arXiv subjects

Adolfo G. Grushin

Publications and source records attributed to Adolfo G. Grushin.

At least 55 records · Page 3Linked to original sources

arXiv2021

Topology and geometry under the nonlinear electromagnetic spotlight

For many materials, a precise knowledge of their dispersion spectra is insufficient to predict their ordered phases and physical responses. Instead, these materials are classified by the geometrical and topological properties of their wavefunctions. A key challenge is to identify and implement experiments that probe or control these quantum properties. In this review, we describe recent progress in this direction, focusing on nonlinear electromagnetic responses that arise directly from quantum geometry and topology. We give an overview of the field by discussing new theoretical ideas, groundbreaking experiments, and the novel materials that drive them. We conclude by discussing how these techniques can be combined with new device architectures to uncover, probe, and ultimately control novel quantum phases with emergent topological and correlated properties.

cond-mat.mtrl-sci↗

arXiv2021

Suppression of second-harmonic generation from linear bands in the topological multifold semimetal RhSi

Recent experiments in the topological Weyl semimetal TaAs have observed record-breaking second-harmonic generation, a non-linear optical response at $2ω$ generated by an incoming light source at $ω$. However, whether second-harmonic generation is enhanced in topological semimetals in general is a challenging open question because their band structure entangles the contributions arising from trivial bands and topological band crossings. In this work, we circumvent this problem by studying RhSi, a chiral topological semimetal with a simple band structure with topological multifold fermions close to the Fermi energy. We measure second-harmonic generation (SHG) in a wide frequency window, $ω\in [0.27,1.5]$eV and, using first principle calculations, we establish that, due to their linear dispersion, the contribution of multifold fermions to SHG is subdominant as compared with other regions in the Brillouin zone. Our calculations suggest that parts of the bands where the dispersion is relatively flat contribute significantly to SHG. As a whole, our results suggest avenues to enhance SHG responses.

cond-mat.mtrl-sci↗

arXiv2021

Topological phases of amorphous matter

Topological phases of matter are often understood and predicted with the help of crystal symmetries, although they don't rely on them to exist. In this chapter we review how topological phases have been recently shown to emerge in amorphous systems. We summarize the properties of topological states and discuss how disposing of translational invariance has motivated the surge of new tools to characterize topological states in amorphous systems, both theoretically and experimentally. The ubiquity of amorphous systems combined with the robustness of topology has the potential to bring new fundamental understanding in our classification of phases of matter, and inspire new technological developments.

cond-mat.dis-nn↗

arXiv2020

Interacting Stochastic Topology and Mott Transition from Light Response

We develop a stochastic description of the topological properties in an interacting Chern insulator. We confirm the Mott transition's first-order nature in the interacting Haldane model on the honeycomb geometry, from a mean-field variational approach, supported by density matrix renormalization group results and Ginzburg-Landau arguments. From the Bloch sphere, we make predictions for circular dichroism of light related to the quantum Hall conductivity on the lattice and in the presence of interactions. This analysis shows that the topological number can be measured from the light response at the Dirac points. Electron-electron interactions can also produce a substantial number of particle-hole pairs above the band gap, which leads us to propose a "stochastic Chern number" as an interacting measure of the topology. The stochastic Chern number can describe disordered situations with a fluctuating staggered potential and we build an analogy between interaction-induced particle-hole pairs and temperature effects. Our stochastic approach is physically intuitive, easy to implement and leads the way to further studies of interaction effects.

cond-mat.str-el↗

arXiv2020

Entanglement Spectrum Crossings Reveal non-Hermitian Dynamical Topology

The development of non-Hermitian topological band theory has led to observations of novel topological phenomena in effectively classical, driven and dissipative systems. However, for open quantum many-body systems, the absence of a ground state presents a challenge to define robust signatures of non-Hermitian topology. We show that such a signature is provided by crossings in the time evolution of the entanglement spectrum. These crossings occur in quenches from the trivial to the topological phase of a driven-dissipative Kitaev chain that is described by a Markovian quantum master equation in Lindblad form. At the topological transition, which can be crossed either by changing parameters of the Hamiltonian of the system or by increasing the strength of dissipation, the time scale at which the first entanglement spectrum crossing occurs diverges with a dynamical critical exponent of $ε= 1/2$. We corroborate these numerical findings with an exact analytical solution of the quench dynamics for a spectrally flat postquench Liouvillian. This exact solution suggests an interpretation of the topological quench dynamics as a fermion parity pump. Our work thus reveals signatures of non-Hermitian topology which are unique to quantum many-body systems and cannot be emulated in classical simulators of non-Hermitian wave physics.

