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Alexander S. Solntsev

Publications and source records attributed to Alexander S. Solntsev.

At least 37 records · Page 2Linked to original sources

Metasurfaces for Quantum Photonics

Rapid progress in the development of metasurfaces allowed to replace bulky optical assemblies with thin nanostructured films, often called metasurfaces, opening a broad range of novel and superior applications to the generation, manipulation, and detection of light in classical optics. Recently, these developments started making a headway in quantum photonics, where novel opportunities arose for the control of nonclassical nature of light, including photon statistics, quantum state superposition, quantum entanglement, and single-photon detection. In this Perspective, we review recent progress in the field of quantum-photonics applications of metasurfaces, focusing on innovative and promising approaches to create, manipulate, and detect nonclassical light.

physics.optics↗

Large few-layer hexagonal boron nitride flakes for nonlinear optics

Hexagonal boron nitride (hBN) is a layered dielectric material with a wide range of applications in optics and photonics. In this work, we demonstrate a fabrication method for few-layer hBN flakes with areas up to 5000 $\rm μm$. We show that hBN in this form can be integrated with photonic microstructures: as an example, we use a circular Bragg grating (CBG). The layer quality of the exfoliated hBN flake on a CBG is confirmed by second-harmonic generation (SHG) microscopy. We show that the SHG signal is uniform across the hBN sample outside the CBG and is amplified in the centre of the CBG.

physics.app-ph↗

Multidimensional synthetic chiral-tube lattices via nonlinear frequency conversion

Geometrical dimensionality plays a fundamentally important role in the topological effects arising in discrete lattices. While direct experiments are limited by three spatial dimensions, the research topic of synthetic dimensions implemented by the frequency degree of freedom in photonics is rapidly advancing. The manipulation of light in such artificial lattices is typically realized through electro-optic modulation, yet their operating bandwidth imposes practical constraints on the range of interactions between different frequency components. Here we propose and experimentally realize all-optical synthetic dimensions involving specially tailored simultaneous short- and long-range interactions between discrete spectral lines mediated by frequency conversion in a nonlinear waveguide. We realize triangular chiral-tube lattices in three-dimensional space and explore their four-dimensional generalization. We implement a synthetic gauge field with nonzero magnetic flux and observe the associated multidimensional dynamics of frequency combs, all within one physical spatial port. We anticipate that our method will provide a new means for the fundamental study of high-dimensional physics and act as an important step towards using topological effects in optical devices operating in the time and frequency domains.

physics.optics↗

Synthetic photonic lattice for single-shot reconstruction of frequency combs

We formulate theoretically and demonstrate experimentally an all-optical method for reconstruction of the amplitude, phase and coherence of frequency combs from a single-shot measurement of the spectral intensity. Our approach exploits synthetic frequency lattices with pump-induced spectral short- and long-range couplings between different signal components across a broad bandwidth of of hundreds GHz in a single nonlinear fiber. When combined with ultra-fast signal conversion techniques, this approach has the potential to provide real-time measurement of pulse-to-pulse variations in the spectral phase and coherence properties of exotic light sources.

physics.optics↗

Second-harmonic generation in multilayer hexagonal boron nitride flakes

We report second-harmonic generation (SHG) from thick hexagonal boron nitride (hBN) flakes with approximately 109-111 layers. The resulting effective second-order susceptibility is similar to previously reported few-layer experiments. This confirms that thick hBN flakes can serve as a platform for nonlinear optics, which is useful because thick flakes are easy to exfoliate while retaining a large flake size. We also show spatial second-harmonic maps revealing that SHG remains a useful tool for the characterization of the layer structure even in the case of a large number of layers.

physics.optics↗

Spontaneous photon-pair generation at the nanoscale

Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far-field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we demonstrate experimentally the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi-photon wavelengths and when excited by a pump beam generates photonpairs with a rate of 35 Hz. Normalized to the pump energy stored by the nanoantenna, this rate corresponds to 1.4 GHz/Wm, being one order of magnitude higher than conventional on-chip or bulk photon-pair sources. Our experiments open the way for multiplexing several antennas for coherent generation of multi-photon quantum states with complex spatial-mode entanglement and applications in free-space quantum communications and sensing.

quant-ph↗

Reconfigurable cluster state generation in specially poled nonlinear waveguide arrays

