arXiv subjects

Adriana Pálffy

Publications and source records attributed to Adriana Pálffy.

At least 37 records · Page 2Linked to original sources

arXiv2022

Nuclear coherent population transfer to the $^{229m}$Th isomer using x-ray pulses

Population of the 8 eV $^{229m}$Th isomer via the second nuclear excited state at 29.19 keV by means of coherent x-ray pulses is investigated theoretically. We focus on two nuclear coherent population transfer schemes using partially overlapping x-ray pulses known from quantum optics: stimulated Raman adiabatic passage (STIRAP), and successive $π$ pulses. Numerical results are presented for three possible experimental setups. Our results identify the Gamma Factory as the most promising scenario, where two ultraviolet pulses combined with relativistically accelerated ions deliver the required intensities for efficient isomer population. Our simulations require knowledge of the in-band and cross-band nuclear transition probabilities. We give theoretically predicted values for the latter and discuss them in the context of recent experiments.

nucl-th↗

arXiv2022

Multiphonon quantum dynamics in cavity optomechanical systems

The multiphonon quantum dynamics in laser-pumped cavity optomechanical samples containing a vibrating mirror is investigated. Especially, we focus on dispersive interaction regimes where the externally applied coherent field frequency detuning from the optical resonator frequency is not equal to the mirror's oscillating frequency or to its multiples. As a result, for moderately strong couplings among the involved subsystems, the quantum dynamics of this complex system is described by multiphonon absorption or emission processes, respectively. Particularly, we demonstrate efficient ways to monitor the phonon quantum dynamics via photon detection. The possibility to extract the relevant sample parameters, for instance, the coupling strength between the mechanical mirror and the electromagnetic field, is also discussed.

quant-ph↗

arXiv2021

Dynamical control of nuclear isomer depletion via electron vortex beams

Long-lived excited states of atomic nuclei can act as energy traps. These states, known as nuclear isomers, can store a large amount of energy over long periods of time, with a very high energy-to-mass ratio. Under natural conditions, the trapped energy is only slowly released, limited by the long isomer lifetimes. Dynamical external control of nuclear state population has proven so far very challenging, despite ground-breaking incentives for a clean and efficient energy storage solution. Here, we describe a protocol to achieve the external control of the isomeric nuclear decay by using electrons whose wavefunction has been especially designed and reshaped on demand. Recombination of these electrons into the atomic shell around the isomer can lead to the controlled release of the stored nuclear energy. On the example of $^{93m}$Mo, we show that the use of tailored electron vortex beams increases the depletion by four orders of magnitude compared to the spontaneous nuclear decay of the isomer. Furthermore, specific orbitals can sustain an enhancement of the recombination cross section for vortex electron beams by as much as six orders of magnitude, providing a handle for manipulating the capture mechanism. These findings open new prospects for controlling the interplay between atomic and nuclear degrees of freedom, with potential energy-related and high-energy radiation sources applications.

physics.atom-ph↗

arXiv2021

Expanding Nuclear Physics Horizons with the Gamma Factory

The Gamma Factory (GF) is an ambitious proposal, currently explored within the CERN Physics Beyond Colliders program, for a source of photons with energies up to $\approx 400\,$MeV and photon fluxes (up to $\approx 10^{17}$ photons per second) exceeding those of the currently available gamma sources by orders of magnitude. The high-energy (secondary) photons are produced via resonant scattering of the primary laser photons by highly relativistic partially-stripped ions circulating in the accelerator. The secondary photons are emitted in a narrow cone and the energy of the beam can be monochromatized, eventually down to the $\approx1$ ppm level, via collimation, at the expense of the photon flux. This paper surveys the new opportunities that may be afforded by the GF in nuclear physics and related fields.

nucl-ex↗

arXiv2021

Laser-nucleus interactions in the sudden regime

The interaction between medium-weight nuclei and a strong zeptosecond laser pulse of MeV photons is investigated theoretically. Multiple absorption of photons competes with nuclear equilibration. We investigate the sudden regime. Here the rate of photon absorption is so strong that there is no time for the nucleus to fully equilibrate after each photon absorption process. We follow the temporal evolution of the system in terms of a set of rate equations. These account for dipole absorption and induced dipole emission, equilibration (modeled in terms of particle-hole states coupled by the residual nuclear interaction), and neutron decay (populating a chain of proton-rich nuclei). Our results are compared with earlier work addressing the adiabatic regime where equilibration is instantaneous. We predict the degree of excitation and the range of nuclei reached by neutron evaporation. These findings are relevant for planning future experiments.

