arXiv subjects

Alessandro Maffini

Publications and source records attributed to Alessandro Maffini.

4 recordsLinked to original sources

arXiv2025

Numerical proof-of-concept of a photon, proton, and positron laser-driven source with nanostructured targets

A source of high-energy photons, ions, and positrons can be attained with the interaction of ultra-intense femtosecond laser pulses with advanced nanostructured targets. We present and characterise a numerical model that mimics the foam deposition process on solid substrates, as it occurs in Double-Layer Target (DLT) manufacturing. The model is integrated into Particle-In-Cell (PIC) simulations in full 3D geometry to study electron acceleration, consequent high-energy photon emission, proton acceleration, and pair production with realistic target and laser parameters. We highlight the importance of realistic foam morphology modelling even at high-laser intensity and the need for specific optimisation of target parameters with realistic PIC simulations to improve radiation production efficiency. Our study shows that the DLT could be a compact multi-purpose scheme to achieve high-brightness photons and high-energy protons and to observe and optimise non-linear Breit-Wheeler pair production.

physics.plasm-ph↗

arXiv2024

Ballistic-aggregated Carbon Nanofoam in Target-side of Pulsed Laser Deposition for Energy Storage Applications

In pulsed laser deposition, along the traditionally exploited deposition on the front-side of the plasma-plume, a coating forms on the surface of the target as well. For reproducibility, this residue is usually cleaned and discarded. Here we instead investigate the target-side coated materials and employ them as a binder-free supercapacitor electrode. The ballistic-aggregated, target-side nanofoam is compact and features a larger fraction of sp2-carbon, higher nitrogen content with higher graphitic-N and lower oxygen content with fewer COOH groups than that of diffusive-aggregated conventional nanofoams. They are highly hydrogenated graphite-like amorphous carbon and superhydrophilic. The resulting symmetric micro-supercapacitor delivers higher volumetric capacitance of 522 mF/cm3 at 100 mV/s and 104% retention after 10000 charge-discharge cycles over conventional nanofoam (215 mF/cm3 and 85% retention) with an areal capacitance of 134 {\mu}F/cm2 at 120 Hz and ultrafast frequency response. Utilizing the normally discarded target-side material can therefore enable high performing devices while reducing waste, cost and energy input per usable product. leading towards a greater sustainability on nanomaterials synthesis and deposition techniques.

physics.app-ph↗

arXiv2020

Fractal Carbon nanofoams by nanosecond and femtosecond pulsed-laser deposition

We report on an investigation on the properties of ultra-low density, fractal, Carbon nanofoams fabricated with the nanosecond and femtosecond pulsed-laser deposition (PLD) techniques. We measure through innovative techniques the foam mean density and the properties of the fractal aggregates composing the film (i.e. nanoparticles diameter, fractal dimension, and gyration radius) as a function of several PLD process parameters, namely the background gas pressure and the laser pulse characteristics (energy, time duration, repetition rate). We discuss the experimental observation on the basis of the existing literature, and we propose an analytical equation, based on the fractal scaling law, to predict the foam density from the aggregates properties. Finally, we use analytical arguments to explain the observed trends in the nanofoam density with respect to the process parameters, useful to gain new insights on the nanofoam growth and to guide experimental work in fabricating ultra-low density films with precisely controlled properties.

cond-mat.mtrl-sci↗

arXiv2019

Reference-free evaluation of thin films mass thickness and composition through energy dispersive x-ray spectroscopy

In this paper we report the development of a new method for the evaluation of thin films mass thickness and composition based on the Energy Dispersive X-Ray Spectroscopy (EDS). The method exploits the theoretical calculation of the in-depth characteristic X-ray generation distribution function, $ϕ$/($ρ$ z), in multilayer samples, obtained by the numerical solution of the electron transport equation, to achieve reliable measurements without the need of a reference sample and multiple voltages acquisitions. The electron transport model is derived from the Boltzmann transport equation and it exploits the most updated and reliable physical parameters in order to obtain an accurate description of the phenomenon. The method for the calculation of film mass thickness and composition is validated with benchmarks from standard techniques. In addition, a model uncertainty and sensitivity analysis is carried out and it indicates that the mass thickness accuracy is in the order of 10 $μ$g/cm$^2$, which is comparable to the nuclear standard techniques resolution. We show the technique peculiarities in one example measurement: two-dimensional mass thickness and composition profiles are obtained for a ultra-low density, high roughness, nanostructured film.

cond-mat.mtrl-sci↗