arXiv subjects

Adrien Bouhon

Publications and source records attributed to Adrien Bouhon.

At least 37 records · Page 2Linked to original sources

arXiv2022

Phase transitions of non-Abelian charged nodal links in a spring-mass system

Although a large class of topological materials have uniformly been identified using symmetry properties of wave functions, the past two years have seen the rise of multi-gap topologies beyond this paradigm. Given recent reports of unexplored features of such phases, platforms that are readily implementable to realize them are therefore desirable. Here, we demonstrate that multi-gap topological phase transitions of non-Abelian charged nodal lines arise in classical phonon waves. By adopting a simple spring-mass system, we construct nodal lines of a three-band system. The braiding process of the nodal lines is readily performed by adjusting the spring constants. The generation and annihilation of the nodal lines are then analyzed using Euler class. Finally, we retrieve topological transitions from trivial nodal lines to a nodal link. Our work provides a simple platform that can offer diverse insights to not only theoretical but also experimental studies on multi-gap topology.

cond-mat.soft↗

arXiv2021

Phonons as a platform for non-Abelian braiding and its manifestation in layered silicates

Topological phases of matter have revolutionised the fundamental understanding of band theory and hold great promise for next-generation technologies such as low-power electronics or quantum computers. Single-gap topologies have been extensively explored, and a large number of materials have been theoretically proposed and experimentally observed. These ideas have recently been extended to multi-gap topologies with band nodes that carry non-Abelian charges, characterised by invariants that arise by the momentum space braiding of such nodes. However, the constraints placed by the Fermi-Dirac distribution to electronic systems have so far prevented the experimental observation of multi-gap topologies in real materials. Here, we show that multi-gap topologies and the accompanying phase transitions driven by braiding processes can be readily observed in the bosonic phonon spectra of known monolayer silicates. The associated braiding process can be controlled by means of an electric field and epitaxial strain, and involves, for the first time, more than three bands. Finally, we propose that the band inversion processes at the $Γ$ point can be tracked by following the evolution of the Raman spectrum, providing a clear signature for the experimental verification of the band inversion accompanied by the braiding process.

cond-mat.mes-hall↗

arXiv2021

Chirality flip of Weyl nodes and its manifestation in strained MoTe$_2$

Due to their topological charge, or chirality, the Weyl cones present in topological semimetals are considered robust against arbitrary perturbations. One well-understood exception to this robustness is the pairwise creation or annihilation of Weyl cones, which involves the overlap of two oppositely charged nodes in energy and momentum. Here we show that their topological charge can in fact change sign, in a process that involves the merging of not two, but three Weyl nodes. This is facilitated by the presence of rotation and time-reversal symmetries, which constrain the relative positions of Weyl cones in momentum space. We analyze the chirality flip process, showing that transport properties distinguish it from the conventional, double Weyl merging. Moreover, we predict that the chirality flip occurs in MoTe$_2$, where experimentally accessible strain leads to the merging of three Weyl cones close to the Fermi level. Our work sets the stage to further investigate and observe such chirality flipping processes in different topological materials.

cond-mat.mes-hall↗

arXiv2021

Multi-gap topology and non-Abelian braiding of phonons from first principles

Non-Abelian states of matter, in which the final state depends on the order of the interchanges of two quasiparticles, can encode information immune from environmental noise with the potential to provide a robust platform for topological quantum computation. We demonstrate that phonons can carry non-Abelian frame charges at the band crossing points of their frequency spectrum, and that external stimuli can drive their braiding. We present a general framework to understand the topological configurations of phonons from first principles calculations using a topological invariant called Euler class, and provide a complete analysis of phonon braiding by combining different topological configurations. Taking a well-known dielectric material, Al$_2$O$_3$, as a representative example, we demonstrate that electrostatic doping gives rise to phonon band inversions that can induce redistribution of the frame charges, leading to non-Abelian braiding of phonons. Our work provides a new quasiparticle platform for realizable non-Abelian braiding in reciprocal space, and expands the toolset for studying braiding processes.

