the Hall angle, at fixed fermion density. From the interplay between YSYK interactions and square-lattice embedding, and the non-Boltzmann frequency-dependent self energies, we find nontrivial evolution of the magnetotransport coefficients as a function of temperature and YSYK interaction strength, notably a superlinear evolution of the Hall-angle cotangent and the inverse carrier mobility with temperature, concomitant with linear-in-temperature resistivity, in an extended crossover regime above the low-temperature Marginal Fermi Liquid (MFL) ground state. Our model and results provide a controlled theoretical framework to interpret magnetotransport experiments, at linear order in applied magnetic field, in strange-metal phases found in strongly correlated solid-state electron systems.

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Critical spin fluctuations across the superconducting dome in La$_{2-x}$Sr$_{x}$CuO$_4$

Overdoped cuprate superconductors are strange metals above their superconducting transition temperature. In such materials, the electrical resistivity has a strong linear dependence on temperature ($T$) and electrical current is not carried by electron quasiparticles as in conventional metals. Here we demonstrate that the strange metal behaviour co-exists with strongly temperature-dependent critical spin fluctuations showing dynamical scaling across the cuprate phase diagram. Our neutron scattering observations and the strange metal behaviour are consistent with a spin density wave quantum phase transition in a metal with spatial disorder in the tuning parameter. Numerical computations using a theory of spin density waves in a disordered metal yield an extended `Griffiths phase' with scaling properties in agreement with experimental observations. Thus we establish that low-energy spin excitations and spatial disorder are central to the strange metal behaviour.

cond-mat.supr-con↗

Strange metals and planckian transport in a gapless phase from spatially random interactions

`Strange' metals that do not follow the predictions of Fermi liquid theory are prevalent in materials that feature superconductivity arising from electron interactions. In recent years, it has been hypothesized that spatial randomness in electron interactions must play a crucial role in strange metals for their hallmark linear-in-temperature ($T$) resistivity to survive down to low temperatures where phonon and Umklapp processes are ineffective, as is observed in experiments. However, a clear picture of how this happens has not yet been provided in a realistic model free from artificial constructions such as large-$N$ limits and replica tricks. We study a realistic model of two-dimensional metals with spatially random antiferromagnetic interactions in a non-perturbative regime, using numerically exact high-performance large-scale hybrid Monte Carlo and exact averages over the quenched spatial randomness. Our simulations reproduce strange metals' key experimental signature of linear-in-$T$ resistivity with a universal `planckian' transport scattering rate $Γ_\mathrm{tr} \sim k_B T/\hbar$ that is independent of coupling constants. We further find that strange metallicity in these systems is not associated with a quantum critical point, and instead arises from a phase of matter with gapless antiferromagnetic fluctuations that lacks long-range correlations and spans an extended region of parameter space: a feature that is also observed in several experiments. These gapless antiferromagnetic fluctuations take the form of spatially localized overdamped modes, whose presence could possibly be detected using recently developed nanoscale magnetometry methods. Our work paves the way for an eventual microscopic understanding of the role of spatial disorder in determining important properties of correlated electron materials.

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Thermopower across Fermi-volume-changing quantum phase transitions without translational symmetry breaking

We describe the evolution of low-temperature thermopower across Fermi-volume-changing quantum phase transitions in Kondo lattice models without translational symmetry breaking. This transition moves from a heavy Fermi liquid with a conventional Luttinger-volume large Fermi surface to a 'FL*' state, characterized by a small Fermi surface and a spin liquid with fractionalized excitations. The onset of the large Fermi surface phase is driven by the condensation of a Higgs field that carries a unit gauge charge under an emergent U(1) gauge field. We consider the case with spatially random Kondo exchange, as this leads to strange metal behavior in electrical transport. We find a large asymmetric thermopower in a 'skewed' marginal Fermi liquid, with similarities to the skewed non-Fermi liquid of Georges and Mravlje (arXiv:2102.13224). Our findings are consistent with recent observations in heavy fermion compounds (Z.-Y. Cao et al., arXiv:2408.13604), and describe an enhancement of thermopower on the large Fermi surface side as well as a non-monotonic behavior on the small Fermi surface side. Our results also apply to single-band Hubbard models and the pseudogap transition in the cuprates. In the ancilla framework, single-band models exhibit an inverted Kondo lattice transition: the small Fermi surface pseudogap state corresponds to the condensed Higgs state. This inversion results in an enhancement of thermopower on the pseudogap side in our theory, consistent with observations in the cuprates (C. Collignon et al., arXiv:2011.14927; A. Gourgout et al., arXiv:2106.05959). We argue that these observations support a non-symmetry-breaking Fermi-volume-changing transition as the underlying description of the onset of the pseudogap in the cuprates.

