arXiv subjects

Achintya Low

Publications and source records attributed to Achintya Low.

12 recordsLinked to original sources

arXiv2025

Extremely Large and Angle-Dependent Magnetoresistance in Kagome Dirac Semimetal RFe$_6$Sn$_6$ (R=Ho, Dy)

We report on the electronic, magnetic, and magneto-transport properties of Fe-based kagome Dirac system, RFe$_6$Sn$_6$ (R = Ho, Dy). Magnetic properties study reveals an antiferromagnetic order with N$\acute{e}$el temperature of $T_N \approx$ 570 K. Additionally, a weak ferromagnetic order emerge at low temperatures. Magnetotransport measurements demonstrate an extremely large magnetoresistance (XMR) reaching as high as $3\times 10^{3} \%$ for HoFe$_6$Sn$_6$ and $ 1\times 10^{3} \%$ for DyFe$_6$Sn$_6$ when measured at 2 K with 9 T of magnetic field. The semi-classical two-band model fitting of the Hall conductivity reveals nearly perfect electron-hole compensation and high carrier mobility, which leads to XMR behaviour in these system. Further, we identify large magnetoresistance anisotropy for the magnetic fields applied in different crystallographic orientations. In addition, considerable modification in the angle-dependent magnetoresistance (ADMR) pattern has been noticed between 2 and 50 K, indicating temperature-dependent changes in the Fermi surface topology of these systems.

cond-mat.mtrl-sci↗

arXiv2025

Spin-reorientation Driven Temperature Dependent Intrinsic Anomalous Hall Conductivity in Fe$_3$Ge, a Ferromagnetic Topological Metal

We investigate the temperature dependence of the intrinsic anomalous Hall conductivity in Fe$_3$Ge, which is a ferromagnetic topological metal. We observe a significant anisotropy in the anomalous Hall conductivity between in-plane and out-of-plane directions. We further identify that the total Hall conductivity is contributed extrinsically due to the skew-scattering mechanism and intrinsically due to nonzero Berry curvature in the momentum space. Most importantly, we demonstrate the temperature dependence of the intrinsic Hall contribution, a rare phenomenon to visualize experimentally, due to tuning the easy-magnetic axis from the out-of-plane to the in-plane with decreasing temperature. We also show that the extrinsic Hall conductivity decreases with temperature as $\sigma_{xy}^{ext}(T)=\frac{\sigma_{xy0}^{ext}}{(aT+1)^2}$ due to electron-phonon scattering.

cond-mat.mtrl-sci↗

arXiv2025

Topological Hall effect in ferromagnetic Weyl semimetal Mn$_5$Ge$_3$ originating in competing dipolar interaction and magnetocrystalline anisotropy

We report the anomalous and topological Hall effect of the ferromagnetic Weyl semimetal Mn$_5$Ge$_3$. We observe a significant anisotropic anomalous Hall effect (AHE) due to nonzero Berry curvature in the momentum space, such that the anomalous Hall conductivity (AHC) is 965 S/cm for the $xy$-plane and 233 S/cm for the $zx$-plane of the single crystal. The band structure calculations predict several Weyl and nodal points span across the momentum space, gapped out under the spin-orbit coupling effect, leading to significant $k$-space Berry curvature and large AHC. Experimentally, we also demonstrate a sizeable topological Hall effect that is originated by the non-coplanar chiral spin structure due to the competition between the out-of-plane uniaxial magnetocrystalline anisotropy and the dipole-dipole interaction between two Mn sublattices. This study hints at the importance of dipole-dipole interactions in producing the skyrmion lattice in Mn$_5$Ge$_3$.

cond-mat.mtrl-sci↗

arXiv2024

Anisotropic Nonsaturating Magnetoresistance Observed in HoMn$_6$Ge$_6$: A Kagome Dirac Semimetal

We report the magnetic and magnetotransport properties and electronic band structure of the kagome Dirac semimetal HoMn$_6$Ge$_6$. Temperature-dependent electrical resistivity demonstrates various magnetic-transition-driven anomalies. Notably, a crossover from negative to positive magnetoresistance (MR) is observed at around 150 K. While the linear nonsaturating positive MR in the low-temperature region is mainly driven by the linear Dirac-like band dispersions as predicted by the first-principles calculations, the negative MR observed in the high-temperature region is due to the spin-flop type magnetic transition. Consistent with anisotropic Fermi surface topology, we observe anisotropic magnetoresistance at low temperatures. A significant anomalous Hall effect has been noticed at high temperatures in addition to a switching of the dominant charge carrier from electron to hole at around 215 K.

