arXiv subjects

Abdul Ahad

Publications and source records attributed to Abdul Ahad.

11 recordsLinked to original sources

arXiv2026

Strain Tuning of Orbital-Driven Giant Magnetoresistance in van der Waals ferrimagnet Mn$_3$Si$_2$Te$_6$

Strain engineering of magnetotransport offers a powerful strategy for uncovering emergent electronic and domain phenomena in quantum magnetic materials, while providing a promising pathway toward next-generation mechanically programmable spintronic technologies. Van der Waals magnets are particularly attractive in this context because their high crystallinity and mechanical flexibility allow exceptionally large, precisely controllable strain, enabling access to strain-induced functionalities unattainable in conventional solids. Here, we report systematic strain control of the van der Waals magnet Mn$_3$Si$_2$Te$_6$, which exhibits an unconventional colossal magnetoresistance whose microscopic origin remains under debate. We demonstrate in situ large-strain modulation of the electrical resistance in bulk crystals and show that the effect can be consistently explained by strain-tunable chiral orbital-current domains. Furthermore, measurements on exfoliated flake devices containing a single chiral domain reveal direct strain control of the electronic structure affected by orbital magnetic moment, establishing a unified microscopic mechanism for the unconventional colossal magnetoresistance. These results identify strain as an exceptionally effective control parameter for tailoring electronic and magnetic states in van der Waals magnets and provide a conceptual framework for realizing spin-straintronic functionalities based on orbital degrees of freedom.

cond-mat.mtrl-sci↗

arXiv2026

Piezomagnetic transport in van der Waals noncoplanar Antiferromagnets

The piezomagnetic effect-strain-induced linear modulation of magnetization, arises in magnets with broken time-reversal symmetry (BTRS), offering a pathway to bidirectional strain-based control of magnetism, which is an essential straintronic and spintronic functionality in solids. Metallic antiferromagnets with BTRS provide an ideal platform to study this effect through transport measurements, yet experimental demonstrations are limited. Van der Waals (vdW) nanomagnets, with their mechanical flexibility, are particularly promising for realizing large piezomagnetic responses and effective transport control. Here we demonstrate piezomagnetic control of electronic transport in nano-devices of the vdW antiferromagnets CoNb$_3$S$_6$ and CoTa$_3$S$_6$, archetypal vdW metals with BTRS that exhibit a spontaneous Hall effect. Applying uniaxial strain linearly modulates both the antiferromagnetic transition temperature and coercive field, consistent with strain-driven tuning of exchange coupling, key signatures of the piezomagnetic effect. Moreover, spontaneous Hall effect is controllable via strain, evidencing piezomagnetic tuning of Berry curvature and its associated geometric transport. These findings establish piezomagnetism as a powerful route to manipulate antiferromagnetic transport, opening avenues for straintronic and spintronic applications in vdW magnetic systems.

cond-mat.mes-hall↗

arXiv2025

Magnetic resonance and microwave resistance modulation in van der Waals colossal-magnetoresistance material

Colossal magnetoresistance (CMR) is a fascinating quantum phenomenon that continues to draw significant interest in condensed matter physics. Mn3Si2Te6 has emerged as a prototypical CMR material, notable for its puzzling magnetoresistance behavior and pronounced directional anisotropy. Despite extensive research, the mechanisms driving CMR in Mn3Si2Te6 remain elusive [1-4]. In this work, we explore the magnetic resonance of Mn3Si2Te6 and observe a reduced g-factor for magnetic fields applied along the crystalline c-axis compared to the ab-plane, indicating a substantial orbital magnetization contribution along the c-axis. Furthermore, we detect resistance modulation under resonance conditions, suggesting that CMR in Mn3Si2Te6 is sensitive to the out-of-the plane spin polarization. These findings shed new light on the role of orbital magnetic moment in Mn3Si2Te6, offering a deeper understanding of the interplay between spin, orbital and lattice degrees of freedom of electrons in this system.

cond-mat.mtrl-sci↗

arXiv2024

In-Context Ensemble Learning from Pseudo Labels Improves Video-Language Models for Low-Level Workflow Understanding

A Standard Operating Procedure (SOP) defines a low-level, step-by-step written guide for a business software workflow. SOP generation is a crucial step towards automating end-to-end software workflows. Manually creating SOPs can be time-consuming. Recent advancements in large video-language models offer the potential for automating SOP generation by analyzing recordings of human demonstrations. However, current large video-language models face challenges with zero-shot SOP generation. In this work, we first explore in-context learning with video-language models for SOP generation. We then propose an exploration-focused strategy called In-Context Ensemble Learning, to aggregate pseudo labels of multiple possible paths of SOPs. The proposed in-context ensemble learning as well enables the models to learn beyond its context window limit with an implicit consistency regularisation. We report that in-context learning helps video-language models to generate more temporally accurate SOP, and the proposed in-context ensemble learning can consistently enhance the capabilities of the video-language models in SOP generation.

