arXiv subjects

Alberto Mercurio

Publications and source records attributed to Alberto Mercurio.

At least 19 recordsLinked to original sources

arXiv2026

Dissipative phase transitions and chaos in two-photon driven quantum optomechanics

We investigate nonequilibrium criticality and chaos in a two-photon-driven optomechanical system. The parametric drive preserves a discrete $\mathbb{Z}_2$ symmetry of the optical field, while radiation-pressure coupling transfers the resulting nonlinear dynamics to a mechanical oscillator. Combining semiclassical stability analysis, exact Liouvillian spectra, and stochastic quantum trajectories, we show that this driven-dissipative optomechanical model supports both first- and second-order dissipative phase transitions. At negative detuning a second-order transition yields spontaneous breaking of the cavity-parity symmetry in the thermodynamic limit. At positive detuning the same symmetry breaking coexists with a first-order transition, signaled by metastability and by an additional symmetric Liouvillian mode. At stronger pump power the mean-field dynamics loses all stable fixed points and develops limit cycles and chaotic attractors with positive Lyapunov exponent. Quantum trajectories in this regime display chaotic-like motion, enhanced steady-state entropy, and delocalization over many entropic Liouvillian modes. These results establish two-photon-driven optomechanics as a platform where dissipative criticality, symmetry breaking, and quantum signatures of chaos emerge within the same experimentally accessible setting.

quant-ph↗

arXiv2026

Density Wave Ordering with Disordered Ultracold Fermions in Optical Cavities

We investigate the interplay between cavity-induced density-wave ordering and controllable disorder in a trapped two-dimensional gas of ultracold fermions. The atoms are dispersively coupled to an optical cavity and transversely driven by a pump beam, while an additional speckle beam spatially modulates the atom-light coupling through an AC-Stark shift of the atomic transition. In momentum space, this disorder converts the usual coupling between the cavity mode and a discrete set of density-wave Fourier components into a coupling to a continuum of fermionic density modes, weighted by the spectrum of the speckle pattern. Using linear response theory, we derive the superradiant threshold and show that the disordered interaction renormalizes the effective light-matter coupling, lowering the critical pump strength on average, with the threshold becoming self-averaging for short speckle correlation lengths. We complement this analysis with a numerical mean-field treatment that gives access to the intracavity photon number and to the real-space fermion density across the transition. These results confirm that the disorder shifts the photonic phase boundary and, above threshold, distorts the density-wave crystal by populating Fourier components beyond those selected by the clean cavity geometry. Our findings identify both the emitted cavity light and in situ density images as probes of engineered disorder in fermionic matter coupled to optical cavities.

cond-mat.quant-gas↗

arXiv2026

Floquet Dissipative Phase Transitions

Dissipative phase transitions (DPTs) are traditionally characterized through the spectrum of a time-independent Liouvillian superoperator. However, this definition does not apply to time-periodic (Floquet) systems that cannot be exactly recast as time-independent problems. Here, we develop a general framework to characterize DPTs in time-periodic open quantum systems through the spectrum of the Floquet propagator. We first study driven-dissipative Kerr resonators, known to display a DPT, showing that counter-rotating terms in the drive shift the critical point and significantly change the time scales associated with the transition. We then investigate DPTs in the driven quantum Rabi model and its time-independent approximation, the driven Jaynes-Cummings model, finding that the Rabi model exhibits distinct critical features as the ultrastrong coupling regime is approached. Moreover, our Floquet analysis unveils the disappearance of the DPT in the deep strong coupling regime, due to light-matter decoupling. Our approach sets the stage for the study of dissipative criticality in a broad class of time-dependent open quantum systems.

quant-ph↗

arXiv2025

Superstrong Dynamics and Directional Emission of a Giant Atom in a Structured Bath

Quantum emitters coupled to waveguides with nonlinear dispersion show rich quantum dynamics with the promise of implementing non-trivial non-Markovian quantum models. Recent advances in engineered photonic environments now allow the realization of discrete-site waveguides with tailored dispersion, yet most implementations of waveguide QED remain limited to a local qubit-waveguide coupling. Here, we study a transmon qubit non-locally coupled to a high-impedance coupled cavity array (CCA), thus implementing a \emph{giant atom} in a structured photonic environment. The non-local coupling produces interference with the CCA modes, selectively enhancing interaction with even and long-wavelength modes, while suppressing coupling to odd and short-wavelength modes. For a subset of symmetric, long-wavelength modes, we reach the superstrong coupling regime. In this regime, measurements of the atomic participation ratio reveal strongly hybridized eigenmodes on a par with a strongly reduced qubit participation at the frequency of maximum hybridization with the qubit, in agreement with theory. Time-domain measurements of the qubit dynamics show clear deviations from the single-mode Jaynes--Cummings model, marked by the emergence of mode--mode interactions. By breaking spatial inversion symmetry of the CCA, the qubit seeds dressed eigenmodes confined to either the right or left of the qubit, which we exploit to implement and characterize a directional photon-emission protocol. These results demonstrate precise control over multimode light--matter interaction in a structured photonic environment.

quant-ph↗

arXiv2025

AlgoTune: Can Language Models Speed Up General-Purpose Numerical Programs?

