arXiv subjects

Alejandro W. Rodriguez

Publications and source records attributed to Alejandro W. Rodriguez.

At least 73 records · Page 4Linked to original sources

arXiv2017

Unifying microscopic and continuum treatments of van der Waals and Casimir interactions

We present an approach for computing long-range van der Waals (vdW) interactions between complex molecular systems and arbitrarily shaped macroscopic bodies, melding atomistic treatments of electronic fluctuations based on density functional theory in the former, with continuum descriptions of strongly shape-dependent electromagnetic fields in the latter, thus capturing many-body and multiple scattering effects to all orders. Such a theory is especially important when considering vdW interactions at mesoscopic scales, i.e. between molecules and structured surfaces with features on the scale of molecular sizes, in which case the finite sizes, complex shapes, and resulting nonlocal electronic excitations of molecules are strongly influenced by electromagnetic retardation and wave effects that depend crucially on the shapes of surrounding macroscopic bodies. We show that these effects together can modify vdW interactions by orders of magnitude compared to previous treatments based on Casimir--Polder or non-retarded approximations, which are valid only at macroscopically large or atomic-scale separations, respectively.

cond-mat.mes-hall↗

arXiv2017

Topology optimization of multi-track ring resonators and 2D microcavities for nonlinear frequency conversion

We exploit recently developed topology-optimization techniques to design complex, wavelength-scale resonators for enhancing various nonlinear $χ^{(2)}$ and $χ^{(3)}$ frequency conversion processes. In particular, we demonstrate aperiodic, multi-track ring resonators and 2D slab microcavities exhibiting long lifetimes $Q \gtrsim 10^4$, small modal volumes $V \gtrsim (λ/2n)^3$, and among the largest nonlinear overlaps (a generalization of phase matching in large-etalon waveguides) possible, paving the way for efficient, compact, and wide-bandwdith integrated nonlinear devices.

physics.optics↗

arXiv2016

Exact formulas for radiative heat transfer between planar bodies under arbitrary temperature profiles: modified asymptotics and sign-flip transitions

We derive exact analytical formulas for the radiative heat transfer between parallel slabs separated by vacuum and subject to arbitrary temperature profiles. We show that, depending on the derivatives of the temperature at points close to the slab--vacuum interfaces, the flux can exhibit one of several different asymptotic low-distance ($d$) behaviors, obeying either $1/d^2$, $1/d$, or logarithmic power laws, or approaching a constant. Tailoring the temperature profile within the slabs could enable unprecedented tunability over heat exchange, leading for instance to sign-flip transitions (where the flux reverses sign) at tunable distances. Our results are relevant to the theoretical description of on-going experiments exploring near-field heat transfer at nanometric distances, where the coupling between radiative and conductive heat transfer could be at the origin of temperature gradients.

cond-mat.mes-hall↗

arXiv2016

General formulation of coupled radiative and conductive heat transfer between compact bodies

We present a general framework for studying strongly coupled radiative and conductive heat transfer between arbitrarily shaped bodies separated by sub-wavelength distances. Our formulation is based on a macroscopic approach that couples our recent fluctuating volume--current (FVC) method of near-field heat transfer to the more well known Fourier conduction transport equation. We apply our technique to consider heat exchange between aluminum-zinc oxide nanorods and show that the presence of bulk plasmon resonances can result in extremely large radiative heat transfer rates (roughly twenty times larger than observed in planar geometries), whose interplay with conductive transport leads to nonlinear temperature profiles along the nanorods.

cond-mat.mes-hall↗

arXiv2016

Strongly coupled near-field radiative and conductive heat transfer between planar objects

