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Alessandro Fedrizzi

Publications and source records attributed to Alessandro Fedrizzi.

At least 19 recordsLinked to original sources

Multi-parameter two-photon polarimetry at the quantum limit

Photonic quantum metrology has demonstrated advantages in precision and resource efficiency for a wide range of applications, with several schemes approaching the fundamental quantum Cram\'er-Rao precision bound (QCRB). However, the intrinsic incompatibility of quantum measurements represents a hurdle in extending these advantages to the simultaneous estimation of multiple parameters. In this paper, we present an experimental protocol approaching the QCRB simultaneously in two polarisation parameters, across a wide range of the parameter space, with as few as $\sim 200$ photon pairs, offering advantages for polarimetric sensing for dim sources such as in X-ray astronomy or photosensitive samples.

quant-ph

Twist-Engineered Nonlinearity in Two-Dimensional Crystals for Tailored Quantum Light

Van der Waals (vdW) materials enable nonlinear-optical engineering with unprecedented resolution: their strong second-order susceptibilities ($\chi^{(2)}$) and twist-tunable interlayer symmetry allow the effective nonlinearity to be shaped continuously, rather than through binary $\pm\chi^{(2)}$ domain inversion as in bulk ferroelectrics. Here, we show that twist-angle domain engineering exploits this continuous degree of freedom to reconstruct target longitudinal nonlinearity profiles with high fidelity. Using spontaneous parametric down-conversion (SPDC) as a benchmark, we demonstrate that twist-engineered vdW crystals yield significantly improved approximations of target phase-matching functions and correspondingly higher single-photon purities, particularly in compact devices where fabrication constraints limit conventional approaches. We further show that this framework remains effective in experimentally relevant vdW materials and demanding non-degenerate wavelength regimes involving mid-infrared photons. More broadly, the ability to continuously and locally program $\chi^{(2)}$ establishes a general framework for tailoring a wide range of SPDC properties, including absolute brightness, joint spectral amplitude structure, signal-idler frequency separation, and temporal wavepacket shape beyond what is accessible in conventional nonlinear crystals. These results position vdW heterostructures as a powerful platform for engineered quantum light sources and open new opportunities for nonlinear-optical devices shaped with monolayer thickness scale.

physics.optics

Decoy-state quantum key distribution over 227 km with a frequency-converted telecom single-photon source

We implement a decoy-state quantum key distribution scheme using a telecom C-band single-emitter source. The decoy states are created by varying the optical excitation of the quantum emitter to modulate the photon number distribution. We provide an analysis of our scheme based on existing security proofs, allowing the calculation of secret key rates including finite key effects. This enables us to demonstrate, with a realistic single-photon source, positive secret key rates using our scheme over 227 km of optical fiber, equivalent to a loss tolerance one order of magnitude greater than non-decoy schemes. This work broadens the scope of single-photon sources in future quantum networks by enabling long-distance QKD with realistic levels of single-photon purity.

quant-ph

Optimised spectral purity of unfiltered photons via pump and nonlinearity shaping

Photonic quantum technologies rely on the efficient generation and interference of indistinguishable photons. Exceptional achievements in this respect have been obtained by domain engineering of quasi-phase-matched parametric down-conversion sources, demonstrating high two-photon interference visibility using only moderate bandpass spectral filtering. Here, we optimised the spectral purity and indistinguishability of photons from telecom-wavelength sources by combining Gaussian quasi-phase-matching with Gaussian pump spectral shaping. Without spectral filtering, we used time-of-flight spectrometry to estimate an upper bound spectral purity of 99.9272(6)%, and achieved visibilities of up to 98.5(8)% in two-photon interference experiments with independent sources.

quant-ph

Quantum-limited optical delay sensing across an enhanced dynamic range by frequency-resolving two-photon interference

Optical sensing schemes that rely on two-photon interference provide a powerful platform for precision metrology, although they are inherently constrained by a trade-off between dynamic range and measurement precision. To overcome this limitation, we sample the frequencies of two interfering photons, which extends the sensitivity in the time domain. This enhances the dynamic range of optical delay estimation by up to twenty times compared to the non-resolved estimates. We demonstrate this approach with independent photon sources and show the behaviour of finite frequency resolving detectors. This technique enables scan-free nanometre resolution depth sensing over a millimetre-scale range, with applications in biological and nanomaterial imaging.

quant-ph

Emulation of satellite up-link quantum communication with entangled photons

Quantum communication rates in terrestrial quantum networks are fundamentally limited by fibre loss, even in the presence of quantum repeaters. Satellites offer a solution for long-distance communication, with the most commonly explored scenario involving prepare-and-measure protocols connecting from orbit to a trusted-node ground station via free-space down-links. In contrast, up-link scenarios allow for entanglement to be distributed between a satellite and remote end users in terrestrial networks, eliminating any trust requirement on the ground station. Here we demonstrate an ultra-bright source of far-non-degenerate entangled photons and perform quantum key distribution in emulated high-loss satellite scenarios. With a loss profile corresponding to that of one of the pioneering Micius up-link experiments, and a terrestrial end user separated by 10~km of telecom fibre we achieve secure key bit accumulation of 5.2~kbit in a single emulated overpass in the asymptotic limit. Our results confirm the viability of upcoming low-Earth orbit receiver satellite missions.

