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Adarsh S. Patri

Publications and source records attributed to Adarsh S. Patri.

At least 19 recordsLinked to original sources

The Sound of Electrons Shattering: Current Noise Composition Laws for Electron Fractionalization

We develop a theory of the non-equilibrium current response for metallic systems near quantum critical points where electronic quasiparticles fractionalize, such as systems near continuous metal-insulator transitions or composite Fermi liquid to Fermi liquid transitions. Applying a generalized response theory within a Keldysh path integral framework, we derive a non-perturbative current noise composition law, wherein the total noise is the sum of the noise of each fractionalized constituent (bosonic holons and fermionic spinons), weighted by their respective resistivities. We demonstrate that the formally derived composition relations can be interpreted in terms of a simple analogy with resistors in series. We leverage this composition rule near certain quantum critical points to show that the shot noise can be suppressed in long nanowires as compared to Fermi liquid expectations due to the collusion of quantum criticality with fractionalization.

cond-mat.str-el

Elastic Response and Instabilities of Anomalous Hall Crystals

Anomalous Hall crystals (AHCs) are exotic phases of matter that simultaneously break continuous translation symmetry and exhibit the quantum anomalous Hall effect. AHCs have recently been proposed to explain the observation of an integer quantum anomalous Hall phase in a multilayer graphene system. Despite intense theoretical and experimental interest, little is known about the mechanical properties of AHCs. We study the elastic properties of AHCs first by using a continuum model with quadratic dispersion and uniform Berry curvature. We find using time-dependent Hartree-Fock that the stiffness of the AHC is an order of magnitude smaller than that of the WC, which we attribute to the finite Chern number of the AHC preventing exponential localization of the charge density. By modifying the dispersion relation to include a local minimum modeled after that of rhombohedral pentalayer graphene (R5G), we find that deformations away from the triangular lattice minimize the AHC's kinetic energy, which overwhelms the small stiffness and triggers a mechanical instability. Using a microscopic model of R5G, we observe a similar mechanical instability over an experimentally relevant parameter regime. We conclude that the topologically limited stiffness of AHCs makes them susceptible to mechanical instabilities, an important consideration when interpreting experiments in terms of AHCs.

cond-mat.str-el

Spontaneous altermagnetism in multi-orbital correlated electron systems

Altermagnets have attracted considerable attention in recent years owing to their potential technological applications in spintronics and magnonics. Recently, a new class of spontaneous altermagnets has been theoretically predicted in a correlated two orbital model, driven by the coexistence of antiferromagnetic spin and staggered orbital ordering, thus broadening the scope of altermagnetic phenomena to systems with strong correlations. It has been noted, however, that the required spin and orbital order violates the well-established Goodenough-Kanamori (GK) rules, which underlie much of our understanding of magnetism in complex systems. Here we show that materials with three active orbitals may offer a more realistic route to this exotic state. Specifically, we consider a two-dimensional system with $t_{2g}^{2}$ electrons and identify a novel microscopic mechanism that allows the formation of a spontaneous altermagnetic Mott insulator. We explain how the GK rules are circumvented and provide the stability criteria by employing unbiased mean-field and density matrix renormalization group calculations. In addition, for the first time, we uncover the presence and microscopic origin of chirally split magnons in these spontaneous altermagnets, with experimentally measurable spin conductivities. Finally, we predict that the application of a small in-plane magnetic field induces, in the presence of weak atomic spin-orbit coupling, an as-yet unreported hybrid chiral magnon-orbiton mode with a non-zero orbital polarization giving rise to finite longitudinal and transverse orbital conductivities under a thermal gradient.

cond-mat.str-el

Unconventional superconductivity mediated by exciton density wave fluctuations

Synthetic platforms afford an unparalleled degree of controllability in realizing strongly-correlated phases of matter. In this work, we study the possibility of electrically tunable exciton-mediated superconductivity arising in charge-imbalanced bilayer semiconductors. Focusing on the case of a bilayer semiconductor heterostructure, we identify the gating conditions required to achieve exciton density wave order within a self-consistent Hartree-Fock approximation. We analyze the role of the coupling of excitonic fluctuations to the fermionic charge carriers to find that the Goldstone mode of the density wave order can mediate attractive interactions leading to superconductivity. Furthermore, when the system is close to the density wave ordering, the interactions mediated by low-energy exciton modes can support an interlayer pair-density wave superconductor of anisotropic character. We discuss experimental signatures associated with these phenomena.

