arXiv subjects

Alessandro Principi

Publications and source records attributed to Alessandro Principi.

At least 73 records · Page 4Linked to original sources

arXiv2019

Enhanced photoenergy harvesting and extreme Thomson effect in hydrodynamic electronic systems

The thermoelectric (TE) properties of a material are dramatically altered when electron-electron interactions become the dominant scattering mechanism. In the degenerate hydrodynamic regime, the thermal conductivity is reduced and becomes a {\it decreasing} function of the electronic temperature, due to a violation of the Wiedemann-Franz (WF) law. We here show how this peculiar temperature dependence gives rise to new striking TE phenomena. These include an 80-fold increase in TE efficiency compared to the WF regime, dramatic qualitative changes in the steady state temperature profile, and an anomalously large Thomson effect. In graphene, which we pay special attention to here, these effects are further amplified due to a doubling of the thermopower.

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arXiv2019

Pseudo-Euler equations from nonlinear optics: plasmon-assisted photodetection beyond hydrodynamics

A great deal of theoretical and experimental efforts have been devoted in the last decades to the study of long-wavelength photodetection mechanisms in field-effect transistors hosting two-dimensional (2D) electron systems. A particularly interesting subclass of these mechanisms is intrinsic and based on the conversion of the incoming electromagnetic radiation into plasmons, which resonantly enhance the photoresponse, and subsequent rectification via hydrodynamic nonlinearities. In this Article we show that such conversion and subsequent rectification occur well beyond the frequency regime in which hydrodynamic theory applies. We consider the nonlinear optical response of generic 2D electron systems and derive pseudo-Euler equations of motion for suitable collective variables. These are solved in one- and two-dimensional geometries for the case of graphene and the results are compared with those of hydrodynamic theory. Significant qualitative differences are found, which are amenable to experimental studies. Our theory expands the knowledge of the fundamental physics behind long-wavelength photodetection.

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arXiv2018

Scanning Gate Microscopy in a Viscous Electron Fluid

We measure transport through a Ga[Al]As heterostructure at temperatures between 0.1 K and 30 K. Increasing the temperature enhances the electron-electron scattering rate and viscous effects in the two-dimensional electron gas arise. To probe this regime we measure so-called vicinity voltages and use a voltage-biased scanning tip to induce a movable local perturbation. We find that the scanning gate images differentiate reliably between the different regimes of electron transport. Our data are in good agreement with recent theories for interacting electron liquids in the ballistic and viscous regimes stimulated by measurements in graphene. However, the range of temperatures and densities where viscous effects are observable in Ga[Al]As are very distinct from the graphene material system.

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arXiv2018

Confining graphene plasmons to the ultimate limit

Graphene plasmons have recently attracted a great deal of attention because of their tunability, long lifetime, and high degree of field confinement in the vertical direction. Nearby metal gates have been shown to modify the graphene plasmon dispersion and further confine their electric field. We study the plasmons of a graphene sheet deposited on a metal, in the regime in which metal bands do not hybridize with massless Dirac fermion bands. We derive exact results for the dispersion and lifetime of the plasmons of such hybrid system, taking into account metal nonlocalities. The graphene plasmon dispersion is found to be acoustic and pushed down in energy towards the upper boundary of the intraband graphene particle-hole continuum, thereby strongly enhancing the vertical confinement of these excitations. Landau damping of such acoustic plasmons due to particle-hole excitations in the metal gate is found to be surprisingly weak, with quality factors exceeding $Q = 10^{2}$.

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arXiv2017

Negative electronic compressibility enables electrically-induced charge density waves in a two-dimensional electron liquid

We show that the negative electronic compressibility of two-dimensional electronic systems at sufficiently low density enables the generation of charge density waves through the application of a uniform force field, provided no current is allowed to flow. The wavelength of the density oscillations is controlled by the magnitude of the (negative) screening length, and their amplitude is proportional to the applied force. Both are electrically tunable.

