SearcharxivSearch

arXiv subjects

Aitor Garcia-Ruiz

Publications and source records attributed to Aitor Garcia-Ruiz.

18 recordsLinked to original sources

Quantum transport across normal-superlattice-normal graphene junctions: Fabry-Pérot interference, Hofstadter butterfly, and supersnake states

Electrostatic modulation of graphene provides a tunable route to engineering miniband structures. We perform quantum transport simulations on a gate-defined graphene superlattice junction, formed by confining a two-dimensional superlattice graphene (SGr) region between two normal graphene (NGr) regions. In the low-field regime at low carrier densities, robust Fabry-Pérot interference fringes emerge even in the unipolar regime due to Fermi-velocity renormalization in the SGr region. At stronger magnetic fields but only up to 3 T, the conductance map clearly reveals the Hofstadter butterfly spectrum. At intermediate fields, our finite-width transport simulations reveal a new type of snake state, the supersnake state, composed of alternating anomalous cyclotron arcs on the SGr side and conventional semicircular arcs on the NGr side, forming a weaving trajectory along the junction. The resulting conductance oscillations agree well with geometrical conditions derived from semiclassical cyclotron orbits. Our results demonstrate that gate-defined NGr-SGr-NGr junctions provide a versatile platform hosting multiple transport regimes within a single device architecture and can be generalized to other types of superlattices not restricted to graphene.

cond-mat.mes-hall

Electronic Reconstruction at the Quasicrystal-Moiré Crossover in Twisted Bilayer Graphene

Large twist angles in twisted bilayer graphene are widely expected to be electronically trivial, with negligible interlayer coupling and no electronic reconstruction, in contrast to the rich moiré-driven band reconstruction and correlated physics that emerge at small twist angles. Here, we show that this paradigm breaks down near a twist angle of 29°, where the system crosses over between quasicrystalline and commensurate order. Atomic-resolution transmission electron microscopy directly reveals the coexistence of near-dodecagonal quasicrystalline symmetry and emerging moiré periodicity, indicating an intermediate, nonperiodic structural regime. Magnetotransport measurements uncover strong interlayer hybridization mediated by Umklapp scattering, manifested by magneto-intersubband oscillations and a highly unconventional Landau-level spectrum. Remarkably, the Landau-level degeneracy evolves from 4- to 12-fold with increasing temperature, a behavior incompatible with two decoupled graphene monolayers. These findings establish large-angle twisted bilayer graphene as a platform where quasiperiodic symmetry fundamentally reshapes low-energy electronic states beyond the conventional moiré framework.

cond-mat.mes-hall

Dimensional and doping stability of Peierls charge density waves in arrays of coupled one-dimensional chains

The Peierls instability, the spontaneous dimerization of a one-dimensional metallic chain at half filling, is a paradigmatic mechanism for charge-density-wave (CDW) formation. Here we test its robustness under finite doping and interchain hybridization in finite-thickness arrays of identical chains. We find that the stacking geometry plays a decisive role in stabilizing CDW order away from half filling. In particular, parallel-coupled chains exhibit a bistable regime where the normal and dimerized states coexist as local minima of the total energy, while skew-coupled chains display reentrant CDW order upon doping. Our results demonstrate that even minimal models of coupled atomic chains host rich phase diagrams controlled by doping, lattice rigidity, and interchain coupling geometry.

cond-mat.mes-hall

Scalable tight-binding model for strained graphene

We generalize the scalable tight-binding model for graphene, which allows for efficient quantum transport simulations in the Dirac regime, to account for elastic strain. We show that the original scalable model with scaling factor $s$ is readily applicable to strained graphene, provided that the displacement fields corresponding to the deformed graphene lattice are properly scaled. In particular, we show that the long-wavelength theory remains invariant when the strain tensor is scaled by $s$. This is achieved in practice by scaling the in-plane displacement fields by $s$ while the out-of-plane displacements have to be scaled by $\sqrt{s}$. We confirm these scaling laws by extensive numerical simulations, starting with the pseudomagnetic field and the local density of states for different scaled lattices. The latter allows us to study pseudo-Landau levels as well as hybrid Landau levels in the presence of an external magnetic field. Finally, we consider quantum transport simulations motivated by a recent experiment, where a uniaxial strain barrier is engineered in monolayer graphene by vertically misaligned gates. Our work generalizes the scalable tight-binding model to allow for efficient modeling of quantum transport in large-scale strained graphene devices.

