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Aidan S. Arnold

Publications and source records attributed to Aidan S. Arnold.

At least 19 recordsLinked to original sources
arXiv2026

Simple tunable phase-locked lasers for quantum technologies

In a wide range of quantum technology applications, ranging from atomic clocks to the creation of ultracold or quantum degenerate samples for atom interferometry, optimal laser sources are critical. In particular, two phase-locked laser sources with a precise difference frequency are needed for efficient coherent population trapping (CPT) clocks, gray molasses laser cooling, or driving Raman transitions. Here we show how a simple cost-effective laser diode can selectively amplify only one sideband of a fiber-electrooptically-modulated seed laser to produce moderate-power phase-locked light with sub-Hz relative linewidth and tunable difference frequencies up to $\approx 15\,$GHz. The architecture is readily scalable to multiple phase-locked lasers and could conceivably be used for future on-chip compact phase-locked laser systems for quantum technologies.

physics.atom-ph↗
arXiv2026

Rapid axial loading of a grating MOT with a cold-atom beam

Laser-cooled atoms are increasingly being used to realise practical quantum devices, motivating the development of compact and robust atom sources. Grating magneto-optical traps (gMOTs) simplify the cold-atom source architecture but are typically vapour-loaded and provide limited atomic flux. Here we explore the loading of gMOTs from cold-atom beams. We numerically simulate loading to show that unbalanced diffracted beams deflect incoming atoms away from the trap centre, thereby strongly constraining radial loading. In contrast, axial loading injects atoms directly into the trapping volume and largely avoids these effects. We experimentally demonstrate rapid axial loading of a gMOT, achieving loading rates of $2.1 \times 10^9$ atoms~s$^{-1}$ using a moving optical molasses to transfer atoms from a 2D MOT into the gMOT. These results establish axial loading as a robust route to high-flux gMOT operation for portable cold-atom systems.

physics.atom-ph↗
arXiv2025

Observation of Rayleigh optical activity for chiral molecules: a new chiroptical tool

By measuring a small circularly polarized component in the scattered light, we report the first observation of Rayleigh optical activity (RayOA) for isotropic samples of chiral molecules, namely the two enantiomers of $α$-pinene in neat liquid form. Our work validates fundamental theoretical predictions made over fifty years ago and expands the chiroptical toolkit.

physics.chem-ph↗
arXiv2025

Practical primary thermometry via alkali-metal-vapour Doppler broadening

Doppler-broadening thermometry (DBT) can be used as a calibration-free primary reference suitable for practical applications, e.g. reliably measuring temperatures over long periods of time in environments where sensor retrieval is impractical. We report on our proof-of-concept investigations into DBT with alkali metal vapour cells, with a particular focus on both absorption and frequency accuracy during scans. We reach sub-kelvin temperature accuracy, and experimental absorption fit residuals below $0.05\,\%$, in a simple setup. The outlook for portable, practical devices is bright, with clear prospects for future improvement.

physics.atom-ph↗
arXiv2024

Single-beam grating-chip 3D and 1D optical lattices

Ultracold atoms are crucial for unlocking truly precise and accurate quantum metrology, and provide an essential platform for quantum computing, communication and memories. One of the largest ongoing challenges is the miniaturization of these quantum devices. Here, we show that the typically macroscopic optical lattice architecture at the heart of many ultra-precise quantum technologies can be realized with a single input laser beam on the same diffractive chip already used to create the ultracold atoms. Moreover, this inherently ultra-stable platform enables access to a plethora of new lattice dimensionalities and geometries, ideally suited for the design of high-accuracy, portable quantum devices.

cond-mat.quant-gas↗
arXiv2023

Optimal binary gratings for multi-wavelength magneto-optical traps

Grating magneto-optical traps are an enabling quantum technology for portable metrological devices with ultracold atoms. However, beam diffraction efficiency and angle are affected by wavelength, creating a single-optic design challenge for laser cooling in two stages at two distinct wavelengths - as commonly used for loading e.g. Sr or Yb atoms into optical lattice or tweezer clocks. Here, we optically characterize a wide variety of binary gratings at different wavelengths to find a simple empirical fit to experimental grating diffraction efficiency data in terms of dimensionless etch depth and period for various duty cycles. The model avoids complex 3D light-grating surface calculations, yet still yields results accurate to a few percent across a broad range of parameters. Gratings optimized for two (or more) wavelengths can now be designed in an informed manner suitable for a wide class of atomic species enabling advanced quantum technologies.

