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Alex Thomson

Publications and source records attributed to Alex Thomson.

At least 19 recordsLinked to original sources

Magnetic Confinement of a Bubble of Supercooled $^3$He-A

We have designed and constructed a magnet surrounding a cylindrical volume of superfluid helium-3 to isolate a region of metastable, supercooled A-phase, entirely surrounded by bulk A-phase - isolating the 'bubble' from rough surfaces that can trigger the transition to the stable B-phase. We outline the design of the experimental cell and magnet, and show that the performance of the magnet is consistent with simulations, including the capability to producing the high field gradient required for generating a bubble. Future plans include the investigation of possible intrinsic mechanisms underpinning the A-B transition, with potential implications for early-universe cosmological phase transitions.

cond-mat.other

Symmetry-broken metallic orders in spin-orbit-coupled Bernal bilayer graphene

We explore Bernal bilayer graphene in the presence of long-range Coulomb interactions, short-range Hund's coupling, and proximity-induced Ising spin-orbit coupling using self-consistent Hartree-Fock simulations. We show that the interplay between these three ingredients produces an intricate phase diagram comprising a multitude of symmetry-broken metallic states tunable via doping and applied displacement field. In particular, we find intervalley coherent and spin-canted ground states that may hold the key to understanding spin-orbit-enabled superconductivity observed in this platform. We also investigate various phase transitions where a continuous $\mathrm{U}(1)$ symmetry is broken to ascertain the possible role of critical fluctuations on pairing.

cond-mat.mes-hall

Imaging inter-valley coherent order in magic-angle twisted trilayer graphene

Magic-angle twisted trilayer graphene (MATTG) exhibits a range of strongly correlated electronic phases that spontaneously break its underlying symmetries. The microscopic nature of these phases and their residual symmetries stands as a key outstanding puzzle whose resolution promises to shed light on the origin of superconductivity in twisted materials. Here we investigate correlated phases of MATTG using scanning tunneling microscopy and identify striking signatures of interaction-driven spatial symmetry breaking. In low-strain samples, over a filling range of about 2-3 electrons or holes per moir\'e unit cell, we observe atomic-scale reconstruction of the graphene lattice that accompanies a correlated gap in the tunneling spectrum. This short-scale restructuring appears as a Kekul\'e supercell -- implying spontaneous inter-valley coherence between electrons -- and persists in a wide range of magnetic fields and temperatures that coincide with the development of the gap. Large-scale maps covering several moir\'e unit cells further reveal a slow evolution of the Kekul\'e pattern, indicating that atomic-scale reconstruction coexists with translation symmetry breaking at the much longer moir\'e scale. We employ auto-correlation and Fourier analyses to extract the intrinsic periodicity of these phases and find that they are consistent with the theoretically proposed incommensurate Kekul\'e spiral order. Moreover, we find that the wavelength characterizing moir\'e-scale modulations monotonically decreases with hole doping away from half-filling of the bands and depends only weakly on the magnetic field. Our results provide essential insights into the nature of MATTG correlated phases in the presence of strain and imply that superconductivity emerges from an inter-valley coherent parent state.

cond-mat.str-el

Andreev reflection spectroscopy in strongly paired superconductors

Motivated by recent experiments on low-carrier-density superconductors, including twisted multilayer graphene, we study signatures of the BCS to BEC evolution in Andreev reflection spectroscopy. We establish that in a standard quantum point contact geometry, Andreev reflection in a BEC superconductor is unable to mediate a zero-bias conductance beyond $e^2/h$ per lead channel. This bound is shown to result from a duality that links the sub-gap conductance of BCS and BEC superconductors. We then demonstrate that sharp signatures of BEC superconductivity, including perfect Andreev reflection, can be recovered by tunneling through a suitably designed potential well. We propose various tunneling spectroscopy setups to experimentally probe this recovery.

