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Alexander Morozov

Publications and source records attributed to Alexander Morozov.

At least 19 recordsLinked to original sources

No need to stay positive: a practical approach to direct numerical simulations of elastic turbulence

Successfully performing direct numerical simulations of polymeric flows remains a major challenge in computational fluid mechanics. In addition to the velocity field, such simulations must resolve polymeric degrees of freedom, often expressed via the conformation tensor, $\mathbf{c}$, which captures the local stretch of polymer molecules. A key difficulty here lies in maintaining the physical requirement $\mathrm{Tr}\, \mathbf{c}>3$, which is not explicitly enforced by the governing equations. Consequently, simulations initiated from physical conditions may silently drift into unphysical states with $\mathrm{Tr}\, \mathbf{c}<0$, indicating a loss of positive-definiteness of the conformation tensor. Existing numerical methods to prevent this are costly, making direct numerical simulations of chaotic polymer flows, such as elastic turbulence, heavily reliant on high-performance computing. Here, we ask whether simulations that violate $\mathrm{Tr}\, \mathbf{c}>3$ can still yield meaningful physical insight into the underlying dynamics. We simulate a model dilute polymer solution driven through a plane channel at low Reynolds number and observe the transition to elastic turbulence. Our simulations exhibit two threshold resolutions: below the first, they become numerically unstable and exhibit a finite-time blow-up; above the second, they maintain positive-definiteness. In between, simulations remain stable and chaotic despite local violations of $\mathrm{Tr}\, \mathbf{c}>3$. Surprisingly, these violations do not affect mid-plane statistics of velocity, its gradients, or polymer stretch, which match results from fully positive-definite simulations. This suggests that resolving flow structures or key flow statistics may not require the extreme resolutions needed to preserve positive-definiteness, potentially lowering computational barriers for studying elastic turbulence.

physics.flu-dyn

All-in-plane image sensors free from readout integrated circuits

High resolution image sensors require electrical access to each individual pixel for signal readout. Such access is especially challenging for ultra-miniaturized pixels, for heterogeneously integrated sensing and readout layers in long-wavelength detectors, and for novel light-sensing materials with unestablished integration to silicon chips. Here, we introduce and experimentally validate a novel imaging approach that does not require electrical connections to individual pixels. The sensor matrix involves photoresistive pixels connected neighbor-to-neighbor and packed into a rectangular lattice. The signal readout is based on electrical impedance tomography applied to the photoresistance: the photovoltage is measured at the matrix boundary at various positions of injected bias current, and the image is reconstructed algorithmically. We present experimental validations for moderate-size infrared imagers based on multilayer graphene (24 pixels) and amorphous vanadium oxide (264 pixels). The reconstruction procedure is mathematically stable, sustainable to variations of pixel resistivity and photosensitivity, and its complexity is that of linear system solution. The proposed method enables unprecedented architecture simplification of imaging devices.

cond-mat.mes-hall

Universal reconstructive polarimetry with graphene-metal infrared photodetectors

Recent advent of smart photodetectors, where in-situ tuning of responsivity enables the reconstruction of light intensity, polarization and spectrum by a single device, has revolutionized the field of optoelectronics. So far, most such reconstructive detectors were realized with non-scalable technology of van der Waals stacking. Here, we demonstrate the infrared reconstructive polarimetry with photodetectors based on conventional gated graphene-metal junctions. The reconstruction exploits the gate tuning of polarization contrast, which enables the determination of both infrared power and polarization angle from photovoltage measurements at two different gate voltages. The physics enabling the polarimetry lies in polarization-dependent shift of the electron hot spot near the contact, and the gate tuning of photosensitive barrier width. We further show the universality of polarization reconstruction, i.e. its feasibility with different geometries of the junction, and with graphene of different quality, from boron-nitride encapsulated flakes to the scalable chemical vapor deposited films.

cond-mat.mes-hall

Targeted synthesis of polycrystalline vanadium dioxide thin films via post-deposition annealing

