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Alessandro Tonello

Publications and source records attributed to Alessandro Tonello.

At least 19 recordsLinked to original sources
arXiv2026

Optical Poling Reveals Hidden Molecular Restructuring in Multimode Fibers, Unlocking Ultra-Efficient Third-Order Nonlinearities

Optical poling is a well-established technique for inducing \chi^{(2)} nonlinearity, yet its impact on silica's molecular structure remains unexplored. Here, we report the first direct observation of molecular restructuring in large-core graded-index multimode fibers (MMFs) induced by optical poling, transforming the silica tetrahedral ring network. Through coherent light beating, this process converts large rings of more than four SiO_4 tetrahedra into smaller ones, altering both linear and nonlinear optical susceptibilities. Contrary to the assumption that poling efficiency stems solely from charge displacement, we show that structural modifications dominate, leading to record enhancements in third-order nonlinear processes, including geometric parametric instabilities (GPIs) and Kerr self-cleaning, despite a low modification of the Kerr coefficient. High-energy poling acts as an in situ annealing process, dynamically modulating the refractive index for unprecedented spatiotemporal light control. These findings provide fundamental insights into silica's molecular dynamics under intense optical fields and open avenues for ultra-efficient nonlinear optical devices, enabling next-generation fiber-based photonics for high-power lasers, broadband light generation, and all-optical signal processing.

physics.optics↗
arXiv2025

Spatio-spectral light-by-light moulding in multimode fibre

Controlling complex light waves to achieve desired behaviours or characteristics on demand presents a significant challenge. This task becomes even more complicated when manipulating speckled light beams owing to their inherently fuzzy intensity and phase structures. Here, we demonstrate that a weak speckled second-harmonic signal in a multimode graded-index fibre can be manipulated via its conservative interaction with a high-power co-propagating fundamental pump wave. Specifically, the spatial quality of the signal can be either enhanced or degraded by varying the pump's power or its modal power distribution. The underlying physical mechanism is the optically induced mode conversion, whose phase-matching can be controlled by the mode power distribution of the pump beam. This phenomenon enables new possibilities for manipulating complex light via material nonlinearities in multimode guiding structures. A striking example of this novel light-by-light control is the experimentally observed enhancement or partial suppression of the visible Raman Stokes cascade regulated by the second harmonic beam, while modulated by the mode power distribution of the fundamental beam.

physics.optics↗
arXiv2024

Concatenation of Kerr solitary waves in Ceramic YAG: application to coherent Raman imaging

A coherent concatenation of multiple Townes solitons may lead to a stable infrared and visible broadband filament in ceramic YAG polycrystal. This self-trapped soliton train is leveraged to implement self-referenced multiplex coherent anti-Stokes Raman scattering imaging. Simulations and experiments illustrating the filamentation process and the concatenation of focusing-defocusing cycles in ceramic and crystal YAG are presented. In addition, our simulations and experiments further examine the dependence of the filamentation onset location and supercontinuum generation upon peak input power. Understanding this dependence is key for implementation of viable CARS imaging techniques, due to the comparatively exceptional ability of YAG to generate supercontinuum which can enable higher-sensitivity imaging without delay lines.

physics.optics↗
arXiv2024

Light tailored by multimode fiber for multiphoton fluorescence microscopy

We study the diffraction of a particular class of beams, composed only by a combination of azimuthally invariant guided modes of an optical fiber. We demonstrate that such beams can be obtained by injecting a Gaussian beam in a small piece of silica graded-index multimode fiber. This minimalistic low-cost method is applied for improving the axial resolution of a two-photon microscope.

physics.optics↗
arXiv2024

Exploitation of the nonresonant background of Multiplex-Coherent anti-Stokes Raman Scattering for label-free discrimination of proteins

We propose a novel approach using Multiplex-Coherent Anti-Stokes Raman Scattering (M-CARS) for la-bel-free discriminations in biomedical tissues. The strategy is based on the evaluation of the contrast be-tween resonant and nonresonant contributions in a M-CARS hyperspectral dataset, and tested to identify and differentiate thin actin filaments from thick myosin filaments in muscle tissue without any labeling. First step consists in ensuring knowledge of the spatial regions containing thick myosin filaments thanks to its endogenous second harmonic signal, deducing expected location for thin actin filaments between myosin filaments. The ratio of resonant and nonresonant contributions for each pixel of the hyperspectral image allows then to discriminate actin from myosin filaments, whose localization is in accordance with the SHG probing. This qualitative imaging represents a proof of principle for highlighting and discriminat-ing purposes in biological microscopy, thanks to the difference in the nonlinear properties of the related proteins. This paves the way for considering label-free imaging through a competition between two third-order nonlinear signatures.