cond-mat.supr-con

Spin-Orbit Enhanced Superconductivity in Bernal Bilayer Graphene

In the presence of a large perpendicular electric field, Bernal-stacked bilayer graphene (BLG) features several broken-symmetry metallic phases as well as magnetic-field-induced superconductivity. The superconducting state is quite fragile, however, appearing only in a narrow window of density and with a maximum critical temperature $T_c\approx30$~mK. Here, we show that placing monolayer tungsten diselenide (WSe$_{2}$) on BLG promotes Cooper pairing to an extraordinary degree: superconductivity appears at zero magnetic field, exhibits an order of magnitude enhancement in $T_c$, and occurs over a density range that is wider by a factor of eight. By mapping quantum oscillations in BLG-WSe$_2$ as a function of electric field and doping, we establish that superconductivity emerges throughout a region whose normal state is polarized, with two out of four spin-valley flavours predominantly populated. In-plane magnetic field measurements further reveal a striking dependence of the critical field on doping, with the Chandrasekhar-Clogston (Pauli) limit roughly obeyed on one end of the superconducting dome yet sharply violated on the other. Moreover, the superconductivity arises only for perpendicular electric fields that push BLG hole wavefunctions towards WSe$_2$ -- suggesting that proximity-induced (Ising) spin-orbit coupling plays a key role in enhancing the pairing. Our results pave the way for engineering robust, highly tunable, and ultra-clean graphene-based superconductors.

cond-mat.supr-con

Ascendance of Superconductivity in Magic-Angle Graphene Multilayers

Graphene moire superlattices have emerged as a platform hosting and abundance of correlated insulating, topological, and superconducting phases. While the origins of strong correlations and non-trivial topology are shown to be directly linked to flat moire bands, the nature and mechanism of superconductivity remain enigmatic. In particular, only alternating twisted stacking geometries of bilayer and trilayer graphene are found to exhibit robust superconductivity manifesting as zero resistance and Fraunhofer interference patterns. Here we demonstrate that magic-angle twisted tri-, quadri-, and pentalayers placed on monolayer tungsten diselenide exhibit flavour polarization and superconductivity. We also observe insulating states in the trilayer and quadrilayer arising at finite electric displacement fields, despite the presence of dispersive bands introduced by additional graphene layers. Moreover, the three multilayer geometries allow us to identify universal features in the family of graphene moire structures arising from the intricate relations between superconducting states, symmetry-breaking transitions, and van Hove singularities. Remarkably, as the number of layers increases, superconductivity emerges over a dramatically enhanced filling-factor range. In particular, in twisted pentalayers, superconductivity extends well beyond the filling of four electrons per moire unit cell, demonstrating the non-trivial role of the additional bands. Our results highlight the importance of the interplay between flat and dispersive bands in extending superconducting regions in graphene moire superlattices and open new frontiers for developing graphene-based superconductors.

cond-mat.supr-con

Spectroscopic Signatures of Strong Correlations and Unconventional Superconductivity in Twisted Trilayer Graphene

Magic-angle twisted trilayer graphene (MATTG) has emerged as a novel moir\'e material that exhibits both strong electronic correlations and unconventional superconductivity. However, spectroscopic studies of its electronic properties are lacking, and the nature of superconductivity and the corresponding order parameter in this system remain elusive. Here we perform high-resolution scanning tunneling microscopy and spectroscopy of MATTG and reveal extensive regions of atomic reconstruction that favor mirror-symmetric stacking. In these regions, we observe a cascade of symmetry-breaking electronic transitions and doping-dependent band structure deformations similar to those realized in magic-angle bilayers, as expected theoretically given the commonality of flat bands. More strikingly, in a density window spanning two to three holes per moire unit cell, spectroscopic signatures of superconductivity are manifest as pronounced dips in the tunneling conductance at the Fermi level accompanied by coherence peaks that become gradually suppressed at elevated temperatures and magnetic fields. The observed evolution of the conductance with doping is consistent with a gate-tunable transition from a gapped to a nodal superconductor, which we show theoretically is compatible with a sharp transition from a Bardeen-Cooper-Schrieffer (BCS) to a Bose-Einstein condensation (BEC) superconductor with a nodal order parameter. Within this doping window, we also detect peak-dip-hump structures suggesting that superconductivity is driven by strong coupling to bosonic modes of MATTG. Our results pave the way for further understanding of superconductivity and correlated states in graphene-based moir\'e structures beyond twisted bilayers, where unconventional superconductivity and nodal pairing were reported.

cond-mat.mes-hall

Gate-defined wires in twisted bilayer graphene: from electrical detection of inter-valley coherence to internally engineered Majorana modes