Implementation of neuromorphic hardware is a promising way to improve the computing efficiency and decrease the energy consumption of artificial neural networks. For this purpose, electronic elements emulating the behavior of synapses and neurons have to be developed. In order to realize electronic artificial neurons, threshold resistive switches or memristors can be efficiently used. One of the most widespread materials for threshold switches is vanadium dioxide due to its property to demonstrate the metal-insulator transition at a temperature about 70 {\deg}C. However, the processes of VO$_{2}$ synthesis are quite restrictive in temperature and gas atmosphere conditions, which hinders its integration into CMOS fabrication. In this work, we propose a new method of VO$_{2}$ synthesis: reactive pulsed laser deposition from metallic V target in oxygen atmosphere at room temperature, followed by vacuum annealing. Our method enables target synthesis of an appropriate VO$_{2}$ phase in a polycrystalline thin film form by finely tuning oxygen pressure during room temperature deposition, which allows to relax the equipment demands, such as high temperature heating in oxygen. Successful targeted VO$_{2}$ synthesis under fabrication conditions close to back-end-of-line CMOS production, achieved in this work, show the way toward its large-scale microelectronic integration for neuromorphic hardware creation.

cond-mat.mtrl-sci

Narwhals and their blessings: exact coherent structures of elastic turbulence in channel flows

Solutions of long, flexible polymer molecules are complex fluids that simultaneously exhibit fluid-like and solid-like behaviour. When subjected to external flows, dilute polymer solutions develop elastic turbulence - a unique chaotic flow state absent in Newtonian fluids such as water. Unlike turbulence in Newtonian fluids, elastic turbulence arises from polymer stretching and alignment in the flow, and can occur even at vanishing inertia. While experimental realisations of elastic turbulence are well documented, its underlying mechanism remains poorly understood. In this paper, we present a perspective on the transition to elastic turbulence in pressure-driven channel flows, drawing on recent computational work from our group. We outline our current understanding of the transition in both two and three spatial dimensions, centred on two key building blocks: (i) narwhals, exact coherent states of the flow, and (ii) blessings, spatio-temporal intermittent states made up of several localised narwhal solutions. This contribution is based on a talk given by one of us (A.M.) at the 2024 APS DFD meeting.

physics.flu-dyn

Pseudo-giant number fluctuations and nematic order in microswimmer suspensions

Giant number fluctuations (GNFs), whereby the standard deviation $\Delta N$ in the local number of particles $\langle N \rangle$ grows faster than $\sqrt{\langle N \rangle}$, are a hallmark property of dry active matter systems with orientational order, such as a collection of granular particles on a vibrated plate. This contrasts with momentum-conserving ("wet") active matter systems, such as suspensions of swimming bacteria, where no theoretical prediction of GNFs exist, although numerous experimental observations of such enhanced fluctuations have been reported. In this Letter, we numerically confirm the emergence of super-Gaussian number fluctuations in a 3-dimensional suspension of pusher microswimmers undergoing a transition to collective motion. These fluctuations emerge sharply above the transition, but only for sufficiently large values of the bacterial persistence length $\ell_p = v_s / \lambda$, where $v_s$ is the bacterial swimming speed and $\lambda$ the tumbling rate. Crucially, these "pseudo-GNFs" differ from true GNFs, as they only occur on length scales shorter than the typical size $\xi$ of nematic patches in the collective motion state, which is in turn proportional to the single-swimmer persistence length $\ell_p$. Our results thus suggest that observations of enhanced density fluctuations in biological active matter systems actually represent transient effects that decay away beyond mesoscopic length scales, and raises the question to what extent "true" GNFs with universal properties can exist in the presence of fluid flows.

cond-mat.soft

3D active nematic disclinations behave as Majorana quasiparticles

Quasiparticles are low-energy excitations with important roles in condensed matter physics. An intriguing example is provided by Majorana fermions, quasiparticles which are identical to their antiparticles. Despite being implicated in neutrino oscillations and topological superconductivity, their experimental realisations remain scarce. Here we propose a purely classical realisation of Majorana fermions, in terms of 3-dimensional disclination lines in active nematics. Activity is required to overcome the elastic cost associated with these excitations, so they can appear in steady state. We combine topology and simulations to show that active nematics under confinement spontaneously create in their interior topologically charged disclination lines and loops, akin to Majorana quasiparticles with finite momentum. Within an elongated channel, we find a phenomenology similar to that of the Kitaev chain, as local Majorana-like excitations appear near surfaces, while a non-local system-spanning helical disclination line can arise along the centre. In unconfined active turbulence, Majorana-like charged loops are instead exceedingly rare, suggesting that boundaries are crucial to generate these quasiparticles, as in quantum condensed matter. We suggest that 3-dimensional active disclinations can be used to probe the physics of Majorana spinors at a much larger scale than traditionally considered, potentially facilitating the experimental observation of their dynamics.

