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Alexander O. Sushkov

Publications and source records attributed to Alexander O. Sushkov.

At least 19 recordsLinked to original sources
arXiv2026

Solid-state nuclear magnetic resonance search for axion-like dark matter with broadband SQUID magnetometry

We report the results of an experimental search for ultralight axion-like dark matter in the mass ranges 19.5--20.5 and 21.5--22 neV. The Cosmic Axion Spin Precession Experiment-electric probes the axion-nuclear electric dipole moment coupling. We perform solid-state nuclear magnetic resonance on $^{207}$Pb spin ensembles which reside in a polarized ferroelectric crystal. The background axion-like dark matter field induces an oscillating torque on the $^{207}$Pb spins via the electric dipole moment coupling $g_{d}$. The experiment is calibrated with pulsed magnetic resonance measurements covering two frequency bands (4.6--5.0 and 5.2--5.3 MHz) that correspond to the axion Compton frequencies associated with the identified axion mass ranges. By sweeping the leading magnetic field applied to the sample, we are able to detect the $^{207}$Pb nuclear magnetic resonance in these frequency ranges using a superconducting quantum interference device, inductively coupled to the sample with a broadband circuit. We establish the upper bounds $|g_{d}| < 4\times 10^{-4}$ GeV$^{-2}$ with 95% confidence in these frequency bands. Our results demonstrate the detection and small-tip angle calibration of low-field $^{207}$Pb nuclear magnetic resonance, allowing for sensitivity to axion-like dark matter in the nanoelectron-volt axion mass range.

hep-ex↗
arXiv2026

Control of relaxation properties of a macroscopic nuclear spin ensemble

Macroscopic spin ensembles in solids are powerful platforms for quantum sensing and precision metrology. A key challenge is controlling the nuclear spin population relaxation time $T_1$, which can become prohibitively long at cryogenic temperatures due to phonon freeze-out. We demonstrate optical control of the $T_1$ relaxation time of the $^{207}$Pb nuclear spin ensemble in lead-containing ferroelectric crystals PbTiO$_3$ (PT) and (PbMg$_{1/3}$Nb$_{2/3}$O$_3$)$_{2/3}$-(PbTiO$_3$)$_{1/3}$ (PMN-PT). Using X-band electron paramagnetic resonance (EPR) spectroscopy at 10 K, we characterize light-induced paramagnetic centers created by 405 nm laser illumination. In PT, we observe paramagnetic Pb$^{3+}$ centers and their hyperfine interaction with nearby nuclear spins. In PMN-PT, we identify two populations: isotropic Pb$^{3+}$ centers and anisotropic Ti$^{3+}$ centers occupying $d$-orbitals, with spin number densities of $(2.5 \pm 1.0) \times 10^{17}$ cm$^{-3}$ and $(4.1 \pm 1.7) \times 10^{17}$ cm$^{-3}$, respectively. Power-dependent EPR measurements enable extraction of spin relaxation times. We investigate the ionization and recombination dynamics of these transient paramagnetic centers. Using saturation-recovery nuclear magnetic resonance, we demonstrate that laser illumination reduces the $^{207}$Pb nuclear $T_1$ by approximately a factor of two, from $(17 \pm 2)$ s to $(7 \pm 1)$ s at 4.6 MHz, and from $(1550 \pm 40)$ s to $(850 \pm 70)$ s at 40 MHz. We develop a model relating the nuclear relaxation rate to the density of photoinduced paramagnetic centers. This optical control of nuclear spin relaxation provides a pathway toward accelerated thermal polarization and dynamic nuclear polarization in solid-state NMR-based precision measurements, including searches for axion-like dark matter.

cond-mat.other↗
arXiv2026

Cavity, lumped-circuit, and spin-based detection of axion dark matter: differences and similarities

