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Adriano Reinaldo Viçoto Benvenho

Publications and source records attributed to Adriano Reinaldo Viçoto Benvenho.

3 recordsLinked to original sources

Enhanced Kadowaki-Woods Ratio and Weak-Coupling Superconductivity in Noncentrosymmetric YPt$_2$Si$_2$ Single Crystals

Superconductivity in noncentrosymmetric RPt2Si2 (R = rare earth) compounds exhibit a rich playground to explore the competition between different ground states, such as unconventional superconductivity, antiferromagnetism and charge density wave. Here, we report the successful single crystal synthesis of noncentrosymmetric YPt2Si2 superconductor, with a transition temperature Tc = 1.67 K, via Sn flux method. The high quality of the prepared single crystals was confirmed using powder and Laue XRD measurements. The superconducting and normal state properties are investigated using electrical transport and heat capacity measurements down to 0.5 K. In the normal state, unlike LaPt2Si2, no charge density wave transition is observed in YPt2Si2, as evidenced by electrical transport and specific heat measurements. A relatively large Kadowaki-Woods ratio and a linear temperature variation of the electrical resistivity in an extended temperature range of 50-300 K suggest an unconventional normal-state in YPt2Si2. The estimated superconducting parameters indicate that YPt2Si2 is a type-II superconductor with weak electron-phonon coupling. The temperature dependence of specific heat in the superconducting state can be explained reasonably well using an isotropic two-gap model. A positive curvature near Tc in the temperature variation of upper critical field also supports the two-gap superconductivity. First-principles DFT calculations suggest a BCS-like superconducting state driven primarily by d-electron contributions. The calculated electron-phonon coupling constant identifies the material as a weak-coupling superconductor, with the McMillan-Allen-Dynes formula yielding a Tc of 1.8 K. Additionally, we provide a comparative analysis of the superconducting and normal-state properties of YPt2Si2 and compositionally similar LaPt2Si2.

cond-mat.supr-con↗

Synthesis and anisotropic magnetism of singlecrystalline GdPt2Si2

Single crystals of GdPt$_2$Si$_2$ were grown using the Sn flux method, crystallizing in the CaBe$_2$Ge$_2$-type tetragonal structure with space group $P4/nmm$. Electrical resistivity, specific heat, and magnetization data revealed the presence of a double magnetic transition with $T_N \approx 8.4$~K and $T_0 \approx 6.8$~K. Analysis of the specific heat data suggest amplitude-modulated and equal-moment antiferromagnetic orderings, respectively. Field-induced magnetization and magnetic susceptibility data show a metamagnetic transition in the $H \parallel a$ direction at 2~K, as well as the suppression of the magnetic transition located at $T_0$ with increasing external magnetic field. Electron Spin Resonance (ESR) shows the Gd$^{3+}$ resonance followed by a small second resonance. Peak-to-peak linewidth ($ΔH_{pp}$) analysis reveals slight broadening at $T \sim 120$~K, indicating an increase in magnetic fluctuations at high temperatures. Ferromagnetic (FM) local polarization at high temperatures is also observed through the $g$-factor analysis, which shows a notable positive shift ($Δg$). Our results establish the fundamental physical properties of this material to aid in further understanding of the magnetism in the RPt$_2$Si$_2$ series and related non-centrosymmetric systems.

cond-mat.str-el↗

Effects of a Flexible Ion Gel as an Active Outer-Layer when in Contact with a Metallic Electrode

In this work the effect of an ion gel outer-layer stuck on top of ITO/PBT/Sn devices was investigated towards its effects on the electrical properties. When this external electrolyte film is in contact with any top permeable electrode it produces a self-biasing effect and changes the charge carriers injection properties. The outer-layer promoted situations where the output current increases up to two orders of magnitude and others where the output current decreases one order of magnitude in comparison to the same samples without it. Admittance spectroscopy measurements were made and the proposed equivalent circuit model indicates that the interfacial electrical properties dominate charge injection face to the bulk properties when the outer-layer is present. All the changes observed here are reversible after the ion gel is detached and replaced, indicating that ions do not diffuse into the active layer. The observed results can contribute to improve the current density in certain sandwich structures as well as notify that electrolyte external films can behave as an active layer promoting electrical changes into sandwich devices and can be extended to cases where the electrolyte film is used as substrate.

physics.chem-ph↗