cond-mat.soft

Combinatorics and topological weights of chromatin loop networks

Polymer physics models suggest that chromatin spontaneously folds into loop networks with transcription units (TUs), such as enhancers and promoters, as anchors. Here we use combinatoric arguments to enumerate the emergent chromatin loop networks, both in the case where TUs are labelled and where they are unlabelled. We then combine these mathematical results with those of computer simulations aimed at finding the inter-TU energy required to form a target loop network. We show that different topologies are vastly different in terms of both their combinatorial weight and energy of formation. We explain the latter result qualitatively by computing the topological weight of a given network -- i.e., its partition function in statistical mechanics language -- in the approximation where excluded volume interactions are neglected. Our results show that networks featuring local loops are statistically more likely with respect to networks including more non-local contacts. We suggest our classification of loop networks, together with our estimate of the combinatorial and topological weight of each network, will be relevant to catalogue 3D structures of chromatin fibres around eukaryotic genes, and to estimate their relative frequency in both simulations and experiments.

physics.bio-ph

Topological spectra and entropy of chromatin loop networks

The 3D folding of a mammalian gene can be studied by a polymer model, where the chromatin fibre is represented by a semiflexible polymer which interacts with multivalent proteins, representing complexes of DNA-binding transcription factors and RNA polymerases. This physical model leads to the natural emergence of clusters of proteins and binding sites, accompanied by the folding of chromatin into a set of topologies, each associated with a different network of loops. Here we combine numerics and analytics to first classify these networks and then find their relative importance or statistical weight, when the properties of the underlying polymer are those relevant to chromatin. Unlike polymer networks previously studied, our chromatin networks have finite average distances between successive binding sites, and this leads to giant differences between the weights of topologies with the same number of edges and nodes but different wiring. These weights strongly favour rosette-like structures with a local cloud of loops with respect to more complicated non-local topologies. Our results suggest that genes should overwhelmingly fold into a small fraction of all possible 3D topologies, which can be robustly characterised by the framework we propose here.

physics.bio-ph

Purely elastic turbulence in pressure-driven channel flows

Solutions of long, flexible polymer molecules are complex fluids that simultaneously exhibit fluid-like and solid-like behaviour. When subjected to an external flow, dilute polymer solutions exhibit elastic turbulence - a unique, chaotic flow state absent in Newtonian fluids, like water. Unlike its Newtonian counterpart, elastic turbulence is caused by polymer molecules stretching and aligning in the flow, and can occur at vanishing inertia. While experimental realisations of elastic turbulence are well-documented, there is currently no understanding of its mechanism. Here, we present large-scale direct numerical simulations of elastic turbulence in pressure-driven flows through straight channels. We demonstrate that the transition to elastic turbulence is sub-critical, giving rise to spot-like flow structures that, further away from the transition, eventually spread throughout the domain. We provide evidence that elastic turbulence is organised around unstable coherent states that are localised close to the channel midplane.

physics.flu-dyn

Collective motion in a sheet of microswimmers

Self-propelled micron-size particles suspended in a fluid, like bacteria or synthetic microswimmers, are strongly non-equilibrium systems where particle motility breaks the microscopic detailed balance, often resulting in large-scale collective motion. Previous theoretical work has identified long-range hydrodynamic interactions as the main driver of collective motion in unbounded dilute suspension of rear-actuated ("pusher") microswimmers. In contrast, most experimental studies of collective motion in microswimmer suspensions have been carried out in quasi-2-dimensional geometries such as in thin films or near solid or fluid interfaces, where both the swimmers' motion and their long-range flow fields become altered due to the proximity of a boundary. Here, we study numerically a minimal model of microswimmers in such a restricted geometry, where the particles move in the midplane between two no-slip walls. For pushers, we demonstrate collective motion with only short-ranged order, in contrast with the long-ranged flows observed in unbounded systems. For front-actuated ("puller") microswimmers, we discover a long-wavelength density instability resulting in the formation of dense microswimmer clusters. Both types of collective motion are fundamentally different from their previously studied counterparts in unbounded domains. Our results illustrate that hydrodynamic screening due to the presence of a wall is subdominant in determining the collective state of the suspension, which is instead dictated by the geometrical restriction of the swimmers' motion.

