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Alexander I. Kuklin

Publications and source records attributed to Alexander I. Kuklin.

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Revised scattering exponents for a power-law distribution of surface and mass fractals

We consider scattering exponents arising in small-angle scattering from power-law polydisperse surface and mass fractals. It is shown that a set of fractals, whose sizes are distributed according to a power-law, can change its fractal dimension when the power-law exponent is sufficiently big. As a result, the scattering exponent corresponding to this dimension appears due to the spatial correlations between positions of different fractals. For large values of the momentum transfer, the correlations do not play any role, and the resulting scattering intensity is given by a sum of intensities of all composing fractals. The restrictions imposed on the power-law exponents are found. The obtained results generalize Martin's formulas for the scattering exponents of the polydisperse fractals.

cond-mat.mtrl-sci

Small-angle scattering from three-phase systems: Investigation of the crossover between mass fractal regimes

In this paper, we construct a three-phase model (that is, a system consisting of three homogeneous regions with various scattering length densities), which illustrate the behavior of small-angle scattering (SAS) scattering curves. Here two phases are a deterministic fractal embedded in another deterministic mass fractal, and they altogether are further embedded in a third phase, which can be a solution or solid matrix. We calculate SAS intensities, derive expressions for the crossover position (that is, the point where the power-law scattering exponent changes) as a function of control parameters, including size, concentration, and volumes of each phase. The corresponding SAS intensities from these models describe a succession of power-law regimes in momentum space where both regimes correspond to mass fractals. The models can be applied to SAS data where the absolute value of the scattering exponent of the first power-law regime is higher than that of the subsequent second power-law regime, that is, the scattering curve of convex kind near the crossover position.

cond-mat.stat-mech