Twisted bilayer graphene (TBG) realizes a highly tunable, strongly interacting system featuring superconductivity and various correlated insulating states. We establish gate-defined wires in TBG with proximity-induced spin-orbit coupling as $(i)$ a tool for revealing the nature of correlated insulators and $(ii)$ a platform for Majorana-based topological qubits. In particular, we show that the band structure of a gate-defined wire immersed in an `inter-valley coherent' correlated insulator inherits electrically detectable fingerprints of symmetry breaking native to the latter. Surrounding the wire by a superconducting TBG region on one side and an inter-valley coherent correlated insulator on the other further enables the formation of Majorana zero modes--possibly even at zero magnetic field depending on the precise symmetry-breaking order present. Our proposal not only introduces a highly gate-tunable topological qubit medium relying on internally generated proximity effects, but can also shed light on the Cooper-pairing mechanism in TBG.

cond-mat.str-el

Deconfined criticality and a gapless $\mathbb{Z}_2$ spin liquid in the square lattice antiferromagnet

The theory for the vanishing of N\'eel order in the spin $S=1/2$ square lattice antiferromagnet has been the focus of attention for many decades. A consensus appears to have emerged in recent numerical studies on the antiferromagnet with first and second neighbor exchange interactions (the $J_1$-$J_2$ model): a gapless spin liquid is present for a narrow window of parameters between the vanishing of the N\'eel order and the onset of a gapped valence bond solid state. We propose a deconfined critical SU(2) gauge theory for a transition into a stable $\mathbb{Z}_2$ spin liquid with massless Dirac spinon excitations; on the other side the critical point, the SU(2) spin liquid (the `$\pi$-flux' phase) is presumed to be unstable to confinement to the N\'eel phase. We identify a dangerously irrelevant coupling in the critical SU(2) gauge theory, which contributes a logarithm-squared renormalization. This critical theory is also not Lorentz invariant, and weakly breaks the SO(5) symmetry which rotates between the N\'eel and valence bond solid order parameters. We also propose a distinct deconfined critical U(1) gauge theory for a transition into the same gapless $\mathbb{Z}_2$ spin liquid; on the other side of the critical point, the U(1) spin liquid (the `staggered flux' phase) is presumed to be unstable to confinement to the valence bond solid. This critical theory has no dangerously irrelevant coupling, dynamic critical exponent $z \neq 1$, and no SO(5) symmetry. All of these phases and critical points are unified in a SU(2) gauge theory with Higgs fields and fermionic spinons which can naturally realize the observed sequence of phases with increasing $J_2/J_1$: N\'eel, gapless $\mathbb{Z}_2$ spin liquid, and valence bond solid.

cond-mat.str-el

Interaction-driven Band Flattening and Correlated Phases in Twisted Bilayer Graphene

Flat electronic bands, characteristic of magic-angle twisted bilayer graphene (TBG), host a wealth of correlated phenomena. Early theoretical considerations suggested that, at the magic angle, the Dirac velocity vanishes and the entire width of the moir\'e bands becomes extremely narrow. Yet, this scenario contradicts experimental studies that reveal a finite Dirac velocity as well as bandwidths significantly larger than predicted. Here we use spatially resolved spectroscopy in finite and zero magnetic fields to examine the electronic structure of moir\'e bands and their intricate connection to correlated phases. By following the relative shifts of Landau levels in finite fields, we detect filling-dependent band flattening, that unexpectedly starts already at ~1.3 degrees, well above the magic angle and hence nominally in the weakly correlated regime. We further show that, as the twist angle is reduced, the moir\'e bands become maximally flat at progressively lower doping levels. Surprisingly, when the twist angles reach values for which the maximal flattening occurs at approximate filling of $-2$, $+1$,$+2$,$+3$ electrons per moir\'e unit cell, the corresponding zero-field correlated phases start to emerge. Our observations are corroborated by calculations that incorporate an interplay between the Coulomb charging energy and exchange interactions; together these effects produce band flattening and hence a significant density-of-states enhancement that facilitates the observed symmetry-breaking cascade transitions. Besides emerging phases pinned to integer fillings, we also experimentally identify a series of pronounced correlation-driven band deformations and soft gaps in a wider doping range around $\pm 2$ filling where superconductivity is expected. Our results highlight the role of interaction-driven band-flattening in forming robust correlated phases in TBG.

