arXiv subjects

Alexander Kubanek

Publications and source records attributed to Alexander Kubanek.

At least 37 records · Page 2Linked to original sources

arXiv2023

All-Optical Spin Initialization via a Cavity Broadened Optical Transition in On-Chip Hybrid Quantum Photonics

Hybrid quantum photonic systems connect classical photonics to the quantum world and promise to deliver efficient light-matter quantum interfaces while leveraging the advantages of both, the classical and the quantum, subsystems. However, combining efficient, scalable photonics and solid state quantum systems with desirable optical and spin properties remains a formidable challenge. In particular the access to individual spin states and coherent mapping to photons remains unsolved for these systems. In this letter, we demonstrate all-optical initialization and readout of the electronic spin of a negatively-charged silicon-vacancy center in a nanodiamond coupled to a silicon nitride photonic crystal cavity. We characterize relevant parameters of the coupled emitter-cavity system and determine the silicon-vacancy center's spin-relaxation and spin-decoherence rate. Our results mark an important step towards the realization of a hybrid spin-photon interface based on silicon nitride photonics and the silicon-vacancy center's electron spin in nanodiamonds with potential use for quantum networks, quantum communication and distributed quantum computation.

quant-ph↗

arXiv2023

Two-Photon Interference from Silicon-Vacancy Centers in Remote Nanodiamonds

The generation of indistinguishable photons is a key requirement for solid-state quantum emitters as a viable source for applications in quantum technologies. Restricting the dimensions of the solid-state host to a size well below the wavelength of light emitted by a defect-center enables efficient external optical coupling, for example for hybrid integration into photonic devices. However, stringent restrictions on the host dimensions result in severe limitations on the spectral properties reducing the indistinguishability of emitted photons. Here, we demonstrate two-photon interference from two negatively-charged Silicon-Vacancy centers located in remote nanodiamonds. The Hong-Ou-Mandel interference efficiency reaches 61% with a coalescence time window of 0.35 ns. We furthermore show a high yield of pairs of Silicon-Vacancy centers with indistinguishable optical transitions. Therefore, our work opens new paths in hybrid quantum technology based on indistinguishable single-photon emitters in nanodiamonds.

physics.optics↗

arXiv2023

Room Temperature Fiber-Coupled single-photon devices based on Colloidal Quantum Dots and SiV centers in Back Excited Nanoantennas

We demonstrate an important step towards on chip integration of single photon sources operating at room temperature fiber coupling of a directional quantum emitter with back-excitation. Directionality is achieved with a hybrid metal-dielectric bullseye antenna, while back-excitation is permitted by placement of the emitter at or in a sub-wavelength hole positioned at the bullseye center. Overall, the unique design enables a direct laser excitation from the back of the on-chip device and very efficient coupling of the highly collimated photon emission to either low numerical aperture (NA) free space optics or directly to an optical fiber from the front. To show the versatility of the concept, we fabricate devices containing either a colloidal quantum dot or a silicon-vacancy center containing nanodiamond, which are accurately coupled to the nano-antenna using two different nano-positioning methods. Both back-excited devices display front collection efficiencies of about 70 % at NAs as low as 0.5. Moreover, the combination of back-excitation with forward low-NA directionality enables direct coupling of the emitted photons into a proximal optical fiber without the need of any coupling optics, thereby facilitating and greatly simplifying future integration.

physics.optics↗

arXiv2022

A Quantum Repeater Platform based on Single SiV$^-$ Centers in Diamond with Cavity-Assisted, All-Optical Spin Access and Fast Coherent Driving