cond-mat.mes-hall

Pseudomagnetotransport in Strained Graphene

In graphene, long-wavelength deformations that result in elastic shear strain couple to the low-energy Dirac electrons as pseudogauge fields. Using a scalable tight-binding model, we consider analogs to magnetotransport in mesoscopic strained graphene devices with nearly uniform pseudomagnetic fields. In particular, we consider transverse pseudomagnetic focusing in a bent graphene ribbon and show that a focused valley-polarized current can be generated with characteristic conductance oscillations. Importantly, our scaling method allows for quantum transport calculations with realistic device geometries, and leaves the Dirac physics and pseudogauge fields invariant as long as the atomic displacements vary slowly with respect to the scaled lattice. Our results show that pseudomagnetotransport is a promising new route for graphene straintronics, and our scaling method provides a new framework for the modeling, design, and interpretation of straintronics experiments and applications.

cond-mat.mes-hall

Substrate, temperature and magnetic field dependence of electric polarisation in mixed-stacking tetralayer graphenes

Polytypes of tetralayer graphene (TLG: Bernal, rhombohedral and mixed stacking) are crystalline structures with different symmetries. Among those, mixed-stacking tetralayers lack inversion symmetry, which allows for intrinsic spontaneous out-of-plane electrical polarisation, inverted in the mirror-image pair, ABCB and ABAC stackings. Here, we compare the intrinsic polarisation of such TLGs with the symmetry-breaking effect of a substrate, which can also generate out-of-plane electric dipole moments with different sizes in all four polytypes, including ABCB and ABAC twins. We analyse their temperature and magnetic field dependence, in view of understanding the origin of the recently measured Kelvin probe force microscopy maps of tetralayer flakes, and notice that the intrinsic contribution could be singled out based on magnetic field dependence of polarisation measured at low temperatures.

cond-mat.mes-hall

Fractal Quantum Transport on MoS2 Superlattices: a System with Tunable Symmetry

Electron doping is an excellent tuning knob to explore different phases of matter in two-dimensional (2D) materials. For example, tuning the Fermi level at a van Hove singularity in twisted bilayer graphene can enhance electron-electron interactions and induce a diverse range of correlated phases. Here, using a single-particle picture, we study the electronic reconstruction of the band edges of a 2D semiconductor, monolayer MoS2, on a hexagonal moire potential induced by another MoS2 monolayer. We find that such system transitions from a honeycomb to a hexagonal symmetry when the Fermi level is tuned from the conduction to the valence side. We also study the system under magnetic fields, and construct the Hofstadter's butterfly in the electron- and hole-doped side. Our findings are confirmed by simulating the conductance across a large-scale two-terminal device. We conclude that this duality is a general property that MoS2 and other transition-metal-dichalcogenides exhibit under non-symmetric superlattice potentials.

cond-mat.mes-hall

Magnetotransport Signatures of the Radial Rashba Spin-Orbit Coupling in Proximitized Graphene

Graphene-based van der Waals heterostructures take advantage of tailoring spin-orbit coupling (SOC) in the graphene layer by proximity effect. At long-wavelength -- saddled by the electronic states near the Dirac points -- the proximitized features can be effectively modelled by the Hamiltonian involving novel SOC terms and allow for an admixture of the tangential and radial spin textures -- by the so-called Rashba angle $θ_{\text{R}}$. Taking such effective models we perform realistic large-scale magneto-transport calculations -- transverse magnetic focusing and Dyakonov-Perel spin relaxation -- and show that there are unique qualitative and quantitative features allowing for an unbiased experimental disentanglement of the conventional Rashba SOC from its novel radial counterpart, called here the radial Rashba SOC. Along with that, we propose a scheme for a direct estimation of the Rashba angle by exploring the magneto-response symmetries when swapping an in-plane magnetic field. To complete the story, we analyze the magneto-transport signatures in the presence of an emergent Dresselhaus SOC and also provide some generic ramifications about possible scenarios of the radial superconducting diode effect.