cond-mat.mes-hall↗

arXiv2021

Topological continuum charges of acoustic phonons in 2D

We analyze the band topology of acoustic phonons in 2D materials by considering the interplay of spatial and internal symmetries with additional constraints that arise from the physical context. These supplemental constraints trace back to the Nambu-Goldstone theorem and the requirements of structural stability. We show that this interplay can give rise to previously unaddressed non-trivial nodal charges that are associated with the crossing of the acoustic phonon branches at the center ($Γ$-point) of the phononic Brillouin zone. We moreover apply our perspective to the concrete context of graphene, where we demonstrate that the phonon spectrum harbors these kinds of non-trivial nodal charges. Apart from its fundamental appeal, this analysis is physically consequential and dictates how the phonon dispersion is affected when graphene is grown on a substrate. Given the generality of our framework, we anticipate that our strategy that thrives on combining physical context with insights from topology should be widely applicable in characterizing systems beyond electronic band theory.

cond-mat.mes-hall↗

arXiv2021

Manipulation and braiding of Weyl nodes using symmetry-constrained phase transitions

Weyl semimetals are arguably the most paradigmatic form of a gapless topological phase. While the stability of Weyl nodes, as quantified by their topological charge, has been extensively investigated, recent interest has shifted to the manipulation of the location of these Weyl nodes for non-Abelian braiding. To accomplish this braiding it is necessary to drive significant Weyl node motion using realistic experimental parameter changes. We show that a family of phase transitions characterized by certain symmetry constraints impose that the Weyl nodes have to reorganise by a large amount, shifting from one high symmetry plane to another. Additionally, for a subset of pairs of nodes with nontrivial Euler class topology, this reorganization can only occur through a braiding process with adjacent nodes. As a result, the Weyl nodes are forced to move a large distance across the Brillouin zone and to braid, all driven by small temperature changes, a process we illustrate with Cd$_2$Re$_2$O$_7$. Our work opens up routes to readily manipulate Weyl nodes using only slight external parameter changes, paving the way for the practical realization of reciprocal space braiding.

cond-mat.mes-hall↗

arXiv2021

Topological correspondence between magnetic space group representations

The past years have seen rapid progress in the classification of topological materials. These diagnostical methods are increasingly getting explored in the pertinent context of magnetic structures. We report on a general class of electronic configurations within a set of anti-ferromagnetic-compatible space groups that are necessarily topological. Interestingly, we find a systematic correspondence between these anti-ferromagnetic phases to necessarily nontrivial topological ferro/ferrimagnetic counterparts that are readily obtained through physically motivated perturbations. Addressing the exhaustive list of magnetic space groups in which this mechanism occurs, we also verify its presence on planes in 3D systems that were deemed trivial in existing classification schemes. This leads to the formulation of the concept of subdimensional topologies, featuring non-triviality within part of the system that coexists with stable Weyl points away from these planes, thereby uncovering novel topological materials in the full 3D sense that have readily observable features in their bulk and surface spectrum.

cond-mat.mes-hall↗

arXiv2021

Observation of non-Abelian topological semimetals and their phase transitions

Topological phases of matter lie at the heart of physics, connecting elegant mathematical principles to real materials that are believed to shape future electronic and quantum computing technologies. To date, studies in this discipline have almost exclusively been restricted to single-gap band topology because of the Fermi-Dirac filling effect. Here, we theoretically analyze and experimentally confirm a novel class of multi-gap topological phases, which we will refer to as non-Abelian topological semimetals, on kagome geometries. These unprecedented forms of matter depend on the notion of Euler class and frame charges which arise due to non-Abelian charge conversion processes when band nodes of different gaps are braided along each other in momentum space. We identify such exotic phenomena in acoustic metamaterials and uncover a rich topological phase diagram induced by the creation, braiding and recombination of band nodes. Using pump-probe measurements, we verify the non-Abelian charge conversion processes where topological charges of nodes are transferred from one gap to another. Moreover, in such processes, we discover symmetry-enforced intermediate phases featuring triply-degenerate band nodes with unique dispersions that are directly linked to the multi-gap topological invariants. Furthermore, we confirm that edge states can faithfully characterize the multi-gap topological phase diagram. Our study unveils a new regime of topological phases where multi-gap topology and non-Abelian charges of band nodes play a crucial role in understanding semimetals with inter-connected multiple bands.