cond-mat.soft

Hydrodynamic instabilities in a 2-D sheet of microswimmers embedded in a 3-D fluid

A collection of microswimmers immersed in an incompressible fluid is characterised by strong interactions due to the long-range nature of the hydrodynamic fields generated by individual organisms. As a result, suspensions of rear-actuated `pusher' swimmers such as bacteria exhibit a collective motion state often referred to as `bacterial turbulence', characterised by large-scale chaotic flows. The onset of collective motion in pusher suspensions is classically understood within the framework of mean-field kinetic theories for dipolar swimmers. In bulk 2-D and 3-D, the theory predicts that the instability leading to bacterial turbulence is due to mutual swimmer reorientation and sets in at the largest length scale available to the suspension. Here, we construct a similar kinetic theory for the case of a dipolar microswimmer suspension restricted to a two-dimensional plane embedded in a three-dimensional incompressible fluid. This setting qualitatively mimics the effect of swimming close to a two-dimensional interface. We show that the in-plane flow fields are effectively compressible in spite of the incompressibility of the 3-D bulk fluid, and that microswimmers on average act as sources (pushers) or sinks (pullers). We analyse stability of the homogeneous and isotropic state, and find two types of instability that are qualitatively different from the bulk, three-dimensional case: First, we show that the analogue of the orientational pusher instability leading to bacterial turbulence in bulk systems instead occurs at the smallest length-scale available to the system. Second, an instability associated with density variations arises in puller suspensions as a generic consequence of the effective in-plane compressibility. We conclude that confinement can have a crucial role in determining the collective behaviour of microswimmer suspensions.

cond-mat.soft

Interplay between Brownian and hydrodynamic tracer diffusion in suspensions of swimming microorganisms

The general problem of tracer diffusion in non-equilibrium baths is important in a wide range of systems, from the cellular level to geographical lengthscales. In this paper, we revisit the archetypical example of such a system: a collection of small passive particles immersed in a dilute suspension of non-interacting dipolar microswimmers, representing bacteria or algae. In particular, we consider the interplay between thermal (Brownian) diffusion and hydrodynamic (active) diffusion due to the persistent advection of tracers by microswimmer flow fields. Previously, it has been argued that even a moderate amount of Brownian diffusion is sufficient to significantly reduce the persistence time of tracer advection, leading to a significantly reduced value of the effective active diffusion coefficient $D_A$ compared to the non-Brownian case. Here, we show by large-scale simulations and kinetic theory that this effect is in fact only practically relevant for microswimmers that effectively remain stationary while still stirring up the surrounding fluid, so-called \emph{shakers}. In contrast, for moderate and high values of the swimming speed $v_s$, relevant for biological microswimmer suspensions, the effect of Brownian motion on $D_A$ is negligible, leading to the effects of advection by microswimmers and Brownian motion being additive. This conclusion contrasts with previous results from the literature, and encourages a reinterpretation of recent experimental measurements of $D_A$ for tracer particles of varying size in bacterial suspensions.

cond-mat.soft

Active turbulence and spontaneous phase separation in inhomogeneous extensile active gels