quant-ph

A Large-Scale Reconfigurable Multiplexed Quantum Photonic Network

Entanglement distribution in quantum networks will enable next-generation technologies for quantum-secured communications, distributed quantum computing and sensing. Future quantum networks will require dense connectivity, allowing multiple users to share entanglement in a reconfigurable and multiplexed manner, while long-distance connections are established through the teleportation of entanglement, or entanglement swapping. While several recent works have demonstrated fully connected, local multi-user networks based on multiplexing, extending this to a global network architecture of interconnected local networks remains an outstanding challenge. Here we demonstrate the next stage in the evolution of multiplexed quantum networks: a prototype global reconfigurable network where entanglement is routed and teleported in a flexible and multiplexed manner between two local multi-user networks composed of four users each. At the heart of our network is a programmable 8x8-dimensional multi-port circuit that harnesses the natural mode-mixing process inside a multi-mode fibre to implement on-demand high-dimensional operations on two independent photons carrying eight transverse-spatial modes. Our circuit design allows us to break away from the limited planar geometry and bypass the control and fabrication challenges of conventional integrated photonic platforms. Our demonstration showcases the potential of this architecture for enabling large-scale, global quantum networks that offer versatile connectivity while being fully compatible with an existing communications infrastructure.

quant-ph

Quantum-private distributed sensing

Quantum networks can enhance both security and privacy conditions for multi-user communication, delegated computation, and distributed sensing tasks. An example quantum protocol is private parameter estimation (PPE) where only the aggregate information is accessible while individual sensor data remain confidential. Specifically, the protocol enables the estimation of a global function of remote sensor parameters without revealing local parameters to any entity. We implement the PPE protocol by distributing a three-photon Greenberger-Horne-Zeilinger (GHZ) state, among three sensors, which is verified using stabilizer measurements to establish privacy and precision bounds for the sensing task. We demonstrate Heisenberg-limited precision scaling of the global parameter while suppressing the metrological information of the local parameters by up to three orders of magnitude. This work, which integrates privacy in distributed quantum sensing, marks a crucial step towards developing advanced quantum-secure-and-private protocols in complex quantum networks.

quant-ph

Purifying quantum-dot light in a coherent frequency interface

Quantum networks typically operate in the telecom wavelengths to take advantage of low-loss transmission in optical fibres. However, bright quantum dots (QDs) emitting highly indistinguishable quantum states of light, such as InGaAs QDs, often emit photons in the near infrared thus necessitating frequency conversion (FC) to the telecom band. Furthermore, the signal quality of quantum emissions is crucial for the effective performance of these networks. In this work we report a method for simultaneously implementing spectral purification and frequency shifting of single photons from QD sources to the C-band in a periodically poled Lithium Niobate waveguide. We consider difference frequency generation in the counter-propagating configuration to implement FC with the output emission bandwidth in units of GHz. Our approach establishes a clear path to integrating high-performance single-emitter sources in a hybrid quantum network.

quant-ph

Guarantees on the structure of experimental quantum networks

Quantum networks connect and supply a large number of nodes with multi-party quantum resources for secure communication, networked quantum computing and distributed sensing. As these networks grow in size, certification tools will be required to answer questions regarding their properties. In this work we demonstrate a general method to guarantee that certain correlations cannot be generated in a given quantum network. We apply quantum inflation methods to data obtained in quantum group encryption experiments, guaranteeing the impossibility of producing the observed results in networks with fewer optical elements. Our results pave the way for scalable methods of obtaining device-independent guarantees on the network structure underlying multipartite quantum protocols.

quant-ph

Experimental anonymous quantum conferencing

Anonymous quantum conference key agreement (AQCKA) allows a group of users within a network to establish a shared cryptographic key without revealing their participation. Although this can be achieved using bi-partite primitives alone, it is costly in the number of network rounds required. By allowing the use of multi-partite entanglement, there is a substantial efficiency improvement. We experimentally implement the AQCKA task in a six-user quantum network using Greenberger-Horne-Zeilinger (GHZ)-state entanglement and obtain a significant resource cost reduction in line with theory when compared to a bi-partite-only approach. We also demonstrate that the protocol retains an advantage in a four-user scenario with finite key effects taken into account.

quant-ph

Photonic implementation of the quantum Morra game

In this paper, we study a faithful translation of a two-player quantum Morra game, which builds on previous work by including the classical game as a special case. We propose a natural deformation of the game in the quantum regime in which Alice has a winning advantage, breaking the balance of the classical game. A Nash equilibrium can be found in some cases by employing a pure strategy, which is impossible in the classical game where a mixed strategy is always required. We prepared our states using photonic qubits on a linear optics setup, with an average deviation less than 2% with respect to the measured outcome probabilities. Finally, we discuss potential applications of the quantum Morra game to the study of quantum information and communication.