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Enhanced Strange Metallicity due to Hubbard-U Coulomb Repulsion

We solve a model of electrons with Hubbard-$U$ Coulomb repulsion and a random Yukawa coupling to a two-dimensional bosonic bath, using an extended dynamical mean field theory scheme. Our model exhibits a quantum critical point, at which the repulsive component of the electron interactions strongly enhances the effects of the quantum critical bosonic fluctuations on the electrons, leading to a breakdown of Fermi liquid physics and the formation of a strange metal with `Planckian' ($\mathcal{O}(k_B T/\hbar)$) quasiparticle decay rates at low temperatures $T\rightarrow 0$. Furthermore, the eventual Mott transition that occurs as the repulsion is increased seemingly bounds the maximum decay rate in the strange metal. Our results provide insight into low-temperature strange metallicity observed in proximity to a Mott transition, as is observed, for instance, in recent experiments on certain moiré materials.

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Strange metal and superconductor in the two-dimensional Yukawa-Sachdev-Ye-Kitaev model

The two-dimensional Yukawa-Sachdev-Ye-Kitaev (2d-YSYK) model provides a universal theory of quantum phase transitions in metals in the presence of quenched random spatial fluctuations in the local position of the quantum critical point. It has a Fermi surface coupled to a scalar field by spatially random Yukawa interactions. We present full numerical solutions of a self-consistent disorder averaged analysis of the 2d-YSYK model in both the normal and superconducting states, obtaining electronic spectral functions, frequency-dependent conductivity, and superfluid stiffness. Our results reproduce key aspects of observations in the cuprates as analyzed by Michon et al. (arXiv:2205.04030). We also find a regime of increasing zero temperature superfluid stiffness with decreasing superconducting critical temperature, as is observed in bulk cuprates.

cond-mat.str-el↗

Localization of overdamped bosonic modes and transport in strange metals

A recent theory described strange metal behavior in a model of a Fermi surface coupled a two-dimensional quantum critical bosonic field with a spatially random Yukawa coupling. With the assumption of self-averaging randomness, similar to that in the Sachdev-Ye-Kitaev model, numerous observed properties of a strange metal were obtained for wide range of intermediate temperatures, including the linear-in-temperature resistivity. The Harris criterion implies that spatial fluctuations in the local position of the critical point must dominate at lower temperatures. For an $M$-component boson with $M \geq 2$, we use multiple graphics processing units (GPUs) to compute the real frequency spectrum of the boson propagator in a self-consistent mean-field treatment of the boson self-interactions, but an exact treatment of multiple realizations of the spatial randomness from the random boson mass. We find that Landau damping from the fermions leads to the emergence of the physics of the random transverse-field Ising model at low temperatures, as has been proposed by Hoyos, Kotabage, and Vojta. This regime is controlled by localized overdamped eigenmodes of the bosonic scalar field, also has a resistivity which is nearly linear-in-temperature, and extends into a `quantum critical phase' away from the quantum critical point, as observed in several cuprates. For the $M = 1$ Ising scalar, the mean-field treatment is not applicable, and so we use Hybrid Monte Carlo simulations running on multiple GPUs; we find a rounded transition and localization physics, with strange metal behavior in an extended region around the transition.

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Cyclotron resonance and quantum oscillations of critical Fermi surfaces

Kohn's theorem places strong constraints on the cyclotron response of Fermi liquids. Recent observations of a doping dependence in the cyclotron mass of La$_{2-x}$Sr$_x$CuO$_4$ (Legros et al., Phys. Rev. B 106, 195110 (2022)) are therefore surprising because the cyclotron mass can only be renormalized by large momentum umklapp interactions which are not expected to vary significantly with doping. We show that a version of Kohn's theorem continues to apply to disorder-free non-Fermi liquids with a critical boson near zero momentum. However, marginal Fermi liquids arising from a spatially random Yukawa coupling between the electrons and bosons do give rise to significant corrections to the cyclotron mass which we compute. This is the same theory which yields linear-in-temperature resistivity and other properties of strange metals at zero fields (Patel et al., Science 381, 790 (2023)).

cond-mat.str-el↗

Theory of shot noise in strange metals

We extend the theory of shot noise in coherent metals to shot noise in strange metals without quasiparticle excitations. This requires a generalization of the Boltzmann equation with a noise source to distribution functions which depend independently on the excitation momentum and energy. We apply this theory to a model of a strange metal with linear in temperature ($T$) resistivity, describing a Fermi surface with a spatially random Yukawa coupling to a critical boson. We find a suppression of the Fano factor in the strange metal, and describe the dependence of the shot noise on temperature and applied voltage. At low temperatures, we obtain a Fano factor equal to $1/6$, in contrast to the $1/3$ Fano factor in diffusive metals with quasiparticles. Our results are in general agreement with recent observations by Chen et al. (arXiv:2206.00673). We further compare the random Yukawa model to quasi-elastic electron-phonon scattering that also generates $T$-linear resistivity, and argue that shot noise observations offer a useful diagnostic to distinguish between them.