cond-mat.mtrl-sci↗

arXiv2024

Unusual Multiple Magnetic Transitions and Anomalous Hall Effect Observed in Antiferromagnetic Weyl Semimetal, Mn$_{2.94}$Ge (Ge-rich)

We report on the magnetic and Hall effect measurements of the magnetic Weyl semimetal, Mn$_{2.94}$Ge (Ge-rich) single crystal. From the magnetic properties study, we identify unusual multiple magnetic transitions below the N$\acute{e}$el temperature of 353 K, such as the spin-reorientation ($T_{SR}$) and ferromagnetic-like transitions. Consistent with the magnetic properties, the Hall effect study shows unusual behavior around the spin-reorientation transition. Specifically, the anomalous Hall conductivity (AHC) increases with increasing temperature, reaching a maximum at $T_{SR}$, which then gradually decreases with increasing temperature. This observation is quite in contrast to the Mn$_{3+\delta}$Ge (Mn-rich) system, though both compositions share the same hexagonal crystal symmetry. This study unravels the sensitivity of magnetic and topological properties on the Mn concentration.

cond-mat.mtrl-sci↗

arXiv2023

Weak Electronic Correlations Observed in Magnetic Weyl Semimetal Mn$_3$Ge

Using angle-resolved photoemission spectroscopy (ARPES) and density functional theory (DFT) calculations, we systematically studied the electronic band structure of Mn$_3$Ge in the vicinity of the Fermi level. We observe several bands crossing the Fermi level, confirming the metallic nature of the studied system. We further observe several flat bands along various high symmetry directions, consistent with the DFT calculations. The calculated partial density of states (PDOS) suggests a dominant Mn $3d$ orbital contribution to the total valence band DOS. With the help of orbital-resolved band structure calculations, we qualitatively identify the orbital information of the experimentally obtained band dispersions. Out-of-plane electronic band dispersions are explored by measuring the ARPES data at various photon energies. Importantly, our study suggests relatively weaker electronic correlations in Mn$_3$Ge compared to Mn$_3$Sn.

cond-mat.mtrl-sci↗

arXiv2023

Investigation of the Anomalous and Topological Hall Effects in Layered Monoclinic Ferromagnet Cr$_{2.76}$Te$_4$

We studied the electrical transport, Hall effect, and magnetic properties of monoclinic layered ferromagnet Cr$_{2.76}$Te$_4$. Our studies demonstrate Cr$_{2.76}$Te$_4$ to be a soft ferromagnet with strong magnetocrystalline anisotropy. Below 50 K, the system shows an antiferromagnetic-like transition. Interestingly, between 50 and 150 K, we observe fluctuating magnetic moments between in-plane and out-of-plane orientations, leading to non-coplanar spin structure. On the other hand, the electrical resistivity data suggest it to be metallic throughout the measured temperature range, except a $kink$ at around 50 K due to AFM ordering. The Rhodes-Wohlfarth ratio $\frac{μ_{eff}}{μ_{s}}=1.89 (>1)$ calculated from our magnetic studies confirms that Cr$_{2.76}$Te$_4$ is an itinerant ferromagnet. Large anomalous Hall effect has been observed due to the skew-scattering of impurities and the topological Hall effect has been observed due to non-coplanar spin-structure in the presence of strong magnetocrystalline anisotropy. We examined the mechanism of anomalous Hall effect by employing the first principles calculations.

cond-mat.mtrl-sci↗

arXiv2023

Effect of Electron-Phonon Scattering on the Anomalous Hall Conductivity of Fe$_3$Sn: A Kagome Ferromagnetic Metal

We report on magnetic and magnetotransport studies of a Kagome ferromagnetic metal, Fe$_3$Sn. Our studies reveal a large anomalous Hall conductivity ($σ_{zx}$) in this system, mainly contributed by temperature independent intrinsic Hall conductivity ($σ^{int}_{zx}$=485$\pm$60 S/cm) and temperature dependent extrinsic Hall conductivity ($σ^{ext}_{zx}$) due to skew-scattering. Although $σ^{ext}_{zx}$ value is large and almost equivalent to the intrinsic Hall conductivity at low temperatures, it drastically decreases with increasing temperature, following the relation $σ^{ext}_{zx}=\frac{σ_{zx0}^{ext}}{(aT+1)^2}$, under the influence of electron-phonon scattering. The presence of electron-phonon scattering in this system is also confirmed by the linear dependence of longitudinal electrical resistivity at higher temperatures [$ρ(T)\propto T$]. We further find that Fe$_3$Sn is a soft ferromagnet with an easy-axis of magnetization lying in the $\it{ab}$ plane of the crystal with magnetocrystalline anisotropy energy density as large as 1.02 $\times$ 10$^6$

cond-mat.mtrl-sci↗

arXiv2023

Tuning of Electrical, Magnetic, and Topological Properties of Magnetic Weyl Semimetal Mn$_{3+x}$Ge by Fe doping

