arXiv subjects

Alex Krasnok

Publications and source records attributed to Alex Krasnok.

80 records · Page 5Linked to original sources

arXiv2018

Localized all-optical control of single semiconductor quantum dots through plasmon-polariton-induced screening

Due to their ability to strongly modify the local electromagnetic (EM) field through the excitation of surface plasmon polaritons (SPPs), plasmonic nanostructures have been often used to reshape the emission direction and enhance the radiative decay rate of quantum emitters, such as semiconductor quantum dots (QDs). These features are essential for quantum information processing, nanoscale photonic circuitry and optoelectronics. However, the modification and enhancement demonstrated thus far often drastically alter the local energy density of the emitters, and hence their intrinsic properties, leaving little room for active control. Here, we demonstrate dynamic tuning of the energy states of a single semiconductor QD by optically modifying its local dielectric environment with a nearby plasmonic structure, instead of directly coupling it to the QD. This method leaves the original intrinsic optical properties of the QD intact, enabling the opportunity of tuning its optical properties in real time. This capability is highly desired in applications requiring ultrafast switching and modulation mechanisms.

cond-mat.mes-hall↗

arXiv2018

Nanophotonics with 2D Transition Metal Dichalcogenides

Two-dimensional transition metal dichalcogenides (TMDCs) have recently become attractive semiconductor materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and lasers. They are particularly appealing because their bandgap lies in the visible and near-IR range, and they possess strong excitonic resonances, high oscillator strengths, and valley-selective response. Coupling these materials to optical nanocavities enhances the quantum yield of exciton emission, enabling advanced quantum optics and nanophotonic devices. Here, we review state-of-the-art advances on hybrid exciton-polariton structures based on monolayer TMDCs coupled to plasmonic and dielectric nanocavities. We first generally discuss the optical properties of 2D WS2, WSe2, MoS2 and MoSe2 materials, paying special attention to their energy and photoluminescence/absorption spectra, excitonic fine structure, and to the dynamics of exciton formation and valley depolarization. We then discuss light-matter interactions in hybrid exciton-polariton structures. Finally, we focus on weak and strong coupling regimes in monolayer TMDCs-based exciton-polariton systems, envisioning research directions and future opportunities based on this novel material platform.

physics.optics↗

arXiv2017

Coherently Enhanced Wireless Power Transfer

Extraction of electromagnetic energy by an antenna from impinging external radiation is at the basis of wireless communications and power transfer (WPT). The maximum of transferred energy is ensured when the antenna is conjugately matched, i.e., when it is resonant and it has an equal coupling with free space and its load, which is not easily implemented in near-field WPT. Here, we introduce the concept of coherently enhanced wireless power transfer. We show that a principle similar to the one underlying the operation of coherent perfect absorbers can be employed to improve the overall performance of WPT and potentially achieve its dynamic control. The concept relies on coherent excitation of the waveguide connected to the antenna load with a backward propagating signal of specific amplitude and phase. This signal creates a suitable interference pattern at the load resulting in a modification of the local wave impedance, which in turn enables conjugate matching and a largely increased amount of energy extracted to the waveguide. We develop an illustrative theoretical model describing this concept, demonstrate it with full-wave numerical simulations for the canonical example of a dipole antenna, and verify it experimentally in both near-field and far-field regimes.

physics.app-ph↗

arXiv2017

Spectroscopy and Biosensing with Optically Resonant Dielectric Nanostructures

Resonant dielectric nanoparticles (RDNs) made of materials with large positive dielectric permittivity, such as Si, GaP, GaAs, have become a powerful platform for modern light science, enabling various fascinating applications in nanophotonics and quantum optics. In addition to light localization at the nanoscale, dielectric nanostructures provide electric and magnetic resonant responses throughout the visible and infrared spectrum, low dissipative losses and optical heating, low doping effect and absence of quenching, which are interesting for spectroscopy and biosensing applications. In this review, we present state-of-the-art applications of optically resonant high-index dielectric nanostructures as a multifunctional platform for light-matter interactions. Nanoscale control of quantum emitters and applications for enhanced spectroscopy including fluorescence spectroscopy, surface-enhanced Raman scattering (SERS), biosensing, and lab-on-a-chip technology are surveyed. We describe the theoretical background underlying these effects, overview realizations of specific resonant dielectric nanostructures and hybrid excitonic systems, and outlook the challenges in this field, which remain open to future research.

