arXiv subjects

Alexander Palevski

Publications and source records attributed to Alexander Palevski.

15 recordsLinked to original sources

arXiv2024

Gapless superconductivity in the low-frequency electrodynamic response of two-dimensional granular In/InO$_x$ composites

We measured the full complex ac conductance of two-dimensional granular In/InO$_x$ composites using the mutual inductance technique to explore the transition from a "failed-superconductor-turned anomalous metal" to a robust superconductor. In this system, room-temperature annealing was adopted to tune the InO$_x$-mediated coupling between In grains, allowing for the observation of both a "true" superconductor-to-insulator transition and the emergence of an intervening anomalous metallic state. In this paper, we show that further annealing increases the inter-grain coupling, which eliminates the anomalous metallic phase, but at the same time prevent the emergence of strong Bose-dominated insulating phase. The complex ac conductance revealed a $T\to0$ saturating dissipative response in a finite magnetic field, coexisting with a robust superfluid density. The anomalous power-law spectra for the dissipative response appear to indicate quantum critical behavior proximate to a quantum superconductor to anomalous-metal transition as probed in the kilo-Hertz range, and point to signatures of gapless superconductivity in our granular superconducting system.

cond-mat.supr-con↗

arXiv2023

Silvanite AuAgTe$_4$: a rare case of gold superconducting material

Gold is one of the most inert metals, forming very few compounds, some with rather interesting properties, and only two of them currently known to be superconducting under certain conditions (AuTe$_2$ and SrAuSi$_3$). Compounds of another noble element, Ag, are also relatively rare, and very few of them are superconducting. Finding new superconducting materials containing gold (and silver) is a challenge - especially having in mind that the best high-$T_c$ superconductors at normal conditions are based upon their rather close ''relative'', Cu. Here we report combined X-ray diffraction, Raman, and resistivity measurements, as well as first-principles calculations, to explore the effect of hydrostatic pressure on the properties of the sylvanite mineral, AuAgTe$_4$. Our experimental results, supported by density functional theory, reveal a structural phase transition at $\sim$5 GPa from a monoclinic $P2/c$ to $P2/m$ phase, resulting in almost identical coordinations of Au and Ag ions, with rather uniform interatomic distances. Further, resistivity measurements show the onset of superconductivity at $\sim$1.5 GPa in the $P2/c$ phase, followed by a linear increase of $T_c$ up to the phase transition, with a maximum in the $P2/m$ phase, and a gradual decrease afterwards. Our calculations indicate phonon-mediated superconductivity, with the electron-phonon coupling coming predominantly from the low-energy phonon modes. Thus, along with the discovery of a new superconducting compound of gold/silver, our results advance understanding of the mechanism of the superconductivity in Au-containing compounds, which may pave the way to the discovery of novel ones.

cond-mat.str-el↗

arXiv2022

Anomalous metals: from "failed superconductor" to "failed insulator"

Resistivity saturation is found on both superconducting and insulating sides of an "avoided" magnetic-field-tuned superconductor-to-insulator transition (H-SIT) in a two-dimensional In/InO$_x$ composite, where the anomalous metallic behaviors cut off conductivity or resistivity divergence in the zero-temperature limit. The granular morphology of the material implies a system of Josephson junctions (JJ) with a broad distribution of Josephson coupling E$_J$ and charging energy E$_C$ , with a H-SIT determined by the competition between E$_J$ and E$_C$ . By virtue of self-duality across the true H-SIT, we invoke macroscopic quantum tunneling effects to explain the temperature-independent resistance where the "failed superconductor" side is a consequence of phase fluctuations and the "failed insulator" side results from charge fluctuations. While true self-duality is lost in the avoided transition, its vestiges are argued to persist, owing to the incipient duality of the percolative nature of the dissipative path in the underlying random JJ system.

cond-mat.supr-con↗

arXiv2021

Superconductor-insulator transitions in three-dimensional indium-oxide at high pressures

Experiments investigating magnetic-field-tuned superconductor-insulator transition (HSIT) mostly focus on two-dimensional material systems where the transition and its proximate ground-state phases, often exhibit features that are seemingly at odds with the expected behavior. Here we present a complementary study of a three-dimensional pressure-packed amorphous indium-oxide (InOx) powder where granularity controls the HSIT. Above a low threshold pressure of ~0.2 GPa, vestiges of superconductivity are detected, although neither a true superconducting transition nor insulating behavior are observed. Instead, a saturation at very high resistivity at low pressure is followed by saturation at very low resistivity at higher pressure. We identify both as different manifestations of anomalous metallic phases dominated by superconducting fluctuations. By analogy with previous identification of the low resistance saturation as a "failed superconductor", our data suggests that the very high resistance saturation is a manifestation of a "failed insulator". Above a threshold pressure of ~6 GPa, the sample becomes fully packed, and superconductivity is robust, with TC tunable with pressure. A quantum critical point at PC~25 GPa marks the complete suppression of superconductivity. For a finite pressure below PC, a magnetic field is shown to induce a HSIT from a true zero-resistance superconducting state to a weakly insulating behavior. Determining the critical field, HC, we show that similar to the 2D behavior, the insulating-like state maintains a superconducting character, which is quenched at higher field, above which the magnetoresistance decreases to its fermionic normal state value.