cond-mat.str-el

Tracing out Correlated Chern Insulators in Magic Angle Twisted Bilayer Graphene

Magic-angle twisted bilayer graphene (MATBG) exhibits a range of correlated phenomena that originate from strong electron-electron interactions. These interactions make the Fermi surface highly susceptible to reconstruction when $ \pm 1, \pm 2, \pm 3$ electrons occupy each moir\' e unit cell and lead to the formation of correlated insulating, superconducting and ferromagnetic phases. While some phases have been shown to carry a non-zero Chern number, the local microscopic properties and topological character of many other phases remain elusive. Here we introduce a set of novel techniques hinging on scanning tunneling microscopy (STM) to map out topological phases in MATBG that emerge in finite magnetic field. By following the evolution of the local density of states (LDOS) at the Fermi level with electrostatic doping and magnetic field, we visualize a local Landau fan diagram that enables us to directly assign Chern numbers to all observed phases. We uncover the existence of six topological phases emanating from integer fillings in finite fields and whose origin relates to a cascade of symmetry-breaking transitions driven by correlations. The spatially resolved and electron-density-tuned LDOS maps further reveal that these topological phases can form only in a small range of twist angles around the magic-angle value. Both the microscopic origin and extreme sensitivity to twist angle differentiate these topological phases from the Landau levels observed near charge neutrality. Moreover, we observe that even the charge-neutrality Landau spectrum taken at low fields is considerably modified by interactions and exhibits an unexpected splitting between zero Landau levels that can be as large as ${\sim }\,3-5$ meV. Our results show how strong electronic interactions affect the band structure of MATBG and lead to the formation of correlation-enabled topological phases.

cond-mat.str-el

Superconductivity without insulating states in twisted bilayer graphene stabilized by monolayer WSe$_2$

Magic-angle twisted bilayer graphene (TBG), with rotational misalignment close to 1.1$^\circ$, features isolated flat electronic bands that host a rich phase diagram of correlated insulating, superconducting, ferromagnetic, and topological phases. The origins of the correlated insulators and superconductivity, and the interplay between them, are particularly elusive. Both states have been previously observed only for angles within $\pm0.1^\circ$ from the magic-angle value and occur in adjacent or overlapping electron density ranges; nevertheless, it is still unclear how the two states are related. Beyond the twist angle and strain, the dependence of the TBG phase diagram on the alignment and thickness of insulating hexagonal boron nitride (hBN) used to encapsulate the graphene sheets indicates the importance of the microscopic dielectric environment. Here we show that adding an insulating tungsten-diselenide (WSe$_2$) monolayer between hBN and TBG stabilizes superconductivity at twist angles much smaller than the established magic-angle value. For the smallest angle of $\theta$ = 0.79$^\circ$, we still observe clear superconducting signatures, despite the complete absence of the correlated insulating states and vanishing gaps between the dispersive and flat bands. These observations demonstrate that, even though electron correlations may be important, superconductivity in TBG can exist even when TBG exhibits metallic behaviour across the whole range of electron density. Finite-magnetic-field measurements further reveal breaking of the four-fold spin-valley symmetry in the system, consistent with large spin-orbit coupling induced in TBG via proximity to WSe$_2$. Our results highlight the importance of symmetry breaking effects in stabilizing electronic states in TBG and open new avenues for engineering quantum phases in moir\'e systems.

cond-mat.supr-con

Recovery of massless Dirac fermions at charge neutrality in strongly interacting twisted bilayer graphene with disorder

Stacking two graphene layers twisted by the 'magic angle' $\theta \approx 1.1^\circ$ generates flat energy bands, which in turn catalyzes various strongly correlated phenomena depending on filling and sample details. At charge neutrality, transport measurements reveal superficially mundane semimetallicity (as expected when correlations are weak) in some samples yet robust insulation in others. We propose that the interplay between interactions and disorder admits either behavior, even when the system is strongly correlated and locally gapped. Specifically, we argue that strong interactions supplemented by weak, smooth disorder stabilize a network of gapped quantum valley Hall domains with spatially varying Chern numbers determined by the disorder landscape--even when an entirely different order is favored in the clean limit. Within this scenario, sufficiently small samples that realize a single domain display insulating transport characteristics. Conversely, multi-domain samples exhibit re-emergent massless Dirac fermions formed by gapless domain-wall modes, yielding semimetallic behavior except on the ultra-long scales at which localization becomes visible. We discuss experimental tests of this proposal via local probes and transport. Our results highlight the crucial role that randomness can play in ground-state selection of twisted heterostructures, an observation that we expect to have further ramifications at other fillings.