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arXiv2017

Ultra-confined acoustic THz graphene plasmons revealed by photocurrent nanoscopy

Terahertz (THz) fields are widely applied for sensing, communication and quality control. In future applications, they could be efficiently confined, enhanced and manipulated - well below the classical diffraction limit - through the excitation of graphene plasmons (GPs). These possibilities emerge from the strongly reduced GP wavelength, lp, compared to the photon wavelength, l0, which can be controlled by modulating the carrier density of graphene via electrical gating. Recently, GPs in a graphene-insulator-metal configuration have been predicted to exhibit a linear dispersion (thus called acoustic plasmons) and a further reduced wavelength, implying an improved field confinement, analogous to plasmons in two-dimensional electron gases (2DEGs) near conductive substrates. While infrared GPs have been visualised by scattering-type scanning near-field optical microscopy (s-SNOM), the real-space imaging of strongly confined THz plasmons in graphene and 2DEGs has been elusive so far - only GPs with nearly free-space wavelength have been observed. Here we demonstrate real-space imaging of acoustic THz plasmons in a graphene photodetector with split-gate architecture. To that end, we introduce nanoscale-resolved THz photocurrent near-field microscopy, where near-field excited GPs are detected thermoelectrically rather than optically. The on-chip GP detection simplifies GP imaging, as sophisticated s-SNOM detection schemes can be avoided. The photocurrent images reveal strongly reduced GP wavelengths (lp = l0/66), a linear dispersion resulting from the coupling of GPs with the metal gate below the graphene, and that plasmon damping at positive carrier densities is dominated by Coulomb impurity scattering. Acoustic GPs could thus strongly benefit the development of deep subwavelength-scale THz devices.

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arXiv2017

Chiral second-sound collective mode at the edge of 2D systems with nontrivial Berry curvature

We study the thermal transport in two-dimensional systems with a nontrivial Berry curvature texture. The physical realizations are many: for a sake of definiteness we consider undoped graphene gapped by the presence of an aligned hexagonal-Boron-Nitride substrate. The same phenomenology applies, i.e., to surface states of 3D topological insulators in the presence of a uniform magnetization. We find that chiral valley-polarized second-sound collective modes propagate along the edges of the system. The localization length of the edge modes has topological origin stemming from the anomalous velocity term in the quasiparticle current. At low temperature, the single-particle contribution to the transverse thermal conductance is exponentially suppressed and only second-sound modes carry heat along the boundary. A sharp change in the behavior of the thermal Hall conductance, extracted from nonlocal measurements of the temperature along the edge, marks the onset of ballistic heat transport due to second-sound edge modes.

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arXiv2016

Fractional quantum Hall effect in strained graphene: stability of Laughlin states in disordered (pseudo)magnetic fields

We address the question of the stability of the (fractional) quantum Hall effect (QHE) in presence of pseudomagnetic disorder generated by mechanical deformations of a graphene sheet. Neglecting the potential disorder and taking into account only strain-induced random pseudomagnetic fields, it is possible to write down a Laughlin-like trial ground-state wave function explicitly. Exploiting the Laughlin plasma analogy, we demonstrate that in the case of fluctuating pseudomagnetic fluxes of relatively small amplitude both the integer and fractional quantum Hall effects are always stable upon the deformations. By contrast, in the case of bubble-induced pseudomagnetic fields in graphene on a substrate (a small number of large fluxes) the disorder can be strong enough to cause a glass transition in the corresponding classical Coulomb plasma, resulting in the destruction of fractional quantum Hall regime and in a quantum phase transition to a non-ergodic state of the lowest Landau level.

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arXiv2016

Super-Planckian electron cooling in a van der Waals stack

Radiative heat transfer (RHT) between macroscopic bodies at separations that are much smaller than the thermal wavelength is ruled by evanescent electromagnetic modes and can be orders of magnitude more efficient than its far-field counterpart, which is described by the Stefan-Boltzmann law. In this Letter we present a microscopic theory of RHT in van der Waals stacks comprising graphene and a natural hyperbolic material, i.e. hexagonal boron nitride (hBN). We demonstrate that RHT between hot carriers in graphene and hyperbolic phonon-polaritons in hBN is extremely efficient at room temperature, leading to picosecond time scales for the carrier cooling dynamics.

