arXiv subjects

Adrian A. Valverde

Publications and source records attributed to Adrian A. Valverde.

4 recordsLinked to original sources

arXiv2026

The mass of $^{101}$Sn and Bayesian extrapolations to the proton drip line

The favorable energy configurations of nuclei at magic numbers of ${N}$ neutrons and ${Z}$ protons are fundamental for understanding the evolution of nuclear structure. The ${Z=50}$ (tin) isotopic chain is a frontier for such studies, with particular interest at and around the doubly-magic \textsuperscript{100}Sn isotope, for which the mass is a topic of debate. Precise mass values for neutron-deficient isotopes provide necessary anchor points for mass models to test extrapolations near the proton drip line, where experimental studies remain out of reach. In this work, we report the first Penning trap mass measurement of \textsuperscript{101}Sn. The determined mass excess of $-59\,889.89(96)$~keV for \textsuperscript{101}Sn represents a factor of 300 improvement over the current precision and indicates that \textsuperscript{101}Sn is less bound than previously thought. Mass predictions from a recently developed Bayesian model combination (BMC) framework employing statistical machine learning and nuclear masses computed within seven global models based on nuclear Density Functional Theory (DFT) agree within 1$σ$ with experimental masses from the $48 \le Z \le 52$ isotopic chains. The framework's resilience to new mass data gave confidence in the extrapolation of tin masses down to $N=46$. Our calculations suggest that \textsuperscript{96}Sn is a two-proton drip line nucleus and predict a mass excess of $-58\,090(800)$~keV for $^{100}$Sn, showing a preference within 1$σ$ for the mass of \textsuperscript{100}Sn derived from the $β$-delayed $Q$-value measured at GSI.

nucl-ex↗

arXiv2025

Fingerprints of triaxiality in the charge radii of neutron-rich Ruthenium

We present the first measurements with a new collinear laser spectroscopy setup at the Argonne Tandem Linac Accelerator System utilizing its unique capability to deliver neutron-rich refractory metal isotopes produced by the spontaneous fission of 252Cf. We measured isotope shifts from optical spectra for nine radioactive ruthenium isotopes 106-114Ru, reaching deep into the mid-shell region. The extracted charge radii are in excellent agreement with predictions from the Brussels-Skyrme-on-a-Grid models that account for the triaxial deformation of nuclear ground states in this region. We show that triaxial deformation impacts charge radii in models that feature shell effects, in contrast to what could be concluded from a liquid drop analysis. This indicates that this exotic type of deformation should not be neglected in regions where it is known to occur, even if its presence cannot be unambiguously inferred through laser spectroscopy.

nucl-ex↗

arXiv2022

Precise Q value measurements of $^{112,113}$Ag and $^{115}$Cd with the Canadian Penning trap for evaluation of potential ultra-low Q value $β$-decays

An ultra-low Q value $β$-decay can occur from a parent nuclide to an excited state in the daughter with $Q_{UL}$ <1 keV. These decays are of interest for nuclear $β$-decay theory and as potential candidates in neutrino mass determination experiments. To date, only one ultra-low Q value $β$-decay has been observed -- that of $^{115}$In with $Q_β$ = 147(10) eV. A number of other potential candidates exist, but improved mass measurements are necessary to determine if the decays are energetically allowed and, in fact, ultra-low. We performed precise $β$-decay Q value measurements of $^{112,113}$Ag and $^{115}$Cd and combined them with nuclear energy level data for the daughter isotopes to determine if the potential UL Q value $β$-decay branches of $^{112,113}$Ag and $^{115}$Cd are energetically allowed and <1 keV. The Canadian Penning Trap at ANL was used to measure the cyclotron frequency ratios of singly-charged $^{112,113}$Ag and $^{115}$Cd ions with respect to their daughters. From these measurements, the ground-state $β$-decay Q values were obtained. The $^{112}$Ag, $^{113}$Ag, and $^{115}$Cd $β$-decay Q values were measured to be 3990.16(22) keV, 2085.7(4.6) keV, and 1451.36(34) keV, respectively. These results were compared to energies of excited states in $^{112}$Cd at 3997.75(14) keV, $^{113}$Cd at 2015.6(2.5) and 2080(10) keV, and $^{115}$In at 1448.787(9) keV, resulting in $Q_{\textrm{UL}}$ values of --7.59(26) keV, 6(11) keV, and 2.57(34) keV, respectively. The potential UL Q value decays of $^{112}$Ag and $^{115}$Cd have been ruled out. $^{113}$Ag is still a possible candidate until a more precise measurement of the 2080(10) keV, 1/2$^{+}$ state of $^{113}$Cd is available. In the course of this work we have found the ground state mass of $^{113}$Ag reported in the 2020AME to be lower than our measurement by 69(17) keV (a 4$σ$ discrepancy).

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arXiv2021

Gaussian mixture model clustering algorithms for the analysis of high-precision mass measurements

The development of the phase-imaging ion-cyclotron resonance (PI-ICR) technique for use in Penning trap mass spectrometry (PTMS) increased the speed and precision with which PTMS experiments can be carried out. In PI-ICR, data sets of the locations of individual ion hits on a detector are created showing how ions cluster together into spots according to their cyclotron frequency. Ideal data sets would consist of a single, 2D-spherical spot with no other noise, but in practice data sets typically contain multiple spots, non-spherical spots, or significant noise, all of which can make determining the locations of spot centers non-trivial. A method for assigning groups of ions to their respective spots and determining the spot centers is therefore essential for further improving precision and confidence in PI-ICR experiments. We present the class of Gaussian mixture model (GMM) clustering algorithms as an optimal solution. We show that on simulated PI-ICR data, several types of GMM clustering algorithms perform better than other clustering algorithms over a variety of typical scenarios encountered in PI-ICR. The mass spectra of $^{163}\text{Gd}$, $^{163m}\text{Gd}$, $^{162}\text{Tb}$, and $^{162m}\text{Tb}$ measured using PI-ICR at the Canadian Penning trap mass spectrometer were checked using GMMs, producing results that were in close agreement with the previously published values.

physics.comp-ph↗