Quantum key distribution enables secure communication based on the principles of quantum mechanics. The distance in fiber-based quantum communication is limited to about a hundred kilometers due to signal attenuation. Thus, quantum repeaters are required to establish large-scale quantum networks. Ideal quantum repeater nodes possess a quantum memory which is efficiently connected to photons, the carrier of quantum information. Color centers in diamond and, in particular, the negatively-charged silicon-vacancy centers are promising candidates to establish such nodes. The major obstacle is an inefficient connection between the color centers spin to the Gaussian optics of fiber networks. Here, we present an efficient spin-photon interface. Individual silicon-vacancy centers coupled to the mode of a hemispherical Fabry-Pérot microcavity show Purcell-factors larger than 1 when operated in a bath of liquid Helium. We demonstrate coherent optical driving with a Rabi frequency of $290\,\mathrm{MHz}$ and all-optical access to the electron spin in strong magnetic fields of up to $3.2\,\mathrm{T}$. Spin initialization within $67\,\mathrm{ns}$ with a fidelity of $80\,\%$ and a lifetime of $350\,\mathrm{ns}$ are reached inside the cavity. The spin-photon interface is passively stable, enabled by placing a color center containing nanodiamond in the hemispherical Fabry-Pérot mirror structure and by choosing short cavity lengths. Therefore, our demonstration opens the way to realize quantum repeater applications.

quant-ph↗

arXiv2022

A first-principles calculation of electron-phonon interactions for the $\text{C}_2\text{C}_\text{N}$ and $\text{V}_\text{N}\text{N}_\text{B}$ defects in hexagonal boron nitride

Quantum emitters in two-dimensional hexagonal boron nitride (h-BN) have generated significant interest due to observations of ultra-bright emission made at room temperature. The expectation that solid-state emitters exhibit broad zero-phonon lines at elevated temperatures has been put in question by recent observations of Fourier transform (FT) limited photons emitted from h-BN flakes at room temperature. The mechanism responsible for the narrow lines has been suggested to be a mechanical decoupling from in-plane phonons due to an out-of-plane distortion of the emitter's orbitals. All decoupled emitters produce photons that are directed in-plane, suggesting that the dipoles are oriented perpendicular to the h-BN plane. Motivated by the promise of an efficient and scalable source of indistinguishable photons that can operate at room temperature, we have developed an approach using density functional theory (DFT) to determine the electron-phonon coupling for defects that have in- and out-of-plane transition dipole moments. Our DFT calculations reveal that the $\text{C}_2 \text{C}_\text{N}$ defect has an in-plane transition dipole moment, and that of the $\text{V}_\text{N} \text{N}_\text{B}$ defect is perpendicular to the plane. We exploit the two-dimensional framework recently implemented in \texttt{QUANTUM ESPRESSO} to determine both the phonon density of states and the electron-phonon matrix elements associated with the h-BN defective structures. We find no indication that an out-of-plane transition dipole is sufficient to obtain FT-limited photons at room temperature. Our work also provides direction to future DFT software developments and adds to the growing list of calculations relevant to researchers in the field of solid-state quantum information processing.

cond-mat.mtrl-sci↗

arXiv2022

Hybrid Quantum Nanophotonics: Interfacing Color Center in Nanodiamonds with Si3N4-Photonics

This chapter covers recent developments in the field of hybrid quantum photonics based on color centers in nanodiamonds and Si3N4-photonics towards a technology platform with applications in quantum information processing and quantum information distribution. The methodological approach can be divided in three main tasks. First, the fabrication and optimization of Si3N4-photonics. Second, the creation, characterization and control of color centers in nanodiamonds. Third, the assembly of hybrid quantum photonics by integrating the nanodiamonds into the photonic structures. One focus will be the efficient interfacing of the color centers done by optimizing the optical coupling. The chapter describes recent progress in all three steps and summarizes the established hybrid platform. We believe, that the hybrid approach provides a promising path to realize quantum photonic applications, such as quantum networks or quantum repeaters, in the near future.

quant-ph↗

arXiv2022

Review on coherent quantum emitters in hexagonal boron nitride

Hexagonal boron nitride is an emerging two-dimensional material with far-reaching applications in fields like nanophotonics or nanomechanics. Its layered architecture plays a key role for new materials such as Van der Waals heterostructures. The layered structure has also unique implications for hosted, optically active defect centers. A very special type of defect center arises from the possibility to host mechanically isolated orbitals localized between the layers. The resulting absence of coupling to low-frequency acoustic phonons turns out to be the essential element to protect the coherence of optical transitions from mechanical interactions with the environment. Consequently, the spectral transition linewidth remains unusually narrow even at room temperature, thus paving a new way towards coherent quantum optics under ambient conditions. In this review, I summarize the state-of-the-art of defect centers in hexagonal boron nitride with a focus on optically coherent defect centers. I discuss the current understanding of the defect centers, remaining questions and potential research directions to overcome pervasive challenges. The field is put into a broad perspective with impact on quantum technology such as quantum optics, quantum photonics as well as spin optomechanics.