cond-mat.mes-hall↗

arXiv2020

Topological Weaire-Thorpe models of amorphous matter

Amorphous solids remain outside of the classification and systematic discovery of new topological materials, partially due to the lack of realistic models that are analytically tractable. Here we introduce the topological Weaire-Thorpe class of models, which are defined on amorphous lattices with fixed coordination number, a realistic feature of covalently bonded amorphous solids. Their short-range properties allow us to analytically predict spectral gaps. Their symmetry under permutation of orbitals allows us to analytically compute topological phase diagrams, which determine quantized observables like circular dichroism, by introducing symmetry indicators for the first time in amorphous systems. These models and our procedures to define invariants are generalizable to higher coordination number and dimensions, opening a route towards a complete classification of amorphous topological states in real space using quasilocal properties.

cond-mat.dis-nn↗

arXiv2020

Fermionic dualities with axial gauge fields

The dualities that map hard-to-solve, interacting theories to free, non-interacting ones often trigger a deeper understanding of the systems to which they apply. However, simplifying assumptions such as Lorentz invariance, low dimensionality, or the absence of axial gauge fields, limit their application to a broad class of systems, including topological semimetals. Here we derive several axial field theory dualities in 2+1 and 3+1 dimensions by developing an axial slave-rotor approach capable of accounting for the axial anomaly. Our 2+1-dimensional duality suggests the existence of a dual, critical surface theory for strained three-dimensional non-symmorphic topological insulators. Our 3+1-dimensional duality maps free Dirac fermions to Dirac fermions coupled to emergent U(1) and Kalb-Ramond vector and axial gauge fields. Upon fixing an axial field configuration that breaks Lorentz invariance, this duality maps free to interacting Weyl semimetals, thereby suggesting that the quantization of the non-linear circular photogalvanic effect can be robust to certain interactions. Our work emphasizes how axial and Lorentz-breaking dualities improve our understanding of topological matter.

cond-mat.mes-hall↗

arXiv2020

Anisotropic electrical and thermal magnetotransport in the magnetic semimetal GdPtBi

The half-Heusler rare-earth intermetallic GdPtBi has recently gained attention due to peculiar magnetotransport phenomena that have been associated with the possible existence of Weyl fermions, thought to arise from the crossings of spin-split conduction and valence bands. On the other hand, similar magnetotransport phenomena observed in other rare-earth intermetallics have often been attributed to the interaction of itinerant carriers with localized magnetic moments stemming from the $4f$-shell of the rare-earth element. In order to address the origin of the magnetotransport phenomena in GdPtBi, we performed a comprehensive study of the magnetization, electrical and thermal magnetoresistivity on two single-crystalline GdPtBi samples. In addition, we performed an analysis of the Fermi surface via Shubnikov-de Haas oscillations in one of the samples and compared the results to \emph{ab initio} band structure calculations. Our findings indicate that the electrical and thermal magnetotransport in GdPtBi cannot be solely explained by Weyl physics and is strongly influenced by the interaction of both itinerant charge carriers and phonons with localized magnetic Gd-ions and possibly also paramagnetic impurities.

cond-mat.mes-hall↗

arXiv2019

Strong bulk photovoltaic effect in chiral crystal in the visible spectrum

Structurally chiral materials hosting multifold fermions with large topological number have attracted considerable attention because of their naturally long surface Fermi arcs and bulk quantized circular photogalvanic effect (CPGE). Multifold fermions only appear in metallic states, and therefore, most studies so far have only focused on the semimetals in compounds with chiral crystal structures. In this work, we show that the structurally chiral topological trivial insulators are also exotic states, which is interesting from the application point of view, owing to their natural advantage to host a large bulk photovoltaic effect in the visible wavelength region. In the last decades, the shift current in the visible wavelength region was limited to be 10 uA/V2 . By scanning the insulators with chiral structure, we found a class of compounds with photoconductivity ranging from 20 to 80 uA/V2 , which is approximately one order of magnitude larger than that reported in other real materials. This work illustrates that the compounds with chiral structure can host both quantum CPGE and a strong shift current in the second order optical response. Moreover, this work offers a good platform for the study of the shift current and its future application by putting the focus on insulator with chiral lattices, so far overlooked in photovoltaic technologies.

cond-mat.mtrl-sci↗

arXiv2019

Quantization in chiral higher order topological insulators: circular dichroism and local Chern marker

