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Alejandro Manjavacas

Publications and source records attributed to Alejandro Manjavacas.

At least 19 recordsLinked to original sources

Rotational Vacuum Friction of Nonabsorbing Particles

A nonabsorbing particle rotating in vacuum can lose angular momentum only by converting mechanical energy into electromagnetic radiation. Here, we develop a quantum theory of rotational vacuum friction for small lossless particles and show that axial symmetry qualitatively changes the leading dissipation channel. At zero temperature, the frictional torque scales as $M\proptoΩ^7$ with rotation frequency $\ Omega$ in anisotropic particles due to the emission of correlated photon pairs whose frequencies sum to $2Ω$, while a contribution to the torque linear in $\ Omega$ is found at finite temperature. In contrast, axisymmetric particles are protected against photon-assisted friction regardless of temperature.

quant-ph

Lattice Resonances in Periodic Arrays of Time-Modulated Scatterers

Lattice resonances are collective optical modes supported by periodic arrays of scatterers, arising from their coherent interaction enabled by the underlying periodicity. Owing to their collective nature, these resonances produce optical responses that are both stronger and spectrally narrower than those of individual scatterers. While such phenomena have been extensively studied in conventional time-invariant systems, recent advances in time-varying photonics present new opportunities to exploit and enhance the extraordinary characteristics of these collective modes. Here, we investigate lattice resonances in periodic arrays of time-modulated scatterers using a simple framework based on the dipolar approximation and time-Floquet theory, where each scatterer is modeled as a harmonic oscillator with periodically varying optical properties. We begin by analyzing the response of an individual scatterer, leveraging our model to identify the complex eigenfrequencies that define its dynamics. We show that, for the appropriate modulation amplitude and frequency, the imaginary part of one of these eigenfrequencies vanishes, leading to amplification. Building on this, we extend our analysis to a periodic array to investigate the effect of the interplay between temporal modulation and lattice resonances. In contrast to isolated scatterers, the collective nature of lattice resonances introduces a markedly more intricate spectral dependence of the amplification regime. Notably, this amplification emerges at substantially lower modulation strengths, facilitated by the enhanced light-matter interaction and increased lifetime provided by these collective resonances. Our work establishes a simple theoretical framework for understanding collective lattice resonances in time-modulated arrays, enabling dynamic control and amplification of these modes.

physics.optics

Quantum Nonlinear Response of Emitter Lattices

We theoretically investigate the emergence of quantum nonlinearities in the optical response of lattices of two-level quantum emitters coherently driven by a laser. For subwavelength lattice periods, where the system behaves as a quantum metasurface, we find that a resonant incident plane wave can populate excitonic Bloch states with parallel wavevectors different from the incident field, including those lying outside the light cone. Closely related to resonance fluorescence, the far-field emission from the system in the strong-driving regime is dominated by a broadband background of photons spanning a wide range of frequencies and wavevectors. Moreover, we show that, for periods approaching the driving wavelength, the emitter lattice enters in a bistable regime due to the renormalization of the driving rate, in striking contrast with its classical (bosonic) analog. This bistable behavior enables the selective activation and deactivation of the optical quantum nonlinearities of the system.

quant-ph

Synthetic crystal rotation with spacetime metamaterials

The interaction of light with rotating bodies has been historically limited to rotation frequencies much smaller than optical frequencies. Here, we investigate synthetic crystal rotations, i.e., spatiotemporal modulations mimicking the rotation of an anisotropic crystal, which grant access to large rotation frequencies. Spatiotemporal modulations change the fundamental symmetries of the electromagnetic field, breaking temporal and rotation symmetries, but preserving a spatiotemporal rotation symmetry that enforces the conservation of a combination of energy and spin angular momentum (SAM). The scattering of optical pulses by synthetically rotating crystals results in spatiotemporal light with intra-pulse SAM changes. The frequency-domain response reveals sidebands with frequency/SAM locking, and negative frequency sideband transitions for large enough rotation frequencies. Our results highlight the qualitatively different light-matter interaction regimes accessed by synthetic rotations.