We study the interplay of conductive and radiative heat transfer (RHT) in planar geometries and predict that temperature gradients induced by radiation can play a significant role on the behavior of RHT with respect to gap sizes, depending largely on geometric and material parameters and not so crucially on operating temperatures. Our findings exploit rigorous calculations based on a closed-form expression for the heat flux between two plates separated by vacuum gaps $d$ and subject to arbitrary temperature profiles, along with an approximate but accurate analytical treatment of coupled conduction--radiation in this geometry. We find that these effects can be prominent in typical materials (e.g. silica and sapphire) at separations of tens of nanometers, and can play an even larger role in metal oxides, which exhibit moderate conductivities and enhanced radiative properties. Broadly speaking, these predictions suggest that the impact of RHT on thermal conduction, and vice versa, could manifest itself as a limit on the possible magnitude of RHT at the nanoscale, which asymptotes to a constant (the conductive transfer rate when the gap is closed) instead of diverging at short separations.

cond-mat.mes-hall↗

arXiv2016

Giant frequency-selective near-field energy transfer in active--passive structures

We apply a fluctuation electrodynamics framework in combination with semianalytical (dipolar) approximations to study amplified spontaneous energy transfer (ASET) between active and passive bodies. We consider near-field energy transfer between semi-infinite planar media and spherical structures (dimers and lattices) subject to gain, and show that the combination of loss compensation and near-field enhancement (achieved by the proximity, enhanced interactions, and tuning of subwavelength resonances) in these structures can result in orders of magnitude ASET enhancements below the lasing threshold. We examine various possible geometric configurations, including realistic materials, and describe optimal conditions for enhancing ASET, showing that the latter depends sensitively on both geometry and gain, enabling efficient and tunable gain-assisted energy extraction from structured surfaces.

cond-mat.mes-hall↗

arXiv2016

Inverse design of third-order Dirac exceptional points in photonic crystals

We propose a novel inverse-design method that enables brute-force discovery of photonic crystal (PhC) structures with complex spectral degeneracies. As a proof of principle, we demonstrate PhCs exhibiting third-order Dirac points formed by the \emph{accidental} degeneracy of modes of monopolar, dipolar, and quadrupolar nature. We show that under suitable conditions, these modes can coalesce and form a third-order exceptional point (EP3), leading to diverging Petermann factors. We show that the spontaneous emission (SE) rate of emitters at such EP3s, related to the local density of states, can be enhanced by a factor of 8 in purely lossy (passive) structures, with larger enhancements $\sim \sqrt{n^3}$ possible at exceptional points of higher order $n$ or in materials with gain.

physics.optics↗

arXiv2016

Non-additivity of van der Waals forces on liquid surfaces

We present an approach for modeling nanoscale wetting and dewetting of liquid surfaces that exploits recently developed, sophisticated techniques for computing van der Waals (vdW) or (more generally) Casimir forces in arbitrary geometries. We solve the variational formulation of the Young--Laplace equation to predict the equilibrium shapes of fluid--vacuum interfaces near solid gratings and show that the non-additivity of vdW interactions can have a significant impact on the shape and wetting properties of the liquid surface, leading to very different surface profiles and wetting transitions compared to predictions based on commonly employed additive approximations, such as Hamaker or Derjaguin approximations.

cond-mat.soft↗

arXiv2015

Amplified and directional spontaneous emission from arbitrary composite bodies: self-consistent treatment of Purcell effect below threshold

We study amplified spontaneous emission (ASE) from wavelength-scale composite bodies--complicated arrangements of active and passive media--demonstrating highly directional and tunable radiation patterns, depending strongly on pump conditions, materials, and object shapes. For instance, we show that under large enough gain, $\mathcal{PT}$ symmetric dielectric spheres radiate mostly along either active or passive regions, depending on the gain distribution. Our predictions are based on a recently proposed fluctuating volume--current (FVC) formulation of electromagnetic radiation that can handle inhomogeneities in the dielectric and fluctuation statistics of active media, e.g. arising from the presence of non-uniform pump or material properties, which we exploit to demonstrate an approach to modelling ASE in regimes where Purcell effect (PE) has a significant impact on the gain, leading to spatial dispersion and/or changes in power requirements. The nonlinear feedback of PE on the active medium, captured by the Maxwell--Bloch equations but often ignored in linear formulations of ASE, is introduced into our linear framework by a self-consistent renormalization of the (dressed) gain parameters, requiring the solution of a large system of nonlinear equations involving many linear scattering calculations.

