arXiv subjects

Alan A. Dzhioev

Publications and source records attributed to Alan A. Dzhioev.

29 records · Page 2Linked to original sources

arXiv2012

Nonequilibrium perturbation theory in Liouville-Fock space for inelastic electron transport

We use a superoperator representation of the quantum kinetic equation to develop nonequilibrium perturbation theory for an inelastic electron current through a quantum dot. We derive a Lindblad-type kinetic equation for an embedded quantum dot (i.e. a quantum dot connected to Lindblad dissipators through a buffer zone). The kinetic equation is converted to non-Hermitian field theory in Liouville-Fock space. The general nonequilibrium many-body perturbation theory is developed and applied to the quantum dot with electron-vibronic and electron-electron interactions. Our perturbation theory becomes equivalent to a Keldysh nonequilibrium Green's function perturbative treatment provided that the buffer zone is large enough to alleviate the problems associated with approximations of the Lindblad kinetic equation.

cond-mat.mes-hall↗

arXiv2012

Solvent induced current-voltage hysteresis and negative differential resistance in molecular junctions

We consider a single molecule circuit embedded into solvent. The Born dielectric solvation model is combined with Keldysh nonequilibrium Green's functions to describe the electron transport properties of the system. Depending on the dielectric constant, the solvent induces multiple nonequilibrium steady states with corresponding hysteresis in molecular current-voltage characteristics as well as negative differential resistance. We identify the physical range of solvent and molecular parameters where the effects are present. The position of the negative differential resistance peak can be controlled by the dielectric constant of the solvent.

cond-mat.mes-hall↗

arXiv2011

Thermal QRPA equations with finite rank separable approximation for residual forces based on the Skyrme type interactions

The approach to study properties of charge-exchange excitations in hot nuclei is presented. The approach is based on the extension of the finite rank separable approximation for Skyrme interactions to finite temperatures employing the TFD formalism. We present the formulae to obtain charge-exchange strength distributions within the Thermal Quasiparticle Random Phase Approximation (TQRPA).

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arXiv2011

Stability analysis of multiple nonequilibrium fixed points in self-consistent electron transport calculations

We present a method to perform stability analysis of nonequilibrium fixed points appearing in self-consistent electron transport calculations. The nonequilibrium fixed points are given by the self-consistent solution of stationary, nonlinear kinetic equation for single-particle density matrix. We obtain the stability matrix by linearizing the kinetic equation around the fixed points and analyze the real part of its spectrum to assess the asymptotic time behavior of the fixed points. We derive expressions for the stability matrices within Hartree-Fock and linear response adiabatic time-dependent density functional theory. The stability analysis of multiple fixed points is performed within the nonequilibrium Hartree-Fock approximation for the electron transport through a molecule with a spin-degenerate single level with local Coulomb interaction.

cond-mat.mes-hall↗

arXiv2011

Kramers problem for nonequilibrium current-induced chemical reactions

We discuss the use of tunneling electron current to control and catalyze chemical reactions. Assuming the separation of time scales for electronic and nuclear dynamics we employ the Langevin equation for the reaction coordinate. The Langevin equation contains current-induced forces and is used to define nonequilibrium, effective potential energy surface for current-carrying molecular systems. The current-induced forces are computed via Keldysh nonequilibrium Green's functions. Once the nonequilibrium, current-depended potential energy surface is defined, the chemical reaction is modeled as an escape of a Brownian particle from the potential well. We demonstrate that the barrier between the reactant and the product states can be controlled by the bias voltage. When the molecule is asymmetrically coupled to the electrodes, the reaction can be catalyzed or stopped depending on the polarity of the tunneling current.

cond-mat.mes-hall↗

arXiv2011

Second-order post-Hartree-Fock perturbation theory for the electron current

Based on the super-fermion representation of quantum kinetic equations we develop nonequilibrium, post-Hartree-Fock many-body perturbation theory for the current through a region of interacting electrons. We apply the theory to out of equilibrium Anderson model and discuss practical implementation of the approach. Our calculations show that nonequilibrium electronic correlations may produce significant quantitative and qualitative corrections to mean-field electronic transport properties. We find that the nonequilibrium leads to enhancement of electronic correlations.

