arXiv subjects

Alberto Bramati

Publications and source records attributed to Alberto Bramati.

At least 19 recordsLinked to original sources

arXiv2026

Modeling Growth and Plasma Oxygen Effects on Metal Purity in Platinum EBID

Electron Beam-Induced Deposition (EBID) enables site-specific nanofabrication but suffers from significant carbon contamination, limiting its applicability in plasmonics, nanoelectronics, and sensing. In this study, we investigate the relationship between EBID process parameters such as beam current, acceleration voltage, and dwell time, and the platinum-to-carbon composition of deposited nanostructures. Using Energy Dispersive X-Ray Spectroscopy (EDX), we establish a hindered exponential growth model that correlates deposit composition with fabrication conditions. To enhance metal purity, we apply plasma oxygen treatment, exposing EBID deposits to a 30 W plasma for 30 minutes in a tabletop plasma generator. Post-treatment EDX analysis confirms a systematic increase in platinum content, while SEM inspection reveals nanostructure shrinkage due to carbon removal. This work aims to provide a framework for optimizing EBID fabrication and post-processing strategies to enhance material performance.

physics.app-ph↗

arXiv2026

Emission of time-ordered photon pairs from a coherently-driven Kerr microcavity

Weakly-interacting many-body systems possess remarkable quantum properties that are essential components of quantum technologies, and constitute a topic of fundamental interest. Here we show that in a solid-state nonlinear microcavity embedding discrete modes of exciton-dressed photons, we can isolate a single eigenmode of quantum fluctuations from the much brighter coherent fraction of the field. In this regime, we perform frequency- and time-resolved correlations measurements between photons on the red and blue side of the fluctuations spectrum. When the average number of fluctuation quanta is smaller than one, we observe the formation of large pairwise time-ordered correlations: red photon first and blue photon second. We show that this peculiar time-ordering correlation emerges spontaneously from the interplay between frequency-resolved detection, and the non-trivial internal quantum structure of the elementary fluctuations.

cond-mat.quant-gas↗

arXiv2025

Momentum correlations of the Hawking effect in a quantum fluid

The Hawking effect -- the amplification of fluctuations at the horizon -- has been detected in quantum fluids through real-space density correlations. However, real-space observables integrate over frequency, mixing distinct scattering channels into a single interference pattern and obscuring the spectral and entanglement structure of the emission. Here, we numerically compute momentum-space two-point correlations in a transcritical quantum fluid, using the truncated Wigner approximation applied to a realistic, driven-dissipative polariton system. We spectrally resolve the Hawking--partner as well as greybody factor channels and find that both carry comparable correlation strength, demonstrating that the well-known real-space ``moustache'' is an interference between these spectrally distinct contributions. The Hawking--partner channel is dominated by negative correlations, a direct signature of quantum-vacuum pair creation. All features reach amplitudes detectable in state-of-the-art experiments. Our results establish that the full three-mode output state must be considered for entanglement characterization, and provide a general framework applicable to any quantum fluid.

cond-mat.quant-gas↗

arXiv2025

Swimming against a superfluid flow: Self-propulsion via vortex-antivortex shedding in a quantum fluid of light

A superfluid flows without friction below a critical velocity, exhibiting zero drag force on impurities. Above this threshold, superfluidity breaks down, and the internal energy is redistributed into incoherent excitations such as vortices. We demonstrate that a finite-mass, mobile impurity immersed in a flowing two-dimensional paraxial superfluid of light can \textit{swim} against the superfluid current when this critical velocity is exceeded. This self-propulsion is achieved by the periodic emission of quantized vortex-antivortex pairs downstream, which impart an upstream recoil momentum that results in a net propulsive force. Analogous to biological systems that minimize effort by exploiting wake turbulence, the impurity harnesses this vortex backreaction as a passive mechanism of locomotion. Reducing the impurity dynamics to the motion of its center of mass and using a point-vortex model, we quantitatively describe how this mechanism depends on the impurity geometry and the surrounding flow velocity. Our findings establish a fundamental link between internal-energy dissipation in quantum fluids and concepts of self-propulsion in active-matter systems, and opens new possibilities for exploiting vortices for controlled quantum transport at the microscale.

