arXiv subjects

Adriana Pálffy

Publications and source records attributed to Adriana Pálffy.

At least 73 records · Page 4Linked to original sources

arXiv2015

Logical operations with single x-ray photons via dynamically-controlled nuclear resonances

The implementation of logical operations on polarization-encoded x-rays via resonant light-nucleus interactions is theoretically investigated. We show that by means of resonant scattering off nuclei and fast rotations of the nuclear hyperfine magnetic field to control the polarization of the output photon, single-qubit logical gates can be simulated. A second control qubit may be employed to trigger the magnetic field rotation, thus allowing several implementation choices for a controlled NOT gate for x-ray photons.

quant-ph↗

arXiv2014

All-Electromagnetic Control of Broadband Quantum Excitations Using Gradient Photon Echoes

A broadband quantum echo effect in a three level $\varLambda$-type system interacting with two laser fields is investigated theoretically. Inspired by the emerging field of nuclear quantum optics which typically deals with very narrow resonances, we consider broadband probe pulses that couple to the system in the presence of an inhomogeneous control field. We show that such a setup provides an all-electromagnetic-field solution to implement high bandwidth photon echoes, which are easy to control, store and shape on a short time scale and therefore may speed up future photonic information processing. The time compression of the echo signal and possible applications for quantum memories are discussed.

quant-ph↗

arXiv2014

Coupling highly excited nuclei to the atomic shell in dense astrophysical plasmas

In dense astrophysical plasmas, neutron capture populates highly excited nuclear states close to the neutron threshold. The impact of additional low-energy nuclear excitations via coupling to the atomic shell on the ability of the so-formed compound nucleus to retain the captured neutron is investigated. We focus on the mechanism of nuclear excitation by electron capture in plasmas characterized by electron fluxes typical for the slow neutron capture process of stellar nucleosynthesis. The small effect of this further excitation on the neutron capture and gamma decay sequence relevant for nucleosynthesis is quantified and compared to the corresponding effect of an additional low-energy photoexcitation step.

nucl-th↗

arXiv2014

Magnetic Quantum-Phase Control between Two Entangled Macroscopic Nuclear Ensembles

Heralded generation and manipulation of quantum entanglement between two macroscopic and spatially separated crystals at room temperature is theoretically studied. We show that by combining an x-ray parametric down-conversion source and x-ray interferometry with nuclear resonant scattering techniques, two macroscopic crystals hosting Mössbauer nuclei located each on an interferometer arm can be entangled for few tens of nanoseconds. The coherence time of the entanglement state can be prolonged up to values comparable to the lifetime of a single nuclear excited state, on the order of hundred nanoseconds. A non-mechanical magnetic control of the quantum phase between the two spatially separated entangled nuclear crystals is put forward.

quant-ph↗

arXiv2014

Field control of single x-ray photons in nuclear forward scattering

Means to coherently control single x-ray photons in resonant scattering of light off nuclei by electric or magnetic fields are investigated theoretically. In order to derive the time response in nuclear forward scattering, we adapt the Maxwell-Bloch equations known from quantum optics to describe the resonant light pulse propagation through a nuclear medium. Two types of time-dependent perturbations of nuclear forward scattering are considered for coherent control of the resonantly scattered x-ray quanta. First, the simultaneous coherent propagation of two pulses through the nuclear sample is addressed. We find that the signal of a weak pulse can be enhanced or suppressed by a stronger pulse simultaneously propagating through the sample in counter-propagating geometry. Second, the effect of a time-dependent hyperfine splitting is investigated and we put forward a scheme that allows parts of the spectrum to be shifted forward in time. This is the inverse effect of coherent photon storage and may become a valuable technique if single x-ray photon wavepackets are to become the information carriers in future photonic circuits.

physics.atom-ph↗

arXiv2014

Dominant Secondary Nuclear Photoexcitation with the X-ray Free Electron Laser

The new regime of resonant nuclear photoexcitation rendered possible by x-ray free electron laser beams interacting with solid state targets is investigated theoretically. Our results unexpectedly show that secondary processes coupling nuclei to the atomic shell in the created cold high-density plasma can dominate direct photoexcitation. As an example we discuss the case of $^{93m}$Mo isomer depletion for which nuclear excitation by electron capture as secondary process is shown to be orders of magnitude more efficient than the direct laser-nucleus interaction. General arguments revisiting the role of the x-ray free electron laser in nuclear experiments involving solid-state targets are further deduced.

nucl-th↗

arXiv2014

Proposed Entanglement of X-ray Nuclear Polaritons as a Potential Method for Probing Matter at the Subatomic Scale