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arXiv2016

Hall viscosity and electromagnetic response of electrons in graphene

We derive an analytic expression for the geometric Hall viscosity of non-interacting electrons in a single graphene layer in the presence of a perpendicular magnetic field. We show that a recently-derived formula in [C. Hoyos and D. T. Son, Phys. Rev. Lett. {\bf 108}, 066805 (2012)], which connects the coefficient of $q^2$ in the wave vector expansion of the Hall conductivity $σ_{xy}(q)$ of the two-dimensional electron gas (2DEG) to the Hall viscosity and the orbital diamagnetic susceptibility of that system, continues to hold for graphene -- in spite of the lack of Galilean invariance -- with a suitable definition of the effective mass. We also show that, for a sufficiently large number of occupied Landau levels in the positive energy sector, the Hall conductivity of electrons in graphene reduces to that of a Galilean-invariant 2DEG with an effective mass given by $\hbar k_F/v_F$ (cyclotron mass). Even in the most demanding case, i.e. when the chemical potential falls between the zero-th and the first Landau level, the cyclotron mass formula gives results accurate to better than 1$\%$. The connection between the Hall conductivity and the viscosity provides a possible avenue to measure the Hall viscosity in graphene.

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arXiv2016

Edge pseudo-magnetoplasmons

We study the properties of edge plasmons in two-component electron liquids in the presence of pseudomagnetic fields, which have opposite signs for the two different electronic populations and therefore preserve the time-reversal symmetry. The physical realizations of such systems are many. We discuss the cases of strained graphene and of electrons in proximity to a Skyrmion lattice, solving the problem with the Wiener-Hopf technique. We show (i) that two charged counter-propagating acoustic edge modes exist at the boundary and (ii) that, in the limit of large pseudomagnetic fields, each of them involves oscillations of only one of the two electronic components. We suggest that the edge pseudo-magnetoplasmons of graphene can be used to selectively address the electrons of one specific valley, a feature relevant for the emerging field of valleytronics. Conversely, the spin-polarized plasmons at the boundary of Skyrmion lattices can be exploited for spintronics applications. Our solution highlights new features missing in previous (similar) results obtained with uncontrolled approximations, namely a logarithmic divergence of the plasmon velocity, and the absence of gapped edge modes inside the bulk-plasmon gap.

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arXiv2016

Self-induced glassiness and pattern formation in spin systems subject to long-range interactions

We study the glass formation in two- and three-dimensional Ising and Heisenberg spin systems subject to competing interactions and uniaxial anisotropy with a mean-field approach. In three dimensions, for sufficiently strong anisotropy the systems always modulates in a striped phase. Below a critical strength of the anisotropy, a glassy phase exists in a finite range of temperature, and it becomes more stable as the system becomes more isotropic. In two dimension the criticality is always avoided and the glassy phase always exists.

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arXiv2015

Stripe glasses in ferromagnetic thin films

Domain walls in magnetic multilayered systems can exhibit a very complex and fascinating behavior. For example, the magnetization of thin films of hard magnetic materials is in general perpendicular to the thin-film plane, thanks to the strong out-of-plane anisotropy, but its direction changes periodically, forming an alternating spin-up and spin-down stripe pattern. The latter is stabilized by the competition between the ferromagnetic coupling and dipole-dipole interactions, and disappears when a moderate in-plane magnetic field is applied. It has been suggested that such a behavior may be understood in terms of a self-induced stripe glassiness. In this paper we show that such a scenario is compatible with the experimental findings. The strong out-of-plane magnetic anisotropy of the film is found to be beneficial for the formation of both the stripe-ordered and glassy phases. At zero magnetic field the system can form a glass only in a narrow interval of fairly large temperatures. An in-plane magnetic field, however, shifts the glass transition towards lower temperatures, therefore enabling it at or below room temperature. In good qualitative agreement with the experimental findings, we show that a moderate in-plane magnetic field of the order of $30~{\rm mT}$ can lead to the formation of defects in the stripe pattern, which sets the onset of the glass transition.

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arXiv2015

Quasiparticle Mass Enhancement and Fermi Surface Shape Modification in Oxide Two-Dimensional Electron Gases

We propose a model intended to qualitatively capture the electron-electron interaction physics of two-dimensional electron gases formed near transition-metal oxide heterojunctions containing $t_{2g}$ electrons with a density much smaller than one electron per metal atom. Two-dimensional electron systems of this type can be described perturbatively using a $GW$ approximation which predicts that Coulomb interactions enhance quasiparticle effective masses more strongly than in simple two-dimensional electron gases, and that they reshape the Fermi surface, reducing its anisotropy.