cond-mat.quant-gas↗

arXiv2025

Spectroscopy on a single nonlinear mode recognizes quantum states

Characterising optical quantum states is essential for the development of quantum technologies. While traditional approaches to perform full quantum state tomography are often experimentally demanding, neuromorphic architectures may provide an effective alternative. In this work, we demonstrate how a quantum nonlinear driven-dissipative mode is sufficient to act as a quantum reservoir. By analyzing the occupations at different frequencies in the emission spectrum, a linear regression suffices in many cases to recognize the relevant parameters of incident squeezed states. Beyond highlighting the general potential of this approach under continuous driving, we illustrate its effectiveness in an explicit nontrivial example where the source is a degenerate optical parametric oscillator (OPO), coupled to a nonlinear polariton microcavity.

quant-ph↗

arXiv2025

Stimulated Hawking effect and quasinormal mode resonance in a polariton simulator of field theory on curved spacetime

The Hawking effect amplifies fluctuations in the vicinity of horizons, both in black holes and in analogue platforms. Here, we consider a polariton simulator and numerically examine the \emph{stimulated} Hawking effect using a coherent probe incident on the horizon from the exterior. We implement an experimentally realistic effective spacetime that supports a quasinormal mode (QNM) in the vicinity of the horizon. We find that the stimulated Hawking effect manifests as transmission into a negative-energy Bogoliubov channel inside the horizon, consistent with pseudo-unitary Bogoliubov scattering. Moreover, transmission across the horizon peaks at the QNM frequency. The computed spectral signatures provide a practical guide for future experimental investigations of the Hawking effect and its interplay with QNMs, an open question in quantum field theory in curved spacetime.

quant-ph↗

arXiv2025

Multiply quantized vortex spectroscopy in a quantum fluid of light

The formation of quantized vortices is a unifying feature of quantum mechanical systems, making it a premier means for fundamental and comparative studies of different quantum fluids. Being excited states of motion, vortices are normally unstable towards relaxation into lower energy states. However, here we exploit the driven-dissipative nature of polaritonic fluids of light to create stationary, multiply charged vortices. We measure the spectrum of collective excitations and observe negative energy modes at the core and positive energy modes at large radii. Their coexistence at the same frequency normally causes the dynamical instability, but here intrinsic losses stabilize the system, allowing for phase pinning by the pump on macroscopic scales. We observe generic features of quantized vortices in quantum fluids and other rotating geometries like astrophysical compact objects, opening the way to the study of generic amplification phenomena.

cond-mat.quant-gas↗

arXiv2025

Deterministic Bottom-Up Fabrication of Plasmonic Nanostructures on Optical Nanofibers via Blurred Electron Beam Deposition

This study introduces a novel method for the deterministic fabrication of metallic nanostructures with controlled geometry and composition on suspended, single mode tapered optical nanofibers (TNFs) using a tailored Blurred Electron Beam Induced Deposition (BEBID) technique. TNFs, owing to their subwavelength diameters and intense evanescent fields, offer a unique platform for enhanced light matter interactions at the nanoscale. However, their mechanical fragility has thus far hindered the integration of plasmonic structures using conventional high energy deposition methods. BEBID addresses this limitation by deliberately defocusing the electron beam to reduce local mechanical stress, minimize vibration, and prevent fiber damage during deposition, thereby enabling the one-step growth of platinum nanopillars with sub 20 nm spatial precision and high structural fidelity directly on suspended TNFs. The fabricated structures were characterized using SEM, EDX, and their optical properties were investigated through broadband scattering spectra and polarization resolved measurements, showing strong agreement with Finite Difference Time Domain (FDTD) simulations. Numerical modeling further reveals that ordered arrays of nanopillars can shape and direct the scattered field along the fiber axis, enabling directional emission. This work establishes BEBID as a versatile bottom up nanofabrication approach for functional photonic architectures on fragile substrates, with direct applications in quantum photonics, nano optics, and on fiber plasmonic sensing.