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Large $N$ theory of critical Fermi surfaces II: conductivity

A Fermi surface coupled to a scalar field can be described in a $1/N$ expansion by choosing the fermion-scalar Yukawa coupling to be random in the $N$-dimensional flavor space, but invariant under translations. We compute the conductivity of such a theory in two spatial dimensions for a critical scalar. We find a Drude contribution, and verify that the proposed $1/ω^{2/3}$ contribution to the optical conductivity at frequency $ω$ has vanishing co-efficient for a convex Fermi surface. We also describe the influence of impurity scattering of the fermions, and find that while the self energy resembles a marginal Fermi liquid, the resistivity and optical conductivity behave like a Fermi liquid.

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Universal theory of strange metals from spatially random interactions

We consider two-dimensional metals of fermions coupled to quantum critical scalars, the latter representing order parameters or emergent gauge fields. We show that at low temperatures ($T$), such metals generically exhibit strange metal behavior with a $T$-linear resistivity arising from spatially random fluctuations in the fermion-scalar Yukawa couplings about a non-zero spatial average. We also find a $T\ln (1/T)$ specific heat, and a rationale for the Planckian bound on the transport scattering time. These results are obtained in the large $N$ expansion of an ensemble of critical metals.

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Pair density wave order from electron repulsion

A pair density wave (PDW) is a superconductor whose order parameter is a periodic function of space, without an accompanying spatially-uniform component. Since PDWs are not the outcome of a weak-coupling instability of a Fermi liquid, a generic pairing mechanism for PDW order has remained elusive. We describe and solve models having robust PDW phases. To access the intermediate coupling limit, we invoke large $N$ limits of Fermi liquids with repulsive BCS interactions that admit saddle point solutions. We show that the requirements for long range PDW order are that the repulsive BCS couplings must be non-monotonic in space and that their strength must exceed a threshold value. We obtain a phase diagram with both finite temperature transitions to PDW order, and a $T=0$ quantum critical point, where non-Fermi liquid behavior occurs.

cond-mat.supr-con↗

Maximal quantum chaos of the critical Fermi surface

We investigate the many-body quantum chaos of non-Fermi liquid states with Fermi surfaces in two spatial dimensions by computing their out-of-time-order correlation functions. Using a recently proposed large $N$ theory for the critical Fermi surface, and the ladder identity of Gu and Kitaev, we show that the chaos Lyapunov exponent takes the maximal value of $2 πk_B T/\hbar$, where $T$ is the absolute temperature. We also examine a phenomenological model in which the chaos exponent becomes smaller than the maximal value precisely when quasiparticles are restored.

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Many-body energy invariant for $T$-linear resistivity

The description of dynamics of strongly correlated quantum matter is a challenge, particularly in physical situations where a quasiparticle description is absent. In such situations, however, the many-body Kubo formula from linear response theory, involving matrix elements of the current operator computed with many-body wavefunctions, remains valid. Working directly in the many-body Hilbert space and not making any reference to quasiparticles (or lack thereof), we address the puzzle of linear in temperature ($T$-linear) resistivity seen in non-Fermi liquid phases that occur in several strongly correlated condensed matter systems. We derive a simple criterion for the occurrence of $T$-linear resistivity based on an analysis of the contributions to the many-body Kubo formula, determined by an energy invariant "$f$-function" involving current matrix elements and energy eigenvalues that describes the DC conductivity of the system in the microcanonical ensemble. Using full diagonalization, we test this criterion for the $f$-function in the spinless nearest neighbor Hubbard model and in a system of Sachdev-Ye-Kitaev dots coupled by weak single particle hopping. We also study the $f$-function for the spin conductivity in the 2D Heisenberg model and arrive at similar conclusions. Our work suggests that a general principle, formulated in terms of many-body Hilbert space concepts, is at the core of the occurrence of $T$-linear resistivity in a wide range of systems, and precisely translates $T$-linear resistivity into a notion of energy scale invariance far beyond what is typically associated with quantum critical points.

cond-mat.str-el↗

Solvable Theory of a Strange Metal at the Breakdown of a Heavy Fermi Liquid

We introduce an effective theory for quantum critical points (QCPs) in heavy fermion systems, involving a change in carrier density without symmetry breaking. Our new theory captures a strongly coupled metallic QCP, leading to robust marginal Fermi liquid transport phenomenology, and associated linear in temperature ($T$) "strange metal" resistivity, all within a controlled large $N$ limit. In the parameter regime of strong damping of emergent bosonic excitations, the QCP also displays a near-universal "Planckian" transport lifetime, $τ_{\mathrm{tr}}\sim\hbar/(k_BT)$. This is contrasted with the conventional so-called "slave boson" theory of the Kondo breakdown, where the large $N$ limit describes a weak coupling fixed point and non-trivial transport behavior may only be obtained through uncontrolled $1/N$ corrections. We also compute the weak-field Hall coefficient within the effective model as the system is tuned across the transition. We further find that between the two plateaus, reflecting the different carrier densities in the two Fermi liquid phases, the Hall coefficient can develop a peak in the critical crossover regime, like in recent experimental findings, in the parameter regime of weak boson damping.

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