cond-mat.supr-con↗

arXiv2021

Robust anomalous metallic states and vestiges of self duality in two-dimensional granular In-InOx composites

Many experiments investigating magnetic field tuned superconductor-insulator transition (H-SIT), often exhibit low-temperature resistance saturation, which is interpreted as an anomalous metallic phase emerging from a "failed superconductor," thus challenging conventional theory. Here we study a random granular array of indium islands grown on a gateable layer of indium-oxide. By tuning the intergrain couplings, we reveal a wide range of magnetic fields where resistance saturation is observed, under conditions of careful electromagnetic filtering and within a wide range of linear response. Exposure to external broadband noise or microwave radiation is shown to strengthen the tendency of superconductivity, where at low field a global superconducting phase is restored. Increasing magnetic field unveils an "avoided H-SIT," that exhibits granularity-induced logarithmic divergence of the resistance/conductance above/below that transition, pointing to possible vestiges of the original emergent duality observed in a true H-SIT. We conclude that anomalous metallic phase is intimately associated with inherent inhomogeneities, exhibiting robust behavior at attainable temperatures for strongly granular two-dimensional systems.

cond-mat.supr-con↗

arXiv2020

Superconductor-Insulator Transition and the Crossover to Non Equilibrium in two-dimensional Indium - Indium-Oxide composite

Magnetic-field tuned superconductor to insulator transition was observed in a novel hybrid system of granular superconducting indium, deposited on indium oxide thin film, which exhibits global superconductivity at low magnetic fields. We have used annealing to tune the coupling to lie just at the borderline where superconductivity in the underlying InOx is suppressed, which is also close to the metal-insulator transition of the InOx. The hybrid system exhibits a "giant" magnetoresistance above the H-SIT, with critical behavior that manifests the duality between Cooper pairs and vortices.

cond-mat.supr-con↗

arXiv2018

Proximity Effect in Superconducting-Ferromagnetic Granular Structures

We examined the proximity effect in granular films made of Pb, a superconductor, and Ni, a ferromagnet, with various compositions. Slow decay of the critical temperature as a function of the relative volume concentration of Ni per sample was demonstrated by our measurements, followed by a saturation of T$_c$. Using an approximate theoretical description of our granular system in terms of a layered one, we show that our data can only be reasonably fitted by a multilayer model. This indicates the importance of the interplay between different ferromagnetic grains; when non-collinearly magnetized they should lead to triplet Cooper pairing.

cond-mat.supr-con↗

arXiv2017

Superconductor-insulator transition in fcc-GeSb2Te4 at elevated pressures

We show that polycrystalline GeSb2Te4 in the fcc phase (f-GST), which is an insulator at low temperature at ambient pressure, becomes a superconductor at elevated pressures. Our study of the superconductor to insulator transition versus pressure at low temperatures reveals a second order quantum phase transition with linear scaling (critical exponent close to unity) of the transition temperature with the pressure above the critical zero-temperature pressure. In addition, we demonstrate that at higher pressures the f-GST goes through a structural phase transition via amorphization to bcc GST (b-GST), which also become superconducting. We also find that the pressure regime where an inhomogeneous mixture of amorphous and b-GST exists, there is an anomalous peak in magnetoresistance, and suggest an explanation for this anomaly.

cond-mat.supr-con↗

arXiv2014

Weak Localization Effects as Evidence for Bulk Quantization in Thin Films Bi2Se3

Strong spin-orbit coupling in topological insulators results in the ubiquitously observed weak antilocalization feature in their magnetoresistance. Here we present magnetoresistance measurements in ultra thin films of the topological insulator Bi_2Se_3, and show that in the 2D quantum limit, in which the topological insulator bulk becomes quantized, an additional negative magnetoresistance feature appears. Detailed analysis associates this feature with weak localization of the quantized bulk channels, providing thus evidence for this quantization. Examination of the dephasing fields at different temperatures indicates different scattering mechanism in the bulk vs the surface states.

cond-mat.mes-hall↗

arXiv2013

Emerging Weak Localization Effects on Topological Insulator-Insulating Ferromagnet (Bi_2Se_3-EuS) Interface