physics.med-ph↗
arXiv2022

Multimode optical fiber beam-by-beam cleanup

We introduce and experimentally demonstrate the concept of all-optical beam switching in graded-index multimode optical fibers. Nonlinear coupling between orthogonally polarized seed and signal beams permits to control the spatial beam quality at the fiber output. Remarkably, we show that even a weak few-mode control beam may substantially enhance the quality of an intense, highly multimode signal beam. We propose a simple geometrical representation of the beam switching operation, whose validity is quantitatively confirmed by the experimental mode decomposition of the output beam. All-optical switching of multimode beams may find important applications in high-power beam delivery and fiber lasers.

physics.optics↗
arXiv2022

Numerical analysis of beam self-cleaning in multimode fiber amplifiers

Recent experimental results have reported the observation of beam self-cleaning or, more generally, nonlinear beam reshaping in active multimode fibers. In this work we present a numerical analysis of these processes, by considering the ideal case of a diode-pumped signal amplifier made of a graded-index multimode fiber with uniform Yb doping. Simulations confirm that beam cleaning of the signal may take place even in amplifying fibers, that is the absence of beam energy conservation. Moreover, we show how the local signal intensity maxima, which are periodically generated by the self-imaging process, may influence the population inversion of the doping atoms, and locally saturate the amplifier gain.

physics.optics↗
arXiv2021

Twin Spotlight Beam Generation in Quadratic Crystals

Optical rogue waves have been extensively studied in the past two decades. However, observations of multidimensional extreme wave events remain surprisingly scarce. In this work we present the experimental demonstration of the spontaneous generation of spatially localized two-dimensional beams in a quadratic nonlinear crystal, which are composed by twin components at the fundamental and the second-harmonic frequencies. These localized spots of light emerge from a wide background beam, and eventually disappear as the laser beam intensity is progressively increased.

physics.optics↗
arXiv2021

Femtosecond nonlinear losses in multimode optical fibers

Research on multimode optical fibers is arousing a growing interest, for their capability to transport high-power laser beams, coupled with novel nonlinear optics-based applications. However, when beam intensities exceed a certain critical value, optical fiber breakdown associated with irreversible modifications of their refractive index occurs, triggered by multiphoton absorption. These processes have been largely exploited for fiber material microstructuration. Here we show that, for intensities slightly below the breakdown threshold, nonlinear absorption strongly affects the dynamics of a propagating beam as well. We experimentally analyze this sub-threshold regime, and highlight the key role played by spatial self-imaging in graded-index fibers for enhancing nonlinear optical losses. We characterize the nonlinear power transmission properties of multimode fibers for femtosecond pulses propagating in the near-infrared spectral range. We show that an effective N-photon absorption analytical model is able to describe well the experimental data.

physics.optics↗
arXiv2020

Spatiotemporal beam self-cleaning for high-resolution nonlinear fluorescence imaging with multimode fibres

Beam self-cleaning (BSC) in graded-index (GRIN) multimode fibres (MMFs) has been recently reported by different research groups. Driven by the interplay between Kerr effect and beam self-imaging, BSC counteracts random mode coupling, and forces laser beams to recover a quasi-single mode profile at the output of GRIN fibres. Here we show that the associated self-induced spatiotemporal reshaping allows for improving the performances of nonlinear fluorescence microscopy and endoscopy using multimode optical fibres. We experimentally demonstrate that the beam brightness increase, induced by self-cleaning, enables two and three-photon imaging of biological samples with high spatial resolution. Temporal pulse shortening accompanying spatial beam clean-up enhances the output peak power, hence the efficiency of nonlinear imaging. We also show that spatiotemporal supercontinuum generation is well-suited for large-band nonlinear fluorescence imaging in visible and infrared domains. We substantiated our findings by multiphoton fluorescence imaging in both microscopy and endoscopy configurations.

physics.optics↗
arXiv2020

Coherent combining of self-cleaned multimode beams

A low intensity light beam emerges from a graded-index, highly multimode optical fibre with a speckled shape, while at higher intensity the Kerr nonlinearity may induce a spontaneous spatial self-cleaning of the beam [1,2]. Here, we reveal that we can generate two self-cleaned beams with a mutual coherence large enough to produce a clear stable fringe pattern at the output of a nonlinear interferometer. The two beams are pumped by the same input laser, yet are self-cleaned into independent multimode fibres. We thus prove that the self-cleaning mechanism preserves the beams' mutual coherence via a noise-free parametric process. While directly related to the initial pump coherence, the emergence of nonlinear spatial coherence is achieved without additional noise, even for self-cleaning obtained on different modes, and in spite of the fibre structural disorder originating from intrinsic imperfections or external perturbations. Our discovery may impact theoretical approaches on wave condensation [3-5], and open new opportunities for coherent beam combining [6-9].