cond-mat.mes-hall↗

arXiv2021

Non-Abelian reciprocal braiding of Weyl points and its manifestation in $\textrm{ZrTe}$

Weyl semimetals in three-dimensional crystals provide the paradigm example of topologically protected band nodes. It is usually taken for granted that a pair of colliding Weyl points annihilate whenever they carry opposite chiral charge. In a stark contrast, here we report that Weyl points in systems symmetric under the composition of time-reversal with a $π$-rotation are characterized by a non-Abelian topological invariant. The topological charges of the Weyl points are transformed via braid phase factors which arise upon exchange inside symmetric planes of the reciprocal momentum space. We elucidate this process with an elementary two-dimensional tight-binding model implementable in cold-atoms setups and in photonic systems. In three dimensions, interplay of the non-Abelian topology with point-group symmetry is shown to enable topological phase transitions in which pairs of Weyl points may scatter or convert into nodal-line rings. By combining our theoretical arguments with first-principles calculations, we predict that Weyl points occurring near the Fermi level of zirconium telluride ($\textrm{ZrTe}$) carry non-trivial values of the non-Abelian charge, and that uniaxial compression strain drives a non-trivial conversion of the Weyl points into nodal lines.

cond-mat.mes-hall↗

arXiv2021

Subdimensional topologies, indicators and higher order phases

The study of topological band structures have sparked prominent research interest the past decade, culminating in the recent formulation of rather prolific classification schemes that encapsulate a large fraction of phases and features. Within this context we recently reported on a class of unexplored topological structures that thrive on the concept of {\it sub-dimensional topology}. Although such phases have trivial indicators and band representations when evaluated over the complete Brillouin zone, they have stable or fragile topologies within sub-dimensional spaces, such as planes or lines. This perspective does not just refine classification pursuits, but can result in observable features in the full dimensional sense. In three spatial dimensions (3D), for example, sub-dimensional topologies can be characterized by non-trivial planes, having general topological invariants, that are compensated by Weyl nodes away from these planes. As a result, such phases have 3D stable characteristics such as Weyl nodes, Fermi arcs and edge states that can be systematically predicted by sub-dimensional analysis. Within this work we further elaborate on these concepts. We present refined representation counting schemes and address distinctive bulk-boundary effects, that include momentum depended (higher order) edge states that have a signature dependence on the perpendicular momentum. As such, we hope that these insights might spur on new activities to further deepen the understanding of these unexplored phases.

cond-mat.mes-hall↗

arXiv2020

Topological Euler class as a dynamical observable in optical lattices

The last years have witnessed rapid progress in the topological characterization of out-of-equilibrium systems. We report on robust signatures of a new type of topology -- the Euler class -- in such a dynamical setting. The enigmatic invariant $(ξ)$ falls outside conventional symmetry-eigenvalue indicated phases and, in simplest incarnation, is described by triples of bands that comprise a gapless pair, featuring $2ξ$ stable band nodes, and a gapped band. These nodes host non-Abelian charges and can be further undone by converting their charge upon intricate braiding mechanisms, revealing that Euler class is a fragile topology. We theoretically demonstrate that quenching with non-trivial Euler Hamiltonian results in stable monopole-antimonopole pairs, which in turn induce a linking of momentum-time trajectories under the first Hopf map, making the invariant experimentally observable. Detailing explicit tomography protocols in a variety of cold-atom setups, our results provide a basis for exploring new topologies and their interplay with crystalline symmetries in optical lattices beyond paradigmatic Chern insulators.

cond-mat.quant-gas↗

arXiv2020

PAI-graphene: a new topological semimetallic two-dimensional carbon allotrope with highly tunable anisotropic Dirac cones