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arXiv2015

Kondo effect and non-Fermi liquid behavior in Dirac and Weyl semimetals

We study the Kondo effect in three-dimensional (3D) Dirac materials and Weyl semimetals. We find the scaling of the Kondo temperature with respect to the doping $n$ and the coupling $J$ between the moment of the magnetic impurity and the carriers of the semimetal. We find that when the temperature is much smaller than the Kondo temperature the resistivity due to the Kondo effect scales as the $n^{-4/3}$.We also study the effect of the interplay of long-range scalar disorder and Kondo effect. In the presence of disorder-induced long-range carrier density inhomogeneities the Kondo effect is not characterized by a Kondo temperature but by a distribution of Kondo temperatures. We obtain the expression of such distribution and show that its features cause the appearance of strong non-Fermi liquid behavior. Finally we compare the properties of the Kondo effect in 3D Dirac materials and 2D Dirac systems like graphene and topological insulators.

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arXiv2015

Bulk and shear viscosities of the 2D electron liquid in a doped graphene sheet

Hydrodynamic flow occurs in an electron liquid when the mean free path for electron-electron collisions is the shortest length scale in the problem. In this regime, transport is described by the Navier-Stokes equation, which contains two fundamental parameters, the bulk and shear viscosities. In this Article we present extensive results for these transport coefficients in the case of the two-dimensional massless Dirac fermion liquid in a doped graphene sheet. Our approach relies on microscopic calculations of the viscosities up to second order in the strength of electron-electron interactions and in the high-frequency limit, where perturbation theory is applicable. We then use simple interpolation formulae that allow to reach the low-frequency hydrodynamic regime where perturbation theory is no longer directly applicable. The key ingredient for the interpolation formulae is the "viscosity transport time" $τ_{\rm v}$, which we calculate in this Article. The transverse nature of the excitations contributing to $τ_{\rm v}$ leads to the suppression of scattering events with small momentum transfer, which are inherently longitudinal. Therefore, contrary to the quasiparticle lifetime, which goes as $-1/[T^2 \ln(T/T_{\rm F})]$, in the low temperature limit we find $τ_{\rm v} \sim 1/T^2$.

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arXiv2015

Accessing phonon polaritons in hyperbolic crystals by ARPES

Recently studied hyperbolic materials host unique phonon-polariton (PP) modes. The ultra-short wavelengths of these modes, which can be much smaller than those of conventional exciton-polaritons, are of high interest for extreme sub-diffraction nanophotonics schemes. Polar hyperbolic materials such as hexagonal boron nitride can be used to realize strong long-range coupling between PP modes and extraneous charge degrees of freedom. The latter, in turn, can be used to control and probe PP modes. Of special interest is coupling between PP modes and plasmons in an adjacent graphene sheet, which opens the door to accessing PP modes by angle-resolved photoemission spectroscopy (ARPES). A rich structure in the graphene ARPES spectrum due to PP modes is predicted, providing a new probe of PP modes and their coupling to graphene plasmons.

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arXiv2015

The intrinsic charge and spin conductivities of doped graphene in the Fermi-Liquid regime

The experimental availability of ultra-high-mobility samples of graphene opens the possibility to realize and study experimentally the "hydrodynamic" regime of the electron liquid. In this regime the rate of electron-electron collisions is extremely high and dominates over the electron-impurity and electron-phonon scattering rates, which are therefore neglected. The system is brought to a local quasi-equilibrium described by a set of smoothly varying (in space and time) functions, {\it i.e.} the density, the velocity field and the local temperature. In this paper we calculate the charge and spin conductivities of doped graphene due solely to electron-electron interactions. We show that, in spite of the linear low-energy band dispersion, graphene behaves in a wide range of temperatures as an effectively Galilean invariant system: the charge conductivity diverges in the limit $T \to 0$, while the spin conductivity remains finite. These results pave the way to the description of charge transport in graphene in terms of Navier-Stokes equations.

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