The robust quantization of observables in units of universal constants is a hallmark of topological phases. We show that chiral higher order topological insulators (HOTIs), bulk insulators with chiral hinge states, present two unusual features related to quantization. First, we show that circular dichroism is quantized to an integer or zero depending on the orientation of the sample. This probe locates the hinge states, and can be used to distinguish different types of chiral HOTIs. Second, we find that the average of the local Chern marker over a single surface, an observable related to the surface Hall conductivity known to be quantized in the infinite slab geometry, is nonuniversal for a finite surface. This is due to a nonuniversal contribution of the hinge states, previously unaccounted for, that distinguishes surfaces of chiral HOTIs from Chern insulators. Our findings are relevant to establish higher order topology in systems such as the axion insulator candidate EuIn$_2$As$_2$, and cold atomic realizations.

cond-mat.mes-hall↗

arXiv2019

Common and not so common high-energy theory methods for condensed matter physics

This chapter is a collection of techniques, warnings, facts and ideas that are sometimes regarded as theoretical curiosities in high-energy physics but have important consequences in condensed matter physics. In particular, we describe theories that have the property of having finite but undetermined radiative corrections that also happen to describe topological semi-metallic phases in condensed matter. In the process, we describe typical methods in high-energy physics that illustrate the working principles to describe a given phase of matter and its response to external fields.

cond-mat.mes-hall↗

arXiv2019

Difference frequency generation in topological semimetals

When two lasers are applied to a non-centrosymmetric material, light can be generated at the difference of the incoming frequencies $Δω$, a phenomenon known as difference frequency generation (DFG), well characterized in semiconductors. In this work, we derive a general expression for DFG in metals, which we use to show that the DFG in chiral topological semimetals under circular polarized light is quantized in units of $e^3/h^2$ and independent of material parameters, including the scattering time $τ$, when $Δω\gg τ^{-1}$. In this regime, DFG provides a simpler alternative to measure a quantized response in metals compared to previous proposals based on single frequency experiments. Our general derivation unmasks, in addition, a free-carrier contribution to the circular DFG beyond the semiclassical one. This contribution can be written as a Fermi surface integral, features strong frequency dependence, and oscillates with a $π/2$ shift with respect to the quantized contribution. We make predictions for the circular DFG of chiral and non-chiral materials using generic effective models, and ab-initio calculations for TaAs and RhSi. Our work provides a complete picture of the DFG in the length gauge approach, in the clean, non-interacting limit, and highlights a plausible experiment to measure topologically quantizated photocurrents in metals.

cond-mat.mes-hall↗

arXiv2019

Spectral and optical properties of Ag$_3$Au(Se$_2$,Te$_2$) and dark matter detection

In this work we study the electronic structure of Ag${}_3$AuSe${}_2$ and Ag${}_3$AuTe${}_2$, two chiral insulators whose gap can be tuned through small changes in the lattice parameter by applying hydrostatic pressure or choosing different growth protocols. Based on first principles calculations we compute their band structure for different values of the lattice parameters and show that while Ag${}_3$AuSe${}_2$ retains its direct narrow gap at the $Γ$ point, Ag${}_3$AuTe${}_2$ can turn into a metal. Focusing on Ag${}_3$AuSe${}_2$ we derive a low energy model around $Γ$ using group theory, which we use to calculate the optical conductivity for different values of the lattice constant. We discuss our results in the context of detection of light dark matter particles, which have masses of the order of a $k$eV, and conclude that Ag${}_3$AuSe${}_2$ satisfies three important requirements for a suitable detector: small Fermi velocities, $m$eV band gap and low photon screening. Our work motivates the growth of high-quality and large samples of Ag${}_3$AuSe${}_2$ to be used as target materials in dark matter detectors.

cond-mat.mtrl-sci↗

arXiv2019

Linear optical conductivity of chiral multifold fermions

Chiral multifold fermions are quasiparticles described by higher spin generalizations of the Weyl equation, and are realized as low energy excitations near symmetry protected band crossings in certain chiral crystals. In this work we calculate the linear optical conductivity of all chiral multifold fermions. We show that it is enhanced with respect to that of Weyl fermions with the same Fermi velocity, and features characteristic activation frequencies for each multifold fermion class, providing an experimental fingerprint to detect them. We calculate the conductivity for realistic chiral multifold semimetals by using lattice tight-binding Hamiltonians that match the effective models of multifold fermions at low energies, for space groups 199 and 198. The latter includes RhSi, for which we give quantitative predictions, and also CoSi and AlPt. Our predictions can be tested in absorption or penetration depth measurements, and are necessary to extract the recently proposed quantized photocurrents from experiments.

