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Alex Hayat

Publications and source records attributed to Alex Hayat.

At least 19 recordsLinked to original sources

Temporal Signature of Bosonic Stimulation Induced by Dark Exciton in a Two-photon Pumped Polariton Condensate

Strongly-coupled light-matter exciton-polaritons constitute an on-chip solid-state platform where the macroscopic quantum phenomenon of condensation is not only achievable at elevated temperatures, but can also be optically controlled, including through their interaction with inaccessible "dark" states. A recent study has shown that polariton condensation can be established under nonlinear two-photon pumping, paving the way towards dark state-condensate coherent control and highly-efficient terahertz (THz) lasing. In this letter, we show for the first time a temporal signature of dark exciton induced bosonic stimulation by investigating one- and two-photon pumped condensation with time-resolved photoluminescence spectroscopy. Our results show a clear difference in the detuning dependence of the buildup and relaxation rates of the condensate-induced blueshifts under one- and two-photon pumping. This difference is associated with the stronger exciton-fraction dependence expected for one-photon pumped condensation, where polariton-polariton stimulation dominates, compared with two-photon pumped condensation, where a 2p-exciton-to-lower-polariton THz transition can provide another stimulation channel, together with various spin-flip, electron-hole exchange and phonon-based mechanisms. These observations indicate the presence of a new dark state originated stimulation channel that could facilitate highly-efficient THz lasing in semiconductor microcavities.

cond-mat.quant-gas

Orbital-Angular-Momentum Entangled Photon Emission from Circular Currents in Semiconductor-Superconductor Structures

We theoretically demonstrate that a superconducting circular current induced in a semiconductor results in emission of orbital-angular-momentum (OAM) entangled photon pairs upon carrier recombination. Combining the macroscopic Ginzburg-Landau theory and the microscopic Bardeen-Cooper-Schrieffer (BCS) theory, we investigate the emission of a superconducting light-emitting diode (SLED) with a spatially varying phase profile in the superconducting order parameter. We show that in the active region of the SLED with a circular supercurrent, radiative recombination processes inherit the order parameter phase and result in photon pairs emitted into modes of different OAM quantum numbers. We demonstrate that coherent superposition of superconducting qubit eigenstates can also be mapped onto a coherent superposition of emitted photon states. We also show that other recombination processes due to thermally excited quasi particles do not significantly degrade the state purity. Our results introduce an original scheme for generating OAM-entangled photons enabling a new method of transmitting superconducting qubit information to photonic channels thereby bridging the gap between solid-state and photon-based platforms for quantum communications and information processing.

quant-ph

Deterministic exciton confinement in 2D semiconductors via local dielectric engineering for scalable quantum light sources

Single-photon emitters are essential building blocks for quantum communication and photonic quantum technologies. However, realizing scalable, on-chip SPEs on a CMOS-compatible platform remains a significant challenge. Here, we propose and theoretically demonstrate a scalable approach to exciton confinement in two-dimensional semiconductors via local dielectric engineering. By introducing a high-dielectric-constant nanopillar above or beneath the 2D material, we create a spatially varying dielectric environment that can support localized exciton states, enabling deterministic, lithography-compatible single-photon emission without relying on strain, defects, or etching of the 2D layer. Using numerical solutions to the 2D excitonic Schrodinger equation, we quantify the resulting confinement through binding energies, wavefunction profiles, and a spatial confinement parameter. These results offer a practical and scalable route for integrating 2D-based quantum emitters into photonic platforms, paving the way for next-generation quantum optoelectronic devices.