We report on the tuning of electrical, magnetic, and topological properties of the magnetic Weyl semimetal (Mn$_{3+x}$Ge) by Fe doping at the Mn site, Mn$_{(3+x)-δ}$Fe$_δ$Ge ($δ$=0, 0.30, and 0.62). Fe doping significantly changes the electrical and magnetic properties of Mn$_{3+x}$Ge. The resistivity of the parent compound displays metallic behavior, the system with $δ$=0.30 of Fe doping exhibits semiconducting or bad-metallic behavior, and the system with $δ$=0.62 of Fe doping demonstrates a metal-insulator transition at around 100 K. Further, we observe that the Fe doping increases in-plane ferromagnetism, magnetocrystalline anisotropy, and induces a spin-glass state at low temperatures. Surprisingly, topological Hall state has been noticed at a Fe doping of $δ$=0.30 that is not found in the parent compound or with $δ$=0.62 of Fe doping. In addition, spontaneous anomalous Hall effect observed in the parent system is significantly reduced with increasing Fe doping concentration.

cond-mat.mtrl-sci↗

arXiv2023

Sn$_{0.06}$Cr$_3$Te$_4$: A Skyrmion Superconductor

Topological superconductors are an exciting class of quantum materials from the point of view of the fundamental sciences and potential technological applications. Here, we report on the successful introduction of superconductivity in a ferromagnetic layered skyrmion system Cr$_3$Te$_4$, obtained by the Sn intercalation, below a transition temperature of $T_c$$\approx$3.5 K. We observe several interesting physical properties, such as superconductivity, magnetism, and the topological Hall effect, simultaneously in this system. Despite the magnetism and Meissner effects being anisotropic, the superconductivity observed from the in-plane electrical resistivity ($\rho_{\it{bc}}$) is nearly isotropic between $H\parallel \it{bc}$ and $H\parallel \it{a}$, suggesting separate channels of conduction electrons responsible for the superconductivity and magnetism of this system, which is also supported by our spin-resolved DFT calculations. We identify two orders of higher carrier density in superconducting Sn$_{0.06}$Cr$_{3}$Te$_4$ than the parent Cr$_3$Te$_4$. A jump in the specific heat is noticed around the $T_c$ with a volume fraction of 33\%, confirming the bulk superconductivity in Sn$_{0.06}$Cr$_{3}$Te$_4$. In addition to the introduction of superconductivity, tuning of topological Hall properties is noticed with Sn intercalation. Our observation of superconductivity in a skyrmion lattice brings up a new class of topological quantum materials.

cond-mat.supr-con↗

arXiv2023

Experimental Realization of Room Temperature Topological Hall Effect in Kagome Antiferromagnet

Magnetic topological semimetals are the manifestations of interplay between electronic and magnetic phases of the matter, leading to peculiar characteristics such as the anomalous Hall effect (AHE) and topological Hall effect (THE). Mn$_3$Sn is a time-reversal symmetry broken (TRS) magnetic Weyl semimetal showing topological characteristics within the Kagome lattice network. In this study, for the first time, we uncover large and pure topological Hall effect in Mn$_3$Sn at the room temperature, which is gradually suppressed by Fe doping at the Mn site of Mn$_{3-x}$Fe$_x$Sn. We further identify that the topological properties of these systems are highly anisotropic. These findings promise the realization of potential topotronic applications at room temperature.

cond-mat.mtrl-sci↗

arXiv2022

Tuning of topological properties in the strongly correlated antiferromagnet Mn$_3$Sn via Fe doping

Magnetic topological materials, in which strong correlations between magnetic and electronic properties of matter, give rise to various exotic phenomena such as anomalous Hall effect (AHE), topological Hall effect (THE), and skyrmion lattice. Here, we report on the electronic, magnetic, and topological properties of Mn$_{3-\it{x}}$Fe$_{\it{x}}$Sn single crystals ($\it{x}$=0, 0.25, and 0.35). Low temperature magnetic properties have been significantly changed with Fe doping. Most importantly, we observe that large uniaxial magnetocrystalline anisotropy that is induced by the Fe doping in combination with competing magnetic interactions at low temperature produce nontrivial spin-texture, leading to large topological Hall effect in the doped systems at low temperatures. Our studies further show that the topological properties of Mn$_{3-\it{x}}$Fe$_{\it{x}}$Sn are very sensitive to the Fe doping.

cond-mat.mtrl-sci↗