physics.atom-ph↗
arXiv2023

Practical Doppler broadening thermometry

We report initial research to develop a compact and practical primary thermometer based on Doppler broadening thermometry (DBT). The DBT sensor uses an intrinsic property of thermalized atoms, namely, the Doppler width of a spectral line characteristic of the atoms being probed. The DBT sensor, being founded on a primary thermometry approach, requires no calibration or reference, and so in principle could achieve reliable long-term in-situ thermodynamic temperature measurement. Here we describe our approach and report on initial proof-of-concept investigations with alkali metal vapour cells. Our focus is to develop long-term stable thermometers based on DBT that can be used to reliably measure temperatures for long periods and in environments where sensor retrieval for re-calibration is impractical such as in nuclear waste storage facilities.

physics.atom-ph↗
arXiv2022

A grating-chip atomic fountain

Cold atom fountain clocks provide exceptional long term stability as they increase interrogation time at the expense of a larger size. We present a compact cold atom fountain using a grating magneto-optical trap (GMOT) to laser cool and launch the atoms in a simplified optical setup. The fountain is evaluated using coherent population trapping and demonstrates improved single-shot stability from the launch. Ramsey times up to 100 ms were measured with a corresponding fringe linewidth of 5 Hz. This technique could improve both short- and long-term stability of cold atom clocks whilst remaining compact for portable applications.

physics.atom-ph↗
arXiv2021

Stand-alone vacuum cell for compact ultracold quantum technologies

Compact vacuum systems are key enabling components for cold atom technologies, facilitating extremely accurate sensing applications. There has been important progress towards a truly portable compact vacuum system, however size, weight and power consumption can be prohibitively large, optical access may be limited, and active pumping is often required. Here, we present a centilitre-scale ceramic vacuum chamber with He-impermeable viewports and an integrated diffractive optic, enabling robust laser cooling with light from a single polarization-maintaining fibre. A cold atom demonstrator based on the vacuum cell delivers $10^7$ laser-cooled $^{87}$Rb atoms per second, using minimal electrical power. With continuous Rb gas emission active pumping yields a $10^{-7}\,$mbar equilibrium pressure, and passive pumping stabilises to $3\times 10^{-6}\,$mbar, with a $17\,$day time constant. A vacuum cell, with no Rb dispensing and only passive pumping, has currently kept a similar pressure for more than \ch{500 days}. The passive-pumping vacuum lifetime is several years, estimated from short-term He throughput, with many foreseeable improvements. This technology enables wide-ranging mobilization of ultracold quantum metrology.

physics.atom-ph↗
arXiv2021

A simple, powerful diode laser system for atomic physics

External-cavity diode lasers are ubiquitous in atomic physics and a wide variety of other scientific disciplines, due to their excellent affordability, coherence length and versatility. However, for higher power applications, the combination of seed lasers, injection-locking and amplifiers can rapidly become expensive and complex. Here we present a useful, high-power, single-diode laser design with specifications: $>210\,$mW, $100\,$ms-linewidth ($427 \pm 7$) kHz, $>99\%$ mode purity, $10\,$GHz mode-hop-free tuning range and $12\,$nm coarse tuning. Simple methods are outlined to determine the spectral purity and linewidth with minimal additional infrastructure. The laser has sufficient power to collect $10^{10}$ $^{87}$Rb atoms in a single-chamber vapour-loaded magneto-optical trap. With appropriate diodes and feedback, the system could be easily adapted to other atomic species and laser formats.

physics.ins-det↗
arXiv2021

Gouy phase-matched angular and radial mode conversion in four-wave mixing

Studying the conversion between transverse light modes via four-wave mixing in a heated rubidium vapour, we demonstrate and explain a transfer between azimuthal and radial mode numbers. These relate to orthogonal modal dimensions, which one would not normally expect to interact. While angular momentum conservation in this nonlinear process dictates the selection rules for the angular mode number, the role of the radial mode number is more esoteric. We demonstrate systematically that the Gouy phase is the key to understanding this conversion, leading to strikingly different conversion behaviour in the thick and thin medium regime. Our experimental investigation of the transition between these regimes bridges the gap between previous experiments in atomic thick media and work in nonlinear crystals. Our work sets a clear starting point to explore new territory in the thick medium regime, allowing efficient radial-to-azimuthal and radial-to-radial mode conversion.

physics.atom-ph↗
arXiv2020

Optical characterisation of micro-fabricated Fresnel zone plates for atomic waveguides

