arXiv subjects

Adrian A. Budini

Publications and source records attributed to Adrian A. Budini.

25 records · Page 2Linked to original sources

arXiv2010

Quantum-jumps and photon-statistic in fluorescent systems coupled to classically fluctuating reservoirs

In this paper, we develop a quantum-jump approach for describing the photon-emission process of single fluorophore systems coupled to complex classically fluctuating reservoirs. The formalism relies on an open quantum system approach where the dynamic of the system and the reservoir fluctuations are described through a density matrix whose evolution is defined by a Lindblad rate equation. For each realization of the photon measurement processes it is possible to define a conditional system state (stochastic density matrix) whose evolution depends on both the photon detection events and the fluctuations between the configurational states of the reservoir. In contrast to standard fluorescent systems the photon-to-photon emission process is not a renewal one, being defined by a (stochastic) waiting time distribution that in each recording event parametrically depends on the conditional state. The formalism allows calculating experimental observables such as the full hierarchy of joint probabilities associated to the time intervals between consecutive photon recording events. These results provide a powerful basis for characterizing different situations arising in single-molecule spectroscopy, such as spectral fluctuations, lifetime fluctuations, and light assisted processes.

quant-ph↗

arXiv2009

Open quantum system approach to single-molecule spectroscopy

In this paper, single-molecule spectroscopy experiments based on continuous laser excitation are characterized through an open quantum system approach. The evolution of the fluorophore system follows from an effective Hamiltonian microscopic dynamic where its characteristic parameters, i.e., its electric dipole, transition frequency, and Rabi frequency, as well as the quantization of the background electromagnetic field and their mutual interaction, are defined in an extended Hilbert space associated to the different configurational states of the local nano-environment. After tracing out the electromagnetic field and the configurational states, the fluorophore density matrix is written in terms of a Lindblad rate equation. Observables associated to the scattered laser field, like optical spectrum, intensity-intensity correlation, and photon-counting statistics, are obtained from a quantum-electrodynamic calculation also based on the effective microscopic dynamic. In contrast with stochastic models, this approach allows to describe in a unified way both the full quantum nature of the scattered laser field as well as the classical nature of the environment fluctuations. By analyzing different processes such as spectral diffusion, lifetime fluctuations, and light assisted processes, we exemplify the power of the present approach.

quant-ph↗

arXiv2008

Langevin approach to synchronization of hyperchaotic time-delay dynamics

In this paper, we characterize the synchronization phenomenon of hyperchaotic scalar non-linear delay dynamics in a fully-developed chaos regime. Our results rely on the observation that, in that regime, the stationary statistical properties of a class of hyperchaotic attractors can be reproduced with a linear Langevin equation, defined by replacing the non-linear delay force by a delta-correlated noise. Therefore, the synchronization phenomenon can be analytically characterized by a set of coupled Langevin equations. We apply this formalism to study anticipated synchronization dynamics subject to external noise fluctuations as well as for characterizing the effects of parameter mismatch in a hyperchaotic communication scheme. The same procedure is applied to second order differential delay equations associated to synchronization in electro-optical devices. In all cases, the departure with respect to perfect synchronization is measured through a similarity function. Numerical simulations in discrete maps associated to the hyperchaotic dynamics support the formalism.

nlin.CD↗

arXiv2006

Lindblad rate equations

In this paper we derive an extra class of non-Markovian master equations where the system state is written as a sum of auxiliary matrixes whose evolution involve Lindblad contributions with local coupling between all of them, resembling the structure of a classical rate equation. The system dynamics may develops strong non-local effects such as the dependence of the stationary properties with the system initialization. These equations are derived from alternative microscopic interactions, such as complex environments described in a generalized Born-Markov approximation and tripartite system-environment interactions, where extra unobserved degrees of freedom mediates the entanglement between the system and a Markovian reservoir. Conditions that guarantees the completely positive condition of the solution map are found. Quantum stochastic processes that recover the system dynamics in average are formulated. We exemplify our results by analyzing the dynamical action of non-trivial structured dephasing and depolarizing reservoirs over a single qubit.

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arXiv2006

Quantum regression theorem for non-Markovian Lindblad equations

We find the conditions under which a quantum regression theorem can be assumed valid for non-Markovian master equations consisting in Lindblad superoperators with memory kernels. Our considerations are based on a generalized Born-Markov approximation, which allows us to obtain our results from an underlying Hamiltonian description. We demonstrate that a non-Markovian quantum regression theorem can only be granted in a stationary regime if the dynamics satisfies a quantum detailed balance condition. As an example we study the correlations of a two level system embedded in a complex structured reservoir and driven by an external coherent field.

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arXiv2005

Random Lindblad equations from complex environments

In this paper we demonstrate that Lindblad equations characterized by a random rate variable arise after tracing out a complex structured reservoir. Our results follows from a generalization of the Born-Markov approximation, which relies in the possibility of splitting the complex environment in a direct sum of sub-reservoirs, each one being able to induce by itself a Markovian system evolution. Strong non-Markovian effects, which microscopically originate from the entanglement with the different sub-reservoirs, characterize the average system decay dynamics. As an example, we study the anomalous irreversible behavior of a quantum tunneling system described in an effective two level approximation. Stretched exponential and power law decay behaviors arise from the interplay between the dissipative and unitary hopping dynamics.

quant-ph↗

arXiv2005

Non-Markovian master equations from entanglement with stationary unobserved degrees of freedom

We deduce a class of non-Markovian completely positive master equations which describe a system in a composite bipartite environment, consisting of a Markovian reservoir and additional stationary unobserved degrees of freedom that modulate the dissipative coupling. The entanglement-induced memory effects can persist for arbitrary long times and affect the relaxation to equilibrium, as well as induce corrections to the quantum-regression theorem. By considering the extra degrees of freedom as a discrete manifold of energy levels, strong non-exponential behavior can arise, as for example power law and stretched exponential decays.

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