Despite progress in language model (LM) capabilities, evaluations have thus far focused on models' performance on tasks that humans have previously solved, including in programming (Jimenez et al., 2024) and mathematics (Glazer et al., 2024). We therefore propose testing models' ability to design and implement algorithms in an open-ended benchmark: We task LMs with writing code that efficiently solves computationally challenging problems in computer science, physics, and mathematics. Our AlgoTune benchmark consists of 154 coding tasks collected from domain experts and a framework for validating and timing LM-synthesized solution code, which is compared to reference implementations from popular open-source packages. In addition, we develop a baseline LM agent, AlgoTuner, and evaluate its performance across a suite of frontier models. AlgoTuner uses a simple, budgeted loop that edits code, compiles and runs it, profiles performance, verifies correctness on tests, and selects the fastest valid version. AlgoTuner achieves an average 1.72x speedup against our reference solvers, which use libraries such as SciPy, sk-learn and CVXPY. However, we find that current models fail to discover algorithmic innovations, instead preferring surface-level optimizations. We hope that AlgoTune catalyzes the development of LM agents exhibiting creative problem solving beyond state-of-the-art human performance.

cs.SE↗

arXiv2025

From Few to Many Emitters Cavity QED: Energy Levels and Emission Spectra From Weak to Deep-Strong Coupling

We present a systematic study of the properties of systems composed of $N$ two-level quantum emitters coupled to a single cavity mode, for light-matter interaction strengths ranging from the weak to the ultrastrong and deep-strong coupling regimes. Beginning with an analysis of the energy spectrum as a function of the light-matter coupling strength, we examine systems with varying numbers of emitters, from a pair to large collections, approaching the thermodynamic limit ($N \to \infty$). Additionally, we explore the emission properties of these systems under incoherent excitation of the emitters, employing a general theoretical framework for open cavity-QED systems, which is valid across all light-matter interaction regimes and preserves gauge invariance within truncated Hilbert spaces. Furthermore, we study the influence of the emitter-environment interaction on the spectral properties of the system. Specifically, when each emitter interacts independently with its own reservoir, we observe the emergence of an emission peak at the cavity's resonant frequency for even values of $N$. Our analysis also clarify the evolution of the system as the number of emitters increases, ultimately converging towards an equivalent system composed of two interacting single-mode bosonic fields.

quant-ph↗

arXiv2025

QuantumToolbox.jl: An efficient Julia framework for simulating open quantum systems

We present QuantumToolbox$.$jl, an open-source Julia package for simulating open quantum systems. Designed with a syntax familiar to users of QuTiP (Quantum Toolbox in Python), it harnesses Julia's high-performance ecosystem to deliver fast and scalable simulations. The package includes a suite of time-evolution solvers supporting distributed computing and GPU acceleration, enabling efficient simulation of large-scale quantum systems. We also show how QuantumToolbox$.$jl can integrate with automatic differentiation tools, making it well-suited for gradient-based optimization tasks such as quantum optimal control. Benchmark comparisons demonstrate substantial performance gains over existing frameworks. With its flexible design and computational efficiency, QuantumToolbox$.$jl serves as a powerful tool for both theoretical studies and practical applications in quantum science.

quant-ph↗

arXiv2025

Chiral cat code: Enhanced error correction induced by higher-order nonlinearities

We introduce a Schr\"odinger chiral cat qubit, a novel bosonic quantum code generalizing Kerr cat qubits that exploits higher-order nonlinearities. Compared to a standard Kerr cat, the chiral cat qubit allows additional correction of bit-flip errors within the Hilbert space of a single bosonic oscillator. Indeed, this code displays optical bistability, i.e., the simultaneous presence of multiple long-lived states. Two of them define the code space and two define an error space. Thanks to the chiral structure of the phase space of this system, the error space can be engineered to ``capture'' bit flip events in the code space (a bit-flip trap), without affecting the quantum information stored in the system. Therefore, it is possible to perform detection and correction of errors. We demonstrate how this topological effect can be particularly efficient in the presence of large dephasing. We provide concrete examples of the performance of the code and show the possibility of applying quantum operations rapidly and efficiently. Beyond the interest in this single technological application, our work demonstrates how the topology of phase space can enhance the performance of bosonic codes.

