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Aleksa Krstić

Publications and source records attributed to Aleksa Krstić.

4 recordsLinked to original sources

Toward Spectral Engineering of Squeezed Light in High-Gain PDC

We investigated the spectral properties of squeezed light generated via parametric down-conversion in the high-gain regime, considering both unapodized and apodized dispersion-engineered waveguides. The gain-dependent evolution of these states is examined starting from the low-gain regime, which includes both highly correlated and nearly uncorrelated cases. For the unapodized configuration, we observe a monotonic increase in spectral purity with gain, whereas the apodized configuration exhibits a nonmonotonic dependence, initially decreasing and then recovering at higher gain. By combining Schmidt-mode analysis with a group-velocity-based interpretation, we explain why different dispersion conditions exhibit distinct gain-dependent behavior, specifically that rapid purification occurs when the pump group velocity lies between those of the signal and idler. Our study shows that the evolution of spectral purity is governed primarily by the underlying dispersion of the waveguide. These results demonstrate that dispersion engineering and parametric gain can be jointly exploited to tailor the spectral-mode structure of squeezed-light sources, enabling their optimization for a broad range of quantum applications.

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Enhancing entangled two-photon absorption of Nile Red via temperature-controlled SPDC

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or photolithography with high axial resolution at minimal exposure intensities. However, most experimental studies on two-photon absorption were not able to show an unambiguous proof of fluorescence emission driven by entangled photon pairs. On the other hand, existing theoretical models struggle to accurately predict the entangled two-photon absorption behavior of chemically complex dyes. In this paper, we introduce an approach to simulate entangled two-photon absorption in common fluorescence dyes considering their chemical properties. Our theoretical model allows a deeper understanding of experimental results and thus the occurrence of entangled two-photon absorption. In particular, we found a remarkable dependency of the absorption probability on the phase-matching temperature of the nonlinear material. Further, we compared results of our theoretical approach to experimental data for Nile Red.

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A hybrid source of quantum light for generation of frequency tunable Fock states

We propose a scheme for quantum-light generation in a nonlinear cavity hybridized with a 2-level system and theoretically show that, when excited by a series of controlled pump pulses, the hybrid source generates Fock states with high probabilities. E.g., 1- and 2-photon states can be generated near-on-demand, and Fock states with up to $7$ photons with a probability above $50\%$. The tailorable nature of the nonlinear cavity allows for generating Fock states with arbitrary frequencies, even with a fixed 2-level system, creating fundamentally new opportunities in all areas of quantum technologies.

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Non-perturbative theory of spontaneous parametric down-conversion in open and dispersive optical systems

We develop a non-perturbative formulation based on the Green-function quantization method, that can describe spontaneous parametric down-conversion in the high-gain regime in nonlinear optical structures with arbitrary amount of loss and dispersion. This formalism opens the way for description and design of arbitrary complex and/or open nanostructured nonlinear optical systems in quantum technology applications, such as squeezed-light generation, nonlinearity-based quantum sensing, and hybrid quantum systems mediated by nonlinear interactions. As an example case, we numerically investigate the scenario of integrated quantum spectroscopy with undetected photons, in the high-gain regime, and uncover novel gain-dependent effects in the performance of the system.

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