Searcharxiv⌕ Search

arXiv subjects

Albert C. Pan

Publications and source records attributed to Albert C. Pan.

5 recordsLinked to original sources
arXiv2006

Lengthscale dependence of dynamic four-point susceptibilities in glass formers

Dynamical four-point susceptibilities measure the extent of spatial correlations in the dynamics of glass forming systems. We show how these susceptibilities depend on the length scales that necessarily form part of their definition. The behaviour of these susceptibilities is estimated by means of an analysis in terms of renewal processes within the context of dynamic facilitation. The analytic results are confirmed by numerical simulations of an atomistic model glass-former, and of two kinetically constrained models. Hence we argue that the scenario predicted by the dynamic facilitation approach is generic.

cond-mat.stat-mech↗
arXiv2005

Rotational correlation and dynamic heterogeneity in a kinetically constrained lattice gas

We study dynamical heterogeneity and glassy dynamics in a kinetically constrained lattice gas model which has both translational and rotational degrees of freedom. We find that the rotational diffusion constant tracks the structural relaxation time as density is increased whereas the translational diffusion constant exhibits a strong decoupling. We investigate distributions of exchange and persistence times for both the rotational and translational degrees of freedom and compare our results on the distributions of rotational exchange times to recent single molecule studies.

cond-mat.soft↗
arXiv2005

Heterogeneity and growing lengthscales in the dynamics of kinetically constrained lattice gases in two dimensions

We study dynamical heterogeneity and growing dynamical lengthscales in two kinetically constrained models, namely, the one- and two-vacancy assisted triangular lattice gases. One of the models is a strong glassformer and the other is a fragile glassformer. Both exhibit heterogeneous dynamics with broadly distributed timescales as seen in the distribution of persistence times. We show that the Stokes-Einstein relation is violated, to a greater degree in the fragile glassformer, and show how this violation is related to dynamic heterogeneity. We extract dynamical lengthscales from structure factors of mobile particles and show, quantitatively, the growth of this lengthscale as density increases. We comment on how the scaling of lengths and times in these models relates to that in facilitated spin models of glasses.

cond-mat.stat-mech↗
arXiv2004

Dynamics of Nucleation in the Ising Model

Reactive pathways to nucleation in a three-dimensional Ising model at 60% of the critical temperature are studied using transition path sampling of single spin flip Monte Carlo dynamics. Analysis of the transition state ensemble (TSE) indicates that the critical nuclei are rough and anisotropic. The TSE, projected onto the free energy surface characterized by cluster size, N, and surface area, S, indicates the significance of other variables in addition to these two traditional reaction coordinates for nucleation. The transmission coefficient along N is ~ 0.35, and this reduction of the transmission coefficient from unity is explained in terms of the stochastic nature of the dynamic model.

cond-mat.stat-mech↗