quant-ph

Entanglement-induced collective many-body interference

Entanglement and interference are both hallmark effects of quantum physics. Particularly rich dynamics arise when multiple (at least partially) indistinguishable particles are subjected to either of these phenomena. By combining both entanglement and many-particle interference, we propose an interferometric setting through which N-particle interference can be observed, while any interference of lower orders is strictly suppressed. We experimentally demonstrate this effect in a four-photon interferometer, where the interference is nonlocal, in principle, as only pairs of photons interfere at two separate and independent beam splitters. A joint detection of all four photons identifies a high-visibility interference pattern varying as a function of their collective four-particle phase, a genuine four-body property.

quant-ph

Conference key agreement in a quantum network

Quantum conference key agreement (QCKA) allows multiple users to establish a secure key from a shared multi-partite entangled state. In a quantum network, this protocol can be efficiently implemented using a single copy of a N-qubit Greenberger-Horne-Zeilinger (GHZ) state to distil a secure N-user conference key bit, whereas up to N-1 entanglement pairs are consumed in the traditional pair-wise protocol. We demonstrate the advantage provided by GHZ states in a testbed consisting of a photonic six-user quantum network, where four users can distil either a GHZ state or the required number of Bell pairs for QCKA using network routing techniques. In the asymptotic limit, we report a more than two-fold enhancement of the conference key rate when comparing the two protocols. We extrapolate our data set to show that the resource advantage for the GHZ protocol persists when taking into account finite-key effects.

quant-ph

Hyper-entanglement between pulse modes and frequency bins

Hyper-entanglement between two or more photonic degrees of freedom (DOF) can enhance and enable new quantum protocols by allowing each DOF to perform the task it is optimally suited for. Here we demonstrate the generation of photon pairs hyper-entangled between pulse modes and frequency bins. The pulse modes are generated via parametric downconversion in a domain-engineered crystal and subsequently entangled to two frequency bins via a spectral mapping technique. The resulting hyper-entangled state is characterized and verified via measurement of its joint spectral intensity and non-classical two-photon interference patterns from which we infer its spectral phase. The protocol combines the robustness to loss, intrinsic high dimensionality and compatibility with standard fiber-optic networks of the energy-time DOF with the ability of hyper-entanglement to increase the capacity and efficiency of the quantum channel, already exploited in recent experimental applications in both quantum information and quantum computation.

quant-ph

Single-emitter quantum key distribution over 175 km of fiber with optimised finite key rates

Quantum key distribution with solid-state single-photon emitters is gaining traction due to their rapidly improving performance and compatibility with future quantum network architectures. In this work, we perform fibre-based quantum key distribution with a quantum dot frequency-converted to telecom wavelength, achieving count rates of 1.6 MHz with $g^{\left(2\right)}\left(0\right) = 3.6 \%$. We demonstrate positive key rates up to 175 km in the asymptotic regime. We then show that the community standard analysis for non-decoy state QKD drastically overestimates the acquisition time required to generate secure finite keys. Our improved analysis using the multiplicative Chernoff bound reduces the required number of received signals by a factor of $10^8$ over existing work, with the finite key rate approaching the asymptotic limit at all achievable distances for acquisition times of one hour. Over a practical distance of 100 km we achieve a finite key rate of 13 kbps after one minute of integration time. This result represents major progress towards the feasibility of long-distance single-emitter QKD networks.

quant-ph

Experimental demonstration of optimal unambiguous two-out-of-four quantum state elimination

A core principle of quantum theory is that non-orthogonal quantum states cannot be perfectly distinguished with single-shot measurements. However, it is possible to exclude a subset of non-orthogonal states without error in certain circumstances. Here we implement a quantum state elimination measurement which unambiguously rules out two of four pure, non-orthogonal quantum states -- ideally without error and with unit success probability. This is a generalised quantum measurement with six outcomes, where each outcome corresponds to excluding a pair of states. Our experimental realisation uses single photons, with information encoded in a four-dimensional state using optical path and polarisation degrees of freedom. The prepared state is incorrectly ruled out up to $3.3(2)\%$ of the time.

quant-ph

Frequency-bin entanglement from domain-engineered down-conversion

Frequency encoding is quickly becoming an attractive prospect for quantum information protocols owing to larger Hilbert spaces and increased resilience to noise compared to other photonic degrees of freedom. To fully make use of frequency encoding as a practical paradigm for QIP, an efficient and simple source of frequency entanglement is required. Here we present a single-pass source of discrete frequency-bin entanglement which does not use filtering or a resonant cavity. We use a domain-engineered nonlinear crystal to generate an eight-mode frequency-bin entangled source at telecommunication wavelengths. Our approach leverages the high heralding efficient and simplicity associated with bulk crystal sources.

quant-ph