cond-mat.str-el

Family of multilayer graphene superconductors with tunable chirality: Momentum-space vortices nucleated by a ring of Berry curvature

Recent experiments in rhombohedrally-stacked multilayer graphene heterostructures have reported signatures of chiral superconductivity, emerging from a spin and valley-polarized normal state with broken time-reversal symmetry and an associated anomalous Hall effect. These findings bring into focus the role of the electronic Bloch wavefunction and the quantum geometric tensor in determining the superconducting pairing channel. In this work, we examine superconducting instabilities of a model of $N$-layer rhombohedral graphene that possesses an enhanced Berry curvature distribution on an extended ring in momentum space $-$ that we dub the 'Berry ring of fire' $-$ in the presence of an isotropic attractive interaction with a parametrically controlled spatial range. We determine that local interactions favor a $N$-fold winding in the order parameter phase for odd-$N$ layered systems, with even-$N$ layers requiring a spatially extended attraction range to achieve pairing. For generic interaction lengths, we discover a family of chiral superconductors and, remarkably, momentum-space vortices nucleated on the Berry ring of fire. The existence of these vortices can be traced to a momentum-space flux quantization condition involving the Berry curvature, with the phase winding dictated by a combination of the Berry flux and a 'statistical flux' to enforce Fermi-Dirac statistics. Such an order parameter structure allows for the possibility of in-situ tuning between various chiral superconducting phases through changes in the electron density or the displacement field. We discuss ways in which these predictions can be experimentally tested and potentially exploited in future devices.

cond-mat.supr-con

Theory of quantum anomalous Hall phases in pentalayer rhombohedral graphene moiré structures

Remarkable recent experiments on the moiré structure formed by pentalayer rhombohedral graphene aligned with a hexagonal Boron-Nitride substrate report the discovery of a zero field fractional quantum hall effect. These "(Fractional) Quantum Anomalous Hall" ((F)QAH) phases occur for one sign of a perpendicular displacement field, and correspond, experimentally, to full or partial filling of a valley polarized Chern-$1$ band. Such a band is absent in the non-interacting band structure. Here we show that electron-electron interactions play a crucial role, and present microscopic theoretical calculations demonstrating the emergence of a nearly flat, isolated, Chern-$1$ band and FQAH phases in this system. We also study the four and six-layer analogs and identify parameters where a nearly flat isolated Chern-$1$ band emerges which may be suitable to host FQAH physics.

cond-mat.str-el

Signatures of hidden octupolar order from nonlinear Hall effects

Detecting symmetry-breaking hidden orders with conventional probes has been a long-standing challenge in the field of magnetism. Higher-rank multipolar ordering $-$ anisotropic charge and magnetization distributions arising from a combination of spin-orbit coupling and crystalline environments $-$ is a quintessential example of such hidden orders, where new protocols of direct detection remain highly desirable. In this work, we propose non-linear Hall effects as a novel probe for multipolar ordering in metallic systems. Taking inspiration from the family of Pr-based heavy-fermion compounds, Pr(Ti,V)$_2$Al$_{20}$, we formulate a minimal cubic-lattice model of conduction electrons coupled to a ferro-octupolar order parameter. The time-reversal-breaking order leads to a band structure that supports strong quadrupolar moments of the Berry curvature (BC). Using a semi-classical Boltzmann formalism in conjunction with a symmetry analysis, we demonstrate that the BC quadrupoles produce a third harmonic generation of the Hall voltage $[V_H(3 ω)]$ measurable in an AC Hall experiment. Properties of the Hall response such as its anisotropy, its dissipationlessness, and its dependence on the order parameter are also examined. Our work encourages a new realm of investigation of multipolar ordering from non-linear transport experiments.

cond-mat.mes-hall

Extended quantum anomalous Hall effect in moiré structures: phase transitions and transport