cond-mat.str-el

Collusion of Interactions and Disorder at the Superfluid-Insulator Transition: A Dirty 2d Quantum Critical Point

We study the stability of the Wilson-Fisher fixed point of the quantum $\mathrm{O}(2N)$ vector model to quenched disorder in the large-$N$ limit. While a random mass is strongly relevant at the Gaussian fixed point, its effect is screened by the strong interactions of the Wilson-Fisher fixed point. This enables a perturbative renormalization group study of the interplay of disorder and interactions about this fixed point. We show that, in contrast to the spiralling flows obtained in earlier double-$\epsilon$ expansions, the theory flows directly to a quantum critical point characterized by finite disorder and interactions. The critical exponents we obtain for this transition are in remarkable agreement with numerical studies of the superfluid-Mott glass transition. We additionally discuss the stability of this fixed point to scalar and vector potential disorder and use proposed boson-fermion dualities to make conjectures regarding the effects of weak disorder on dual Abelian Higgs and Chern-Simons-Dirac fermion theories when $N=1$.

cond-mat.str-el

Imaging Electronic Correlations in Twisted Bilayer Graphene near the Magic Angle

Twisted bilayer graphene with a twist angle of around 1.1{\deg} features a pair of isolated flat electronic bands and forms a strongly correlated electronic platform. Here, we use scanning tunneling microscopy to probe local properties of highly tunable twisted bilayer graphene devices and show that the flat bands strongly deform when aligned with the Fermi level. At half filling of the bands, we observe the development of gaps originating from correlated insulating states. Near charge neutrality, we find a previously unidentified correlated regime featuring a substantially enhanced flat band splitting that we describe within a microscopic model predicting a strong tendency towards nematic ordering. Our results provide insights into symmetry breaking correlation effects and highlight the importance of electronic interactions for all filling factors in twisted bilayer graphene.

cond-mat.mes-hall

Simulating spin systems with Majorana networks

With the discovery of Majorana quasiparticles in semiconductor-superconductor hybrid structures, topologically protected qubits have emerged as a promising contender for quantum information processing. While the construction of a universal quantum computer with topological protection likely requires significant advances in materials science, intermediate-scale devices are nearly within the reach of current technology. As a near-term milestone for topological qubits, we propose a network of topological superconductors as a simulator of a large variety of quantum spin systems, including those with frustration. Our proposal is founded on existing technology, combining advantages of semiconducting and superconducting qubits. We identify local measurement protocols that give access to information about ground and excited states as well as dynamic correlations. The topological protection of the qubits results in longer coherence times, and relaxation to the groundstate can be controlled by coupling the network an external bath. We conclude by pointing out specific applications of the quantum simulator, e.g., spin liquids, quantum criticality, and thermalization.

cond-mat.mes-hall

Triangular antiferromagnetism on the honeycomb lattice of twisted bilayer graphene

We present the electronic band structures of states with the same symmetry as the three-sublattice planar antiferromagnetic order of the triangular lattice. Such states can also be defined on the honeycomb lattice provided the spin density waves lie on the bonds. We identify cases which are consistent with observations on twisted bilayer graphene: a correlated insulator with an energy gap, yielding a single doubly-degenerate Fermi surface upon hole doping. We also discuss extensions to metallic states which preserve spin rotation invariance, with fluctuating spin density waves and bulk $\mathbb{Z}_2$ topological order.

cond-mat.str-el

Deconfined Quantum Critical Point on the Triangular Lattice

We first propose a topological term that captures the "intertwinement" between the standard "$\sqrt{3} \times \sqrt{3}$" antiferromagnetic order (or the so-called 120$^\circ$ state) and the "$\sqrt{12}\times \sqrt{12}$" valence solid bond (VBS) order for spin-1/2 systems on a triangular lattice. Then using a controlled renormalization group calculation, we demonstrate that there exists an unfine-tuned direct continuous deconfined quantum critical point (dQCP) between the two ordered phases mentioned above. This dQCP is described by the $N_f = 4$ quantum electrodynamics (QED) with an emergent PSU(4)=SU(4)/$Z_4$ symmetry only at the critical point. The topological term aforementioned is also naturally derived from the $N_f = 4 $ QED. We also point out that physics around this dQCP is analogous to the boundary of a $3d$ bosonic symmetry protected topological state with on-site symmetries only.

cond-mat.str-el