cond-mat.mes-hall↗

arXiv2015

Giant near-field mediated heat flux at the nanometer scale

In this Letter, we report on quantitative measurements of the absolute near-field mediated heat flux between a gold coated near-field scanning thermal microscope (NSThM) tip and a planar gold sample at nanometer distances of 0.2 nm- 7 nm. We find an extraordinary large heat flux which is more than five orders of magnitude larger than black-body radiation and four orders of magnitude larger than the values predicted by conventional theory of fluctuational electrodynamics. Additionally, we compare our data with different theories of phonon tunneling which might explain a drastically increased heat flux, but are found not to be able to reproduce the distance dependence observed in our experiment. The findings demand modified or even new models of heat transfer across vacuum gaps at nanometer distances.

cond-mat.mes-hall↗

arXiv2015

Shape-Independent Limits to Near-Field Radiative Heat Transfer

We derive shape-independent limits to the spectral radiative heat-transfer rate between two closely spaced bodies, generalizing the concept of a black body to the case of near-field energy transfer. Through conservation of energy and reciprocity, we show that each body of susceptibility $χ$ can emit and absorb radiation at enhanced rates bounded by $|χ|^2 / \textrm{Im} χ$, optimally mediated by near-field photon transfer proportional to $1/d^2$ across a separation distance $d$. Dipole--dipole and dipole--plate structures approach restricted versions of the limit, but common large-area structures do not exhibit the material enhancement factor and thus fall short of the general limit. By contrast, we find that particle arrays interacting in an idealized Born approximation (i.e., neglecting multiple scattering) exhibit both enhancement factors, suggesting the possibility of orders-of-magnitude improvement beyond previous designs and the potential for radiative heat transfer to be comparable to conductive heat transfer through air at room temperature, and significantly greater at higher temperatures.

physics.optics↗

arXiv2015

Dynamical laser spike processing

Novel materials and devices in photonics have the potential to revolutionize optical information processing, beyond conventional binary-logic approaches. Laser systems offer a rich repertoire of useful dynamical behaviors, including the excitable dynamics also found in the time-resolved "spiking" of neurons. Spiking reconciles the expressiveness and efficiency of analog processing with the robustness and scalability of digital processing. We demonstrate that graphene-coupled laser systems offer a unified low-level spike optical processing paradigm that goes well beyond previously studied laser dynamics. We show that this platform can simultaneously exhibit logic-level restoration, cascadability and input-output isolation---fundamental challenges in optical information processing. We also implement low-level spike-processing tasks that are critical for higher level processing: temporal pattern detection and stable recurrent memory. We study these properties in the context of a fiber laser system, but the addition of graphene leads to a number of advantages which stem from its unique properties, including high absorption and fast carrier relaxation. These could lead to significant speed and efficiency improvements in unconventional laser processing devices, and ongoing research on graphene microfabrication promises compatibility with integrated laser platforms.

physics.optics↗

arXiv2015

Temperature control of thermal radiation from heterogeneous bodies

We demonstrate that recent advances in nanoscale thermal transport and temperature manipulation can be brought to bear on the problem of tailoring thermal radiation from compact emitters. We show that wavelength-scale composite bodies involving complicated arrangements of phase-change chalcogenide (GST) glasses and metals or semiconductors can exhibit large emissivities and partial directivities at mid-infrared wavelengths, a consequence of temperature localization within the GST. We consider multiple object topologies, including spherical, cylindrical, and mushroom-like composites, and show that partial directivity follows from a complicated interplay between particle shape, material dispersion, and temperature localization. Our calculations exploit a recently developed fluctuating-volume current formulation of electromagnetic fluctuations that rigorously captures radiation phenomena in structures with both temperature and dielectric inhomogeneities.