Recent experiments on multilayer rhombohedral graphene have unearthed a number of interesting phenomena in the regime where Integer and Fractional Quantum Anomalous Hall phenomena were previously reported. Specifically at low temperature ($T$) and low applied currents, an "Extended" Integer Quantum Anomalous Hall (EIQAH) is seen over a wide range of the phase diagram. As the current is increased, at low $T$, the EIQAH undergoes a phase transition to a metallic state at generic fillings, and to the fractional quantum anomalous Hall (FQAH) state at the Jain fillings. Increasing temperature at the Jain fillings also leads to an evolution out of the EIQAH to the Jain state. Here we provide an interpretation of many of these observations. We describe the EIQAH as a crystalline state (either of holes doped into the $ν= 1$ state, or an Anomalous Hall Crystal of electrons) that breaks moiré translation symmetry. At generic fillings, we show how an electric current-induced depinning transition of the crystalline order leads to peculiar non-linear current-voltage curves consistent with the experiment. At Jain fillings, we propose that the depinning transition is pre-empted by an equilibrium transition between EIQAH and Jain FQAH states. This transition occurs due to the large polarizability of the Jain FQAH states which enables them to lower their energy effectively in an applied electric field compared to the crystal states. We also discuss the finite temperature evolution in terms of the relative entropies of the crystalline and FQAH states.

cond-mat.str-el

Stability of Anomalous Hall Crystals in multilayer rhombohedral graphene

Recent experiments showing an integer quantum anomalous Hall effect in pentalayer rhombohedral graphene have been interpreted in terms of a valley-polarized interaction-induced Chern band. The resulting many-body state can be viewed as an Anomalous Hall Crystal (AHC), with a further coupling to a weak moiré potential. We explain the origin of the Chern band and the corresponding AHC in the pentalayer system. To describe the competition between AHC and Wigner Crystal (WC) phases, we propose a simplified low-energy description that predicts the Hartree-Fock phase diagram to good accuracy. This theory can be fruitfully viewed as `superconducting ring' in momentum space, where the emergence of Chern number is analogous to the flux quantization in a Little-Parks experiment. We discuss the possible role of the moiré potential, and emphasize that even if in the moiré-less limit, the AHC is not favored (beyond Hartree-Fock) over a correlated Fermi liquid, the moiré potential will push the system into a `moiré-enabled AHC'. We also suggest that there is a range of alignment angles between R5G and hBN where a $C = 2$ insulator may be found at integer filling.

cond-mat.str-el

Strong correlations in ABC-stacked trilayer graphene: Moiré is important

Recent experiments on multilayer graphene materials have discovered a plethora of correlated phases, including ferromagnetism and superconductivity, in the absence of a moiré potential. These findings pose an intriguing question of whether an underlying moiré potential plays a key role in determining the phases realizable in tunable two-dimensional quantum materials, or whether it merely acts as a weak periodic potential that perturbs an underlying correlated many body state. In this work, employing a Hartree-Fock mean field analysis, we examine this question theoretically by quantitatively studying the effects of an hexagonal Boron Nitride (h-BN) substrate on ABC-stacked trilayer graphene (ABC-TLG). For the topologically trivial regime, we find that the moiré potential leads to a strong suppression of the ferromagnetism of the underlying metal. Further, band insulators appear solely at full filling of the moiré unit cell, with a moiré potential stronger than is conventionally assumed. Thus the observed correlated insulating phases in ABC-TLG aligned with h-BN cannot be understood through band folding of the ferromagnetic metal found without the moiré potential. For the topologically non-trivial regime, we discover the appearance of prominent incompressible states when fractional hole fillings (of the moiré unit cell) coincide with the occurrence of fractional-metallic states in the moiré-less setting, as well as a slight weakening of the ferromagnetic nature of the phases; however this once again requires a moiré potential stronger than is conventionally assumed. Our findings highlight the importance of interactions in renormalizing the electronic bandstructure, and emphasizes the key role played by the moiré potential in determining the strong correlation physics.

cond-mat.str-el

Uncovering footprints of dipolar-octupolar quantum spin ice from neutron scattering signatures