physics.optics

Two-photon pumped exciton-polariton condensation

Two-photon absorption (TPA) allows accessing dark states of matter otherwise inaccessible to light, which serve as important building blocks for quantum information processing. In a semiconductor microcavity, TPA driven condensation of strongly-coupled light-matter exciton-polaritons can enable new solid-state quantum simulations of dark state-condensate interactions, and was predicted to stimulate THz emission. Here, we report the first observation of two-photon pumped polariton condensation, demonstrated by angle-resolved photoluminescence in a GaAs-based microcavity. TPA is evidenced in the quadratic emission dependence on pump power below and above the condensation threshold, and second-harmonic generation is ruled out by both this threshold behaviour and by the emission peak energy showing no dependence on pump photon energy. Our results pave the way towards novel polariton-based sources and solid-state coherent control of collective quantum states with individual two-level systems.

cond-mat.mes-hall

Andreev Reflection Enhancement in Semiconductor-Superconductor Structures

We develop a new theoretical approach for modelling a wide range of semiconductor-superconductor structures with arbitrary potential barriers and a spatially-dependent superconducting order parameter. We demonstrate asymmetry in the conductance spectrum as a result of a Schottky barrier shape. We further show that Andreev reflection process can be significantly enhanced through resonant tunneling with appropriate barrier configuration, which can incorporate the Schottky barrier as a contributing component of the device. Moreover, we show that resonant tunneling can be achieved in superlattice structures as well. These theoretically demonstrated effects along with our modelling approach enable much more efficient Cooper pair injection into semiconductor-superconductor structures, including superconducting optoelectronic devices.

cond-mat.supr-con

Andreev Reflection without Fermi surface alignment in High T$_{c}$-Topological heterostructures

We address the controversy over the proximity effect between topological materials and high T$_{c}$ superconductors. Junctions are produced between Bi$_{2}$Sr$_{2}$CaCu$_{2}$O$_{8+\delta}$ and materials with different Fermi surfaces (Bi$_{2}$Te$_{3}$ \& graphite). Both cases reveal tunneling spectra consistent with Andreev reflection. This is confirmed by magnetic field that shifts features via the Doppler effect. This is modeled with a single parameter that accounts for tunneling into a screening supercurrent. Thus the tunneling involves Cooper pairs crossing the heterostructure, showing the Fermi surface mis-match does not hinder the ability to form transparent interfaces, which is accounted for by the extended Brillouin zone and different lattice symmetries.

cond-mat.supr-con

Photon Bell-State Analysis Based on Semiconductor-Superconductor Structures

We propose a compact and highly-efficient scheme for complete Bell-state analysis using two-photon absorption in a superconducting proximity region of a semiconductor avalanche photodiode. One-photon transitions to the superconducting Cooper-pair based condensate in the conduction band are forbidden, whereas two-photon transitions are allowed and are strongly enhanced by superconductivity. This Cooper-pair based two-photon absorption results in a strong detection preference of a specified entangled state. Our analysis shows high detection purity of the desired Bell state with negligible false detection probability. The theoretically-demonstrated concept can pave the way towards practical realizations of advanced quantum information schemes.

quant-ph

Light Amplification in Semiconductor-Superconductor Structures

We study a new effect of Cooper-pair-based two-photon gain in semiconductor-superconductor structures, showing broadband enhancement of ultrafast two-photon amplification. We further show that with the superconducting enhancement, at moderately high seed intensities the two-photon gain contribution approaches that of the one-photon gain. A full quantum-optical model of singly- and fully-stimulated two-photon emission is developed. Our results provide new insights on nonlinear light-matter interaction in the superconducting state, including the possibility of coherent control in two-photon semiconductor-superconductor devices. The theoretically demonstrated effects can have important implications in optoelectronics and in coherent control applications.

cond-mat.supr-con

Quantum control of population transfer between vibrational states in an optical lattice