quant-ph↗

arXiv2021

On-chip single-photon subtraction by individual silicon vacancy centers in a laser-written diamond waveguide

Modifying light fields at single-photon level is a key challenge for upcoming quantum technologies and can be realized in a scalable manner through integrated quantum photonics. Laser-written diamond photonics offers three-dimensional fabrication capabilities and large mode-field diameters matched to fiber optic technology, though limiting the cooperativity at the single-emitter level. To realize large cooperativities, we combine excitation of single shallow-implanted silicon vacancy centers via large numerical aperture optics with detection assisted by laser-written type-II waveguides. We demonstrate single-emitter extinction measurements with a cooperativity of 0.153 and a beta factor of 13% yielding 15.3% as lower bound for the quantum efficiency of a single emitter. The transmission of resonant photons reveals single-photon subtraction from a quasi-coherent field resulting in super-Poissonian light statistics. Our architecture enables single quantum level light field engineering in an integrated design which can be fabricated in three dimensions and with a natural connectivity to optical fiber arrays.

quant-ph↗

arXiv2021

Prolonged orbital relaxation by locally modified phonon density of states for SiV$^-$ center in nanodiamonds

Coherent quantum systems are a key resource for emerging quantum technology. Solid-state spin systems are of particular importance for compact and scalable devices. However, interaction with the solid-state host degrades the coherence properties. The negatively-charged silicon vacancy center in diamond is such an example. While spectral properties are outstanding, with optical coherence protected by the defects symmetry, the spin coherence is susceptible to rapid orbital relaxation limiting the spin dephasing time. A prolongation of the orbital relaxation time is therefore of utmost urgency and has been tackled by operating at very low temperatures or by introducing large strain. However, both methods have significant drawbacks, the former requires use of dilution refrigerators and the latter affects intrinsic symmetries. Here, a novel method is presented to prolong the orbital relaxation with a locally modified phonon density of states in the relevant frequency range, by restricting the diamond host to below 100 nm. The method works at liquid Helium temperatures of few Kelvin and in the low-strain regime.

quant-ph↗

arXiv2021

A Robust Coherent Single-Photon Interface for Moderate- NA Optics Based on SiV Center in Nanodiamonds and a Plasmonic Bullseye Antenna

Coherent exchange of single photons is at the heart of applied Quantum Optics. The negatively-charged silicon vacancy center in diamond is among most promising sources for coherent single photons. Its large Debye-Waller factor, short lifetime and extraordinary spectral stability is unique in the field of solid-state single photon sources. However, the excitation and detection of individual centers requires high numerical aperture optics which, combined with the need for cryogenic temperatures, puts technical overhead on experimental realizations. Here, we investigate a hybrid quantum photonics platform based on silicon-vacancy center in nanodiamonds and metallic bullseye antenna to realize a coherent single-photon interface that operates efficiently down to low numerical aperture optics with an inherent resistance to misalignment.

physics.optics↗

arXiv2021

Single photon randomness originating from the symmetry of dipole emission and the unpredictability of spontaneous emission

Quantum random number generation is a key ingredient for quantum cryptography and fundamental quantum optics and could advance Monte-Carlo simulations and machine learning. An established generation scheme is based on single photons impinging on a beam splitter. Here, we experimentally demonstrate quantum random number generation solely based on the spontaneous emission process in combination with the symmetric emission profile of a dipole aligned orthogonal to the laboratory frame. The demonstration builds on defect centers in hexagonal boron nitride and benefits from the ability to manipulate and align the emission directionality. We prove the randomness in the correlated photon detection events making use of the NIST randomness test suite and show that the randomness remains for two independently emitting defect centers. The scheme can be extended to random number generation by coherent single photons with potential applications in solid-state based quantum communication at room temperature.