We present a new approach for generating cluster states on-chip, with the state encoded in the spatial component of the photonic wavefunction. We show that for spatial encoding, a change of measurement basis can improve the practicality of cluster state algorithm implementation, and demonstrate this by simulating Grover's search algorithm. Our state generation scheme involves shaping the wavefunction produced by spontaneous parametric down-conversion in on-chip waveguides using specially tailored nonlinear poling patterns. Furthermore the form of the cluster state can be reconfigured quickly by driving different waveguides in the array.

physics.optics↗

Suppression of Spectral Diffusion by Anti-Stokes Excitation of Quantum Emitters in Hexagonal Boron Nitride

Solid-state quantum emitters are garnering a lot of attention due to their role in scalable quantum photonics. A notable majority of these emitters, however, exhibit spectral diffusion due to local, fluctuating electromagnetic fields. In this work, we demonstrate efficient Anti-Stokes (AS) excitation of quantum emitters in hexagonal boron nitride (hBN), and show that the process results in the suppression of a specific mechanism responsible for spectral diffusion of the emitters. We also demonstrate an all-optical gating scheme that exploits Stokes and Anti-Stokes excitation to manipulate spectral diffusion so as to switch and lock the emission energy of the photon source. In this scheme, reversible spectral jumps are deliberately enabled by pumping the emitter with high energy (Stokes) excitation; AS excitation is then used to lock the system into a fixed state characterized by a fixed emission energy. Our results provide important insights into the photophysical properties of quantum emitters in hBN, and introduce a new strategy for controlling the emission wavelength of quantum emitters.

physics.optics↗

Anti-Stokes excitation of solid-state quantum emitters for nanoscale thermometry

Color centers in solids are the fundamental constituents of a plethora of applications such as lasers, light emitting diodes and sensors, as well as the foundation of advanced quantum information and communication technologies. Their photoluminescence properties are usually studied under Stokes excitation, in which the emitted photons are at a lower energy than the excitation ones. In this work, we explore the opposite Anti-Stokes process, where excitation is performed with lower energy photons. We report that the process is sufficiently efficient to excite even a single quantum system, namely the germanium-vacancy center in diamond. Consequently, we leverage the temperature-dependent, phonon-assisted mechanism to realize an all-optical nanoscale thermometry scheme that outperforms any homologous optical method employed to date. Our results frame a promising approach for exploring fundamental light-matter interactions in isolated quantum systems, and harness it towards the realization of practical nanoscale thermometry and sensing.

physics.app-ph↗

Quantum metasurface for multi-photon interference and state reconstruction

Metasurfaces based on resonant nanophotonic structures have enabled novel types of flat-optics devices often outperforming the capabilities of bulk components, yet these advances remain largely unexplored for quantum applications. We show that non-classical multi-photon interferences can be achieved at the subwavelength scale in all-dielectric metasurfaces. We simultaneously image multiple projections of quantum states with a single metasurface, enabling a robust reconstruction of amplitude, phase, coherence, and entanglement of multi-photon polarization-encoded states. One- and two-photon states are reconstructed through nonlocal photon correlation measurements with polarization-insensitive click-detectors positioned after the metasurface, and the scalability to higher photon numbers is established theoretically. Our work illustrates the feasibility of ultra-thin quantum metadevices for the manipulation and measurement of multi-photon quantum states with applications in free-space quantum imaging and communications.

quant-ph↗

Spectral photonic lattices with complex long-range coupling

We suggest and experimentally realize a spectral photonic lattice - a signal can hop between discrete frequency channels, driven by nonlinear interaction with stronger pump lasers. By controlling the complex envelope and frequency separations of multiple pumps, it is possible to introduce non- local hopping and to break time-reversal symmetry, which opens up new possibilities for photonic quantum simulation. As two examples, we observe a spectral quantum walk and demonstrate the discrete Talbot effect in the spectral domain, where we find novel instances containing asymmetry and periodicities not possible in spatial lattices.

physics.optics↗

Non-reciprocal geometric phase in nonlinear frequency conversion

We describe analytically and numerically the geometric phase arising from nonlinear frequency conversion and show that such a phase can be made non-reciprocal by momentum-dependent photonic transition. Such non-reciprocity is immune to the shortcomings imposed by dynamic reciprocity in Kerr and Kerr-like devices. We propose a simple and practical implementation, requiring only a single waveguide and one pump, while the geometric phase is controllable by the pump and promises robustness against fabrication errors.

physics.optics↗

Direct characterization of a nonlinear photonic circuit's wave function with laser light