A setup for generating the special superposition of a simultaneously forward- and backward-propagating collective excitation in a nuclear sample is studied. We show that by actively manipulating the scattering channels of single x-ray quanta with the help of a normal incidence x-ray mirror, a nuclear polariton which propagates in two opposite directions can be generated. The two counterpropagating polariton branches are entangled by a single x-ray photon. The quantum nature of the nuclear excitation entanglement gives rise to a subangstrom-wavelength standing wave excitation pattern that can be used as a flexible tool to probe matter dynamically on the subatomic scale.

quant-ph↗

arXiv2013

Nuclear Level Densities at High Excitation Energies and for Large Particle Numbers

Starting from an independent-particle model with a finite and arbitrary set of single-particle energies, we develop an analytical approximation to the many-body level density $ρ_A(E)$ and to particle-hole densities. We use exact expressions for the low-order moments and cumulants to derive approximate expressions for the coefficients of an expansion of these densities in terms of orthogonal polynomials. The approach is asymptotically (mass number $A \gg 1$) convergent and, for large $A$, covers about 20 orders of magnitude near the maximum of $ρ_A(E)$ (i.e., about half the spectrum). Densities of accessible states are calculated using the Fermi-gas model.

nucl-th↗

arXiv2013

Quantum interference effects in an ensemble of $^{229}$Th nuclei interacting with coherent light

As a unique feature, the $^{229}$Th nucleus has an isomeric transition in the vacuum ultraviolet that can be accessed by optical lasers. The interference effects occurring in the interaction between coherent optical light and an ensemble of $^{229}$Th nuclei are investigated theoretically. We consider the scenario of nuclei doped in vacuum ultraviolet-vacuum ultraviolet transparent crystals and take into account the effect of different doping sites and therefore different lattice fields that broaden the nuclear transition width. This effect is shown to come in interplay with interference effects due to the hyperfine splitting of the ground and isomeric nuclear states. We investigate possible experimentally available situations involving two-, three- and four-level schemes of quadrupole sublevels of the ground and isomeric nuclear states coupling to one or two coherent fields. Specific configurations which offer clear signatures of the isomer excitation advantageous for the more precise experimental determination of the transition energy are identified. Furthermore, it is shown that population trapping into the isomeric state can be achieved. This paves the way for further nuclear quantum optics applications with $^{229}$Th such as nuclear coherent control.

physics.atom-ph↗

arXiv2013

A three-beam setup for coherently controlling nuclear state population

The controlled transfer of nuclear state population using two x-ray laser pulses is investigated theoretically. The laser pulses drive two nuclear transitions in a nuclear three-level system facilitating coherent population transfer via the quantum optics technique of stimulated Raman adiabatic passage. To overcome present limitations of the x-ray laser frequency, we envisage accelerated nuclei interacting with two copropagating or crossed x-ray laser pulses in a three-beam setup. We present a systematic study of this setup providing both pulse temporal sequence and laser pulse intensity for optimized control of the nuclear state population. The tolerance for geometrical parameters such as laser beam divergence of the three-beam setup as well as for the velocity spread of the nuclear beam are studied and a two-photon resonance condition to account for experimental uncertainties is deduced. This additional condition gives a less strict requirement for the experimental implementation of the three-beam setup. Present experimental state of the art and future prospects are discussed.

physics.optics↗

arXiv2013

Nuclear Level Densities in the Constant-Spacing Model

A new method to calculate level densities for non-interacting Fermions within the constant-spacing model with a finite number of states is developed. We show that asymptotically (for large numbers of particles or holes) the densities have Gaussian form. We improve on the Gaussian distribution by using analytical expressions for moments higher than the second. Comparison with numerical results shows that the resulting sixth-moment approximation is excellent except near the boundaries of the spectra and works globally for all particle/hole numbers and all excitation energies.

nucl-th↗

arXiv2013

Nuclear recollisions in laser-assisted $α$ decay

Laser-induced nuclear recollisions following $α$ decay in the presence of an intense laser field are investigated theoretically. We show that while an intense optical laser does not influence notably the tunneling rate in $α$ decay, it can completely change the $α$ particle spectrum. For intensities of $10^{22}-10^{23}$ W/cm$^{2}$, the field is strong enough to induce recollisions between the emitted $α$ particle and the daughter nucleus. The energy gained by the $α$ particle in the field can reach 20 MeV and suffice to trigger several types of nuclear reactions on a femtosecond time scale. Similar conclusions can be drawn about laser-induced recollisions after proton emission. Prospects for the experimental realization of laser-induced nuclear recollisions are discussed.

nucl-th↗

arXiv2013

Coherent storage and phase modulation of single hard x-ray photons using nuclear excitons