cond-mat.mes-hall↗

arXiv2011

Super-fermion representation of the Lindblad master equation for the electron transport problem

We discuss the use of super-fermion formalism to represent and solve quantum kinetic equations for the electron transport problem. Starting with the Lindblad master equation for the molecule connected to two metal electrodes, we convert the problem of finding the nonequilibrium steady state to the many-body problem with non-Hermitian Liouvillian in super-Fock space. We transform the Liouvillian to the normal ordered form, introduce nonequilibrium quasiparticles by a set of canonical nonunitary transformations and develop general many-body theory for the electron transport through the interacting region. The approach is applied to the electron transport through a single level. We consider a minimal basis hydrogen atom attached to two metal leads in Coulomb blockade regime (out of equilibrium Anderson model) within the nonequilibrium Hartree-Fock approximation as an example of the system with electron interaction. Our approach agrees with exact results given by the Landauer theory for the considered models.

cond-mat.mes-hall↗

arXiv2010

Thermal effects on neutrino-nucleus inelastic scattering in stellar environments

Thermal effects for inelastic neutrino-nucleus scattering off even-even nuclei in the iron region are studied. Allowed and first-forbidden contributions to the cross sections are calculated within the quasiparticle random phase approximation, extended to finite temperatures within the Thermo-Field-Dynamics formalism. The GT$_0$ strength distribution at finite temperatures is calculated for the sample nucleus $^{54}$Fe. The neutral-current neutrino-nucleus inelastic cross section is calculated for relevant temperatures during the supernova core collapse. The thermal population of the excited states significantly enhances the cross section at low neutrino energies. In agreement with studies using a large scale shell-model approach the enhancement is mainly due to neutrino up-scattering at finite temperatures.

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arXiv2010

Thermal Bogoliubov transformation in nuclear structure theory

Thermal Bogoliubov transformation is an essential ingredient of the thermo field dynamics -- the real time formalism in quantum field and many-body theories at finite temperatures developed by H. Umezawa and coworkers. The approach to study properties of hot nuclei which is based on the extension of the well-known Quasiparticle-Phonon Model to finite temperatures employing the TFD formalism is presented. A distinctive feature of the QPM-TFD combination is a possibility to go beyond the standard approximations like the thermal Hartree-Fock or the thermal RPA ones.

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arXiv2009

Gamow-Teller strength distributions at finite temperatures and electron capture in stellar environments

We propose a new method to calculate stellar weak-interaction rates. It is based on the Thermo-Field-Dynamics formalism and allows the calculation of the weak-interaction response of nuclei at finite temperatures. The thermal evolution of the GT$_+$ distributions is presented for the sample nuclei $^{54, 56}$Fe and ~$^{76,78,80}$Ge. For Ge we also calculate the strength distribution of first-forbidden transitions. We show that thermal effects shift the GT$_+$ centroid to lower excitation energies and make possible negative- and low-energy transitions. In our model we demonstrate that the unblocking effect for GT$_+$ transitions in neutron-rich nuclei is sensitive to increasing temperature. The results are used to calculate electron capture rates and are compared to those obtained from the shell model.

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arXiv2008

On the TFD treatment of collective vibrations in hot nuclei

The approach in a theory of collective excitations in hot nuclei exploring the formalism of thermo field dynamics and the model Hamiltonian consisting of a mean field, the BCS paring interaction and long-range particle-hole effective forces is reexamined. In contrast with earlier studies it is found that a wave function of a thermal phonon is depended not only on the Fermi-Dirac thermal occupation numbers of Bogoliubov quasiparticles consisting the phonon but on the Bose thermal occupation numbers of the phonon as well. This strongly affects a thermal phonon couplings due to renormalizing of a phonon-phonon interaction and enlarging the number of thermal two-phonon configurations coupled with one-phonon ones. Moreover, it is shown that the formulation of the double tilde conjugation rule for fermions proposed by I.Ojima is more appropriate in the context of the present study than the original one by H.Umezawa and coworkers.

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