Thin films of topological insulator Bi_2Se_3 were deposited directly on insulating ferromagnetic EuS. Unusual negative magnetoresistance was observed near the zero field below the Curie temperature (T_C), resembling the weak localization effect; whereas the usual positive magnetoresistance was recovered above T_C. Such negative magnetoresistance was only observed for Bi_2Se_3 layers thinner than t~4nm, when its top and bottom surfaces are coupled. These results provide evidence for a proximity effect between a topological insulator and an insulating ferromagnet, laying the foundation for future realization of the half-integer quantized anomalous Hall effect in three-dimensional topological insulators.

cond-mat.mtrl-sci↗

arXiv2013

Anomalous response to gate voltage application in mesoscopic LaAlO_3/SrTiO_3 devices

We report on resistivity and Hall measurements performed on a series of narrow mesa devices fabricated from LaAlO_3/SrTiO_3 single interface heterostructure with a bridge width range of 1.5-10 microns. Upon applying back-gate voltage of the order of a few Volts, a strong increase in the sample resistance (up to factor of 35) is observed, suggesting a relatively large capacitance between the Hall-bar and the gate. The high value of this capacitance is due to the device geometry, and can be explained within an electrostatic model using the Thomas Fermi approximation. The Hall coefficient is sometimes a non-monotonic function of the gate voltage. This behavior is inconsistent with a single conduction band model. We show that a theoretical two-band model is consistent with this transport behavior, and indicates a metal to insulator transition in at least one of these bands.

cond-mat.mes-hall↗

arXiv2012

High Quality Ultrathin Bi2Se3 Films on CaF2 and CaF2/Si by Molecular Beam Epitaxy with a Radio Frequency Cracker Cell

Here we report a method to fabricate high quality Bi2Se3 thin films using molecular beam epitaxy with a radio frequency cracker cell as an atomic selenium source. With rates close to exact stoichiometry, optimal layer-by-layer growth of high quality Bi2Se3 thin films with smooth surfaces, has been achieved on CaF2(111) substrates and Si(111) substrates with a thin CaF2 buffer layer(CaF2/Si). Transport measurements show a characteristic weak antilocalization mangnetoresistance, with emergence of weak localization in the ultrathin film limit. Quantum Oscillations attributed to the topological surface states have been observed, including in films on CaF2/Si.

cond-mat.mtrl-sci↗

arXiv2012

Weak antilocalization and disorder-enhanced electron interactions in crystalline GeSbTe

Phase change materials can be reversibly switched between amorphous and crystalline states and often show strong contrast in the optical and electrical properties of these two phases. They are now in widespread use for optical data storage, and their fast switching and a pronounced change of resistivity upon crystallization are also very attractive for nonvolatile electronic data storage. Nevertheless there are still several open questions regarding the electronic states and charge transport in these compounds. In this work we study electrical transport in thin metallic films of the disordered, crystalline phase change material Ge$_1$Sb$_2$Te$_4$. We observe weak antilocalization and disorder enhanced Coulomb interaction effects at low temperatures, and separate the contributions of these two phenomena to the temperature dependence of the resistivity, Hall effect, and magnetoresistance. Strong spin-orbit scattering causes positive magnetoresistance at all temperatures, and a careful analysis of the low-field magnetoresistance allows us to extract the temperature dependent electron dephasing rate and study other scattering phenomena. We find electron dephasing due to inelastic electron-phonon scattering at higher temperatures, electron-electron scattering dephasing at intermediate temperatures, and a crossover to weak temperature dependence below 1 K.

cond-mat.mes-hall↗

arXiv2009

Polar Kerr Effect as Probe for Time-Reversal Symmetry Breaking in Unconventional Superconductors

The search for broken time reversal symmetry (TRSB) in unconventional superconductors intensified in the past year as more systems have been predicted to possess such a state. Following our pioneering study of TRSB states in Sr$_2$RuO$_4$ using magneto-optic probes, we embarked on a systematic study of several other of these candidate systems. The primary instrument for our studies is the Sagnac magneto-optic interferometer, which we recently developed. This instrument can measure magneto-optic Faraday or Kerr effects with an unprecedented sensitivity of 10 nanoradians at temperatures as low as 100 mK. In this paper we review our recent studies of TRSB in several systems, emphasizing the study of the pseudogap state of high temperature superconductors and the inverse proximity effect in superconductor/ferromagnet proximity structures.

cond-mat.str-el↗

arXiv1996

Inductive Probing of the Integer Quantum Hall Effect

We investigated the Integer Quantum Hall Effect (IQHE) using an inductive method. The following conclusions can be derived from our study: (i) when the Fermi energy is located between Landau levels the only extended states at the Fermi energy are located at the physical edges of the sample. (ii) the extended states located at the bulk of the sample below the Fermi energy are capable of carrying a substantial amount of Hall current, but cannot screen an external electrostatic potential.

cond-mat↗