quant-ph↗

arXiv2025

Renormalization and Low-Energy Effective Models in Cavity and Circuit QED

The quantum Rabi model (QRM) is a cornerstone in the study of light-matter interactions within cavity and circuit quantum electrodynamics (QED). It effectively captures the dynamics of a two-level system coupled to a single-mode resonator, serving as a foundation for understanding quantum optical phenomena in a great variety of systems. However, this model may produce inaccurate results for large coupling strengths, even in systems with high anharmonicity. Moreover, issues of gauge invariance further undermine its reliability. In this work, we introduce a renormalized QRM that incorporates the effective influence of higher atomic energy levels, providing a significantly more accurate representation of the system while still maintaining a two-level description. To demonstrate the versatility of this approach, we present two different examples: an atom in a double-well potential and a superconducting artificial atom (fluxonium qubit). This procedure opens new possibilities for precisely engineering and understanding cavity and circuit QED systems, which are highly sought-after, especially for quantum information processing.

quant-ph↗

arXiv2024

Circuit QED Spectra in the Ultrastrong Coupling Regime: How They Differ from Cavity QED

Cavity quantum electrodynamics (QED) studies the interaction between resonator-confined radiation and natural atoms or other formally equivalent quantum excitations, under conditions where the quantum nature of photons is relevant. Phenomena studied in cavity QED can also be explored using superconducting artificial atoms and microwave photons in superconducting resonators. These circuit QED systems offer the possibility to reach the ultrastrong coupling regime with individual artificial atoms, unlike their natural counterparts. In this regime, the light-matter coupling strength reaches a considerable fraction of the bare resonance frequencies in the system. Here, we provide a careful analysis of both incoherent and coherent spectra in circuit QED systems consisting of a flux qubit interacting with an LC resonator. Despite these systems can be effectively described by the quantum Rabi model, as the corresponding cavity QED ones, we find distinctive features, depending on how the system is coupled to the output port, which become evident in the ultrastrong coupling regime.

quant-ph↗

arXiv2024

Nonperturbative cavity quantum electrodynamics: is the Jaynes-Cummings model still relevant?

In this tutorial review, we briefly discuss the role that the Jaynes-Cummings model occupies in present-day research in cavity quantum electrodynamics with a particular focus on the so-called ultrastrong coupling regime. We start by critically analyzing the various approximations required to distill such a simple model from standard quantum electrodynamics. We then discuss how many of those approximations can, and often have been broken in recent experiments. The consequence of these failures has been the need to abandon the Jaynes-Cummings model for more complex models. In this, the quantum Rabi model has the most prominent role and we will rapidly survey its rich and peculiar phenomenology. We conclude the paper by showing how the Jaynes-Cummings model still plays a crucial role even in non-perturbative light-matter coupling regimes.

quant-ph↗

arXiv2024

Bilateral photon emission from a vibrating mirror and multiphoton entanglement generation

Entanglement plays a crucial role in the development of quantum-enabled devices. One significant objective is the deterministic creation and distribution of entangled states, achieved, for example, through a mechanical oscillator interacting with confined electromagnetic fields. In this study, we explore a cavity resonator containing a two-sided perfect mirror. Although the mirror separates the cavity modes into two independent confined electromagnetic fields, the radiation pressure interaction gives rise to high-order effective interactions across all subsystems. Depending on the chosen resonant conditions, which are also related to the position of the mirror, we study $2n$-photon entanglement generation and bilateral photon pair emission. Demonstrating the non-classical nature of the mechanical oscillator, we provide a pathway to control these phenomena, opening potential applications in quantum technologies. Looking ahead, similar integrated devices could be used to entangle subsystems across vastly different energy scales, such as microwave and optical photons.

quant-ph↗

arXiv2024

Strong coupling between a single-photon and a two-photon Fock state

The realization of strong nonlinear coupling between single photons has been a long-standing goal in quantum optics and quantum information science, promising wide impact applications, such as all-optical deterministic quantum logic and single-photon frequency conversion. Here, we report an experimental observation of the strong coupling between a single-photon and a two-photon Fock state in an ultrastrongly-coupled circuit-QED system. This strong nonlinear interaction is realized by introducing a detuned flux qubit working as an effective coupler between two modes of a superconducting coplanar waveguide resonator. The ultrastrong light--matter interaction breaks the excitation number conservation, and an external flux bias breaks the parity conservation. The combined effect of the two enables the strong one--two-photon coupling. Quantum Rabi-like avoided crossing is resolved when tuning the two-photon resonance frequency of the first mode across the single-photon resonance frequency of the second mode. Within this new photonic regime, we observe the thresholdless second harmonic generation for a mean photon number below one. Our results represent a key step towards a new regime of quantum nonlinear optics, where individual photons can deterministically and coherently interact with each other in the absence of any stimulating fields.