Recent experiments on Ce$_2$Zr$_2$O$_7$ suggest that this material may host a novel form of quantum spin ice, a three-dimensional quantum spin liquid with an emergent photon. The Ce$^{3+}$ local moments on the pyrochlore lattice are described by pseudospin 1/2 degrees of freedom, whose components transform as dipolar and octupolar moments under symmetry operations. In principle, there exist four possible quantum spin ice regimes, depending on whether the Ising component is in the dipolar/octupolar channel, and two possible flux configurations of the emergent gauge field. In this work, using exact diagonalization and molecular dynamics, we investigate the equal-time and dynamical spin structure factors in all four quantum spin ice regimes using quantum and classical computations. Contrasting the distinct signatures of quantum and classical results for the four possible quantum spin ice regimes and elucidating the role of quantum fluctuations, we show that the quantum structure factor computed for the $π$-flux octupolar quantum spin ice regime is most compatible with the neutron scattering results on Ce$_2$Zr$_2$O$_7$.

cond-mat.str-el

Ultrasound detection of emergent photons in generic quantum spin ice

Experimental identification of quantum spin ice (QSI), a U(1) quantum spin liquid on the pyrochlore lattice hosting emergent photons, is a major challenge in frustrated magnets. In this work, we propose ultrasound measurements as a novel tool for probing the emergent photons of various QSI phases. Our analysis includes QSI phases in non-Kramers doublet compounds such as $\rm{Pr}_2 \rm{Zr}_2 \rm{O}_7$ as well as dipolar-octupolar Kramers doublet compounds such as $\rm{Ce}_2 \rm{Zr}_2 \rm{O}_7$. The latter may host emergent photons associated with an octupolar component which renders them difficult to detect with inelastic neutron scattering. We demonstrate theoretically how the speed of the emergent photons can be obtained from the renormalization of the phonon spectrum and show that ultrasound measurements provide a means of distinguishing the dipolar from the octupolar QSI phase in dipolar-octupolar materials.

cond-mat.str-el

Pairing symmetry of twisted bilayer graphene: a phenomenological synthesis

One of the outstanding questions in the study of twisted bilayer graphene -- from both experimental and theoretical points of view -- is the nature of its superconducting phase. In this work we perform a comprehensive synthesis of existing experiments, and argue that experimental constraints are strong enough to allow the structure of the superconducting order parameter to be nearly uniquely determined. In particular, we argue that the order parameter is nodal, and is formed from an admixture of spin-singlet and spin-triplet Cooper pairs. This argument is made on phenomenological grounds, without committing to any particular microscopic model of the superconductor. Existing data is insufficient to determine the orbital parity of the order parameter, which could be either p-wave or d-wave. We propose a way in which the measurement of Andreev edge states can be used to distinguish between the two.

cond-mat.supr-con

Realization of fractonic quantum phases in the breathing pyrochlore lattice

Fractonic phases of matter are novel quantum ground states supporting sub-dimensional emergent excitations with mobility restrictions. Due to a sub-extensive ground state degeneracy that is dependent on the geometry of the underlying lattice, fractonic phases are considered as models for quantum memory or quantum glass. While there exist a number of exactly solvable models with interactions between multiple particles/spins, the realization of such models in real materials is extremely challenging. In this work, we provide a realistic quantum model of quadratic spin interactions on the breathing pyrochlore lattice of existing materials. We show that the emergent "cluster charge" excitations arise as vacuum fluctuations residing on the boundary of membrane objects, and move in a sub-dimensional space. Using the membrane operators, we demonstrate the existence of a sub-extensive ground state degeneracy explicitly depending on the lattice geometry, which is a useful resource for novel quantum memory.

cond-mat.str-el

Non-Trivial Fixed Points and Truncated SU(4) Kondo Models in a Quasi-Quartet Multipolar Quantum Impurity Problem

The multipolar Kondo problem, wherein the quantum impurity carries higher-rank multipolar moments, has seen recent theoretical and experimental interest due to proposals of novel non-Fermi liquid states and the availability of a variety of material platforms. The multipolar nature of local moments, in conjunction with constraining crystal field symmetries, leads to a vast array of possible interactions and resulting non-Fermi liquid ground states. Previous works on Kondo physics have typically focussed on impurities that have two degenerate internal states. In this work, inspired by recent experiments on the tetragonal material YbRu$_{2}$Ge$_{2}$, which has been shown to exhibit a local moment with a quasi-fourfold degenerate ground state, we consider the Kondo effect for such a quasi-quartet multipolar impurity. In the tetragonal crystal field environment, the local moment supports dipolar, quadrupolar, and octupolar moments, which interact with conduction electrons in entangled spin and orbital states. Using renormalization group analysis, we uncover a number of emergent quantum ground states characterized by non-trivial fixed points. It is shown that these previously unidentified fixed points are described by truncated SU(4) Kondo models, where only some of the SU(4) generators (representing the impurity degrees of freedom) are coupled to conduction electrons. Such novel non-trivial fixed points are unique to the quasi-quartet multipolar impurity, reinforcing the idea that an unexplored rich diversity of phenomena may be produced by multipolar quantum impurity systems.