Axions and axion-like particles are compelling candidates for ultralight bosonic dark matter, forming coherent oscillating fields that can be probed by experiments known as haloscopes. A broad range of haloscope concepts has been developed, including resonant cavity haloscopes, lumped-element circuit detectors, and spin-based experiments, each sensitive to different axion couplings and mass ranges. Rather than attempting an exhaustive survey of all existing approaches, this comparative review provides a unified framework for the major haloscope classes, establishing a common language for the descriptions of signal generation, noise properties, data analysis, and scanning strategies. Key properties of ultralight bosonic dark matter relevant for detection are summarized first, including coherence time, spectral linewidth, and stochasticity under the standard halo model. The discussion then compares cavity, Earth-scale, lumped-element, and spin haloscopes, focusing on expected signal shapes, dominant noise sources, and statistical frameworks for axion searches. Particular emphasis is placed on consistent definitions of signal-to-noise ratio and on how detector bandwidth, axion coherence, and noise characteristics determine optimal scan strategies. By systematically comparing operating principles and performance metrics across these detector families, this framework clarifies shared concepts as well as the essential differences that govern sensitivity in different mass and coupling regimes. The resulting perspective synthesizes current search methodologies and offers guidance for optimizing future haloscope experiments.

hep-ph↗
arXiv2025

Search for Axionlike Dark Matter Using Liquid-State Nuclear Magnetic Resonance

We search for dark matter in the form of axionlike particles (ALPs) in the mass range $5.576741 \,\mathrm{neV/c^2}$ - $5.577733\,\mathrm{neV/c^2}$ by probing their possible coupling to fermion spins through the ALP field gradient. This is achieved by performing proton nuclear magnetic resonance spectroscopy on a sample of methanol as a technical demonstration of the Cosmic Axion Spin Precession Experiment Gradient (CASPEr-Gradient) Low-Field apparatus. Searching for spin-coupled ALP dark matter in this mass range with associated Compton frequencies in a 240 Hz window centered at 1.348570 MHz resulted in a sensitivity to the ALP-proton coupling constant of $g_{\mathrm{ap}} \approx 3 \times 10^{-2}\,\mathrm{GeV}^{-1}$. This narrow-bandwidth search serves as a proof-of-principle and a commissioning measurement, validating our methodology and demonstrating the experiment's capabilities. CASPEr-Gradient Low-Field will probe the mass range from $4.1\,\mathrm{\peV/c^2}$ to $17\,\mathrm{\neV/c^2}$ with hyperpolarized samples to boost the sensitivity beyond the astronomical limits.

hep-ex↗
arXiv2025

Spin Squeezing of Macroscopic Nuclear Spin Ensembles

Spin squeezing has been explored in atomic systems as a tool for quantum sensing, improving experimental sensitivity beyond the spin standard quantum limit for certain measurements. To optimize absolute metrological sensitivity, it is beneficial to consider macroscopic spin ensembles, such as nuclear spins in solids and liquids. Coupling a macroscopic spin ensemble to a parametrically-modulated resonant circuit can create collective spin squeezing by generating spin correlations mediated by the circuit. We analyze the squeezing dynamics in the presence of decoherence and finite spin polarization, showing that achieving 7 dB spin squeezing is feasible in several nuclear spin systems. The metrological benefit of squeezing a macroscopic spin ensemble lies in the suppression of technical noise sources in the spin detection system relative to the spin projection noise. This expands the experimental sensitivity bandwidth when searching for signals of unknown frequency and can improve the resonant signal-to-noise ratio. Squeezing macroscopic spin ensembles may prove to be a useful technique for fundamental physics experiments aimed at detecting spin interactions with oscillating background fields, such as ultralight dark matter.

hep-ph↗
arXiv2024

Ultralight dark matter detection with levitated ferromagnets

Levitated ferromagnets act as ultraprecise magnetometers, which can exhibit high quality factors due to their excellent isolation from the environment. These instruments can be utilized in searches for ultralight dark matter candidates, such as axionlike dark matter or dark-photon dark matter. In addition to being sensitive to an axion-photon coupling or kinetic mixing, which produce physical magnetic fields, ferromagnets are also sensitive to the effective magnetic field (or "axion wind") produced by an axion-electron coupling. While the dynamics of a levitated ferromagnet in response to a DC magnetic field have been well studied, all of these couplings would produce AC fields. In this work, we study the response of a ferromagnet to an applied AC magnetic field and use these results to project their sensitivity to axion and dark-photon dark matter. We pay special attention to the direction of motion induced by an applied AC field, in particular, whether it precesses around the applied field (similar to an electron spin) or librates in the plane of the field (similar to a compass needle). We show that existing levitated ferromagnet setups can already have comparable sensitivity to an axion-electron coupling as comagnetometer or torsion balance experiments. In addition, future setups can become sensitive probes of axion-electron coupling, dark-photon kinetic mixing, and axion-photon coupling, for ultralight dark matter masses $m_\mathrm{DM}\lesssim\mathrm{feV}$.