quant-ph↗

arXiv2023

Phonon Pumping by Modulating the Ultrastrong Vacuum

The vacuum (i.e., the ground state) of a system in ultrastrong light-matter coupling contains particles that cannot be emitted without any dynamical perturbation and is thus called virtual. We propose a protocol for inducing and observing real mechanical excitations of a mirror enabled by the virtual photons in the ground state of a tripartite system, where a resonant optical cavity is ultrastrongly coupled to a two-level system (qubit) and, at the same time, optomechanically coupled to a mechanical resonator. Real phonons are coherently emitted when the frequency of the two-level system is modulated at a frequency comparable to that of the mechanical resonator and, therefore much lower than the optical frequency. We demonstrate that this hybrid effect is a direct consequence of the virtual photon population in the ground state. Within a classical physics analogy, attaching a weight to a spring only changes its resting position, whereas dynamically modulating the weight makes the system oscillate. In our case, however, the weight is the vacuum itself. We propose and accurately characterize a hybrid superconducting-optomechanical setup based on available state-of-the-art technology, where this effect can be experimentally observed.

quant-ph↗

arXiv2023

Photon condensation, Van Vleck paramagnetism, and chiral cavities

We introduce a gauge-invariant model of planar, square molecules coupled to a quantized spatially-varying cavity electromagnetic vector potential A(r). Specifically, we choose a temporally chiral cavity hosting a uniform magnetic field B, as this is the simplest instance in which a transverse spatially-varying A(r) is at play. We show that when the molecules are in the Van Vleck paramagnetic regime, an equilibrium quantum phase transition to a photon condensate state occurs.

cond-mat.mes-hall↗

arXiv2023

Ultrastrong Magnon-Photon Coupling Achieved by Magnetic Films in Contact with Superconducting Resonators

Coherent coupling between spin wave excitations (magnons) and microwave photons in a cavity may disclose new paths to unconventional phenomena as well as for novel applications. Here, we present a systematic investigation on YIG (Yttrium Iron Garnet) films on top of coplanar waveguide resonators made of superconducting YBCO. We first show that spin wave excitations with frequency higher than the Kittel mode can be excited by putting in direct contact a 5~$\mu$m thick YIG film with the YBCO coplanar resonator (cavity frequency $\omega_c/2 \pi = 8.65$~GHz). With this configuration, we obtain very large values of the collective coupling strength $\lambda/2 \pi \approx 2$~GHz and cooperativity $C=5 \times 10^4$. Transmission spectra are analyzed by a modified Hopfield model for which we provide an exact solution that allows us to well reproduce spectra by introducing a limited number of free parameters. It turns out that the coupling of the dominant magnon mode with photons exceeds 0.2 times the cavity frequency, thus demonstrating the achievement of the ultrastrong coupling regime with this architecture. Our analysis also shows a vanishing contribution of the diamagnetic term which is a peculiarity of pure spin systems.

cond-mat.mes-hall↗

arXiv2022

Flying atom back-reaction and mechanically generated photons from vacuum

We investigate the dynamics of a two-level atom flying through a photonic cavity when the light-matter interaction is in the ultrastrong coupling regime. We adopt a closed full quantum description that takes into account the quantization of the atom center-of-mass motion in addition to its internal degree of freedom and to the quantized photonic cavity field. We find that multiple qualitatively different dynamical regimes are achievable according to two key figures of merit: the ratio between the kinetic energy and the bare excitation energies, and the product of these bare energies with the time the atom takes to fly through the cavity. According to the values of those figures of merit, the atom can be reflected by the \emph{dressed} vacuum, or can convert part of its kinetic energy into real excitations which might be emitted out of the cavity. In the first case, the atom experiences a \emph{quantum regenerative braking} mechanism, based on temporary storage of energy into virtual excitations.

quant-ph↗

arXiv2022

Optomechanical Two-Photon Hopping

The hopping mechanism plays a key role in collective phenomena emerging in many-body physics. The ability to create and control systems that display this feature is important for next generation quantum technologies. Here we study two cavities separated by a vibrating two-sided perfect mirror and show that, within currently available experimental parameters, this system displays photon-pair hopping between the two electromagnetic resonators. In particular, the two-photon hopping is not due to tunneling, but rather to higher order resonant processes. Starting from the classical problem, where the vibrating mirror perfectly separates the two sides of the cavity, we quantize the system and then the two sides can interact. This opens the possibility to investigate a new mechanism of photon-pair propagation in optomechanical lattices.

quant-ph↗