We study quantum control techniques, specifically Adiabatic Rapid Passage (ARP) and Gradient Ascent Pulse Engineering (GRAPE), for transferring atoms trapped in an optical lattice between different vibrational states. We compare them with each other and with previously studied coupling schemes in terms of performance. In our study of ARP, we realize control of the vibrational states by tuning the frequency of a spatial modulation through the inhomogeneously broadened vibrational absorption spectrum. We show that due to the presence of multiple crossings, the population transfer depends on the direction of the frequency sweep, in contrast to traditional ARP. In a second study, we control these states by applying a pulse sequence involving both the displacement of the optical lattice and modulation of the lattice depth. This pulse is engineered via the GRAPE algorithm to maximize the number of atoms transferred from the initial (ground) state to the first excited state. We find that the ARP and the GRAPE techniques are superior to the previously tested techniques at transferring population into the first excited state from the ground state: $38.9\pm0.2\%$ and $39\pm2\%$ respectively. GRAPE outperforms ARP in leaving the higher excited states unpopulated (less than $3.3\%$ of the ground state population, at $84\%$ confidence level), while $18.7\pm0.3\%$ of the ground state population is transferred into higher excited states by using ARP. On the other hand, ARP creates a normalized population inversion of $0.21\pm0.02$, which is the highest obtained by any of the control techniques we have investigated.

quant-ph

Observation of EIT-enhanced cross-phase modulation in the short-pulse regime

We present an experiment using a sample of laser-cooled Rb atoms to show that cross-phase modulation schemes continue to benefit from electromagnetically-induced transparency (EIT) even as the transparency window is made narrower than the signal bandwidth (i.e., for signal pulses much shorter than the response time of the EIT system). Addressing concerns that narrow EIT windows might not prove useful for such applications, we show that while the peak phase shift saturates in this regime, it does not drop, and the time-integrated effect continues to scale inversely with EIT window width. This integrated phase shift is an important figure of merit for tasks such as the detection of single-photon-induced cross phase shifts.

quant-ph

Evidence for a New Excitation at the Interface Between a High-Tc Superconductor and a Topological Insulator

High-temperature superconductors exhibit a wide variety of novel excitations. If contacted with a topological insulator, the lifting of spin rotation symmetry in the surface states can lead to the emergence of unconventional superconductivity and novel particles. In pursuit of this possibility, we fabricated high critical-temperature (Tc ~ 85 K) superconductor/topological insulator (Bi2Sr2CaCu2O8+delta/Bi2Te2Se) junctions. Below 75 K, a zero-bias conductance peak (ZBCP) emerges in the differential conductance spectra of this junction. The magnitude of the ZBCP is suppressed at the same rate for magnetic fields applied parallel or perpendicular to the junction. Furthermore, it can still be observed and does not split up to at least 8.5 T. The temperature and magnetic field dependence of the excitation we observe appears to fall outside the known paradigms for a ZBCP.

cond-mat.supr-con

Characterizing an Entangled-Photon Source with Classical Detectors and Measurements

Quantum state tomography (QST) is a universal tool for the design and optimization of entangled-photon sources. It typically requires single-photon detectors and coincidence measurements. Recently, it was suggested that the information provided by the QST of photon pairs generated by spontaneous parametric down-conversion could be obtained by exploiting the stimulated version of this process, namely difference frequency generation. In this protocol, so-called "stimulated-emission tomography" (SET), a seed field is injected along with the pump pulse, and the resulting stimulated emission is measured. Since the intensity of the stimulated field can be several orders of magnitude larger than the intensity of the corresponding spontaneous emission, measurements can be made with simple classical detectors. Here, we experimentally demonstrate SET and compare it with QST. We show that one can accurately reconstruct the polarization density matrix, and predict the purity and concurrence of the polarization state of photon pairs without performing any single-photon measurements.

quant-ph

Quantum Data Compression of a Qubit Ensemble

Data compression is a ubiquitous aspect of modern information technology, and the advent of quantum information raises the question of what types of compression are feasible for quantum data, where it is especially relevant given the extreme difficulty involved in creating reliable quantum memories. We present a protocol in which an ensemble of quantum bits (qubits) can in principle be perfectly compressed into exponentially fewer qubits. We then experimentally implement our algorithm, compressing three photonic qubits into two. This protocol sheds light on the subtle differences between quantum and classical information. Furthermore, since data compression stores all of the available information about the quantum state in fewer physical qubits, it could provide a vast reduction in the amount of quantum memory required to store a quantum ensemble, making even today's limited quantum memories far more powerful than previously recognized.