cond-mat.mes-hall↗

arXiv2015

Cavity-enhanced second harmonic generation via nonlinear-overlap optimization

We describe an approach based on topology optimization that enables automatic discovery of wavelength-scale photonic structures for achieving high-efficiency second-harmonic generation (SHG). A key distinction from previous formulation and designs that seek to maximize Purcell factors at individual frequencies is that our method not only aims to achieve frequency matching (across an entire octave) and large radiative lifetimes, but also optimizes the equally important nonlinear--coupling figure of merit $\barβ$, involving a complicated spatial overlap-integral between modes. We apply this method to the particular problem of optimizing micropost and grating-slab cavities (one-dimensional multilayered structures) and demonstrate that a variety of material platforms can support modes with the requisite frequencies, large lifetimes $Q > 10^4$, small modal volumes $\sim (λ/n)^3$, and extremely large $\barβ \gtrsim 10^{-2}$, leading to orders of magnitude enhancements in SHG efficiency compared to state of the art photonic designs. Such giant $\barβ$ alleviate the need for ultra-narrow linewidths and thus pave the way for wavelength-scale SHG devices with faster operating timescales and higher tolerance to fabrication imperfections.

physics.optics↗

arXiv2015

Ab-initio multimode linewidth theory for arbitrary inhomogeneous laser cavities

We present a multimode laser-linewidth theory for arbitrary cavity structures and geometries that contains nearly all previously known effects and also finds new nonlinear and multimode corrections, e.g. a bad-cavity correction to the Henry $α$ factor and a multimode Schawlow--Townes relation (each linewidth is proportional to a sum of inverse powers of all lasing modes). Our theory produces a quantitatively accurate formula for the linewidth, with no free parameters, including the full spatial degrees of freedom of the system. Starting with the Maxwell--Bloch equations, we handle quantum and thermal noise by introducing random currents whose correlations are given by the fluctuation--dissipation theorem. We derive coupled-mode equations for the lasing-mode amplitudes and obtain a formula for the linewidths in terms of simple integrals over the steady-state lasing modes.

physics.optics↗

arXiv2015

Design of diamond microcavities for single photon frequency down-conversion

We propose monolithic diamond cavities that can be used to convert color-center Fock-state single photons from emission wavelengths to telecommunication bands. We present a detailed theoretical description of the conversion process, analyzing important practical concerns such as nonlinear phase shifts and frequency mismatch. Our analysis predicts sustainable power requirements ($ \lesssim 1~\mathrm{W}$) for a chipscale nonlinear device with high conversion efficiencies.

physics.optics↗

arXiv2015

Thermal radiation from optically driven Kerr ($χ^{(3)}$) photonic cavities

We study thermal radiation from nonlinear ($χ^{(3)}$) photonic cavities coupled to external channels and subject to incident monochromatic light. Our work extends related work on nonlinear mechanical oscillators [Phys. Rev. Lett. 97, 110602 (2006)] to the problem of thermal radiation, demonstrating that bistability can enhance thermal radiation by orders of magnitude and result in strong lineshape alternations, including "super-narrow spectral peaks" occurring at the onset of kinetic phase transitions. We show that when the cavities are designed so as to have perfect linear absorptivity (rate matching), such thermally activated transitions can be exploited to dramatically tune the output power and radiative properties of the cavity, leading to a kind of Kerr-mediated thermo-optic effect. Finally, we demonstrate that in certain parameter regimes, the output radiation exhibits Stokes and anti-Stokes side peaks whose relative magnitudes can be altered by tuning the internal temperature of the cavity relative to its surroundings, a consequence of strong correlations and interference between the emitted and reflected radiation.

cond-mat.mes-hall↗

arXiv2015

Radiative heat transfer in nonlinear Kerr media

We obtain a fluctuation--dissipation theorem describing thermal electromagnetic fluctuation effects in nonlinear media that we exploit in conjunction with a stochastic Langevin framework to study thermal radiation from Kerr ($χ^{(3)}$) photonic cavities coupled to external environments at and out of equilibrium. We show that that in addition to thermal broadening due to two-photon absorption,the emissivity of such cavities can exhibit asymmetric,non-Lorentzian lineshapes due to self-phase modulation. When the local temperature of the cavity is larger than that of the external bath, we find that the heat transfer into the bath exceeds the radiation from a corresponding linear black body at the same local temperature. We predict that these temperature-tunable thermal processes can be observed in practical, nanophotonic cavities operating at relatively small temperatures.

cond-mat.mes-hall↗