cs.AI↗

arXiv2023

Random magnetic anisotropy driven transitions in layered perovskite LaSrCoO$_4$

Attempts to unravel the nature of magnetic ordering in LaSrCoO$_4$ (Co$^{3+}$), a compound intermediate between antiferromagnetic (AFM) La$_2$CoO$_4$ (Co$^{2+}$) and ferromagnetic (FM) Sr$_2$CoO$_4$ (Co$^{4+}$), have met with a limited success so far. In this report, the results of a thorough investigation of dc magnetization and ac susceptibility (ACS) in single-phase LaSrCoO$_4$ provide clinching evidence for a thermodynamic paramagnetic (PM) - ferromagnetic (FM) phase transition at T$_{c}$ = 220.5 K, followed at lower temperature (T$_{g}$ = 7.7 K) by a transition to the cluster spin glass (CSG) state. Analysis of the low-field Arrott plot isotherms, in the critical region near T$_{c}$, in terms of the Aharony-Pytte scaling equation of state clearly establishes that the PM-FM transition is basically driven by random magnetic anisotropy (RMA). For temperatures below $\approx$ 30 K, large enough RMA destroys long-range FM order by breaking up the infinite FM network into FM clusters of finite size and leads to the formation of a CSG state at temperatures T $\lesssim$ 8 K by promoting freezing of finite FM clusters in random orientations. Increasing strength of the single-ion magnetocrystalline anisotropy (and hence RMA) with decreasing temperature is taken to reflect an increase in the number of low-spin (LS) Co$^{3+}$ ions at the expense of that of high-spin (HS) Co$^{3+}$ ions. At intermediate temperatures (30 K $\lesssim T \lesssim$ 180 K), spin dynamics has contributions from the infinite FM network (fast relaxation governed by a single anisotropy energy barrier) and finite FM clusters (extremely slow stretched exponential relaxation due to hierarchical energy barriers).

cond-mat.mtrl-sci↗

arXiv2022

Coexistence of local structural heterogeneities and long-range ferroelectricity in Pb-free (1-x)Ba(Zr0.2Ti0.8)O3-x(Ba0.7Ca0.3)TiO3 ceramics

Environmentally benign (1-x)Ba(Ti$_{0.8}$Zr$_{0.2}$)O$_3$-x(Ba$_{0.7}$Ca$_{0.3}$)TiO$_3$ (BZT-BCT) ceramics are promising materials due to their remarkable high piezoresponse [Liu and Ren, Phys. Rev. Lett. \textbf{103}, 257602 (2009)]. In this Letter, by focusing on local and average structure in combination with macroscopic electromechanical and dielectric measurements we demonstrate the structure property relationship in the tetragonal BZT-BCT ceramic. During high-temperature cubic to tetragonal phase transformation, polar nanoregions are manifested through the spontaneous volume ferroelectrostriction at temperatures below $\sim$ 477 K. Temperature-dependent local structural investigations across the Zr K edge extended x-ray absorption fine structure spectroscopy reveal an anomalous collaboration between the ZrO$_{6}$ and TiO$_6$ octahedra. These octahedra compromise their individuality during polarization development. The presence of domains of submicron size embedded inside the macroscopic ferroelectric regions below T$_{m}$, as well as their hierarchical arrangement, is observed by piezo-response force microscopy. Effects of the existence of the structural/polar heterogeneities below T$_{m}$ are observed also when polarizibilities of the poled and the unpoled samples are compared; the poled sample is found to be more susceptible to the electric field. In addition, by using electric field dependent x-ray diffraction studies we also show that this ceramic under field exhibits reduction of tetragonal distortion, which is consistent with earlier reports.

cond-mat.mtrl-sci↗

arXiv2020

Magnetic correlations in subsystems of the misfit [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$] cobaltate

[Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$], a two dimensional misfit metallic compound, is famous for its rich phases accessed by temperature, $i.e.$ high temperature spin-state transition, metal-insulator transition (MIT) at intermediate temperature ($\sim$ 100 K) and low temperature spin density wave (SDW). It enters into SDW phase below T$_{MIT}$ which becomes long range at 27 K. Information on the independent role of misfit layers (rocksalt/Ca$_2$CoO$_3$ \& triangular/CoO$_2$) in these phases is scarce. By combining a set of complementary macroscopic (DC magnetization and resistivity) and microscopic (neutron diffraction and X-ray absorption fine structure spectroscopy) measurements on pure (CCO) and Tb substituted in the rocksalt layer of CCO (CCO1), magnetic correlations in both subsystems of this misfit compound are unraveled. CCO is found to exhibit glassiness, as well as exchange bias (EB) effects, while CCO1 does not exhibit glassiness, albeit it shows weaker EB effect. By combining local structure investigations from extended X-ray absorption fine structure (EXAFS) spectroscopy and neutron diffraction results on CCO, we confirm that the SDW arises in the CoO$_2$ layer. Our results show that the magnetocrystalline anisotropy associated with the rocksalt layer acts as a source of pinning, which is responsible for EB effect. Ferromagnetic clusters in the Ca$_2$CoO$_3$ affects SDW in CoO$_2$ and ultimately glassiness arises.

cond-mat.mtrl-sci↗

arXiv2020

Origin of the high Seebeck coefficient of the misfit [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$] cobaltate from site-specific valency and spin-state determinations

Layered misfit cobaltate [Ca$_2$CoO$_3$]$_{0.62}$[CoO$_2$], which emerged as an important thermoelectric material~[A. C. Masset et al. Phys. Rev. B, 62, 166 (2000)], has been explored extensively in the last decade for the exact mechanism behind its high Seebeck coefficient. Its complex crystal and electronic structures have inhibited consensus among such investigations. This situation has arisen mainly due to difficulties in accurate identification of the chemical state, spin state, and site symmetries in its two subsystems (rocksalt [Ca$_2$CoO$_3$] and triangular [CoO$_2$]). By employing resonant photoemission spectroscopy and x-ray absorption spectroscopy along with charge transfer multiplet simulations (at the Co ions), we have successfully identified the site symmetries, valencies and spin states of the Co in both layers. Our site-symmetry observations explain the experimental value of the high Seebeck coefficient and also confirm that the carriers hop within the rocksalt layer, which is in contrast to earlier reports where hopping within triangular CoO$_2$ layer has been held responsible for the large Seebeck coefficient.

cond-mat.str-el↗

arXiv2020

Hierarchical Tensor Ring Completion

Tensor completion can estimate missing values of a high-order data from its partially observed entries. Recent works show that low rank tensor ring approximation is one of the most powerful tools to solve tensor completion problem. However, existing algorithms need predefined tensor ring rank which may be hard to determine in practice. To address the issue, we propose a hierarchical tensor ring decomposition for more compact representation. We use the standard tensor ring to decompose a tensor into several 3-order sub-tensors in the first layer, and each sub-tensor is further factorized by tensor singular value decomposition (t-SVD) in the second layer. In the low rank tensor completion based on the proposed decomposition, the zero elements in the 3-order core tensor are pruned in the second layer, which helps to automatically determinate the tensor ring rank. To further enhance the recovery performance, we use total variation to exploit the locally piece-wise smoothness data structure. The alternating direction method of multiplier can divide the optimization model into several subproblems, and each one can be solved efficiently. Numerical experiments on color images and hyperspectral images demonstrate that the proposed algorithm outperforms state-of-the-arts ones in terms of recovery accuracy.

math.NA↗

arXiv2019

A setup for Seebeck coefficient measurement through controlled heat pulses

A setup is designed for measuring the Seebeck coefficient (S) of materials in form of thin film, bar and wire. The main feature of this setup is control in heating and cooling cycles. In this setup heat pulse is used to generate the temperature gradient. To demonstrate the capabilities of this setup, S vs T of standard wire samples such as Au-Fe (0.07 \%), chromel, Pt and thin films of Pt and F doped SnO$_2$ are presented. The standard uncertainty of the repeatability in S measurement is found to be $\sim$ $\pm 0.056~μV/K$ while temperature stability is $\sim$ $\pm 10~mK$ (at 320 K), estimated for a chromel wire sample. We have tested the setup in temperature range 100 K to 320 K, while it does not have any intrinsic limitation in going down to liquid He temperatures. For temperatures above 320 K limitation is due to gluing material like varnish.

physics.ins-det↗

arXiv2019

Non thermal isostructural electrically driven insulator-metal transition and electro-strain in layered cobaltate

We report here a discovery of electrically driven insulator to metal transition (IMT) and concomitant isostructural volume expansion in the layered cobaltates which otherwise do not exhibit temperature dependent IMT. These findings are demonstrated at macroscopic, microscopic and atomic scales. With application of voltage growth of metallic regions have been observed in the 2D layered La2-xSrxCoO4. Growth of metallic regions is associated with volume increase (strain as high as 0.3%). Non thermal IMT and electro-strain are proposed to be caused by electro-proliferation of the Co3+ high spin states.

cond-mat.str-el↗