Searcharxiv⌕ Search

arXiv subjects

Akashdeep Kamra

Publications and source records attributed to Akashdeep Kamra.

At least 37 records · Page 2Linked to original sources
arXiv2024

Superconducting spin valves based on antiferromagnet/superconductor/antiferromagnet heterostructures

Proximity effect at superconductor/antiferromagnet (S/AF) interfaces, which manifests itself as generation of Neel-type triplet correlations, leads to sensitivity of the superconducting critical temperature to the mutual orientation of the AF Neel vectors in AF/S/AF trilayers, which is called the spin-valve effect. Here we predict that the spin-valve effect in AF/S/AF heterostructures crucially depends on the value of the chemical potential of the superconducting interlayer due to the occurrence of the finite-momentum Neel triplet correlations. In addition we investigate equal-spin triplet correlations, which appear in AF/S/AF structures for non-aligned Neel vectors of the AFs, and their role in the nonmonotonic dependence of the superconducting critical temperature of the AF/S/AF structure on the mutual orientation of the AF Neel vectors. The influence of impurities on the spin-valve effect is also investigated.

cond-mat.supr-con↗
arXiv2024

Unconventional magnetism mediated by spin-phonon-photon coupling

Magnetic order typically emerges due to the short-range exchange interaction between the constituent electronic spins. Recent discoveries have found a crucial role for spin-phonon coupling in various phenomena from optical ultrafast magnetization switching to dynamical control of the magnetic state. Here, we demonstrate theoretically the emergence of a biquadratic long-range interaction between spins mediated by their coupling to phonons hybridized with vacuum photons into polaritons. The resulting ordered state enabled by the exchange of virtual polaritons between spins is reminiscent of superconductivity mediated by the exchange of virtual phonons. The biquadratic nature of the spin-spin interaction promotes ordering without favoring ferro- or antiferromagnetism. It further makes the phase transition to magnetic order a first-order transition, unlike in conventional magnets. Consequently, a large magnetization develops abruptly on lowering the temperature which \aknew{could} enable magnetic memories admitting ultralow-power thermally-assisted writing while maintaining a high data stability. The role of photons in the phenomenon further enables an in-situ static control over the magnetism. These unique features make our predicted spin-spin interaction and magnetism highly unconventional paving the way for novel scientific and technological opportunities.

cond-mat.mes-hall↗
arXiv2024

Quantum Sensing of Antiferromagnetic Magnon Two-Mode Squeezed Vacuum

Néel ordered antiferromagnets exhibit two-mode squeezing such that their ground state is a nonclassical superposition of magnon Fock states. Here we theoretically demonstrate that antiferromagnets can couple to spin qubits via direct dispersive interaction stemming from, e.g., interfacial exchange. We demonstrate that this kind of coupling induces a magnon number dependent level splitting of the excited state resulting in multiple system excitation energies. This series of level splittings manifests itself as nontrivial excitation peaks in qubit spectroscopy thereby revealing the underlying nonclassical magnon composition of the antiferromagnetic quantum state. By appropriately choosing the drive or excitation energy, the magnonic state can be controlled via the qubit, suggesting that Fock states of magnon pairs can be generated deterministically. This enables achieving states useful for quantum computing and quantum information science protocols.

cond-mat.mes-hall↗
arXiv2024

Inductive magnon noise spectroscopy

State tomography allows to characterize quantum states, and was recently applied to reveal the dynamic magnetization state of a parametrically driven magnet. The identification of non-classical states, such as squeezed states, relies on a careful analysis of their emission and their distinction from thermal and vacuum fluctuations. A technique allowing to detect equilibrium magnetization fluctuations is a crucial first step in this regard. In this Letter, we show that inductive magnon noise spectroscopy (iMNS) allows to characterize the thermal magnetization fluctuations of a ferromagnetic thin film in a broadband coplanar waveguide-based scheme. Relative to a cold microwave background, the microwaves emitted by the equilibrium magnetization fluctuations can be detected via spectrum analysis. We provide a comprehensive picture of our microwave system by quantitatively modeling its response, including the thermalizing influence of the cables. The model allows for direct comparison to low-power broadband ferromagnetic resonance measurements with excellent agreement, corroborating the equilibrium character of the iMNS measurement by probing the linear response of the equilibrium state. Our work thus demonstrates broadband access to the equilibrium properties of magnetization fluctuations using a purely inductive approach.