physics.optics

Thermal Radiation Force and Torque on Moving Nanostructures with Anisotropic Optical Response

Nanoscale objects moving relative to a thermal radiation bath experience a drag force due to the imbalance in their interaction with the blue- and redshifted components of the electromagnetic field. Here, we show that, in addition to this drag force, moving nanostructures with an anisotropic optical response experience a lateral force and a torque that substantially modify their trajectory. These phenomena emerge from the additional coupling between the electromagnetic field components polarized parallel and perpendicular to the trajectory, enabled by the anisotropic response of the nanostructure. This work unveils the intricate dynamics of anisotropic nanostructures moving in a thermal radiation bath.

physics.optics

Chiral Light-Matter Interactions with Thermal Magnetoplasmons in Graphene Nanodisks

We investigate the emergence of self-hybridized thermal magnetoplasmons in doped graphene nanodisks at finite temperatures when subjected to an external magnetic field. Using a semianalytical approach, which fully describes the eigenmodes and polarizability of the graphene nanodisks, we show that the hybridization originates from the coupling of transitions between thermally populated Landau levels and localized magnetoplasmon resonances of the nanodisks. Owing to their origin, these modes combine the extraordinary magneto-optical response of graphene with the strong field enhancement of plasmons, making them an ideal tool for achieving strong chiral light-matter interactions, with the additional advantage of being tunable through carrier concentration, magnetic field, and temperature. As a demonstration of their capabilities, we show that the thermal magnetoplasmons supported by an array of graphene nanodisks enable chiral perfect absorption and chiral thermal emission.

cond-mat.mes-hall

Geometric Antibunching and Directional Shaping of Photon Anticorrelations

We investigate the directional characteristics of photon statistics in dimers of quantum emitters. For their analysis, we construct a two-point second-order correlation function that allows us to find a new mechanism for photon anticorrelation, termed as geometric antibunching. This phenomenon is completely agnostic to the quantum state of the emitters and emerges from quantum interference effects due to the indistinguishability of different two-photon optical pathways. Finally, we explore its occurrence in emitters placed in the vicinity of a flat substrate and a nanosphere, demonstrating its tunnability through the different material and geometric parameters of these structures.

quant-ph

Thermal radiation forces on planar structures with asymmetric optical response

Light carries momentum and, upon interaction with material structures, can exert forces on them. Here, we show that a planar structure with asymmetric optical response is spontaneously accelerated when placed in an environment at a different temperature. This phenomenon originates from the imbalance in the exchange rates of photons between both sides of the structure and the environment. Using a simple theoretical model, we calculate the force acting on the planar structure and its terminal velocity in vacuum, and analyze their dependence on the initial temperature and the geometrical properties of the system for different realistic materials. Our results unravel an alternative approach to manipulating objects in the nano and microscale that does not require an external source of radiation.

physics.optics

Control of the Radiative Heat Transfer in a Pair of Rotating Nanostructures

The fluctuations of the electromagnetic field are at the origin of the near-field radiative heat transfer between nanostructures, as well as the Casimir forces and torques that they exert on each other. Here, working within the formalism of fluctuational electrodynamics, we investigate the simultaneous transfer of energy and angular momentum in a pair of rotating nanostructures. We demonstrate that, due to the rotation of the nanostructures, the radiative heat transfer between them can be increased, decreased, or even reversed with respect to the transfer that occurs in absence of rotation, which is solely determined by the difference in the temperature of the nanostructures. This work unravels the unintuitive phenomena arising from the simultaneous transfer of energy and angular momentum in pairs of rotating nanostructures.