nucl-th↗

arXiv2021

Transient nuclear inversion by X-Ray Free Electron Laser in a tapered x-ray waveguid

By restricting the spatial energy transmission of an electromagnetic wave, dielectric waveguides transmit light over long distances at sustained intensity. Waveguides have been used in the microwave and optical range to maintain strong signal intensities in connection with lasers, but guiding of intense short-wavelength radiation such as x-rays has proven more cumbersome. Here we investigate theoretically how tapered x-ray waveguides can focus and guide radiation from x-ray free electron lasers. Elliptical waveguides using a cladding material with high atomic number such as platinum can maintain an x-ray intensity up to three orders of magnitude larger than in free space. This feature can be used to significantly enhance resonant interactions of x-rays, for instance driving nuclear transitions up to transient nuclear population inversion. This could be the first breakthrough in nuclear state population control. Our results anticipate the important role of tapered x-ray waveguides in the emerging field of x-ray quantum optics with nuclear transitions.

physics.optics↗

arXiv2021

Superradiance and anomalous hyperfine splitting in inhomogeneous ensembles

Collective effects in the interaction of light with ensembles of identical scatterers play an important role in many fields of physics. However, often the term ``identical'' is not accurate due to the presence of hyperfine fields which induce inhomogeneous transition shifts and splittings. Here we develop a formalism based on the Green function method to model the linear response of such inhomogeneous ensembles in one-dimensional waveguides. We obtain a compact formula for the collective spectrum, which exhibits deviations from the uniform frequency shift and broadening expected of two level systems. In particular, if the coherent contribution to the collective coupling is large, the effect of inhomogeneous broadening can be suppressed, with the linewidth approaching that of the superradiant value. We apply this formalism to describe collective effects in x-ray scattering off thin-film waveguides for inhomogeneous hyperfine parameters.

quant-ph↗

arXiv2021

$^{229m}$Th isomer from a nuclear model perspective

The physical conditions for the emergence of the extremely low-lying nuclear isomer $^{229m}$Th at approximately 8 eV are investigated in the framework of our recently proposed nuclear structure model. Our theoretical approach explains the $^{229m}$Th-isomer phenomenon as the result of a very fine interplay between collective quadrupole-octupole and single-particle dynamics in the nucleus. We find that the isomeric state can only appear in a rather limited model space of quadrupole-octupole deformations in the single-particle potential, with the octupole deformation being of a crucial importance for its formation. Within this deformation space the model-described quantities exhibit a rather smooth behaviour close to the line of isomer-ground state quasi-degeneracy determined by the crossing of the corresponding single-particle orbitals. Our comprehensive analysis confirms the previous model predictions for reduced transition probabilities and the isomer magnetic moment, while showing a possibility for limited variation in the ground-state magnetic moment theoretical value. These findings prove the reliability of the model and suggest that the same dynamical mechanism could manifest in other actinide nuclei giving a general prescription for the search and exploration of similar isomer phenomena.

nucl-th↗

arXiv2020

Green function formalism for resonant interaction of x-rays with nuclei in structured media

The resonant interaction between x-ray photons and nuclei is one of the most exciting subjects of the burgeoning field of x-ray quantum optics. A resourceful platform used so far are thin-film x-ray cavities with embedded layers or Mössbauer nuclei such as $^{57}\mathrm{Fe}$. A new quantum optical model based on the classical electromagnetic Green's function is developed to investigate theoretically the nuclear response inside the x-ray cavity. The model is versatile and provides an intuitive picture about the influence of the cavity structure on the resulting spectra. We test its predictive powers with the help of the semiclassical coherent scattering formalism simulations and discuss our results for increasing complexity of layer structures.