physics.optics↗

arXiv2024

Room-temperature efficient single-photon generation from CdSe/ZnS nanoplateletes

In the search for materials for quantum information science applications, colloidal semiconductor nanoplatelets (NPLs) have emerged as a highly promising new class of materials due to their interesting optical properties, such as narrow emission linewidth and fast photoluminescence (PL) lifetimes at room temperature. So far only few works focused on the quantum properties of their emission, however, NPLs, with their atomic-scale thickness and one-dimensional quantum confinement, are promising candidates for single-photon sources. Here, we demonstrate room-temperature single-photon emission from core/shell CdSe/ZnS NPLs, which feature 8$x$20 nm$^2$ surface area and 1 nm shell. The limited surface area ensures effective Auger non-radiative recombination, resulting in highly efficient single-photon generation with values of photon purity as low as $g^{(2)}(\tau)=0.04$. The observed long-period blinking and bleaching, typical of such thin shells, can be easily reduced by increasing the shell thickness. This work establishes NPLs as new single-photon sources very well suited for integration into quantum photonic systems.

quant-ph↗

arXiv2023

Polariton Fluids as Quantum Field Theory Simulators on Tailored Curved Spacetimes

Quantum fields in curved spacetime exhibit a wealth of effects like Hawking radiation from black holes. While quantum field theory in black holes can only be studied theoretically, it can be tested in controlled laboratory experiments. In experiments, a fluid going from sub- to supersonic speed creates an effectively curved spacetime for the acoustic field, with a horizon where the speed of the fluid equals the speed of sound. The challenge to test predictions like the Hawking effect in such systems lies in the control of the spacetime curvature and access to the field spectrum thereon. Here, we create tailored stationary effective curved spacetimes in a polaritonic quantum fluid of light in which either massless or massive excitations can be created, with smooth and steep horizons and various supersonic fluid speeds. Using a recently developed spectroscopy method we measure the spectrum of collective excitations on these spacetimes, crucially observing negative energy modes in the supersonic regions, which signals the formation of a horizon. Control over the horizon curvature and access to the spectrum on either side demonstrates the potential of quantum fluids of light for the study of field theories on curved spacetimes, and we discuss the possibility of investigating emission and spectral instabilities with a horizon or in an effective Exotic Compact Object configuration.

cond-mat.quant-gas↗

arXiv2023

Entanglement from superradiance and rotating quantum fluids of light

The amplification of radiation by superradiance is a universal phenomenon observed in numerous physical systems. We demonstrate that superradiant scattering generates entanglement for different input states, including coherent states, thereby establishing the inherently quantum nature of this phenomenon. To put these concepts to the test, we propose a novel approach to create horizonless ergoregions, which are nonetheless dynamically stable thanks to the dissipative dynamics of a polaritonic fluid of light. We numerically simulate the system to demonstrate the creation of a stable ergoregion. Subsequently, we investigate rotational superradiance within this system, with a primary focus on entanglement generation and the possibilities for its enhancement using current techniques. Our methods permit the investigation of quantum emission by rotational superradiance in state-of-the-art experiments, in which the input state can be controlled at will.

gr-qc↗

arXiv2023

Observation of the diffusive Nambu-Goldstone mode of a non-equilibrium phase transition

Second-order phase transitions are governed by spontaneous symmetry breaking, which yield collective excitations with a gapless spectrum called Nambu-Goldstone (NG) modes. While NG modes in conservative systems are propagating excitations, non-equilibrium phase transitions have been predicted to feature a diffusive NG mode. We present the first experimental evidence of a diffusive NG mode in a non-equilibrium Bose-Einstein condensate of microcavity polaritons. The NG mode is observed as a spectral narrowing in the spectroscopic response of the condensate. Additionally, explicitly breaking the symmetry causes the opening of a gap in the spectrum and the disappearance of the NG mode. Our observations confirm the diffusive dynamics of the NG mode of non-equilibrium phase transitions and establish a promising framework to investigate fundamental questions in statistical mechanics.

cond-mat.quant-gas↗

arXiv2023

Highly photostable Zn-treated halide perovskite nanocrystals for efficient single photon generation

Achieving pure single-photon emission is essential for a range of quantum technologies, from optical quantum computing to quantum key distribution to quantum metrology. Among solid-state quantum emitters, colloidal lead halide perovskite (LHP) nanocrystals (NCs) have garnered significant attention due to their interesting structural and optical properties, which make them appealing single-photon sources (SPSs). However, their practical utilization for quantum technology applications has been hampered by environment-induced instabilities. In this study, we fabricate and characterize in a systematic manner Zn-treated $CsPbBr_3$ colloidal NCs obtained through $Zn^{2+}$ ion doping at the Pb-site, demonstrating improved stability under dilution and illumination. These doped NCs exhibit high single-photon purity, reduced blinking on a sub-millisecond timescale and stability of the bright state for excitation powers well above the saturation levels. Our findings highlight the potential of this synthesis approach to optimize the performance of LHP-based SPSs, opening up interesting prospects for their integration into nanophotonic systems for quantum technology applications.