Using evolutionary algorithm for crystal structure prediction, we present a new stable two-dimensional (2D) carbon allotrope composed of polymerized as-indacenes (PAI) in a zigzag pattern, namely PAI-graphene whose energy is lower than most of the reported 2D allotropes of graphene. Crucially, the crystal structure realizes a nonsymmorphic layer group that enforces a nontrivial global topology of the band structure with two Dirac cones lying perfectly at the Fermi level. The absence of electron/hole pockets makes PAI-graphene a pristine crystalline topological semimetal having anisotropic Fermi velocities with a high value of $7.0 \times 10^{5}$ m/s. We show that while the semimetallic property of the allotrope is robust against the application of strain, the positions of the Dirac cone and the Fermi velocities can be modified significantly with strain. Moreover, by combining strain along both the x- and y-directions, two band inversions take place at $Γ$ leading to the annihilation of the Dirac nodes demonstrating the possibility of strain-controlled conversion of a topological semimetal into a semiconductor. Finally we formulate the bulk-boundary correspondence of the topological nodal phase in the form of a generalized Zak-phase argument finding a perfect agreement with the topological edge states computed for different edge-terminations.

cond-mat.mtrl-sci↗

arXiv2020

Geometric approach to fragile topology beyond symmetry indicators

We present a framework to systematically address topological phases when finer partitionings of bands are taken into account, rather than only considering the two subspaces spanned by valence and conduction bands. Focusing on $C_2\mathcal{T}$-symmetric systems that have gained recent attention, for example in the context of layered van-der-Waals graphene heterostructures, we relate these insights to homotopy groups of Grassmannians and flag varieties, which in turn correspond to cohomology classes and Wilson-flow approaches. We furthermore make use of a geometric construction, the so-called Plücker embedding, to induce windings in the band structure necessary to facilitate non-trivial topology. Specifically, this directly relates to the parametrization of the Grassmannian, which describes partitioning of an arbitrary band structure and is embedded in a better manageable exterior product space. From a physical perspective, our construction encapsulates and elucidates the concepts of fragile topological phases beyond symmetry indicators as well as non-Abelian reciprocal braiding of band nodes that arises when the multiple gaps are taken into account. The adopted geometric viewpoint most importantly culminates in a direct and easily implementable method to construct model Hamiltonians to study such phases, constituting a versatile theoretical tool.

cond-mat.mes-hall↗

arXiv2019

Fractional corner charges in spin-orbit coupled crystals

We study two-dimensional spinful insulating phases of matter that are protected by time-reversal and crystalline symmetries. To characterize these phases we employ the concept of corner charge fractionalization: Corners can carry charges that are fractions of even multiples of the electric charge. The charges are quantized and topologically stable as long as all symmetries are preserved. We classify the different corner charge configurations for all point groups, and match them with the corresponding bulk topology. For this we employ symmetry indicators and (nested) Wilson loop invariants. We provide formulas that allow for a convenient calculation of the corner charge from Bloch wavefunctions and illustrate our results using the example of arsenic and antimony monolayers. Depending on the degree of structural buckling, these materials can exhibit two distinct obstructed atomic limits. We present density functional theory calculations for open flakes to support our findings.

cond-mat.str-el↗

arXiv2019

Wilson loop approach to fragile topology of split elementary band representations and topological crystalline insulators with time reversal symmetry