quant-ph

Ultra-Fast Stark-Induced Control of Polaritonic States

A laser pulse, several meV red-detuned from the excitonic line of a quantum well, has been shown to induce an almost instantaneous and rigid shift of the lower and upper polariton branches. Here we demonstrate that through this shift, ultra-fast all-optical control of the polariton population in a semiconductor microcavity should be achievable. In the proposed setup a Stark field is used to bring the lower polariton branch in or out of resonance with a quasi-resonant continuous-wave laser, thereby favoring or inhibiting the injection of polaritons into the cavity. Moreover we show that this technique allows for the implementation of optical switches with extremely high repetition rates.

cond-mat.mes-hall

Scalable Spatial Super-Resolution using Entangled Photons

N00N states -- maximally path-entangled states of N photons -- exhibit spatial interference patterns sharper than any classical interference pattern. This is known as super-resolution. However, even with perfectly efficient number-resolving detectors, the detection efficiency of all previously demonstrated methods to measure such interference decreases exponentially with the number of photons in the N00N state, often leading to the conclusion that N00N states are unsuitable for spatial measurements. Here, we create spatial super-resolution fringes with two-, three-, and four-photon N00N states, and demonstrate a scalable implementation of the so-called ``optical centroid measurement'' which provides an in-principle perfect detection efficiency. Moreover, we compare the N00N-state interference to the corresponding classical super-resolution interference. Although both provide the same increase in spatial frequency, the visibility of the classical fringes decreases exponentially with the number of detected photons, while the visibility of our experimentally measured N00N-state super-resolution fringes remains approximately constant with N. Our implementation of the optical centroid measurement is a scalable method to measure high photon-number quantum interference, an essential step forward for quantum-enhanced measurements, overcoming what was believed to be a fundamental challenge to quantum metrology.

quant-ph

Enhanced Probing of Fermion Interaction Using Weak Value Amplification

We propose a scheme for enhanced probing of an interaction between two single fermions based on weak-value amplification. The scheme is applied to measuring the anisotropic electron-hole exchange interaction strength in semiconductor quantum dots, where both spin and energy are mapped onto emitted photons. We study the effect of dephasing of the probe on the weak-value-enhanced measurement. We find that in the limit of slow noise, weak-value amplification provides a unique tool for enhanced-precision measurement of few-fermion systems.

quant-ph

Macroscopic coherence between quantum condensates formed at different times

We demonstrate macroscopic coherence between quantum condensates generated at different times, separated by more than the particle dephasing time. This is possible due to the dressed light-matter nature of exciton-polaritons, which can be injected resonantly by optical excitation at well-defined momenta. We show that the build-up of coherence between condensates depends on the interaction between the particles, particle density, as well as temperature despite the non-equilibrium nature of the condensate, whereas the mass of the particles plays no role in the condensation of resonantly injected polaritons. This experiment also makes it possible for us to measure directly the large nonlinear phase shift resulting from the polariton-polariton interaction energy. Our results provide direct evidence for coherence between different condensates and demonstrate a new approach for probing their ultrafast dynamics, opening new directions in the study of matter coherence as well as in practical applications such as quantum information and ultrafast logic.

cond-mat.quant-gas

Experimental demonstration of a time-domain multidimensional quantum channel

We present the first experimental realization of a flexible multidimensional quantum channel where the Hilbert space dimensionality can be controlled electronically. Using electro-optical modulators (EOM) and narrow-band optical filters, quantum information is encoded and decoded in the temporal degrees of freedom of photons from a long-coherence-time single-photon source. Our results demonstrate the feasibility of a generic scheme for encoding and transmitting multidimensional quantum information over the existing fiber-optical telecommunications infrastructure.

quant-ph