Integrated photonics is a leading platform for quantum technologies including nonclassical state generation \cite{Vergyris:2016-35975:SRP, Solntsev:2014-31007:PRX, Silverstone:2014-104:NPHOT, Solntsev:2016:RPH}, demonstration of quantum computational complexity \cite{Lamitral_NJP2016} and secure quantum communications \cite{Zhang:2014-130501:PRL}. As photonic circuits grow in complexity, full quantum tomography becomes impractical, and therefore an efficient method for their characterization \cite{Lobino:2008-563:SCI, Rahimi-Keshari:2011-13006:NJP} is essential. Here we propose and demonstrate a fast, reliable method for reconstructing the two-photon state produced by an arbitrary quadratically nonlinear optical circuit. By establishing a rigorous correspondence between the generated quantum state and classical sum-frequency generation measurements from laser light, we overcome the limitations of previous approaches for lossy multimode devices \cite{Liscidini:2013-193602:PRL, Helt:2015-1460:OL}. We applied this protocol to a multi-channel nonlinear waveguide network, and measured a 99.28$\pm$0.31\% fidelity between classical and quantum characterization. This technique enables fast and precise evaluation of nonlinear quantum photonic networks, a crucial step towards complex, large-scale, device production.

quant-ph↗

Tunable generation of entangled photons in a nonlinear directional coupler

The on-chip integration of quantum light sources has enabled the realization of complex quantum photonic circuits. However, for the practical implementation of such circuits in quantum information applications it is crucial to develop sources delivering entangled quantum photon states with on-demand tunability. Here we propose and experimentally demonstrate the concept of a widely tunable quantum light source based on spontaneous parametric down-conversion in a nonlinear directional coupler. We show that spatial photon-pair correlations and entanglement can be reconfigured on-demand by tuning the phase difference between the pump beams and the phase mismatch inside the structure. We demonstrate the generation of split states, robust N00N states, various intermediate regimes and biphoton steering. This fundamental scheme provides an important advance towards the realization of reconfigurable quantum circuitry.

quant-ph↗

Cascaded third harmonic generation in hybrid graphene-semiconductor waveguides

We study cascaded harmonic generation of hybrid surface plasmons in integrated planar waveguides composed of a graphene layer and a doped-semiconductor slab. We derive a comprehensive model of cascaded third harmonic generation through phase-matched nonlinear interaction of fundamental, second harmonic and third harmonic plasmonic modes supported by the structure. We show that hybrid graphene-semiconductor waveguides can simultaneously phase-match these three interacting harmonics, increasing the total third-harmonic output by a factor of 5 compared to the non-cascaded regime.

physics.optics↗

Modulated coupled nanowires for ultrashort pulses

We predict analytically and confirm with numerical simulations that inter-mode dispersion in nanowire waveguide arrays can be tailored through periodic waveguide bending, facilitating flexible spatio-temporal reshaping without break-up of femtosecond pulses. This approach allows simulta- neous and independent control of temporal dispersion and spatial diffraction that are often strongly connected in nanophotonic structures.

physics.optics↗

Parity-Time Anti-Symmetric Parametric Amplifier

We describe the process of parametric amplification in a directional coupler of quadratically nonlinear and lossy waveguides, which belong to a class of optical systems with spatial parity-time (PT) symmetry in the linear regime. We identify a distinct spectral parity-time anti-symmetry associated with optical parametric interactions, and show that pump-controlled symmetry breaking can facilitate spectrally selective mode amplification in analogy with PT lasers. We also establish a connection between breaking of spectral and spatial mode symmetries, revealing the potential to implement unconventional regimes of spatial light switching through ultrafast control of PT breaking by pump pulses.

physics.optics↗

Lattice topology and spontaneous parametric down-conversion in quadratic nonlinear waveguide arrays

We analyze spontaneous parametric down-conversion in various experimentally feasible 1D quadratic nonlinear waveguide arrays, with emphasis on the relationship between the lattice's topological invariants and the biphoton correlations. Nontrivial topology results in a nontrivial "winding" of the array's Bloch waves, which introduces additional selection rules for the generation of biphotons. These selection rules are in addition to, and independent of existing control using the pump beam's spatial profile and phase matching conditions. In finite lattices, nontrivial topology produces single photon edge modes, resulting in "hybrid" biphoton edge modes, with one photon localized at the edge and the other propagating into the bulk. When the single photon band gap is sufficiently large, these hybrid biphoton modes reside in a band gap of the bulk biphoton Bloch wave spectrum. Numerical simulations support our analytical results.

physics.optics↗