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Adam T. Heiniger

Publications and source records attributed to Adam T. Heiniger.

3 recordsLinked to original sources

Suspended thin-film lithium niobate modulator for broadband mid-infrared light modulation and frequency comb generation

The mid-infrared (MIR) spectral regime is central to applications including remote sensing, precision spectroscopy, higher harmonic generation, and free-space optical communication. However, coherent and broadband MIR modulation remains challenging owing to high optical loss, limited bandwidth, and large drive voltages in existing platforms. Here, we overcome these challenges by deploying a suspended thin-film lithium-niobate (TFLN) based electro-optic (EO) platform co-designed with high-performance traveling-wave microwave (MW) electrodes. We demonstrate a record-low Vpi,DC of 2.3 to 4.3 V over a broadband MIR bandwidth from 2.4 to 3.6 um, and a 2.7 dB EO bandwidth of 40 GHz (extracted 3 dB bandwidth of 50 GHz), yielding a figure of merit of 17.4 GHz/V, more than an order of magnitude higher than the state of the art. We demonstrate, for the first time, high-frequency Vpi,MW of 4.5 to 6.5 V in the 25 to 35 GHz range, and frequency-agile MIR EO frequency comb generation with a 10 dB optical bandwidth over 0.8 THz using a suspended phase modulator of 4 cm active modulation length. We further validate the platform in a free-space optical communication link. Our results establish a monolithic MIR photonic platform capable of powerful EO modulation and spectral synthesis, and represent a significant step toward reconfigurable MIR sensing and communication systems on chip.

physics.optics

High power, frequency agile comb spectroscopy in the mid-infrared enabled by a continuous-wave optical parametric oscillator

While mid-infrared optical frequency combs have been widely utilized in areas such as trace gas sensing, chemical kinetics, and combustion science, the relatively low power per comb tooth has limited acquisition times and sensitivities. We have developed a new approach in which an electro-optic frequency comb is utilized to pump a continuous-wave singly-resonant optical parametric oscillator in order to spectrally translate the comb into the mid-infrared. Through the use of electro-optic combs produced via chirped waveforms we have produced mid-infrared combs containing up to 2400 comb teeth. We show that a comb can be generated on the non-resonant idler when the pump modulation is non-synchronous, and we use these combs to perform high resolution spectroscopy on methane. In addition, we describe the underlying theory of this method and demonstrate that phase matching should allow for combs as broad as several THz to be spectrally translated to the mid-infrared. The high power and mutual coherence as well as the relatively low complexity of this approach should allow for broad application in areas such as chemical dynamics, quantum information, and photochemistry.

physics.optics

Nanosecond time-resolved dual-comb absorption spectroscopy

Frequency combs have revolutionized the field of optical spectroscopy, enabling researchers to probe molecular systems with a multitude of accurate and precise optical frequencies. While there have been tremendous strides in direct frequency comb spectroscopy, these approaches have been unable to record high resolution spectra on the nanosecond timescale characteristic of many physiochemical processes. Here we demonstrate a new approach to optical frequency comb generation in which a pair of electro-optic combs is produced in the near-infrared and subsequently transferred with high mutual coherence and efficiency into the mid-infrared within a single optical parametric oscillator. The high power, mutual coherence, and agile repetition rates of these combs as well as the large mid-infrared absorption of many molecular species enable fully resolved spectral transitions to be recorded in timescales as short as 20 ns. We have applied this approach to study the rapid dynamics occurring within a supersonic pulsed jet, however we note that this method is widely applicable to fields such as chemical and quantum physics, atmospheric chemistry, combustion science, and biology.

physics.optics