physics.optics↗
arXiv2020

Nonlinear beam self-imaging and self-focusing dynamics in a GRIN multimode optical fiber: theory and experiments

Beam self-imaging in nonlinear graded-index multimode optical fibers is of interest for many applications, such as implementing a fast saturable absorber mechanism in fiber lasers via multimode interference. We obtain an exact solution for the nonlinear evolution of first and second order moments of a laser beam carried by a graded-index multimode fiber, predicting that the spatial self-imaging period does not vary with power. Whereas the amplitude of the oscillation of the beam width is power-dependent. We have experimentally studied the longitudinal evolution of beam self-imaging by means of femtosecond laser pulse propagation in both the anomalous and the normal dispersion regime of a standard telecom graded-index multimode optical fiber. Light scattering out of the fiber core via visible fluorescence emission and harmonic wave generation permits us to directly confirm that the self-imaging period is invariant with power. Spatial shift and splitting of the self-imaging process under the action of self-focusing are also emphasized.

physics.optics↗
arXiv2019

Spatial beam self-cleaning in multimode lanthanum aluminum silicate glass fiber

We demonstrated that spatial Kerr beam self-cleaning can be obtained in a highly multimode multicomponent optical fiber based on lanthanum aluminum silicate oxide glasses (SiO2-Al2O3-La2O3), which was made by using the modified powder in tube technology (MIPT). We show how such fabrication method can provide interesting potentialities to design doped multimode optical fibers with homogeneous and quasi-parabolic refractive-index core profile for nonlinear optics applications.

physics.optics↗
arXiv2018

Refractive index profile tailoring of multimode optical fibers for the spatial and spectral shaping of parametric sidebands

We introduce the concept of spatial and spectral control of nonlinear parametric sidebands in multimode optical fibers by tailoring their linear refractive index profile. In all cases, the pump experiences Kerr self-cleaning, leading to a bell-shaped profile close to the fundamental mode. Geometric parametric instability, owing to quasi-phase-matching from the grating generated via the Kerr effect by pump self-imaging, leads to frequency multicasting of beam self-cleaning across a wideband array of sidebands. Our experiments show that introducing a gaussian dip in the refractive index profile of a graded index fiber permits to dramatically change the spatial content of spectral sidebands into higher-order modes. This is due to the breaking of oscillation synchronism among fundamental and higher-order modes. Hence modal-four-wave mixing prevails over geometric parametric instability as the main sideband generation mechanism. Observations agree well with theoretical predictions based on a perturbative analysis, and with full numerical solutions of the (3D + 1) nonlinear Schrodinger equation.

physics.optics↗
arXiv2018

Spatiotemporal light-beam compression from nonlinear mode coupling

We experimentally demonstrate simultaneous spatial and temporal compression in the propagation of light pulses in multimode nonlinear optical fibers. We reveal that the spatial beam self-cleaning recently discovered in graded-index multimode fibers is accompanied by significant temporal reshaping and up to four-fold shortening of the injected sub-nanosecond laser pulses. Since the nonlinear coupling among the modes strongly depends on the instantaneous power, we explore the entire range of the nonlinear dynamics with a single optical pulse, where the optical power is continuously varied across the pulse profile.

physics.optics↗
arXiv2018

Nonlinear dynamics in multimode optical fibers

We overview recent advances in the research on spatiotemporal beam shaping in nonlinear multimode optical fibers. An intense light beam coupled to a graded index (GRIN) highly multimode fiber undergoes a series of complex nonlinear processes when its power grows larger. Among them, the lowest threshold effect is the Kerr-induced beam self-cleaning, that redistributes most of the beam energy into a robust bell-shaped beam close to the fundamental mode. At higher powers a series of spectral sidebands is generated, thanks to the phase matching induced by the long period grating due to the periodic self-imaging of the beam and the Kerr effect. Subsequently a broadband and spectrally flat supercontinuum is generated, extending from the visible to the mid-infrared.

physics.optics↗
arXiv2017

Spatial beam self-cleaning in multimode fiber

Multimode optical fibres are enjoying a renewed attention, boosted by the urgent need to overcome the current capacity crunch of single-mode fibre systems and by recent advances in multimode complex nonlinear optics [1-13]. In this work, we demonstrate that standard multimode fibres can be used as ultrafast all-optical tool for transverse beam manipulation of high power laser pulses. Our experimental data show that the Kerr effect in a graded-index multimode fibre is the driving mechanism for overcoming speckle distortions, leading to a somewhat counter-intuitive effect resulting in a spatially clean output beam robust against fibre bending. Our observations demonstrate that nonlinear beam reshaping into the fundamental mode of a multimode fibre can be achieved even in the absence of a dissipative process such as stimulated scattering (Raman or Brillouin) [14,15].

physics.optics↗