We report numerical results for the hydrodynamics of inhomogeneous lyotropic and extensile active nematic gels. By simulating the coupled Cahn-Hilliard, Navier-Stokes, and Beris-Edwards equation for the evolution of the composition, flow and orientational order of an active nematic, we ask whether composition variations are important to determine its emergent physics. As in active gels of uniform composition, we find that increasing either activity or nematic tendency (e.g., overall active matter concentration) triggers a transition between an isotropic passive phase and an active nematic one. We show that composition inhomogeneities are important in the latter phase, where we find three types of possible dynamical regimes. First, we observe regular patterns with defects and vortices: these exist close to the passive-active transition. Second, for larger activity, or deeper in the nematic phase, we find active turbulence, as in active gels of uniform composition, but with exceedingly large composition variation. In the third regime, which is uniquely associated with inhomogeneity and occurs for large nematic tendency and low activity, we observe spontaneous microphase separation into active and passive domains. The microphase separated regime is notable in view of the absence of an explicit demixing term in the underlying free energy which we use, and we provide a theoretical analysis based on the common tangent construction which explains its existence. We hope this regime can be probed experimentally in the future.

cond-mat.soft

Linear stability analysis of purely elastic travelling wave solutions in pressure driven channel flows

Recent studies of pressure-driven flows of dilute polymer solutions in straight channels demonstrated the existence of two-dimensional coherent structures that are disconnected from the laminar state and appear through a sub-critical bifurcation from infinity. These travelling-wave solutions were suggested to organise the phase-space dynamics of purely elastic and elasto-inertial chaotic channel flows. Here, we consider a wide range of parameters, covering the purely-elastic and elasto-inertial cases, and demonstrate that the two-dimensional travelling-wave solutions are unstable when embedded in sufficiently wide three-dimensional domains. Our work demonstrates that studies of purely elastic and elasto-inertial turbulence in straight channels require three-dimensional simulations, and no reliable conclusions can be drawn from studying strictly two-dimensional channel flows.

physics.flu-dyn

Polymers in Swarming Bacterial Turbulence

We experimentally investigate the effects of polymer additives on the collective dynamics of swarming Serratia marcescens in quasi two-dimensional (2D) liquid films. We find that even minute amounts of polymers (< 20 ppm) can significantly enhance swimming speed and promote largescale coherent structures. Velocity statistics show that polymers suppress large velocity fluctuation, transforming the velocity distributions from super-Gaussian to Gaussian. Spatial and temporal correlation functions suggest that polymers increase both the size and lifetime of flow structures. The energy spectra show an exponential decay at low wavenumbers, with a characteristic length scale increasing with polymer concentration. Overall, these result show polymers can mediate bacteria interaction and promote large-scale coherence in dense active suspensions.

cond-mat.soft

Coherent structures in plane channel flow of dilute polymer solutions with vanishing inertia

When subjected to sufficiently strong velocity gradients, solutions of long, flexible polymers exhibit flow instabilities and chaotic motion, often referred to as elastic turbulence. Its mechanism differs from the familiar, inertia-driven turbulence in Newtonian fluids, and is poorly understood. Here, we demonstrate that the dynamics of purely elastic pressure-driven channel flows of dilute polymer solutions are organised by exact coherent structures that take the form of two-dimensional travelling waves. Our results demonstrate that no linear instability is required to sustain such travelling wave solutions, and that their origin is purely elastic in nature. We show that the associated stress profiles are characterised by thin, filament-like arrangements of polymer stretch, which is sustained by a solitary pair of vortices. We discuss the implications of the travelling wave solutions for the transition to elastic turbulence in straight channels, and propose ways for their detection in experiments.

physics.flu-dyn

Yield-stress transition in suspensions of deformable droplets

Yield-stress materials, which require a sufficiently large forcing to flow, are currently ill-understood theoretically. To gain insight into their yielding transition, here we study numerically the rheology of a suspension of deformable droplets under pressure-driven flow. We show that the suspension displays yield-stress behaviour, with the droplets remaining motionless when the applied body-force is below a critical value. In the non-flowing phase, droplets jam to form an amorphous structure, whereas they order in the flowing phase. Yielding is linked to a percolation transition in the contacts of droplet-droplet overlaps, and requires suitable wetting boundary conditions and strict conservation of the droplet area to exist. Close to the yielding transition, we find strong oscillations in the droplet motion which closely resemble those found experimentally in confined colloidal glasses under flow. We show that even when droplets are static the underlying solvent moves by permeation, so that the viscosity of the composite system is never truly infinite, and, as we discuss, its precise value ceases to be a bulk material property of the system.

cond-mat.soft