hep-ph↗
arXiv2024

Searching for dark matter with a 1000 km baseline interferometer

Axion-like particles (ALPs) arise from well-motivated extensions to the Standard Model and could account for dark matter. ALP dark matter would manifest as a field oscillating at an (as of yet) unknown frequency. The frequency depends linearly on the ALP mass and plausibly ranges from $10^{-22}$ to $10$ eV/$c^2$. This motivates broadband search approaches. We report on a direct search for ALP dark matter with an interferometer composed of two atomic K-Rb-$^3$He comagnetometers, one situated in Mainz, Germany, and the other in Kraków, Poland. We leverage the anticipated spatio-temporal coherence properties of the ALP field and probe all ALP-gradient-spin interactions covering a mass range of nine orders of magnitude. No significant evidence of an ALP signal is found. We thus place new upper limits on the ALP-neutron, ALP-proton and ALP-electron couplings reaching below $g_{aNN}<10^{-9}$ GeV$^{-1}$, $g_{aPP}<10^{-7}$ GeV$^{-1}$ and $g_{aee}<10^{-6}$ GeV$^{-1}$, respectively. These limits improve upon previous laboratory constraints for neutron and proton couplings by up to three orders of magnitude.

hep-ph↗
arXiv2024

An Improved Bound on Nonlinear Quantum Mechanics using a Cryogenic Radio Frequency Experiment

There are strong arguments that quantum mechanics may be nonlinear in its dynamics. A discovery of nonlinearity would hint at a novel understanding of the interplay between gravity and quantum field theory, for example. As such, experiments searching for potential nonlinear effects in the electromagnetic sector are important. Here we outline such an experiment, consisting of a stream of random bits (which were generated using Rigetti's Aspen-M-3 chip) as input to an RF signal generator coupled to a cryogenic detector. Projective measurements of the qubit state, which is originally prepared in an equal superposition, serve as the random binary output of a signal generator. Thereafter, spectral analysis of the RF detector would yield a detectable excess signal predicted to arise from such a nonlinear effect. A comparison between the projective measurements of the quantum bits vs the classical baseline showed no power excess. This sets a new limit on the electromagnetic nonlinearity parameter $|ε| \lessapprox 1.15 \times 10^{-12}$, at a 90.0% confidence level. This is the most stringent limit on nonlinear quantum mechanics thus far and an improvement by nearly a factor of 50 over the previous experimental limit.

quant-ph↗
arXiv2023

Understanding the dynamics of randomly positioned dipolar spin ensembles

Dipolar spin ensembles with random spin positions attract much attention currently because they help to understand decoherence as it occurs in solid state quantum bits in contact with spin baths. Also, these ensembles are systems which may show many-body localization, at least in the sense of very slow spin dynamics. We present measurements of the autocorrelations of spins on diamond surfaces in a doubly-rotating frame which eliminates local disorder. Strikingly, the time scales in the longitudinal and the transversal channel differ by more than one order of magnitude which is a factor much greater than one would have expected from simulations of spins on lattices. A previously developed dynamic mean-field theory for spins (spinDMFT) fails to explain this phenomenon. Thus, we improve it by extending it to clusters (CspinDMFT). This theory does capture the striking mismatch up to two orders of magnitude for random ensembles. Without positional disorder, however, the mismatch is only moderate with a factor below 4. The pivotal role of positional disorder suggests that the strong mismatch is linked to precursors of many-body localization.

cond-mat.dis-nn↗
arXiv2023

Quantum Sensors for High Energy Physics

Strong motivation for investing in quantum sensing arises from the need to investigate phenomena that are very weakly coupled to the matter and fields well described by the Standard Model. These can be related to the problems of dark matter, dark sectors not necessarily related to dark matter (for example sterile neutrinos), dark energy and gravity, fundamental constants, and problems with the Standard Model itself including the Strong CP problem in QCD. Resulting experimental needs typically involve the measurement of very low energy impulses or low power periodic signals that are normally buried under large backgrounds. This report documents the findings of the 2023 Quantum Sensors for High Energy Physics workshop which identified enabling quantum information science technologies that could be utilized in future particle physics experiments, targeting high energy physics science goals.