physics.optics↗

arXiv2017

Tunable Resonance Coupling in Single Si Nanoparticle-Monolayer WS2 Structures

Two-dimensional semiconducting transition metal dichalcogenides (TMDCs) are extremely attractive materials for optoelectronic applications in the visible and near-IR range. Here, we address for the first time to the best of our knowledge the issue of resonance coupling in hybrid exciton-polariton structures based on single Si nanoparticles coupled to monolayer WS2. We predict a transition from weak to strong coupling regime , with a Rabi splitting energy exceeding 200 meV for a Si nanoparticle covered by monolayer WS 2 at the magnetic optical Mie resonance. This large transition is achieved due to the symmetry of magnetic dipole Mie mode and by changing the surrounding dielectric material from air to water. The prediction is based on the experimental estimation of TMDC dipole moment variation obtained from measured photoluminescence (PL) spectra of WS2 monolayers in different solvents. An ability of such a system to tune the resonance coupling is realized experimentally for optically resonant spherical Si nanoparticles placed on a WS2 monolayer. The Rabi splitting energy obtained for this scenario increases from 49.6 meV to 86.6 meV after replacing air by water. Our findings pave the way to develop high-efficiency optoelectronic, nanophotonic and quantum optical devices.

physics.optics↗

arXiv2017

Coherent Virtual Absorption Based on Complex Zero Excitation for Ideal Light Capturing

Absorption of light is directly associated with dissipative processes in a material. In suitably tailored resonators, a specific level of dissipation can support coherent perfect absorption, the time-reversed analogue of lasing, which enables total absorption and zero scattering in open cavities. On the contrary, the scattering zeros of lossless objects strictly occur at complex frequencies. While usually considered non-physical due to their divergent response in time, these zeros play a crucial role in the overall scattering dispersion. Here, we introduce the concept of coherent virtual absorption, accessing these modes by temporally shaping the incident waveform. We show that engaging these complex zeros enables storing and releasing the electromagnetic energy at will within a lossless structure for arbitrary amounts of time, under the control of the impinging field. The effect is robust with respect to inevitable material dissipation and can be realized in systems with any number of input ports. The observed effect may have important implications for flexible control of light propagation and storage, low-energy memory, and optical modulation.

physics.optics↗

arXiv2017

Enhancement of inherent Raman scattering in dielectric nanostructures with electric and magnetic Mie resonances

Resonantly enhanced Raman scattering in dielectric nanostructures has been recently proven to be an effcient tool for developing nanothermometry and experimental determination of their mode- composition. In this paper, we develop a rigorous analytical theory based on the Green's function approach to calculate the Raman emission from crystalline high-index dielectric nanoparticles. As an example, we consider silicon nanoparticles which have a strong Raman response due to active optical phonon modes. We relate enhancement of Raman signal emission to Purcell effect due to the excitation of Mie modes inside the nanoparticles. We also employ the numerical approach to the calculation of inelastic Raman emission in more sophisticated geometries, which do not allow a straightforward analytical form of the Green's function description. The Raman response from a silicon nanodisk has been analyzed within the proposed method, and the contribution of the various Mie modes has been revealed.

physics.optics↗

arXiv2017

Coherent perfect absorbers: linear control of light with light

Absorption of electromagnetic energy by a material is a phenomenon that underlies many applied problems, including molecular sensing, photocurrent generation and photodetection. Commonly, the incident energy is delivered to the system through a single channel, for example by a plane wave incident on one side of an absorber. However, absorption can be made much more efficient by exploiting wave interference. A coherent perfect absorber is a system in which complete absorption of electromagnetic radiation is achieved by controlling the interference of multiple incident waves. Here, we review recent advances in the design and applications of such devices. We present the theoretical principles underlying the phenomenon of coherent perfect absorption and give an overview of the photonic structures in which it can be realized, including planar and guided-mode structures, graphene-based systems, parity- and time-symmetric structures, 3D structures and quantum-mechanical systems. We then discuss possible applications of coherent perfect absorption in nanophotonics and, finally, we survey the perspectives for the future of this field.

physics.optics↗