quant-ph↗

arXiv2020

Nuclear excitation of the $^{229}$Th isomer via defect states in doped crystals

When Th nuclei are doped in CaF$_2$ crystals, a set of electronic defect states appears in the crystal bandgap which would otherwise provide complete transparency to vacuum-ultraviolet radiation. The coupling of these defect states to the 8 eV $^{229m}$Th nuclear isomer in the CaF$_2$ crystal is investigated theoretically. We show that although previously viewed as a nuisance, the defect states provide a starting point for nuclear excitation via electronic bridge mechanisms involving stimulated emission or absorption using an optical laser. The rates of these processes are at least two orders of magnitude larger than direct photoexcitation of the isomeric state using available light sources. The nuclear isomer population can also undergo quenching when triggered by the reverse mechanism, leading to a fast and controlled decay via the electronic shell. These findings are relevant for a possible solid-state nuclear clock based on the $^{229m}$Th isomeric transition.

cond-mat.mtrl-sci↗

arXiv2020

The theory of direct laser excitation of nuclear transitions

A comprehensive theoretical study of direct laser excitation of a nuclear state based on the density matrix formalism is presented. The nuclear clock isomer $^{229\text{m}}$Th is discussed in detail, as it could allow for direct laser excitation using existing technology and provides the motivation for this work. The optical Bloch equations are derived for the simplest case of a pure nuclear two-level system and for the more complex cases taking into account the presence of magnetic sub-states, hyperfine-structure and Zeeman splitting in external fields. Nuclear level splitting for free atoms and ions as well as for nuclei in a solid-state environment is discussed individually. Based on the obtained equations, nuclear population transfer in the low-saturation limit is reviewed. Further, nuclear Rabi oscillations, power broadening and nuclear two-photon excitation are considered. Finally, the theory is applied to the special cases of $^{229\text{m}}$Th and $^{235\text{m}}$U, being the nuclear excited states of lowest known excitation energies. The paper aims to be a didactic review with many calculations given explicitly.

nucl-th↗

arXiv2020

Rate for Laser-Induced Nuclear Dipole Absorption

Using the Brink-Axel hypothesis we derive the rate $R$ for nuclear dipole excitation by a laser pulse carrying $N \gg 1$ photons with average energy $\hbar ω_0 \approx 5$ MeV. As expected $R \propto (\hbar ω_0)^3$. The rate is also proportional to the aperure $α$ of the laser pulse. Perhaps less expected is the fact that $R \propto N$, irrespective of the degree of coherence of the laser pulse. The expression for $R$, derived for a nearly stationary laser pulse, is valid also for short times and can, thus, be used in simulations via rate equations of multiple nuclear dipole excitations by a single pulse. The explicit dependence of $R$ on the parameters of the laser pulse and on nuclear parameters given in the paper should help to optimize experiments on laser-nucleus reactions.

nucl-th↗

arXiv2020

Electronic bridge excitation in highly charged Th-229 ions

The excitation of the 8 eV $^{229m}$Th isomer through the electronic bridge mechanism in highly charged ions is investigated theoretically. By exploiting the rich level scheme of open $4f$ orbitals and the robustness of highly charged ions against photoionization, a pulsed high-intensity optical laser can be used to efficiently drive the nuclear transition by coupling it to the electronic shell. We show how to implement a promising electronic bridge scheme in an electron beam ion trap starting from a metastable electronic state. This setup would avoid the need for a tunable vacuum ultraviolet laser. Based on our theoretical predictions, determining the isomer energy with an uncertainty of $10^{-5}$ eV could be achieved in one day of measurement time using realistic laser parameters.

physics.atom-ph↗

arXiv2019

X-ray assisted nuclear excitation by electron capture in optical laser-generated plasmas

X-ray assisted nuclear excitation by electron capture (NEEC) into inner-shell atomic holes in a plasma environment generated by strong optical lasers is investigated theoretically. The considered scenario involves the interaction of a strong optical laser with a solid-state nuclear target leading to the generation of a plasma. In addition, intense x-ray radiation from an X-ray Free Electron Laser (XFEL) produces inner-shell holes in the plasma ions, into which NEEC may occur. As case study we consider the $4.85$-keV transition starting from the 2.4 MeV long-lived $^{\mathrm{93m}}$Mo isomer that can be used to release the energy stored in this metastable nuclear state. We find that the recombination into $2p_{1/2}$ inner-shell holes is most efficient in driving the nuclear transition. Already at few hundred eV plasma temperature, the generation of inner-shell holes can allow optimal conditions for NEEC, otherwise reached for steady-state plasma conditions in thermodynamical equilibrium only at few keV. The combination of x-ray and optical lasers presents two advantages: first, NEEC rates can be maximized at plasma temperatures where the photoexcitation rate remains low. Second, with mJ-class optical lasers and an XFEL repetition rate of $10$ kHz, the NEEC excitation number can reach $\sim 1$ depleted isomer per second and is competitive with scenarios recently envisaged at petawatt-class lasers.

physics.plasm-ph↗

arXiv2019

Can extreme electromagnetic fields accelerate the $α$ decay of nuclei?

