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Alexander Mistonov

Publications and source records attributed to Alexander Mistonov.

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Probing bulk superconductivity in centrosymmetric Te-doped PtBi$_2$ single crystals

The Weyl semimetal $\gamma$-PtBi$_2$ has been shown to be one of the most promising novel materials, recently proposed as a topological i-wave superconductor. A crucial requirement for observing this physics is the absence of inversion symmetry in its trigonal $P31m$ crystal structure. Centrosymmetry has been reported to be readily restored in the $P\overline{3}m1$ structure upon electron doping, partially substituting Bi with as little as 2% Te. In this work, we synthesized Te-doped PtBi$_{2-x}$Te$_{x}$ samples and thoroughly investigated the bulk superconductivity of selected single crystals with nominal composition PtBi$_{1.96}$Te$_{0.04}$, exhibiting the highest superconducting volume fraction of $\sim100$%. Single crystal XRD measurements confirm the centrosymmetric $P\overline{3}m1$ structure in our samples, whereas bulk superconductivity with a critical temperature of $T_\mathrm{c} \approx 2.4\,$K was observed in magnetization and specific heat measurements. The upper critical fields for two different orientations were determined as $H^{\parallel}_{\mathrm{c2}}(0)\approx 6.3\,$kOe for in-plane and $H^{\perp}_{\mathrm{c2}}(0)\approx 4.7\,$kOe for out-of-plane magnetic fields. Robust superconductivity was also found in resistance and point contact measurements, where the latter showed a slight enhancement of the critical temperature up to $T_\mathrm{c} \sim 3\,$K. Finally, ARPES measurements corroborate the centrosymmetric structure of our samples, showing a single surface termination and the absence of Fermi arcs.

cond-mat.supr-con

Disentangling the unusual magnetic anisotropy of the near-room-temperature ferromagnet Fe$_{4}$GeTe$_{2}$

In the quest for two-dimensional conducting materials with high ferromagnetic ordering temperature the new family of the layered Fe$_{n}$GeTe$_{2}$ compounds, especially the near-room-temperature ferromagnet Fe$_{4}$GeTe$_{2}$, receives a significant attention. Fe$_{4}$GeTe$_{2}$ features a peculiar spin reorientation transition at $T_\mathrm{SR} \sim 110$ K suggesting a non-trivial temperature evolution of the magnetic anisotropy (MA) - one of the main contributors to the stabilization of the magnetic order in the low-D systems. An electron spin resonance (ESR) spectroscopic study reported here provides quantitative insights into the unusual magnetic anisotropy of Fe$_{4}$GeTe$_{2}$. At high temperatures the total MA is mostly given by the demagnetization effect with a small contribution of the counteracting intrinsic magnetic anisotropy of an easy-axis type, whose growth below a characteristic temperature $T_{\rm shape} \sim 150$ K renders the sample seemingly isotropic at $T_\mathrm{SR}$. Below one further temperature $T_{\rm d} \sim 50$ K the intrinsic MA becomes even more complex. Importantly, all the characteristic temperatures found in the ESR experiment match those observed in transport measurements, suggesting an inherent coupling between magnetic and electronic degrees of freedom in Fe$_{4}$GeTe$_{2}$. This finding together with the observed signatures of the intrinsic two-dimensionality should facilitate optimization routes for the use of Fe$_{4}$GeTe$_{2}$ in the magneto-electronic devices, potentially even in the monolayer limit.

cond-mat.str-el

Disordered ground state in the three-dimensional face-centred frustrated spin-$\frac{5}{2}$ system MnSn(OH)$_\text{6}$

Frustrated magnetism in face-centred cubic (fcc) magnetic sublattices remains underexplored but holds considerable potential for exotic magnetic behaviour. Here we report on the crystal structure, magnetic and thermodynamic properties of the $A$-site-vacant double hydroxide perovskite MnSn(OH)$_6$. Despite dominant antiferromagnetic interactions among Mn$^{2+}$ moments, evidenced by a negative Curie-Weiss temperature, the lack of a sharp thermodynamic transition down to 350$\,$mK implies the absence of long-range magnetic order. However, a broad hump in the specific heat at 1.6$\,$K suggests short-range correlations. Neutron diffraction at low temperatures confirms the presence of three-dimensional antiferromagnetic correlations, manifested as diffuse magnetic scattering with a correlation length $\xi = 24.66\,${\AA} and magnetic propagation vectors $\mathbf{k}=(\frac{1}{2}\,\frac{1}{2}\,\frac{1}{2})$ and $(0\,0.625\,0)$ at 20$\,$mK.

cond-mat.str-el