hep-ex↗
arXiv2023

Frequency-scanning considerations in axionlike dark matter spin-precession experiments

Galactic dark matter may consist of axionlike particles (ALPs) that can be described as an "ultralight bosonic field" oscillating at the ALP Compton frequency. The ALP field can be searched for using nuclear magnetic resonance (NMR), where resonant precession of spins of a polarized sample can be sensitively detected. The ALP mass to which the experiment is sensitive is scanned by sweeping the bias magnetic field. The scanning either results in detection of ALP dark matter or rules out ALP dark matter with sufficiently strong couplings to nuclear spins over the range of ALP masses corresponding to the covered span of Larmor frequencies. In this work, scanning strategies are analyzed with the goal of optimizing the parameter-space coverage via a proper choice of experimental parameters (e.g., the effective transverse relaxation time).

physics.atom-ph↗
arXiv2023

Probing dynamics of a two-dimensional dipolar spin ensemble using single qubit sensor

Understanding the thermalization dynamics of quantum many-body systems at the microscopic level is among the central challenges of modern statistical physics. Here we experimentally investigate individual spin dynamics in a two-dimensional ensemble of electron spins on the surface of a diamond crystal. We use a near-surface NV center as a nanoscale magnetic sensor to probe correlation dynamics of individual spins in a dipolar interacting surface spin ensemble. We observe that the relaxation rate for each spin is significantly slower than the naive expectation based on independently estimated dipolar interaction strengths with nearest neighbors and is strongly correlated with the timescale of the local magnetic field fluctuation. We show that this anomalously slow relaxation rate is due to the presence of strong dynamical disorder and present a quantitative explanation based on dynamic resonance counting. Finally, we use resonant spin-lock driving to control the effective strength of the local magnetic fields and reveal the role of the dynamical disorder in different regimes. Our work paves the way towards microscopic study and control of quantum thermalization in strongly interacting disordered spin ensembles.

quant-ph↗
arXiv2023

Directional Detection of Dark Matter Using Solid-State Quantum Sensing

Next-generation dark matter (DM) detectors searching for weakly interacting massive particles (WIMPs) will be sensitive to coherent scattering from solar neutrinos, demanding an efficient background-signal discrimination tool. Directional detectors improve sensitivity to WIMP DM despite the irreducible neutrino background. Wide-bandgap semiconductors offer a path to directional detection in a high-density target material. A detector of this type operates in a hybrid mode. The WIMP or neutrino-induced nuclear recoil is detected using real-time charge, phonon, or photon collection. The directional signal, however, is imprinted as a durable sub-micron damage track in the lattice structure. This directional signal can be read out by a variety of atomic physics techniques, from point defect quantum sensing to x-ray microscopy. In this white paper, we present the detector principle and review the status of the experimental techniques required for directional readout of nuclear recoil tracks. Specifically, we focus on diamond as a target material; it is both a leading platform for emerging quantum technologies and a promising component of next-generation semiconductor electronics. Based on the development and demonstration of directional readout in diamond over the next decade, a future WIMP detector will leverage or motivate advances in multiple disciplines towards precision dark matter and neutrino physics.

physics.ins-det↗
arXiv2023

Intensity interferometry for ultralight bosonic dark matter detection

Ultralight bosonic dark matter (UBDM) can be described by a classical wave-like field oscillating near the Compton frequency of the bosons. If a measurement scheme for the direct detection of UBDM interactions is sensitive to a signature quadratic in the field, then there is a near-zero-frequency (dc) component of the signal. Thus, a detector with a given finite bandwidth can be used to search for bosons with Compton frequencies many orders of magnitude larger than its bandwidth. This opens the possibility of a detection scheme analogous to Hanbury Brown and Twiss intensity interferometry. Assuming that the UBDM is virialized in the galactic gravitational potential, the random velocities produce slight deviations from the Compton frequency. These result in stochastic fluctuations of the intensity on a time scale determined by the spread in kinetic energies. In order to mitigate ubiquitous local low-frequency noise, a network of sensors can be used to search for the stochastic intensity fluctuations by measuring cross-correlation between the sensors. This method is inherently broadband, since a large range of Compton frequencies will yield near-zero-frequency components within the sensor bandwidth that can be searched for simultaneously. Measurements with existing sensor networks have sufficient sensitivity to search experimentally unexplored parameter space.