The possibility to control the $α$ decay channel of atomic nuclei with electromagnetic fields of extreme intensities envisaged for the near future at multi-petawatt and exawatt laser facilities is investigated theoretically. Using both analytic arguments based on the Wentzel-Kramers-Brillouin approximation and numerical calculations for the imaginary time method applied in the framework of the $α$ decay precluster model, we show that no experimentally detectable modification of the $α$ decay rate can be observed with super-intense lasers at any so-far available wavelength. Comparing our predictions with those reported in several recent publications, where a considerable or even giant laser-induced enhancement of the decay rate has been claimed, we identify there the misuse of a standard approximation.

nucl-th↗

arXiv2019

Roadmap on STIRAP applications

STIRAP (Stimulated Raman Adiabatic Passage) is a powerful laser-based method, usually involving two photons, for efficient and selective transfer of population between quantum states. A particularly interesting feature is the fact that the coupling between the initial and the final quantum states is via an intermediate state even though the lifetime of the latter can be much shorter than the interaction time with the laser radiation. Nevertheless, spontaneous emission from the intermediate state is prevented by quantum interference. Maintaining the coherence between the initial and final state throughout the transfer process is crucial. STIRAP was initially developed with applications in chemical dynamics in mind. That is why the original paper of 1990 was published in The Journal of Chemical Physics. However, as of about the year 2000, the unique capabilities of STIRAP and its robustness with respect to small variations of some experimental parameters stimulated many researchers to apply the scheme in a variety of other fields of physics. The successes of these efforts are documented in this collection of articles.

quant-ph↗

arXiv2019

$^{93m}$Mo isomer depletion via beam-based nuclear excitation by electron capture

A recent nuclear physics experiment [C. J. Chiara {\it et al.}, Nature (London) {\bf 554}, 216 (2018)] reports the first direct observation of nuclear excitation by electron capture (NEEC) in the depletion of the $^{93m}$Mo isomer. The experiment used a beam-based setup in which Mo highly charged ions with nuclei in the isomeric state $^{93m}$Mo at 2.4 MeV excitation energy were slowed down in a solid-state target. In this process, nuclear excitation to a higher triggering level led to isomer depletion. The reported excitation probability $P_{\rm{exc}} = 0.01$ was solely attributed to the so-far unobserved process of NEEC in lack of a different known channel of comparable efficiency. In this work, we investigate theoretically the beam-based setup and calculate excitation rates via NEEC using state-of-the-art atomic structure and ion stopping power models. For all scenarios, our results disagree with the experimental data by approximately nine orders of magnitude. This stands in conflict with the conclusion that NEEC was the excitation mechanism behind the observed depletion rate.

nucl-th↗

arXiv2019

Energy of the $^{229}$Th nuclear clock transition

The first nuclear excited state of $^{229}$Th offers the unique opportunity for laser-based optical control of a nucleus. Its exceptional properties allow for the development of a nuclear optical clock which offers a complementary technology and is expected to outperform current electronic-shell based atomic clocks. The development of a nuclear clock was so far impeded by an imprecise knowledge of the energy of the $^{229}$Th nuclear excited state. In this letter we report a direct excitation energy measurement of this elusive state and constrain this to 8.28$\pm$0.17 eV. The energy is determined by spectroscopy of the internal conversion electrons emitted in-flight during the decay of the excited nucleus in neutral $^{229}$Th atoms. The nuclear excitation energy is measured via the valence electronic shell, thereby merging the fields of nuclear- and atomic physics to advance precision metrology. The transition energy between ground and excited state corresponds to a wavelength of 149.7$\pm$3.1 nm. These findings set the starting point for high-resolution nuclear laser spectroscopy and thus the development of a nuclear optical clock of unprecedented accuracy. A nuclear clock is expected to have a large variety of applications, ranging from relativistic geodesy over dark matter research to the observation of potential temporal variation of fundamental constants.

nucl-ex↗