cond-mat.mes-hall

Green Tensor Analysis of Lattice Resonances in Periodic Arrays of Nanoparticles

When arranged in a periodic geometry, arrays of metallic nanostructures are capable of supporting collective modes known as lattice resonances. These modes, which originate from the coherent multiple scattering between the elements of the array, give rise to very strong and spectrally narrow optical responses. Here, we show that, thanks to their collective nature, the lattice resonances of a periodic array of metallic nanoparticles can mediate an efficient long-range coupling between dipole emitters placed near the array. Specifically, using a coupled dipole approach, we calculate the Green tensor of the array connecting two points and analyze its spectral and spatial characteristics. This quantity represents the electromagnetic field produced by the array at a given position when excited by a unit dipole emitter located at another one. We find that, when a lattice resonance is excited, the Green tensor is significantly larger and decays more slowly with distance than the Green tensor of vacuum. Therefore, in addition to advancing the fundamental understanding of lattice resonances, our results show that periodic arrays of nanostructures are capable of enhancing the long-range coupling between collections of dipole emitters, which makes them a promising platform for applications such as nanoscale energy transfer and quantum information processing.

physics.optics

Near-Field Radiative Heat Transfer Eigenmodes

The near-field electromagnetic interaction between nanoscale objects produces enhanced radiative heat transfer that can greatly surpass the limits established by far-field black-body radiation. Here, we present a theoretical framework to describe the temporal dynamics of the radiative heat transfer in ensembles of nanostructures, which is based on the use of an eigenmode expansion of the equations that govern this process. Using this formalism, we identify the fundamental principles that determine the thermalization of collections of nanostructures, revealing general but often unintuitive dynamics. Our results provide an elegant and precise approach to efficiently analyze the temporal dynamics of the near-field radiative heat transfer in systems containing a large number of nanoparticles.

cond-mat.mes-hall

Nanoscale transfer of angular momentum mediated by the Casimir torque

Casimir interactions play an important role in the dynamics of nanoscale objects. Here, we investigate the noncontact transfer of angular momentum at the nanoscale through the analysis of the Casimir torque acting on a chain of rotating nanoparticles. We show that this interaction, which arises from the vacuum and thermal fluctuations of the electromagnetic field, enables an efficient transfer of angular momentum between the elements of the chain. Working within the framework of fluctuational electrodynamics, we derive analytical expressions for the Casimir torque acting on each nanoparticle in the chain, which we use to study the synchronization of chains with different geometries and to predict unexpected dynamics, including a rattleback-like behavior. Our results provide new insights into the Casimir torque and how it can be exploited to achieve efficient noncontact transfer of angular momentum at the nanoscale, and therefore have important implications for the control and manipulation of nanomechanical devices.

cond-mat.mes-hall

High-harmonic generation from an epsilon-near-zero material

High-harmonic generation (HHG) from a compact, solid-state medium is highly desirable for applications such as coherent attosecond pulse generation and extreme ultra-violet (EUV) spectroscopy, yet the typically weak conversion of pump light to HHG can largely hinder its applications. Here, we use a material operating in its epsilon-near-zero (ENZ) region, where the real part of its permittivity vanishes, to greatly boost the efficiency of the HHG process at the microscopic level. In experiments, we report high-harmonic emission up to the 9th order directly from a low-loss, solid-state ENZ medium: indium-doped cadmium oxide, with an excitation intensity at the GW cm-2 level. Furthermore, the observed HHG signal exhibits a pronounced spectral red-shift as well as linewidth broadening, resulting from the photo-induced electron heating and the consequent time-dependent resonant frequency of the ENZ film. Our results provide a novel nanophotonic platform for strong field physics, reveal new degrees of freedom for spectral and temporal control of HHG, and open up possibilities of compact solid-state attosecond light sources.

physics.app-ph

Finite-Size Effects on Periodic Arrays of Nanostructures

Arrays of nanostructures have emerged as exceptional tools for the manipulation and control of light. Oftentimes, despite the fact that real implementations of nanostructure arrays must be finite, these systems are modeled as perfectly periodic, and therefore infinite. Here, we investigate the legitimacy of this approximation by studying the evolution of the optical response of finite arrays of nanostructures as their number of elements is increased. We find that the number of elements necessary to reach the infinite array limit is determined by the strength of the coupling between them, and that, even when that limit is reached, the individual responses of the elements may still display significant variations. In addition, we show that, when retardation is negligible, the resonance frequency for the infinite array is always redshifted compared to the single particle. However, in the opposite situation, there could be either a blue- or a redshift. We also study the effects of inhomogeneity in size and position of the elements on the optical response of the array. This work advances the understanding of the behavior of finite and infinite arrays of nanostructures, and therefore provides guidance to design applications that utilize these systems.