Coherent storage and phase modulation of x-ray single-photon wave packets in resonant scattering of light off nuclei is investigated theoretically. We show that by switching off and on again the magnetic field in the nuclear sample, phase-sensitive storage of photons in the keV regime can be achieved. Corresponding $π$ phase modulation of the stored photon can be accomplished if the retrieving magnetic field is rotated by $180^{\circ}$. The development of such x-ray single-photon control techniques is a first step towards forwarding quantum optics and quantum information to shorter wavelengths and more compact photonic devices.

physics.atom-ph↗

arXiv2013

Coherence-enhanced optical determination of the $^{229}$Th isomeric transition

The impact of coherent light propagation on the excitation and fluorescence of thorium nuclei in a crystal lattice environment is investigated theoretically. We find that in the forward direction the fluorescence signal exhibits characteristic intensity modulations dominated by an orders of magnitude faster, sped-up initial decay signal. This feature can be exploited for the optical determination of the isomeric transition energy. In order to obtain a unmistakable signature of the isomeric nuclear fluorescence, we put forward a novel scheme for the direct measurement of the transition energy via electromagnetically modified nuclear forward scattering involving two fields that couple three nuclear states.

physics.atom-ph↗

arXiv2012

Cooperative effects in nuclear excitation with coherent x-ray light

The interaction between super-intense coherent x-ray light and nuclei is studied theoretically. One of the main difficulties with driving nuclear transitions arises from the very narrow nuclear excited state widths which limit the coupling between laser and nuclei. In the context of direct laser-nucleus interaction, we consider the nuclear width broadening that occurs when in solid targets, the excitation caused by a single photon is shared by a large number of nuclei, forming a collective excited state. Our results show that for certain isotopes, cooperative effects may lead to an enhancement of the nuclear excited state population by almost two orders of magnitude. Additionally, an update of previous estimates for nuclear excited state population and signal photons taking into account the experimental advances of the x-ray coherent light sources is given. The presented values are an improvement by orders of magnitude and are encouraging for the future prospects of nuclear quantum optics.

quant-ph↗

arXiv2012

Overlapping resonances in nuclei coupling to the atomic shells

The resonant process of nuclear excitation by electron transition (NEET) in highly charged ions is investigated. In NEET, a bound electronic decay transition occurs with the simultaneous excitation of the nucleus, provided that the energies of the atomic and nuclear transition match. By varying the atomic charge state, the atomic transition energy can be tuned to a better match of the nuclear transition energy. We propose a new way to create the atomic hole in highly charged ions by dielectronic capture of a free electron. In order to derive the cross section for the three-step process composed by dielectronic capture, NEET, and the subsequent nuclear decay, a Feshbach projection operator formalism is developed. With the help of this formalism, the resonances in nuclei coupling to the atomic shell and the possible interference between several direct and resonant electronic and nuclear processes such as radiative recombination, dielectronic recombination and nuclear excitation by electron capture are described.

physics.atom-ph↗

arXiv2011

Nuclear coherent population transfer with x-ray laser pulses

Coherent population transfer between nuclear states using x-ray laser pulses is studied. The laser pulses drive two nuclear transitions between three nuclear states in a setup reminding of stimulated Raman adiabatic passage used for atomic coherent population transfer. To compensate for the lack of $γ$-ray laser sources, we envisage accelerated nuclei interacting with two copropagating or crossed x-ray laser pulses. The parameter regime for nuclear coherent population transfer using fully coherent light generated by future X-Ray Free-Electron Laser facilities and moderate or strong acceleration of nuclei is determined. We find that the most promising case requires laser intensities of $10^{17}$-$10^{19}$ W/cm$^{2}$ for complete nuclear population transfer. As relevant application, the controlled pumping or release of energy stored in long-lived nuclear states is discussed.

quant-ph↗

arXiv2011

Nuclear effects in atomic transitions

Atomic electrons are sensitive to the properties of the nucleus they are bound to, such as nuclear mass, charge distribution, spin, magnetization distribution, or even excited level scheme. These nuclear parameters are reflected in the atomic transition energies. A very precise determination of atomic spectra may thus reveal information about the nucleus, otherwise hardly accessible via nuclear physics experiments. This work reviews theoretical and experimental aspects of the nuclear effects that can be identified in atomic structure data. An introduction to the theory of isotope shifts and hyperfine splitting of atomic spectra is given, together with an overview of the typical experimental techniques used in high-precision atomic spectroscopy. More exotic effects at the borderline between atomic and nuclear physics, such as parity violation in atomic transitions due to the weak interaction, or nuclear polarization and nuclear excitation by electron capture, are also addressed.

physics.atom-ph↗