hep-ph↗
arXiv2023

EuCl$_3\cdot 6$H$_2$O as the solid-state platform for searches for new P,T-odd physics

Condensed matter systems offer the opportunity to maximize the number of spins, probed in magnetic resonance experiments that search for physics beyond the standard model. EuCl$_3\cdot 6$H$_2$O is a promising solid-state platform for such searches. The narrow inhomogeneous linewidth of the Eu optical $^7\hspace{-0.1em}F_0 \leftrightarrow\,^5\hspace{-0.1em}D_0$ transition in this material opens the opportunity to optically pump the $^{153}$Eu nuclear spin ensemble into a single hyperfine sublevel. The closely-spaced opposite-parity nuclear energy levels, and the low-energy collective octupole mode, or a possible static octupole deformation, enhance the $^{153}$Eu nuclear Schiff moment. The optimistic estimate of the effective electric field is $E^*=10\,$MV/cm. With this estimate, the CASPEr-electric search for the gluon interaction of axion dark matter can reach QCD axion sensitivity with a 3~cm sample.

cond-mat.other↗
arXiv2023

Quantum Science and the Search for Axion Dark Matter

The dark matter puzzle is one of the most important open problems in modern physics. The ultra-light axion is a well-motivated dark matter candidate, conceived to resolve the strong-CP problem of quantum chromodynamics. Numerous precision experiments are searching for the three non-gravitational interactions of axion-like dark matter. Some of the searches are approaching fundamental quantum limits on their sensitivity. This Perspective describes several approaches that use quantum engineering to circumvent these limits. Squeezing and single-photon counting can enhance searches for the axion-photon interaction. Optimization of quantum spin ensemble properties is needed to realize the full potential of spin-based searches for the electric-dipole-moment and the gradient interactions of axion dark matter. Several metrological and sensing techniques, developed in the field of quantum information science, are finding natural applications in this area of experimental fundamental physics.

hep-ph↗
arXiv2023

Effective electric field: quantifying the sensitivity of searches for new P,T-odd physics with EuCl$_3\cdot$6H$_2$O

Laboratory-scale precision experiments are a promising approach to searching for physics beyond the standard model. Non-centrosymmetric solids offer favorable statistical sensitivity for efforts that search for new fields, whose interactions violate the discrete parity and time-reversal symmetries. One example is the electric Cosmic Axion Spin Precession Experiment (CASPEr-e), which is sensitive to the defining interaction of the QCD axion dark matter with gluons in atomic nuclei. The effective electric field is the parameter that quantifies the sensitivity of such experiments to new physics. We describe the theoretical approach to calculating the effective electric field for non-centrosymmetric sites in ionic insulating solids. We consider the specific example of the EuCl$_3\cdot$6H$_2$O crystal, which is a particularly promising material. The optimistic estimate of the effective electric field for the $^{153}$Eu isotope in this crystal is 10 MV/cm. The calculation uncertainty is estimated to be two orders of magnitude, dominated by the evaluation of the Europium nuclear Schiff moment.

physics.atom-ph↗
arXiv2022

Quantum Sensors for High Precision Measurements of Spin-dependent Interactions

The applications of spin-based quantum sensors to measurements probing fundamental physics are surveyed. Experimental methods and technologies developed for quantum information science have rapidly advanced in recent years, and these tools enable increasingly precise control and measurement of spin dynamics. Theories of beyond-the-Standard-Model physics predict, for example, symmetry violating electromagnetic moments aligned with particle spins, exotic spin-dependent forces, coupling of spins to ultralight bosonic dark matter fields, and changes to the local environment that affect spins. Spin-based quantum sensors can be used to search for these myriad phenomena, and offer a methodology for tests of fundamental physics that is complementary to particle colliders and large scale particle detectors. Areas of technological development that can significantly enhance the sensitivity of spin-based quantum sensors to new physics are highlighted.

quant-ph↗