quant-ph↗

arXiv2021

Hybrid quantum photonics based on artificial atoms placed inside one hole of a photonic crystal cavity

Spin-based quantum photonics promise to realize distributed quantum computing and quantum networks. The performance depends on efficient entanglement distribution, where the efficiency can be boosted by means of cavity quantum electrodynamics. The central challenge is the development of compact devices with large spin-photon coupling rates and high operation bandwidth. Photonic crystal cavities comprise strong field confinement but put high demands on accurate positioning of an atomic system in the mode field maximum. Color center in diamond, and in particular the negatively-charged Silicon-Vacancy center, emerged as a promising atom-like systems. Large spectral stability and access to long-lived, nuclear spin memories enabled elementary demonstrations of quantum network nodes including memory-enhanced quantum communication. In a hybrid approach, we deterministically place SiV$^-$-containing nanodiamonds inside one hole of a one-dimensional, free-standing, Si$_3$N$_4$-based photonic crystal cavity and coherently couple individual optical transitions to the cavity mode. We optimize the light-matter coupling by utilizing two-mode composition, waveguiding, Purcell-enhancement and cavity resonance tuning. The resulting photon flux is increased by more than a factor of 14 as compared to free-space. The corresponding lifetime shortening to below 460 ps puts the potential operation bandwidth beyond GHz rates. Our results mark an important step to realize quantum network nodes based on hybrid quantum photonics with SiV$^-$- center in nanodiamonds.

cond-mat.mtrl-sci↗

arXiv2020

An integrated magnetometry platform with stackable waveguide-assisted detection channels for sensing arrays

The negatively-charged NV$^-$-center in diamond has shown great success in nanoscale, high-sensitivity magnetometry. Efficient fluorescence detection is crucial for improving the sensitivity. Furthermore, integrated devices enable practicable sensors. Here, we present a novel architecture which allows us to create NV$^-$-centers a few nanometers below the diamond surface, and at the same time in the mode field maximum of femtosecond-laser-written type-II waveguides. We experimentally verify the coupling efficiency, showcase the detection of magnetic resonance signals through the waveguides and perform first proof-of-principle experiments in magnetic field and temperature sensing. The sensing task can be operated via the waveguide without direct light illumination through the sample, which marks an important step for magnetometry in biological systems which are fragile to light. In the future, our approach will enable the development of two-dimensional sensing arrays facilitating spatially and temporally correlated magnetometry.

physics.optics↗

arXiv2020

Tunable quantum photonics platform based on fiber-cavity enhanced single photon emission from two-dimensional hBN

Realization of quantum photonic devices requires coupling single quantum emitters to the mode of optical resonators. In this work we present a hybrid system consisting of defect centers in few-layer hBN grown by chemical vapor deposition and a fiber-based Fabry-Perot cavity. The sub 10 nm thickness of hBN and its smooth surface enables efficient integration into the cavity mode. We operate our hybrid platform over a broad spectral range larger than 30 nm and use its tuneability to explore different coupling regimes. Consequently, we achieve very large cavity-assisted signal enhancement up to 50-fold and equally strong linewidth narrowing owing to cavity funneling, both records for hBN-cavity systems. Additionally, we implement an excitation and readout scheme for resonant excitation that allows us to establish cavity-assisted PLE spectroscopy. Our work marks an important milestone for the deployment of 2D materials coupled to fiber-based cavities in practical quantum technologies.

physics.app-ph↗

arXiv2020

Purcell-Enhanced Emission from Individual SiV$^-$ Center in Nanodiamonds Coupled to a Si$_3$N$_4$-Based, Photonic Crystal Cavity

Hybrid quantum photonics combines classical photonics with quantum emitters in a postprocessing step. It facilitates to link ideal quantum light sources to optimized photonic platforms. Optical cavities enable to harness the Purcell-effect boosting the device efficiency. Here, we postprocess a free-standing, crossed-waveguide photonic crystal cavity based on Si$_3$N$_4$ with SiV$^-$ center in nanodiamonds. We develop a routine that holds the capability to optimize all degrees of freedom of the evanescent coupling term utilizing AFM nanomanipulation. After a few optimization cycles we resolve the fine-structure of individual SiV$^-$ centers and achieve a Purcell enhancement of more than 4 on individual optical transitions, meaning that four out of five spontaneously emitted photons are channeled into the photonic device. Our work opens up new avenues to construct efficient quantum photonic devices.