cond-mat.mes-hall

Mixed-Stacking Few-Layer Graphene as an Elemental Weak Ferroelectric Material

Ferroelectricity (Valasek, J. Phys. Rev. 1921, 17, 475) - a spontaneous formation of electric polarisation - is a solid state phenomenon, usually, associated with ionic compounds or complex materials. Here we show that, atypically for elemental solids, few-layer graphenes can host an equilibrium out-of-plane electric polarisation, switchable by sliding the constituent graphene sheets. The systems hosting such effect include mixed-stacking tetralayers and thicker (5-9 layers) rhombohedral graphitic films with a twin boundary in the middle of a flake. The predicted electric polarisation would also appear in marginally (small-angle) twisted few-layer flakes, where lattice reconstruction would give rise to networks of mesoscale domains with alternating value and sign of out-of-plane polarisation.

cond-mat.mtrl-sci

Kagomé quantum oscillations in graphene superlattices

Periodic systems feature the Hofstadter butterfly spectrum produced by Brown--Zak minibands of electrons formed when magnetic field flux through the lattice unit cell is commensurate with flux quantum and manifested by magneto-transport oscillations. Quantum oscillations, such as Shubnikov -- de Haas effect and Aharonov--Bohm effect, are also characteristic for electronic systems with closed orbits in real space and reciprocal space. Here we show the intricate relation between these two phenomena by tracing quantum magneto-oscillations to Lifshitz transitions in graphene superlattices, where they persist even at relatively low fields and very much above liquid-helium temperatures. The oscillations originate from Aharonov--Bohm interference on cyclotron trajectories that form a kagomé-shaped network characteristic for Lifshitz transitions. In contrast to Shubnikov - de Haas oscillations, the kagomé oscillations are robust against thermal smearing and they can be detected even when the Hofstadter butterfly spectrum is undermined by electron's scattering. We expect that kagomé quantum oscillations are generic to rotationally-symmetric two-dimensional crystals close to Lifshitz transitions.

cond-mat.mes-hall

Spectroscopic signatures of tetralayer graphene polytypes

Tetralayer graphene has recently become a new addition to the family of few-layer graphene with versatile electronic properties. This material can be realised in three distinctive stacking configurations, for which we determine spectroscopic signatures in angle-resolved photoemission spectroscopy (ARPES), dynamical optical conductivity, and Raman spectra of inter-band excitations. The reported library of spectral features of tetralayer graphenes can be used for the non-invasive identification of the stacking order realised in a particular film.

cond-mat.mes-hall

Flat bands for electrons in rhombohedral graphene multilayers with a twin boundary

Topologically protected flat surface bands make thin films of rhombohedral graphite an appealing platform for searching for strongly correlated states of 2D electrons. In this work, we study rhombohedral graphite with a twin boundary stacking fault and analyse the semimetallic and topological properties of low-energy bands localised at the surfaces and at the twinned interface. We derive an effective 4-band low energy model, where we implement the full set of Slonczewski-Weiss-McClure (SWMcC) parameters, and find the conditions for the bands to be localised at the twin boundary, protected from the environment-induced disorder. This protection together with a high density of states at the charge neutrality point, in some cases -- due to a Lifshitz transition, makes this system a promising candidate for hosting strongly-correlated effects.

cond-mat.mes-hall

Band Gap Opening in Bilayer Graphene-CrCl$_3$/CrBr$_3$/CrI$_3$ van der Waals Interfaces

We report experimental investigations of transport through bilayer graphene (BLG)/chromium trihalide (CrX$_3$; X=Cl, Br, I) van der Waals interfaces. In all cases, a large charge transfer from BLG to CrX$_3$ takes place (reaching densities in excess of $10^{13}$ cm$^{-2}$), and generates an electric field perpendicular to the interface that opens a band gap in BLG. We determine the gap from the activation energy of the conductivity and find excellent agreement with the latest theory accounting for the contribution of the $σ$ bands to the BLG dielectric susceptibility. We further show that for BLG/CrCl$_3$ and BLG/CrBr$_3$ the band gap can be extracted from the gate voltage dependence of the low-temperature conductivity, and use this finding to refine the gap dependence on the magnetic field. Our results allow a quantitative comparison of the electronic properties of BLG with theoretical predictions and indicate that electrons occupying the CrX$_3$ conduction band are correlated.