We optically assess Fresnel zone plates (FZPs) that are designed to guide cold atoms. Imaging of various ring patterns produced by the FZPs gives an average RMS error in the brightest part of the ring of 3% with respect to trap depth. This residue will be due to the imaging system, incident beam shape and FZP manufacturing tolerances. Axial propagation of the potentials is presented experimentally and through numerical simulations, illustrating prospects for atom guiding without requiring light sheets.

physics.atom-ph↗
arXiv2020

Cold-atom clock based on a diffractive optic

Clocks based on cold atoms offer unbeatable accuracy and long-term stability, but their use in portable quantum technologies is hampered by a large physical footprint. Here, we use the compact optical layout of a grating magneto-optical trap (gMOT) for a precise frequency reference. The gMOT collects $10^7$ $^{87}$Rb atoms, which are subsequently cooled to $20\,μ$K in optical molasses. We optically probe the microwave atomic ground-state splitting using lin$\perp$lin polarised coherent population trapping and a Raman-Ramsey sequence. With ballistic drop distances of only $0.5\,$mm, the measured short-term fractional frequency stability is $2 \times 10 ^{-11} /\sqrtτ$.

physics.atom-ph↗
arXiv2018

Spiral bandwidth of four-wave mixing in Rb vapour

Laguerre-Gauss beams, and more generally the orbital angular momentum of light (OAM) provide valuable research tools for optical manipulation, processing, imaging and communication. Here we explore the high-efficiency frequency conversion of OAM in a four-wave mixing process in rubidium vapour. Conservation of the OAM in the two pump beams determines the total OAM shared by the generated light fields at 420 nm and 5.2 um - but not its distribution between them. We experimentally investigate the spiral bandwidth of the generated light modes as a function of pump OAM. A small pump OAM is transferred almost completely to the 420 nm beam. Increasing the total pump OAM broadens the OAM spectrum of the generated light, indicating OAM entanglement between the generated light fields. This clears the path to high-efficiency OAM entanglement between widely disparate wavelengths.

physics.atom-ph↗
arXiv2018

Holographically controlled three-dimensional atomic population patterns

The interaction of spatially structured light fields with atomic media can generate spatial structures inscribed in the atomic populations and coherences, allowing for example the storage of optical images in atomic vapours. Typically, this involves coherent optical processes based on Raman or EIT transitions. Here we study the simpler situation of shaping atomic populations via spatially dependent optical depletion. Using a near resonant laser beam with a holographically controlled 3D intensity profile, we imprint 3D population structures into a thermal rubidium vapour. This 3D population structure is simultaneously read out by recording the spatially resolved fluorescence of an unshaped probe laser. We find that the reconstructed atomic population structure is largely complementary to the intensity structure of the control beam, however appears blurred due to global repopulation processes. We identify and model these mechanisms which limit the achievable resolution of the 3D atomic population. We expect this work to set design criteria for future 2D and 3D atomic memories.

physics.atom-ph↗
arXiv2018

Vector Magnetometry Exploiting Phase-Geometry Effects in a Double-Resonance Alignment Magnetometer

Double-resonance optically pumped magnetometers are an attractive instrument for unshielded magnetic field measurements due to their wide dynamic range and high sensitivity. Use of linearly polarised pump light creates alignment in the atomic sample, which evolves in the local static magnetic field, and is driven by a resonant applied field perturbation, modulating the polarisation of transmitted light. We show for the first time that the amplitude and phase of observed first- and second-harmonic components in the transmitted polarisation signal contain sufficient information to measure static magnetic field magnitude and orientation. We describe a laboratory system for experimental measurements of these effects and verify a theoretical derivation of the observed signal. We demonstrate vector field tracking under varying static field orientations and show that the static field magnitude and orientation may be observed simultaneously, with experimentally realised resolution of 1.7 pT and 0.63 mrad in the most sensitive field orientation.

physics.atom-ph↗
arXiv2017

Detection of Applied and Ambient Forces with a Matterwave Magnetic-Gradiometer

An atom interferometer using a Bose-Einstein condensate of $^{87}$Rb atoms is utilized for the measurement of magnetic field gradients. Composite optical pulses are used to construct a spatially symmetric Mach-Zehnder geometry. Using a biased interferometer we demonstrate the ability to measure small residual forces in our system at the position of the atoms. These are a residual magnetic field gradient of 15$\pm$2 mG/cm and and an inertial acceleration of 0.08$\pm$0.02 m/s$^2$. Our method has important applications in the calibration of precision measurement devices and the reduction of systematic errors.

physics.atom-ph↗