cond-mat.mes-hall↗
arXiv2024

Thermodynamic properties of a superconductor interfaced with an altermagnet

Recently introduced magnetic materials called altermagnets (AM) feature zero net magnetization but a momentum dependent magnetic exchange field, which can have intriguing implications when combined with superconductivity. In our work, we use the quasiclassical framework to study the effects of such a material on a conventional superconductor (S) in an AM/S bilayer. We discuss the superconducting phase diagram and heat capacity of AM/S while making a comparison with a ferromagnet-superconductor bilayer. Furthermore, we examine the density of states and analyze the system's response to an external magnetic field. We illustrate the anisotropy of spin-susceptibility and magnetization of AM/S by considering an external field in the in-plane and out-of-plane direction, thereby facilitating the scope of experimental detection and characterization of an AM in an AM/S hybrid system.

cond-mat.supr-con↗
arXiv2024

Standing spin waves in Permalloy-NiO bilayers as a probe of the interfacial exchange coupling

Ferromagnetic/Antiferromagnetic (FM/AFM) bilayers dynamics have been a recent topic of interest due to the interaction occurring at the interface, where the magnetic moments of the AFM can be imprinted into the FM, and the exchange bias field can affect these dynamics. Here, we investigate Permalloy (Py) and NiO (Py/NiO) hybrids and for comparison single Py films in the broad Py thickness range varied from few nm to 200 nm by using static (Kerr effect) and dynamic (spin waves) measurements along with micromagnetic simulations. We observe hybrid modes between uniform (ferromagnetic resonance FMR, n=0) and perpendicular standing spin waves (PSSWs, n=1, 2) and a clear enhancement of the PSSWs modes frequencies upon interfacing Py with NiO both from experiments and simulations. This enhancement becomes less pronounced as the thickness of the film increases, demonstrating its interfacial origin rooted in the exchange coupling between the FM and AFM layers. Besides, through micromagnetic simulations, we investigate and correlate changes in spatial profiles of the PSSWs with the interfacial exchange coupling. As the thickness is increased, we see that the n=1 and n=2 modes begin to couple with the fundamental FMR mode, resulting in asymmetric (with respect the Py layer center) modes. Our results suggest that PSSWs detection in a ferromagnet offers a means of probing the interfacial exchange coupling with the adjacent AFM layer. Furthermore, the controlled spatial symmetry breaking by the AFM layer enables engineering of PSSWs with different spatial profiles in the FM.

cond-mat.mes-hall↗
arXiv2023

Electrically induced angular momentum flow between separated ferromagnets

Converting angular momentum between different degrees of freedom within a magnetic material results from a dynamic interplay between electrons, magnons and phonons. This interplay is pivotal to implementing spintronic device concepts that rely on spin angular momentum transport. We establish a new concept for long-range angular momentum transport that further allows to address and isolate the magnonic contribution to angular momentum transport in a nanostructured metallic ferromagnet. To this end, we electrically excite and detect spin transport between two parallel and electrically insulated ferromagnetic metal strips on top of a diamagnetic substrate. Charge-to-spin current conversion within the ferromagnetic strip generates electronic spin angular momentum that is transferred to magnons via electron-magnon coupling. We observe a finite angular momentum flow to the second ferromagnetic strip across a diamagnetic substrate over micron distances, which is electrically detected in the second strip by the inverse charge-to-spin current conversion process. We discuss phononic and dipolar interactions as the likely cause to transfer angular momentum between the two strips. Moreover, our work provides the experimental basis to separate the electronic and magnonic spin transport and thereby paves the way towards magnonic device concepts that do not rely on magnetic insulators.

cond-mat.mes-hall↗
arXiv2023

Electrostatic nature of cavity-mediated interactions between low-energy matter excitations

The use of cavity quantum electrodynamical effects, i.e., of vacuum electromagnetic fields, to modify material properties in cavities has rapidly gained popularity and interest in the last few years. However, there is still a scarcity of general results that provide guidelines for intuitive understanding and limitations of what kind of effects can be achieved. We provide such a result for the effective interactions between low-energy matter excitations induced either directly by their mutual coupling to the cavity electromagnetic (EM) field or indirectly through coupling to mediator modes that couple to the EM field. We demonstrate that the induced interactions are purely electrostatic in nature and are thus fully described by the EM Green's function evaluated at zero frequency. Our findings imply that reduced models with one or a few cavity modes can easily give misleading results.

quant-ph↗
arXiv2023

Complete $T_c$ suppression and Néel triplets-mediated exchange in antiferromagnet-superconductor-antiferromagnet trilayers

An antiferromagnetic insulator (AFI) bearing a compensated interface to an adjacent conventional superconductor (S) has recently been predicted to generate Néel triplet Cooper pairs, whose amplitude alternates sign in space. Here, we theoretically demonstrate that such Néel triplets enable control of the superconducting critical temperature in an S layer via the angle between the Néel vectors of two enclosing AFI layers. This angle dependence changes sign with the number of S monolayers providing a distinct signature of the Néel triplets. Furthermore, we show that the latter mediate a similarly distinct exchange interaction between the two AFIs' Néel vectors.