physics.optics

How To Identify Plasmons from the Optical Response of Nanostructures

A promising trend in plasmonics involves shrinking the size of plasmon-supporting structures down to a few nanometers, thus enabling control over light-matter interaction at extreme-subwavelength scales. In this limit, quantum mechanical effects, such as nonlocal screening and size quantization, strongly affect the plasmonic response, rendering it substantially different from classical predictions. For very small clusters and molecules, collective plasmonic modes are hard to distinguish from other excitations such as single-electron transitions. Using rigorous quantum mechanical computational techniques for a wide variety of physical systems, we describe how an optical resonance of a nanostructure can be classified as either plasmonic or nonplasmonic. More precisely, we define a universal metric for such classification, the generalized plasmonicity index (GPI), which can be straightforwardly implemented in any computational electronic-structure method or classical electromagnetic approach to discriminate plasmons from single-particle excitations and photonic modes. Using the GPI, we investigate the plasmonicity of optical resonances in a wide range of systems including: the emergence of plasmonic behavior in small jellium spheres as the size and the number of electrons increase; atomic-scale metallic clusters as a function of the number of atoms; and nanostructured graphene as a function of size and doping down to the molecular plasmons in polycyclic aromatic hydrocarbons. Our study provides a rigorous foundation for the further development of ultrasmall nanostructures based on molecular plasmonics

cond-mat.mes-hall

Lateral Casimir force on a rotating particle near a planar surface

We study the lateral Casimir force experienced by a particle that rotates near a planar surface. The origin of this force lies in the symmetry breaking induced by the particle rotation in the vacuum and thermal fluctuations of its dipole moment, and, therefore, in contrast to lateral Casimir forces previously described in the literature for corrugated surfaces, it exists despite the translational invariance of the planar surface. Working within the framework of fluctuational electrodynamics, we derive analytical expressions for the lateral force and analyze its dependence on the geometrical and material properties of the system. In particular, we show that the direction of the force can be controlled by adjusting the particle-surface distance, which may be exploited as a new mechanism to manipulate nanoscale objects.

cond-mat.other

Graphene optical-to-thermal converter

Infrared plasmons in doped graphene nanostructures produce large optical absorption that can be used for narrow-band thermal light emission at tunable frequencies that strongly depend on the doping charge. By virtue of Kirchhoff's law, thermal light emission is proportional to the absorption, thus resulting in narrow emission lines associated with the electrically controlled plasmons of heated graphene. Here we show that realistic designs of graphene plasmonic structures can release over 90% of the emission through individual infrared lines with 1% bandwidth. We examine anisotropic graphene structures in which efficient heating can be produced upon optical pumping tuned to a plasmonic absorption resonance situated in the blue region relative to the thermal emission. An incoherent thermal light converter is thus achieved. Our results open a radically different approach for designing tunable nanoscale infrared light sources.

cond-mat.mes-hall

Plasmonics in Atomically Thin Materials

The observation and electrical manipulation of infrared surface plasmons in graphene have triggered a search for similar photonic capabilities in other atomically thin materials that enable electrical modulation of light at visible and near-infrared frequencies, as well as strong interaction with optical quantum emitters. Here, we present a simple analytical description of the optical response of such kinds of structures, which we exploit to investigate their application to light modulation and quantum optics. Specifically, we show that plasmons in one-atom-thick noble-metal layers can be used both to produce complete tunable optical absorption and to reach the strong-coupling regime in the interaction with neighboring quantum emitters. Our methods are applicable to any plasmon-supporting thin materials, and in particular, we provide parameters that allow us to readily calculate the response of silver, gold, and graphene islands. Besides their interest for nanoscale electro-optics, the present study emphasizes the great potential of these structures for the design of quantum nanophotonics devices.

cond-mat.mes-hall