quant-ph↗

arXiv2022

Spectrum of collective excitations of a quantum fluid of polaritons

We use a recently developed high-resolution coherent probe spectroscopy method to investigate the dispersion of collective excitations of a polaritonic quantum fluid. We measure the dispersion relation with high energy and wavenumber resolution, which allows us to determine the speed of sound in the fluid and to evidence the contribution of an excitonic reservoir. We report on the generation of collective excitations at negative energies, on the ghost branch of the dispersion curve. Precursors of dynamical instabilities are also identified. Our methods open the way to the precise study of quantum hydrodynamics of quantum fluids of light.

cond-mat.quant-gas↗

arXiv2022

Turbulent dynamics in two-dimensional paraxial fluid of light

Turbulence in quantum fluids has, surprisingly, a lot in common with its classical counterpart. Recently, cold atomic gases has emerged as a well controlled experimental platform to study turbulent dynamics. In this work, we introduce a novel system to study quantum turbulence in optics, with the major advantage of having access to a wide range of characterization tools available for light fields. In particular we report the temporal dynamics of density and phase and we show the emergence of isotropy in momentum space and the presence of different scaling laws in the incompressible kinetic energy spectrum. The microscopic origin of the algebraic exponents in the energy spectrum is discussed by studying the internal structure of quantized vortices within the healing length and their clustering at larger length scales. These results are obtained using two counter-streaming fluids of light, which allows for a precise preparation of the initial state and the in-situ measurement of the compressible and incompressible fluid velocity.

cond-mat.quant-gas↗

arXiv2022

Color-Tunable Mixed-Cation Perovskite Single Photon Emitters

Quantum photonics technologies like wavelength division multiplexing (WDM) for high-rate quantum key distribution require narrowband, spectrally tunable single photon emitters. Physical methods that rely on the application of large mechanical strain to epitaxial quantum dots or electric and magnetic fields to color centers in 2D metal dichalcogenides provide limited spectral tunability. Here we adopt a chemical approach to synthesize a family of colloidal mixed-cation perovskite quantum dots ($\text{Cs}_{1-x}\text{FA}_{x}\text{PbBr}_3$) that show highly photo-stable, compositionally tunable single photon emission at room temperature - spanning more than 30 nm in the visible wavelength spectral range. We find that, tailoring the stoichiometry of the organic formamidinium (FA) cation in all-inorganic cesium lead bromide ($\text{CsPbBr}_3$) perovskite quantum dots detunes the electronic band structure while preserving their excellent single photon emission characteristics. We argue that the mixed-cation perovskite quantum dots studied in this work offer a new platform for the realization of color-tunable single photon emitters that could be readily integrated in a diversity of quantum photonic devices.

quant-ph↗

arXiv2022

Transit effects for non-linear index measurement in hot atomic vapors

Hot atomic vapors are widely used in non-linear and quantum optics due to their large Kerr non-linearity. While the linear refractive index and the transmission are precisely measured and well modeled theoretically, similar characterization remains partial for the $\chi^{(3)}$ non-linear part of the susceptibility. In this work, we present a set of tools to measure and estimate numerically the non-linear index of hot atomic vapors both in the steady state and during the transient response of the medium. We apply these techniques for the characterization of a hot vapor of rubidium and we evidence the critical role played by transit effects, due to finite beam sizes, in the measurement of the non-linear index.

quant-ph↗

arXiv2022

Analogue quantum simulation of the Hawking effect in a polariton superfluid

Quantum effects of fields on curved spacetimes may be studied in the laboratory thanks to quantum fluids. Here we use a polariton fluid to study the Hawking effect, the correlated emission from the quantum vacuum at the acoustic horizon. We show how out-of-equilibrium physics affects the dispersion relation, and hence the emission and propagation of correlated waves: the fluid properties on either side of the horizon are critical to observing the Hawking effect. We find that emission may be optimised by supporting the phase and density of the fluid upstream of the horizon in a regime of optical bistability. This opens new avenues for the observation of the Hawking effect in out-of-equilibrium systems as well as for the study of new phenomenology of fields on curved spacetimes.

quant-ph↗