cond-mat.mes-hall↗
arXiv2023

Resolving nonclassical magnon composition of a magnetic ground state via a qubit

Recently gained insights into equilibrium squeezing and entanglement harbored by magnets point towards exciting opportunities for quantum science and technology, while concrete protocols for exploiting these are needed. Here, we theoretically demonstrate that a direct dispersive coupling between a qubit and a noneigenmode magnon enables detecting the magnonic number states' quantum superposition that forms the ground state of the actual eigenmode - squeezed-magnon - via qubit excitation spectroscopy. Furthermore, this unique coupling is found to enable control over the equilibrium magnon squeezing and a deterministic generation of squeezed even Fock states via the qubit state and its excitation. Our work demonstrates direct dispersive coupling to noneigenmodes, realizable in spin systems, as a general pathway to exploiting the equilibrium squeezing and related quantum properties thereby motivating a search for similar realizations in other platforms.

cond-mat.mes-hall↗
arXiv2023

Ferromagnetic interlayer coupling in CrSBr crystals irradiated by ions

Layered magnetic materials are becoming a major platform for future spin-based applications. Particularly the air-stable van der Waals compound CrSBr is attracting considerable interest due to its prominent magneto-transport and magneto-optical properties. In this work, we observe a transition from antiferromagnetic to ferromagnetic behavior in CrSBr crystals exposed to high-energy, non-magnetic ions. Already at moderate fluences, ion irradiation induces a remanent magnetization with hysteresis adapting to the easy-axis anisotropy of the pristine magnetic order up to a critical temperature of 110 K. Structure analysis of the irradiated crystals in conjunction with density functional theory calculations suggest that the displacement of constituent atoms due to collisions with ions and the formation of interstitials favors ferromagnetic order between the layers.

cond-mat.mtrl-sci↗
arXiv2023

Using superconductivity to control magnetism: a facet of superconducting spintronics

Magnets are used in electronics to store and read information. A magnetic moment is rotated to a desired direction, so that information can later be retrieved by reading this orientation. Controlling the moment via electric currents causes resistive losses and heating, a major bottleneck in advancing computing technologies. Superconducting spintronics can resolve this using the unique features of superconductors.

cond-mat.mes-hall↗
arXiv2023

Electrical detectability of magnon-mediated spin current shot noise

A magnonic spin current crossing a ferromagnet-metal interface is accompanied by spin current shot noise arising from the discrete quanta of spin carried by magnons. In thin films, e.g., the spin of so-called squeezed magnons have been shown to deviate from the common value $\hbar$, with corresponding changes in the spin noise. In experiments, spin currents are typically converted to charge currents via the inverse spin Hall effect. We here analyze the magnitude of the spin current shot noise in the charge channel for a typical electrically detected spin pumping experiment, and find that the voltage noise originating from the spin current shot noise is much smaller than the inevitable Johnson-Nyquist noise. Furthermore, we find that due to the local nature of the spin-charge conversion, the ratio of spin current shot noise and Johnson-Nyquist noise cannot be systematically enhanced by tuning the sample geometry, in contrast to the linear increase in dc spin pumping voltage with sample length. Instead, the ratio depends sensitively on material-specific transport properties. Our analysis thus provides guidance for the experimental detection of squeezed magnons through spin pumping shot noise.

cond-mat.mes-hall↗
arXiv2023

Magnon-Cooparons in magnet-superconductor hybrids

Generation and detection of spinful Cooper pairs in conventional superconductors has been intensely pursued by designing increasingly complex magnet-superconductor hybrids. Here, we demonstrate theoretically that magnons with nonzero wavenumbers universally induce a cloud of spinful triplet Cooper pairs around them in an adjacent conventional superconductor. The resulting composite quasiparticle, termed magnon-cooparon, consists of a spin flip in the magnet screened by a cloud of the spinful superfluid condensate. Thus, it inherits a large effective mass, which can be measured experimentally. Furthermore, we demonstrate that two magnetic wires deposited on a superconductor serve as a controllable magnonic directional coupler mediated by the nonlocal and composite nature of magnon-cooparons. Our analysis predicts a quasiparticle that enables generation, control, and use of spinful triplet Cooper pairs in the simplest magnet-superconductor heterostructures.