cond-mat.mes-hall↗

arXiv2019

Landau levels, Bardeen polynomials and Fermi arcs in Weyl semimetals: the who's who of the chiral anomaly

Condensed matter systems realizing Weyl fermions exhibit striking phenomenology derived from their topologically protected surface states as well as chiral anomalies induced by electromagnetic fields. More recently, inhomogeneous strain or magnetization were predicted to result in chiral electric $\mathbf{E}_5$ and magnetic $\mathbf{B}_5$ fields, which modify and enrich the chiral anomaly with additional terms. In this work, we develop a lattice-based approach to describe the chiral anomaly, which involves Landau and pseudo-Landau levels and treats all anomalous terms on equal footing, while naturally incorporating Fermi arcs. We exemplify its potential by physically interpreting the largely overlooked role of Fermi arcs in the covariant (Fermi level) contribution to the anomaly and revisiting the factor of $1/3$ difference between the covariant and consistent (complete band) contributions to the $\mathbf{E}_5\cdot\mathbf{B}_5$ term in the anomaly. Our framework provides a versatile tool for the analysis of anomalies in realistic lattice models as well as a source of simple physical intuition for understanding strained and magnetized inhomogeneous Weyl semimetals.

cond-mat.mes-hall↗

arXiv2019

Pseudo-electromagnetic fields in topological semimetals

Dirac and Weyl semimetals, materials where electrons behave as relativistic fermions, react to position- and time-dependent perturbations, such as strain, as if emergent electromagnetic fields were applied. Since they differ from external electromagnetic fields in their symmetries and phenomenology they are called pseudo-electromagnetic fields, and enable a simple and unified description of a variety of inhomogeneous systems involving topological semimetals. We review the different physical ways to create effective pseudo-fields, their observable consequences as well as their similarities and differences compared to electromagnetic fields. Among these difference is their effect on quantum anomalies, the absence of a classical symmetry in the quantum theory, which we revisit from a quantum field theory and a semiclassical viewpoint. We conclude with predicted observable signatures of the pseudo-fields and the nascent experimental status.

cond-mat.mes-hall↗

arXiv2018

Charge excitation dynamics in bosonic fractional Chern insulators

The experimental realization of the Harper-Hofstadter model in ultra-cold atomic gases has placed fractional states of matter in these systems within reach---a fractional Chern insulator state (FCI) is expected to emerge for sufficiently strong interactions when half-filling the lowest band. The experimental setups naturally allow to probe the dynamics of this topological state, yet little is known about its out-of-equilibrium properties. We explore, using density matrix renormalization group (DMRG) simulations, the response of the FCI state to spatially localized perturbations. After confirming the static properties of the phase we show that the characteristic, gapless features are clearly visible in the edge dynamics. We find that a local edge perturbation in this model propagates chirally independent of the perturbation strength. This contrasts the behavior of single particle models with counter-propagating edge states, such as the non-interacting Harper-Hofstadter model, where the chirality is manifest only for weak perturbations. Additionally, our simulations show that there is inevitable density leakage from the first row of sites into the bulk, preventing a naive chiral Luttinger theory interpretation of the dynamics.

cond-mat.str-el↗

arXiv2018

Chiral Optical Response of Multifold Fermions

Multifold fermions are generalizations of two-fold degenerate Weyl fermions with three-, four-, six- or eight-fold degeneracies protected by crystal symmetries, of which only the last type is necessarily non-chiral. Their low energy degrees of freedom can be described as emergent particles not present in the Standard Model of particle physics. We propose a range of experimental probes for multifold fermions in chiral symmetry groups based on the gyrotropic magnetic effect (GME) and the circular photo-galvanic effect (CPGE). We find that, in contrast to Weyl fermions, multifold fermions can have zero Berry curvature yet a finite GME, leading to an enhanced response. The CPGE is quantized and independent of frequency provided that the frequency region at which it is probed defines closed optically-activated momentum surfaces. We confirm the above properties by calculations in symmetry-restricted tight binding models with realistic density functional theory parameters. We identify a range of previously-unidentified ternary compounds able to exhibit chiral multifold fermions of all types (including a range of materials in the families AsBaPt and Gd$_3$Cl$_3$C), and provide specific predictions for the known multifold material RhSi.

cond-mat.mes-hall↗