cond-mat.mtrl-sci↗

arXiv2020

Mechanical Decoupling of Quantum Emitters in Hexagonal Boron Nitride from Low-Energy Phonon Modes

Quantum emitters in hexagonal Boron Nitride (hBN) were recently reported to hol a homogeneous linewidth according to the Fourier-Transform limit up to room temperature. This unusual observation was traced back to decoupling from in-plane phonon modes which can arise if the emitter is located between two planes of the hBN host material. In this work, we investigate the origins for the mechanical decoupling. Improved sample preparation enabled a reduced background and a 70-fold decrease of spectral diffusion which was so far the major drawback of defect center in hBN and allowed us to reveal a gap in the electron-phonon spectral density for low phonon frequencies. This decoupling from phonons persists at room temperature and explains the observed Fourier Transform limited lines up to 300K. Furthermore, we investigate the dipole emission directionality and show a preferred photon emission through the side of the hBN flakes supporting the claim for an out-of-plane distortion of the defect center. Our work lays the foundation to a deeper understanding of the underlying physics for the persistence of Fourier-Transform limit lines up to room temperature. It furthermore provides a description on how to identify the mechanically isolated emitter within the large number of defect centers in hBN. Therefore, it paves the way for quantum optics applications with defect centers in hBN at room temperature.

cond-mat.mes-hall↗

arXiv2019

Preparing single SiV$^{-}$ center in nanodiamonds for external, optical coupling with access to all degrees of freedom

Optical coupling enables intermediate- and long-range interactions between distant quantum emitters. Such interaction may be the basic element in bottom-up approaches of coupled spin systems or for integrated quantum photonics and quantum plasmonics. Here, we prepare nanodiamonds carrying single, negatively-charged silicon-vacancy centers for evanescent optical coupling with access to all degrees of freedom by means of atomic force nanomanipulation. The color centers feature excellent optical properties, comparable to silicon-vacancy centers in bulk diamond, resulting in a resolvable fine structure splitting, a linewidth close to the Fourier-Transform limit under resonant excitation and a good polarization contrast. We determine the orbital relaxation time $T_{1}$ of the orbitally split ground states and show that all optical properties are conserved during translational nanomanipulation. Furthermore, we demonstrate the rotation of the nanodiamonds. In contrast to the translational operation, the rotation leads to a change in polarization contrast. We utilize the change in polarization contrast before and after nanomanipulation to determine the rotation angle. Finally, we evaluate the likelihood for indistinguishable, single photon emission of silicon-vacancy centers located in different nanodiamonds. Our work enables ideal evanescent, optical coupling of distant nanodiamonds containing silicon-vacancy centers with applications in the realization of quantum networks, quantum repeaters or complex quantum systems.

cond-mat.mtrl-sci↗

arXiv2019

A Diamond-Photonics Platform Based on Silicon-Vacancy Centers in a Single Crystal Diamond Membrane and a Fiber-Cavity

We realize a potential platform for an efficient spin-photon interface, namely negatively-charged silicon-vacancy centers in a diamond membrane coupled to the mode of a fully-tunable, fiber-based, optical resonator. We demonstrate that introducing the thin ($\sim 200 \, \text{nm}$), single crystal diamond membrane into the mode of the resonator does not change the cavity properties, which is one of the crucial points for an efficient spin-photon interface. In particular, we observe constantly high Finesse values of up to $3000$ and a linear dispersion in the presence of the membrane. We observe cavity-coupled fluorescence froman ensemble of SiV$^{-}$ centers with an enhancement factor of $\sim 1.9$. Furthermore from our investigations we extract the ensemble absorption and extrapolate an absorption cross section of $(2.9 \, \pm \, 2) \, \cdot \, 10^{-12} \, \text{cm}^{2}$ for a single SiV$^{-}$ center, much higher than previously reported.

physics.app-ph↗