cond-mat.supr-con↗
arXiv2023

Generation of spin-triplet Cooper pairs via a canted antiferromagnet

Spinful triplet Cooper pairs can be generated from their singlet counterparts available in a conventional superconductor (S) using two or more noncollinear magnetic moments, typically contributed by different magnets in a multilayered heterostructure. Here, we theoretically demonstrate that an S interfaced with a canted antiferromagnet (AF) harbors spinful triplet Cooper pairs capitalizing on the intrinsic noncollinearity between the two AF sublattice magnetizations. As the AF canting can be controlled by an applied field, our work proposes a simple bilayer structure that admits controllable generation of spin-triplet Cooper pairs. Employing the Bogoliubov-de Gennes framework, we delineate the spatial dependence of the spin-triplet correlations. We further evaluate the superconducting critical temperature as a function of the AF canting, which provides one experimental observable associated with the emergence of these triplet correlations.

cond-mat.mes-hall↗
arXiv2023

Impact of magnetic anisotropy on the magnon Hanle effect in $α$-Fe$_2$O$_3$

In easy-plane antiferromagnets, the nature of the elementary excitations of the spin system is captured by the precession of the magnon pseudospin around its equilibrium pseudofield, manifesting itself in the magnon Hanle effect. Here, we investigate the impact of growth-induced changes in the magnetic anisotropy on this effect in the antiferromagnetic insulator $α$-Fe$_2$O$_3$ (hematite). To this end, we compare the structural, magnetic, and magnon-based spin transport properties of $α$-Fe$_2$O$_3$ films with different thicknesses grown by pulsed laser deposition in molecular and atomic oxygen atmospheres. While in films grown with molecular oxygen a spin-reorientation transition (Morin transition) is absent down to $10\,$K, we observe a Morin transition for those grown by atomic-oxygen-assisted deposition, indicating a change in magnetic anisotropy. Interestingly, even for a $19\,$nm thin $α$-Fe$_2$O$_3$ film grown with atomic oxygen we still detect a Morin transition at $125\,$K. We characterize the magnon Hanle effect in these $α$-Fe$_2$O$_3$ films via all-electrical magnon transport measurements. The films grown with atomic oxygen show a markedly different magnon spin signal from those grown in molecular oxygen atmospheres. Most importantly, the maximum magnon Hanle signal is significantly enhanced and the Hanle peak is shifted to lower magnetic field values for films grown with atomic oxygen. These observations suggest a change of magnetic anisotropy for $α$-Fe$_2$O$_3$ films fabricated by atomic-oxygen-assisted deposition resulting in an increased oxygen content in these films. Our findings provide new insights into the possibility to fine-tune the magnetic anisotropy in $α$-Fe$_2$O$_3$ and thereby to engineer the magnon Hanle effect.

cond-mat.mes-hall↗
arXiv2023

Ubiquitous Superconducting Diode Effect in Superconductor Thin Films

The macroscopic coherence in superconductors supports dissipationless supercurrents which could play a central role in emerging quantum technologies. Accomplishing unequal supercurrents in the forward and backward directions would enable unprecedented functionalities. This nonreciprocity of critical supercurrents is called superconducting (SC) diode effect. We demonstrate strong SC diode effect in conventional SC thin films, such as niobium and vanadium, employing external magnetic fields as small as 1 Oe. Interfacing the SC layer with a ferromagnetic semiconductor EuS, we further accomplish non-volatile SC diode effect reaching a giant efficiency of 65%. By careful control experiments and theoretical modeling, we demonstrate that the critical supercurrent nonreciprocity in SC thin films could be easily accomplished with asymmetrical vortex edge/surface barriers and the universal Meissner screening current governing the critical currents. Our engineering of the SC diode effect in simple systems opens door for novel technologies. Meanwhile, we reveal the ubiquity of Meissner screening effect induced SC diode effect in superconducting films, which should be eliminated with great care in the search of exotic superconducting states harboring finite-momentum Cooper pairing.

cond-mat.supr-con↗
arXiv2022

Rotationally invariant formulation of spin-lattice coupling in multi-scale modeling

In the spirit of multi-scale modeling, we develop a theoretical framework for spin-lattice coupling that connects, on the one hand, to ab initio calculations of spin-lattice coupling parameters and, on the other hand, to the magneto-elastic continuum theory. The derived Hamiltonian describes a closed system of spin and lattice degrees of freedom and explicitly conserves the total momentum, angular momentum and energy. Using a new numerical implementation that corrects earlier Suzuki-Trotter decompositions we perform simulations on the basis of the resulting equations of motion to investigate the combined magnetic and mechanical motion of a ferromagnetic nanoparticle, thereby validating our developed method. In addition to the ferromagnetic resonance mode of the spin system we find another low-frequency mechanical response and a rotation of the particle according to the Einstein-de-Haas effect. The framework developed herein will enable the use of multi-scale modeling for investigating and understanding a broad range of magneto-mechanical phenomena from slow to ultrafast time scales.

cond-mat.mtrl-sci↗