cond-mat.mes-hall

Out-of-plane dielectric susceptibility of graphene in twistronic and Bernal bilayers

We describe how the out-of-plane dielectric polarizability of monolayer graphene influences the electrostatics of bilayer graphene -- both Bernal (BLG) and twisted (tBLG). We compare the polarizability value computed using density functional theory with the output from previously published experimental data on the electrostatically controlled interlayer asymmetry potential in BLG and data on the on-layer density distribution in tBLG. We show that monolayers in tBLG are described well by polarizability $α_{exp} = 10.8 \unicode{x212B}^3$ and effective out-of-plane dielectric susceptibility $ε_z = 2.5$, including their on-layer electron density distribution at zero magnetic field and the inter-layer Landau level pinning at quantizing magnetic fields.

cond-mat.mes-hall

Scattering between minivalleys in a moiré material

A unique feature of the complex band structures of moiré materials is the presence of minivalleys, their hybridization, and scattering between them. Here we investigate magneto-transport oscillations caused by scattering between minivalleys - a phenomenon analogous to magneto-intersubband oscillations - in a twisted double bilayer graphene sample with a twist angle of 1.94°. We study and discuss the potential scattering mechanisms and find an electron-phonon mechanism and valley conserving scattering to be likely. Finally, we discuss the relevance of our findings for different materials and twist angles.

cond-mat.mes-hall

Full Slonczewski-Weiss-McClure parametrization of few-layer twistronic graphene

We use a hybrid k dot p theory - tight binding (HkpTB) model to describe interlayer coupling simultaneously in both Bernal and twisted graphene structures. For Bernal-aligned interfaces, HkpTB is parametrized using the full Slonczewski-Weiss-McClure (SWMcC) Hamiltonian of graphite, which is then used to refine the commonly used minimal model for twisted interfaces, by deriving additional terms that reflect all details of the full SWMcC model of graphite. We find that these terms introduce some electron-hole asymmetry in the band structure of twisted bilayers, but in twistronic multilayer graphene, they produce only a subtle change of moire miniband spectra, confirming the broad applicability of the minimal model for implementing the twisted interface coupling in such systems.

cond-mat.mes-hall

Coherent Jetting behind a gate-defined Channel in Bilayer Graphene

Graphene has evolved as a platform for quantum transport that can compete with the best and cleanest semiconductor systems. Recently, many interesting local properties of carrier transport in graphene have been investigated by various scanning probe techniques. Here, we report on the observation of distinct electronic jets emanating from a narrow split-gate defined channel in bilayer graphene. We find that these jets, which are visible via their interference patterns, occur predominantly with an angle of 60° between each other. This observation is related to the specific bandstructure of bilayer graphene, in particular trigonal warping, which leads to a valley-dependent selection of momenta for low-energy conduction channels. This experimental observation of electron jetting has consequences for carrier transport in graphene in general as well as for devices relying on ballistic and valley selective transport.

cond-mat.mes-hall

Tunable van Hove Singularities and Correlated States in Twisted Trilayer Graphene

Understanding and tuning correlated states is of great interest and significance to modern condensed matter physics. The recent discovery of unconventional superconductivity and Mott-like insulating states in magic-angle twisted bilayer graphene (tBLG) presents a unique platform to study correlation phenomena, in which the Coulomb energy dominates over the quenched kinetic energy as a result of hybridized flat bands. Extending this approach to the case of twisted multilayer graphene would allow even higher control over the band structure because of the reduced symmetry of the system. Here, we study electronic transport properties in twisted trilayer graphene (tTLG, bilayer on top of monolayer graphene heterostructure). We observed the formation of van Hove singularities which are highly tunable by twist angle and displacement field and can cause strong correlation effects under optimum conditions, including superconducting states. We provide basic theoretical interpretation of the observed electronic structure.

cond-mat.mes-hall