arXiv subjects

Aki Takahashi

Publications and source records attributed to Aki Takahashi.

3 recordsLinked to original sources

arXiv2023

Evaluating feasibility of batteries for second-life applications using machine learning

This paper presents a combination of machine learning techniques to enable prompt evaluation of retired electric vehicle batteries as to either retain those batteries for a second-life application and extend their operation beyond the original and first intent or send them to recycle facilities. The proposed algorithm generates features from available battery current and voltage measurements with simple statistics, selects and ranks the features using correlation analysis, and employs Gaussian Process Regression enhanced with bagging. This approach is validated over publicly available aging datasets of more than 200 cells with slow and fast charging, with different cathode chemistries, and for diverse operating conditions. Promising results are observed based on multiple training-test partitions, wherein the mean of Root Mean Squared Percent Error and Mean Percent Error performance errors are found to be less than 1.48% and 1.29%, respectively, in the worst-case scenarios.

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arXiv2022

Core-shell enhanced single particle model for lithium iron phosphate batteries: model formulation and analysis of numerical solutions

In this paper, a core-shell enhanced single particle model for iron-phosphate battery cells is formulated, implemented, and verified. Starting from the description of the positive and negative electrodes charge and mass transport dynamics, the positive electrode intercalation and deintercalation phenomena and associated phase transitions are described with the core-shell modeling paradigm. Assuming two phases are formed in the positive electrode, one rich and one poor in lithium, a core-shrinking problem is formulated and the phase transition is modeled through a shell phase that covers the core one. A careful discretization of the coupled partial differential equations is proposed and used to convert the model into a system of ordinary differential equations. To ensure robust and accurate numerical solutions of the governing equations, a sensitivity analysis of numerical solutions is performed and the best setting, in terms of solver tolerances, solid phase concentration discretization points, and input current sampling time, is determined in a newly developed probabilistic framework. Finally, unknown model parameters are identified at different C-rate scenarios and the model is verified against experimental data.

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arXiv2022

Core-shell enhanced single particle model for LiFePO$_4$ batteries

In this paper, a novel electrochemical model for LiFePO$_4$ battery cells that accounts for the positive particle lithium intercalation and deintercalation dynamics is proposed. Starting from the enhanced single particle model, mass transport and balance equations along with suitable boundary conditions are introduced to model the phase transformation phenomena during lithiation and delithiation in the positive electrode material. The lithium-poor and lithium-rich phases are modeled using the core-shell principle, where a core composition is encapsulated with a shell composition. The coupled partial differential equations describing the phase transformation are discretized using the finite difference method, from which a system of ordinary differential equations written in state-space representation is obtained. Finally, model parameter identification is performed using experimental data from a 49Ah LFP pouch cell.

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