cond-mat.str-el

Rise and Fall of Non-Fermi Liquid Fixed Points in Multipolar Kondo Problems

Recently it was shown that the multipolar Kondo problem, wherein a quantum impurity carrying higher-rank multipolar moments interacts with conduction electrons, leads to novel non-Fermi liquid states. Because of the multipolar character of the local moments, the form of the interaction with conduction electrons is strongly dependent on the orbital-symmetry of the conduction electrons via crystalline symmetry constraints. This suggests that there may exist a variety of different non-Fermi liquid states in generic multipolar Kondo problems depending on the character of conduction electrons. In this work, using renormalization group analysis, we investigate a model where the multipolar local moment is coupled to conduction electrons with two different orbital-symmetry components, namely $p$-wave and $f$-wave symmetries. When each orbital-symmetry component is present alone, non-Fermi liquid states with exactly the same thermodynamic singularities appear. When both orbital-symmetry components are allowed, however, a completely different non-Fermi liquid state arises via the quantum fluctuations in the mixed scattering channels. This remarkable result suggests that the multipolar Kondo problem presents novel opportunities for the discovery of unexpected non-Fermi liquid states.

cond-mat.str-el

Unconventional Superconductivity arising from Multipolar Kondo Interactions

The nature of unconventional superconductivity is intimately linked to the microscopic nature of the pairing interactions. In this work, motivated by cubic heavy fermion compounds with embedded multipolar moments, we theoretically investigate superconducting instabilities instigated by multipolar Kondo interactions. Employing multipolar fluctuations (mediated by RKKY interaction) coupled to conduction electrons via two-channel Kondo and novel multipolar Kondo interactions, we uncover a variety of superconducting states characterized by higher-angular momentum Cooper pairs, $J=0,1,2,3$. We demonstrate that both odd and even parity pairing functions are possible, regardless of the total angular momentum of the Cooper pairs, which can be traced back to the atypical nature of the multipolar Kondo interaction that intertwines conduction electron spin and orbital degrees of freedom. We determine that different (point-group) irrep classified pairing functions may coexist with each other, with some of them characterized by gapped and point node structures in their corresponding quasiparticle spectra. This work lays the foundation for discovery and classification of superconducting states in rare-earth metallic compounds with multipolar local moments.

cond-mat.supr-con

Critical theory of non-Fermi liquid fixed point in multipolar Kondo problem

When the ground state of a localized ion is a non-Kramers doublet, such localized ions may carry multipolar moments. For example, Pr$^{3+}$ ions in a cubic environment would possess quadrupolar and octupolar, but no magnetic dipole, moments. When such multipolar moments are placed in a metallic host, unusual interactions between these local moments and conduction electrons arise, in contrast to the familiar magnetic dipole interactions in the classic Kondo problem. In this work, we consider the interaction between a single quadrupolar-octupolar local moment and conduction electrons with $p$-orbital symmetry as a concrete model for the multipolar Kondo problem. We show that this model can be written most naturally in the spin-orbital entangled basis of conduction electrons. Using this basis, the perturbative renormalization group (RG) fixed points are readily identified. There are two kinds of fixed points, one for the two-channel Kondo and the other for a novel fixed point. We investigate the nature of the novel fixed point non-perturbatively using non-abelian bosonization, current algebra and conformal field theory approaches. It is shown that the novel fixed point leads to a, previously unidentified, non-Fermi liquid state with entangled spin and orbital degrees of freedom, which shows resistivity $ρ\sim T^Δ$ and diverging specific heat coefficient $C/T \sim T^{-1 + 2Δ}$ with $Δ=1/5$. Our results open up the possibility of myriads of non-Fermi liquid states, depending on the choices of multipolar moments and conduction electron orbitals, which would be relevant for many rare-earth metallic systems.

cond-mat.str-el