We present a general methodology towards the systematic characterization of crystalline topological insulating phases with time reversal symmetry (TRS).~In particular, taking the two-dimensional spinful hexagonal lattice as a proof of principle we study windings of Wilson loop spectra over cuts in the Brillouin zone that are dictated by the underlying lattice symmetries.~Our approach finds a prominent use in elucidating and quantifying the recently proposed ``topological quantum chemistry" (TQC) concept.~Namely, we prove that the split of an elementary band representation (EBR) by a band gap must lead to a topological phase.~For this we first show that in addition to the Fu-Kane-Mele $\mathbb{Z}_2$ classification, there is $C_2\mathcal{T}$-symmetry protected $\mathbb{Z}$ classification of two-band subspaces that is obstructed by the other crystalline symmetries, i.e.~forbidding the trivial phase. This accounts for all nontrivial Wilson loop windings of split EBRs \textit{that are independent of the parameterization of the flow of Wilson loops}.~Then, we show that while Wilson loop winding of split EBRs can unwind when embedded in higher-dimensional band space, two-band subspaces that remain separated by a band gap from the other bands conserve their Wilson loop winding, hence revealing that split EBRs are at least "stably trivial", i.e. necessarily non-trivial in the non-stable (few-band) limit but possibly trivial in the stable (many-band) limit.~This clarifies the nature of \textit{fragile} topology that has appeared very recently.~We then argue that in the many-band limit the stable Wilson loop winding is only determined by the Fu-Kane-Mele $\mathbb{Z}_2$ invariant implying that further stable topological phases must belong to the class of higher-order topological insulators.

cond-mat.mes-hall↗

arXiv2018

Spin Hall effect in 2D metallic delafossite PtCoO$_2$ and vicinity topology

The two-dimensional (2D) metal PtCoO$_2$ is renowned for the lowest room temperature resistivity among all oxides, close to that of the top two materials Ag and Cu. In addition, we theoretically predict a strong intrinsic spin Hall effect. This originates from six strongly-tilted Dirac cones that we find in the electronic structure near the Fermi surface, where a gap is opened by large spin-orbit coupling (SOC). This is underpinned by rich topological properties; in particular, the phenomenology of a mirror Chern metal is realized not exactly, but very accurately, on account of an approximate crystalline symmetry. We expect that such 'vicinity topology' to be a feature of relevance well beyond this material. Our Wilson loop analysis indicates further elaborate features such as fragile topology. These findings highlight PtCoO$_2$ as a promising material for spintronic applications as well as a platform to study the interplay of symmetry and topology.

cond-mat.mes-hall↗

arXiv2018

Spontaneous surface flux pattern in chiral p-wave superconductors - revisited

In chiral $p$-wave superconductors, magnetic flux patterns may appear spontaneously when translational symmetry is broken such as at surfaces, domain walls, or impurities. However, in the candidate material Sr$_2$RuO$_4$ no direct signs of such magnetic fields have been detected experimentally. In this paper, the flux pattern at the edge of a disk-shaped sample is examined using the phenomenological Ginzburg Landau approach. The detailed shape of the flux pattern, including self-screening, is computed numerically for different surface types by systematically scanning a range of boundary conditions. Moreover, specific features of the electronic structure are included qualitatively through the coefficients in the Ginzburg Landau functional. Both the shape and the magnitude of the flux pattern are found to be highly sensitive to all considered parameters. In conclusion, such spontaneous magnetic flux patterns are not a universal feature of chiral $p$-wave superconductors.

cond-mat.supr-con↗

arXiv2018

Topological nodal superconducting phases and topological phase transition in the hyperhoneycomb lattice

We establish the topology of the spin-singlet superconducting states in the bare hyperhoneycomb lattice and derive analytically the full phase diagram using only symmetry and topology in combination with simple energy arguments. The phase diagram is dominated by two states preserving time-reversal symmetry. We find that the line-nodal state dominating at low doping levels is topologically nontrivial and exhibits surface Majorana flat bands, which we show perfectly match the bulk-boundary correspondence using Berry phase approach. At higher doping levels we find a fully gapped state with trivial topology. By analytically calculating the topological invariant of the line nodes, we derive the critical point between the line-nodal and fully gapped states as a function of both pairing parameters and doping. We find that the line-nodal state is favored not only at lower doping levels but also if symmetry-allowed deformations of the lattice is present. Adding simple energy arguments we establish that a fully gapped state with broken time-reversal symmetry likely appears covering the actual phase transition. We find this time-reversal symmetry broken state to be topologically trivial, while we find an additional point nodal state at very low doping levels to have nontrivial topology with associated Fermi surface arcs. We eventually address the robustness of the phase diagram to generalized models also including adiabatic spin-orbit coupling, and show how all but the point nodal state are reasonably stable.

cond-mat.supr-con↗